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RESEARCH PAPER · Nature Communications · 2022

Rapid atom-efficient polyolefin plastics hydrogenolysis mediated by a well-defined single-site electrophilic/cationic organo-zirconium catalyst

Alexander H. Mason, Alessandro Motta, Anusheela Das, Qing Ma, Michael J. Bedzyk, Yosi Kratish, Tobin Jay Marks

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Rapid atom-efficient polyolefin plastics hydrogenolysis mediated by a well-defined single-site electrophilic/cationic organo-zirconium catalystOriginalDual-Pathway Polyolefin Upcycling over an Unexpectedly Bifunctional Low-Loading Ru/TiO2-Anatase Catalyst54Enabling resource circularity through thermo-catalytic and solvent-based conversion of waste plastics49Cationic Tantalum Hydrides Catalyze Hydrogenolysis and Alkane Metathesis Reactions of Paraffins and Polyethylene38Highly Efficient Polyolefin Hydrogenolysis Enabled by a Single-Site Organo-Tantalum Catalyst on a Super-Acidic Support0Sustainable developments in polyolefin chemistry: Progress, challenges, and outlook204Investigation into the Reaction Pathways and Catalyst Deactivation for Polyethylene Hydrogenolysis over Silica-Supported Cobalt Catalysts58Structure–Property Relationships for Nickel Aluminate Catalysts in Polyethylene Hydrogenolysis with Low Methane Selectivity61MAO- and Borate-Free Activating Supports for Group 4 Metallocene and Post-Metallocene Catalysts of α-Olefin Polymerization and Oligomerization11Upcycling of polyethylenes by catalysis0Polypropylene Degradation Catalyzed by Tantalum Hydrides Supported on Sulfated Alumina23Treasuring trash: Pt/SrTiO3 catalysts process plastic waste into high-value materials25Molecular Alumo- and Gallosilicate Hydrides Functionalized with Terminal M(NR2)3 and Bridging M(NR2)2 (M = Ti, Zr, Hf; R = Me, Et) Moieties2Atomically‐Dispersed Metal Heterocatalysts: A Practical Step Toward Sustainability2Chemically recyclable polyolefin-like multiblock polymers201A Supported Ziegler-Type Organohafnium Site Metabolizes Polypropylene8Rapid Polyolefin Hydrogenolysis by a Single‐Site Organo‐Tantalum Catalyst on a Super‐Acidic Support: Structure and Mechanism14Rapid Polyolefin Hydrogenolysis by a Single‐Site Organo‐Tantalum Catalyst on a Super‐Acidic Support: Structure and Mechanism5Isoreticular Metal–Organic Frameworks Confined Mononuclear Ru-Hydrides Enable Highly Efficient Shape-Selective Hydrogenolysis of Polyolefins39Rapid Polyolefin Plastic Hydrogenolysis Mediated by Single-Site Heterogeneous Electrophilic/Cationic Organo-group IV Catalysts19Depolymerization of waste polyethylene to linear alkenes via sequential dehydrogenation and metathesis19Modern mechanistic approaches for the depolymerization of commodity plastics via organometallic catalysis0Review on Catalytic Depolymerization of Polyolefin Waste by Hydrogenolysis: State-of-the-Art and Outlook57Highly Selective Upgrading of Polyethylene into Light Aromatics via a Low-Temperature Melting-Catalysis Strategy55Emerging green approaches for valorization of plastics with saturated carbon backbones42Dynamic Chemistry Toolbox for Advanced Sustainable Materials24Catalytic Strategies for the Upcycling of Polyolefin Plastic Waste30Circular olefin copolymers made de novo from ethylene and α-olefins83Temperature-Dependent NiFeAl catalysts for efficient microwave-assisted catalytic pyrolysis of polyethylene into value-added hydrogen and carbon nanotubes24The Overlooked Potential of Sulfated Zirconia: Reexamining Solid Superacidity Toward the Controlled Depolymerization of Polyolefins11A US perspective on closing the carbon cycle to defossilize difficult-to-electrify segments of our economy60Molecular engineering of a MOF with an ionic liquid sheath for direct air separation at ambient conditions12Catalytic chemical recycling and upcycling of polyolefin plastics27Demystifying group-4 polyolefin hydrogenolysis catalysis: Gaseous propane hydrogenolysis mechanism over the same catalysts5Mild Catalytic Degradation of Crystalline Polyethylene Units in a Solid State Assisted by Carboxylic Acid Groups23Pyrolytic Depolymerization of Polyolefins Catalysed by Zirconium‐based UiO‐66 Metal–Organic Frameworks38Pyrolytic Depolymerization of Polyolefins Catalysed by Zirconium‐based UiO‐66 Metal–Organic Frameworks10Catalytic Upcycling of Polyolefins316The role of size and structure of catalytic active sites in polyolefin hydrogenolysis12Assessment of transport phenomena in catalyst effectiveness for chemical polyolefin recycling45Hydroborative Depolymerization of Polyesters and Polycarbonates to Diols Catalyzed by Heterogeneous Lanthanum Materials La(CH2C6H4NMe2-o)3@SBA-155Upcycling of polyethylene waste to biodegradable adhesive and coating via Baeyer-Villiger reaction: A new view on oxidation-fracture mechanism and structure-function relationship10Hydrogenolysis of Polyethylene by Metal–Organic Framework Confined Single-Site Ruthenium Catalysts16Chemically Recyclable, Reprocessable, and Mechanically Robust Reversible Cross-Linked Polyurea Plastics for Fully Recyclable Aramid Fiber Reinforced Composites15Investigation on the role of hydrogen in polyethylene hydropyrolysis process via ReaxFF molecular dynamic simulation2Microwave‐Powered Liquid Metal Degradation of Polyolefins30Sustainability in Polyolefins0Upgrading of waste polyolefins with non-noble metal catalysts21Conversion of Polypropylene to Light Olefins by HMFI Catalysts below Pyrolytic Temperature: Catalytic, Spectroscopic, and Theoretical Studies3Advances and Challenges in Low‐Temperature Upcycling of Waste Polyolefins via Tandem Catalysis25Advances and Challenges in Low‐Temperature Upcycling of Waste Polyolefins via Tandem Catalysis2Reductive Upcycling of Polyolefins, Polyesters and Mixed Plastic Wastes to Valuable Chemicals: Bridging Chemical Catalysis With Plastic Waste Management35Enhancing Waste Plastic Hydrogenolysis on Ru/CeO 2 Through Concurrent Incorporation of Fe Single Atoms and FeO x Nanoclusters27Enhancing Waste Plastic Hydrogenolysis on Ru/CeO 2 Through Concurrent Incorporation of Fe Single Atoms and FeO x Nanoclusters4Synergistic Catalysis for Recycling and Upcycling of Plastics35Predicting a generalized mechanism of branched alkane hydrogenolysis on Ru, Ir, and Pt surfaces relevant to polymer upcycling applications3A Broad-Spectrum Catalyst for Aliphatic Polymer Breakdown4Stable single-site organonickel catalyst preferentially hydrogenolyses branched polyolefin C–C bonds12Single-site catalyst cuts branched polyolefins to pieces2Polymer Upcycling by Catalytic Hydrogenolysis: The Role of Polyolefin Short-Chain Branching3Atomically dispersed zirconium hydroxide promotes the selective transfer hydrogenolysis of aromatic alcohols to methyl aromatics0From waste to value: A review of emerging plastic valorization technologies3Surface and Interface Properties of Metal Species for Waste Plastic Hydroconversion6Catalytic valorization of polyolefins: from catalysts and processes to reactors0Acid sites in hydrogen-involved polyolefin upcycling: mechanistic insights and design principles0Reductive catalytic upcycling of polyolefins for sustainable fuel production0Recent advancements in catalytic processes for plastic upcycling into fuels: a major step in sustainable waste management and energy production3Thermo-chemical upgrading of waste polyethylene and polypropylene plastics0Hydrogenolysis Versus Hydrocracking for Polyolefin Upcycling0Cleavage Alkylation Coupling with Versatile Amide-Based Eutectic Catalytic Systems0Catalytic Upcycling of Polyolefins and Polystyrene: Integrating Active Site Design With Mass Transfer Considerations4Engineering Interfacial Compatibility and Dynamic Active Hydrogen Pools to Accelerate Polyolefin Hydrogenolysis0Emerging Dynamic Polymers for Sustainable Materials0From waste to wealth: Advanced strategies and mechanisms for chemical recycling and upcycling of polymeric materials1Atomically precise catalysts design toward efficient waste plastic hydrogenolysis2Advances in Catalytic Hydrogenolysis of Waste Plastics to Value-Added Products0Controlling Polyolefin Hydrogenolysis Selectivity by Engineering Single-Site Nickel(II) Hydride Active Catalytic Species0A Review on Catalyst Chemical Recycling Technologies for Production of Light Gaseous Compounds from Polyolefin Waste1Machine learning induced tandem catalysis for high-value recovery of polyolefins: pathways, mechanisms and products0Comprehensive quantitative analysis of polyolefin hydrogenolysis toward plastic waste management0Catalytic pyrolysis of waste plastics to liquid fuels: pathways, mechanisms, and challenges0Homogeneous Ru/La2O2CO3 Catalyst for Efficient Thermal Cracking of Crosslinked Polyethylene0Challenges in polyolefin re/upcycling catalysis specific to polymer feedstock0

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  1. Dual-Pathway Polyolefin Upcycling over an Unexpectedly Bifunctional Low-Loading Ru/TiO2-Anatase Catalyst

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  3. Cationic Tantalum Hydrides Catalyze Hydrogenolysis and Alkane Metathesis Reactions of Paraffins and Polyethylene

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  4. Highly Efficient Polyolefin Hydrogenolysis Enabled by a Single-Site Organo-Tantalum Catalyst on a Super-Acidic Support

    ChemRxiv · 2023-03-15

    Qingheng Lai, Alexander H. Mason, Amol Agarwal, Wilson C. Edenfield, Xinrui Zhang, Takeshi Kobayashi, Yosi Kratish, Tobin Jay Marks

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  5. Sustainable developments in polyolefin chemistry: Progress, challenges, and outlook

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  6. Investigation into the Reaction Pathways and Catalyst Deactivation for Polyethylene Hydrogenolysis over Silica-Supported Cobalt Catalysts

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  7. Structure–Property Relationships for Nickel Aluminate Catalysts in Polyethylene Hydrogenolysis with Low Methane Selectivity

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  8. MAO- and Borate-Free Activating Supports for Group 4 Metallocene and Post-Metallocene Catalysts of α-Olefin Polymerization and Oligomerization

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  9. Upcycling of polyethylenes by catalysis

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  10. Polypropylene Degradation Catalyzed by Tantalum Hydrides Supported on Sulfated Alumina

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  11. Treasuring trash: Pt/SrTiO3 catalysts process plastic waste into high-value materials

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  12. Molecular Alumo- and Gallosilicate Hydrides Functionalized with Terminal M(NR2)3 and Bridging M(NR2)2 (M = Ti, Zr, Hf; R = Me, Et) Moieties

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  13. Atomically‐Dispersed Metal Heterocatalysts: A Practical Step Toward Sustainability

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  14. Chemically recyclable polyolefin-like multiblock polymers

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  15. A Supported Ziegler-Type Organohafnium Site Metabolizes Polypropylene

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  16. Rapid Polyolefin Hydrogenolysis by a Single‐Site Organo‐Tantalum Catalyst on a Super‐Acidic Support: Structure and Mechanism

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  17. Rapid Polyolefin Hydrogenolysis by a Single‐Site Organo‐Tantalum Catalyst on a Super‐Acidic Support: Structure and Mechanism

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  18. Isoreticular Metal–Organic Frameworks Confined Mononuclear Ru-Hydrides Enable Highly Efficient Shape-Selective Hydrogenolysis of Polyolefins

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  19. Rapid Polyolefin Plastic Hydrogenolysis Mediated by Single-Site Heterogeneous Electrophilic/Cationic Organo-group IV Catalysts

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  20. Depolymerization of waste polyethylene to linear alkenes via sequential dehydrogenation and metathesis

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  28. Temperature-Dependent NiFeAl catalysts for efficient microwave-assisted catalytic pyrolysis of polyethylene into value-added hydrogen and carbon nanotubes

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  31. Molecular engineering of a MOF with an ionic liquid sheath for direct air separation at ambient conditions

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  32. Catalytic chemical recycling and upcycling of polyolefin plastics

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  33. Demystifying group-4 polyolefin hydrogenolysis catalysis: Gaseous propane hydrogenolysis mechanism over the same catalysts

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