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RESEARCH PAPER · Annual Review of Chemical and Biomolecular Engineering · 2022

The Critical Role of Process Analysis in Chemical Recycling and Upcycling of Waste Plastics

Scott R. Nicholson, Julie E. Rorrer, Avantika Singh, Mikhail O. Konev, Nicholas A. Rorrer, Alberta C. Carpenter, Alan J. Jacobsen, Yuriy Román‐Leshkov, Gregg T. Beckham

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The Critical Role of Process Analysis in Chemical Recycling and Upcycling of Waste PlasticsOriginalLife cycle assessment of enzymatic poly(ethylene terephthalate) recycling156Systemic approaches to model plastics circularity0TOWARDS A CIRCULAR ECONOMY: LIQUID-FED FAST PYROLYSIS OF WASTE POLYOLEFIN PLASTICS1Quantification and evaluation of plastic waste in the United States189Plastic Waste Valorization by Leveraging Multidisciplinary Catalytic Technologies169Material Flow Analysis and Life Cycle Assessment of Polyethylene Terephthalate and Polyolefin Plastics Supply Chains in the United States54Enabling resource circularity through thermo-catalytic and solvent-based conversion of waste plastics49Nachhaltiges Design von Struktur‐ und Funktionspolymeren für die Kreislaufwirtschaft6RETRACTED: Hydrogenolysis of Polyethylene and Polypropylene into Propane over Cobalt-Based Catalysts72Sustainable Design of Structural and Functional Polymers for a Circular Economy159Mixed plastics waste valorization through tandem chemical oxidation and biological funneling635Competing Time Scales in Surface-Driven Solution Depolymerization2Economic and environmental analysis of plastics pyrolysis after secondary sortation of mixed plastic waste88Circular Upcycling of Bottlebrush Thermosets14Circular Upcycling of Bottlebrush Thermosets3Selective deconstruction of mixed plastics by a tailored organocatalyst70Solvent based dissolution–precipitation of waste polyethylene terephthalate: economic and environmental performance metrics40Techno-economic analysis and life cycle assessment for catalytic fast pyrolysis of mixed plastic waste210Techno-economic analysis and life cycle assessment of mixed plastic waste gasification for production of methanol and hydrogen139Technical, Economic, and Environmental Comparison of Closed-Loop Recycling Technologies for Common Plastics425The contribution of high-resolution GC separations in plastic recycling research14Manufacturing Energy and Greenhouse Gas Emissions Associated with United States Consumption of Organic Petrochemicals64Trends in Polyester Upcycling for Diversifying a Problematic Waste Stream50Towards circular plastics within planetary boundaries392Mass transfer in catalytic depolymerization: External effectiveness factors and serendipitous processivity in stagnant and stirred melts31Bifunctional tandem catalytic upcycling of polyethylene to surfactant-range alkylaromatics101Transitioning to a Sustainable, Circular Economy for Plastics [Workshop Report]0A focused review on recycling and hydrolysis techniques of polyethylene terephthalate205Sustainable utilization of alkane resources toward carbon neutrality2Hydrogen-free catalytic depolymerization of waste polyolefins at mild temperatures43Closed-Loop Recycling of Polyols from Thermoset Polyurethanes by tert -Amyl Alcohol-Mediated Depolymerization of Flexible Foams52Ionic-Liquid-Mediated Deconstruction of Polymers for Advanced Recycling and Upcycling45Review and recommendations for sustainable pathways of recycling commodity plastic waste across different economic regions51Circular plastics technologies: open loop recycling of waste plastics into new chemicals0Additive manufacturing for sustainability and circular economy: needs, challenges, and opportunities for 3D printing of recycled polymeric waste151Valorization of waste plastics and waste oases of Gabes-Tunisia to prepare polymeric membrane for oily wastewater treatment3Upcycling plastic polymers into single-walled carbon nanotubes from a magnesia supported iron catalyst27Dynamics, uncertainty and control in circular supply chains8Rapid Polyolefin Hydrogenolysis by a Single‐Site Organo‐Tantalum Catalyst on a Super‐Acidic Support: Structure and Mechanism14Rapid Polyolefin Hydrogenolysis by a Single‐Site Organo‐Tantalum Catalyst on a Super‐Acidic Support: Structure and Mechanism5Converting Waste Plastic to Liquid Organic Hydrogen Carriers16Converting Waste Plastic to Liquid Organic Hydrogen Carriers1Optimización de las propiedades de tenacidad e impacto de formulaciones de ácido poliláctico (PLA), mediante mezclas con polímeros flexibles y optimización de los sistemas de compatibilización0Chemical recycling of plastic wastes via homogeneous catalysis: A review78Models for Decarbonization in the Chemical Industry38Pyrolysis of mixed engineering plastics: Economic challenges for automotive plastic waste39Development of Enzyme-Based Approaches for Recycling PET on an Industrial Scale34Chlorinated plastics offer unique opportunities and challenges in upcycling25Depolymerization within a Circular Plastics System387Biobased de novo synthesis, upcycling, and recycling — the heartbeat toward a green and sustainable polyethylene terephthalate industry26Sorting plastics waste for a circular economy: Perspectives for lanthanide luminescent markers26Effect of reaction media on hydrogenolysis of polyethylene plastic waste: Polymer-surface interactions in small alkane/polymer blends35Bio-based lactone acrylic plastics with performance and recyclability advantages10Perspective on the Development of Monomer Recovery Technologies from Plastics Designed to Last28Terpenoid-based high-performance polyester with tacticity-independent crystallinity and chemical circularity21Chemical upcycling of polyolefins into liquid refinery feedstock from the circularity and chemical engineering aspects11High Molecular Weight Product Formation in Polyolefin Chemical Recycling: A Comprehensive Review on Primary and Secondary Products18Depolymerization mechanisms and closed-loop assessment in polyester waste recycling144PVC Modification through Sequential Dehydrochlorination–Hydrogenation Reaction Cycles Facilitated via Fractionation by Green Solvents17Catalytic Upcycling of Polyolefins316The environmental impact of end-of-life PVC flex banners and its potential upcycling opportunities12Quantification and Categorization of Macroplastics (Plastic Debris) within a Headwaters Basin in Western North Carolina, USA: Implications to the Potential Impacts of Plastic Pollution on Biota11Cross-Linked Polyolefins: Opportunities for Fostering Circularity Throughout the Materials Lifecycle28Analyses of circular solutions for advanced plastics waste recycling88Circular Economy and Chemical Conversion for Polyester Wastes23Mixed polyester recycling can enable a circular plastic economy with environmental benefits38Chemistry in Plastic Recycling: Breaking Down Polymers3Advances and Challenges for Catalytic Recycling and Upgrading of Real-World Mixed Plastic Waste100Upcycling of waste plastics: strategies, status-quo, and prospects3Intensification & Scale-up of Waste Plastic Upcycling to Lubricants Conversion0Is it possible to distinguish virgin versus pyrolytic recycled styrene by determining the intramolecular 13 C distribution?0Tuning solvent strength can fractionate PVC into ultra-low molecular weight material with low dispersity6Waving the green flag: incorporating sustainable and green chemistry practices into research and education8Recent Advances in Electrochemical Organic Waste Reforming: Highlights on Anodic Chemistry, Materials Design, and System Integration11Stereomicrostructure-regulated biodegradable adhesives104Scalable, biologically sourced depolymerizable polydienes with intrinsically weakened carbon–carbon bonds14Photocatalytic Upgrading of Plastic Waste into High-Value-Added Chemicals and Fuels: Advances and Perspectives49Towards Circular Economy: Integrating Polymer Recycling and 3D Printing for Economic Regeneration11Technological trajectories in circular economy: Bridging patent analytics with sustainable development goals19Global trends and strategic pathways for waste plastics depolymerization in the circular economy3Co-recycling of plastics and other waste materials70Process innovations to enable viable enzymatic poly(ethylene terephthalate) recycling41Population Balance Models for Catalytic Depolymerization: From Elementary Steps to Multiphase Reactors8Process Systems Engineering Approaches for Sustainable Plastics Management9Recent Advances in the Thermo-Catalytic Upcycling of Polyethylene Waste13Acetolysis for epoxy-amine carbon fibre-reinforced polymer recycling84Light-Responsive Star Polymers for Reprocessable Network Formation and Deconstruction6Carbon-fibre composites can be broken down into reusable components0Accelerated Acid-Assisted Degradability and Tunable Properties of 1,1-Diphenylethylene Copolymers2Life cycle climate change and economic impact of biodegradable biopolymer poly(3-hydroxybutyrate-co-3-hydroxyhexanoate) (PHBH) for production expansion2Methods for Carbon Mass Closure in Polyolefin Hydrocracking6Circular economy strategies for converting waste plastics into surfactants6Closed-loop recycling of mixed polyesters via catalytic methanolysis and monomer separations22Degradation-catalysis of polypropylene into liquid fuel-range iso-olefins using Zn and Ni-incorporated microporous carbon3Composites from Postconsumer Polypropylene Carpet and Bottle-Waste Polyolefins3Ultra-high selective adsorbents for per- and polyfluoroalkyl substances (PFAS) destruction: Bridging the gap between adsorption and catalytic degradation for excellent performance in persistent environmental contaminants14Optimizing the use of pyrolysis waste oil as a feedstock for the naphtha cracking process by hydrotreating and hydrocracking4Mechanically Accelerated Depolymerization of Entangled Linear Polymer Melts2Life cycle assessment of plastics waste management technologies0Low-Carbon Thermochemical Upcycling of Plastic Waste with Steel Slag at Elevated Temperatures1Selective polyethylene hydrocracking to liquid and gaseous hydrocarbons over Co–Ni catalysts supported on H-BEA zeolite10Boosting the brightness of short-wave infrared emission in YPO 4 :Yb 3+ /Er 3+ phosphors: optimal photoluminescence quantum yield versus particle size1Carbon–carbon bond cleavage for lignin and plastics deconstruction0Recent advances in chemical recycling and upcycling of plastic waste into valuable materials, chemicals, and energy: a comprehensive review18Sustainable additive manufacturing: A review on 3D printing using recycled waste polymers0Tunable ether-functionalized protic ionic liquid for efficient glycolysis of polyethylene terephthalate5Techno-economic analysis and life cycle assessment for the catalytic hydrogenolysis and hydrocracking of polyethylene6Alcoholysis of nylon 6 waste to ε-caprolactam promoted by phosphoric acid4Lifetime-Adjusted LCA of Biochemical and Thermochemical Circular Plastic Pathways0Technoeconomic Analysis of Plastic Chemical Upcycling via Nitric Acid Thermal Oxidation0Coupled Population Balance Models for Evolution of Alkane, α ‐Olefin, and α, ω ‐Olefin Molecular Weight Distributions During Polypropylene Thermal Pyrolysis0Selective Oxidative Upcycling of Polyethylene Pyrolyzed Wax to High‐Performance Surfactants Using Synthesized Co and Mn–Co Stearate Catalysts0Advanced Sustainable Process Integration and Comprehensive Techno-Economic Evaluation of Polystyrene Waste Upcycling into Methanol as a Clean Alternative Fuel0Advances and technical challenges in mono-material plastics design for sustainability0

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  2. Systemic approaches to model plastics circularity

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  4. Quantification and evaluation of plastic waste in the United States

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  5. Plastic Waste Valorization by Leveraging Multidisciplinary Catalytic Technologies

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