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RESEARCH PAPER · ChemSusChem · 2021

Electrochemical Activation of C−C Bonds through Mediated Hydrogen Atom Transfer Reactions

Bing Yan, Changxia Shi, Gregg T. Beckham, Eugene Y.‐X. Chen, Yuriy Román‐Leshkov

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Electrochemical Activation of C−C Bonds through Mediated Hydrogen Atom Transfer ReactionsOriginalZ-Scheme nanocomposite with high redox ability for efficient cleavage of lignin C–C bonds under simulated solar light69Hydrogenolysis of Polypropylene and Mixed Polyolefin Plastic Waste over Ru/C to Produce Liquid Alkanes288Chemical Upcycling of Commercial Polystyrene via Catalyst-Controlled Photooxidation361Recent Advances in the Electrochemical Functionalization of Isocyanides28A Horseradish Peroxidase–Mediator System for Benzylic C–H Activation28Electrocatalytic upcycling of plastic waste79HAT‐Promoted Electrochemical Amination: C(sp2)−H/N−H Cross Dehydrogenative Coupling20Recent Advances in Catalytic Chemical Recycling of Polyolefins104Electrochemically Driven Hydrogen Atom Transfer Catalysis: A Tool for C(sp 3 )/Si–H Functionalization and Hydrofunctionalization of Alkenes98Unique Raoultella species isolated from petroleum contaminated soil degrades polystyrene and polyethylene24Mechanistic Insights Enable Divergent Product Selectivity in Catalyst-Controlled Photooxidative Degradation of Polystyrene90Selective Electrocatalytic Degradation of Ether‐Containing Polymers31Selective Electrocatalytic Degradation of Ether‐Containing Polymers1Precise activation of C–C bonds for recycling and upcycling of plastics81Electrochemical C−H/C−C Bond Oxygenation: A Potential Technology for Plastic Depolymerization13Recent advances in oxidative degradation of plastics227Biomass valorization via electrocatalytic carbon–carbon bond cleavage46Plastic Waste Conversion by Leveraging Renewable Photo/Electro‐Catalytic Technologies27Recent progress in upcycling of plastic wastes into value-added chemicals via photo-, electro- and photoelectro-catalytic strategies19Emerging green approaches for valorization of plastics with saturated carbon backbones42Recent Progress in Electrochemical Conversion from Biomass Derivatives into High‐Value‐Added Chemicals39Progress and Challenges in Polystyrene Recycling and Upcycling87Advancements and future directions in waste plastics recycling: From mechanical methods to innovative chemical processes136Photochemical Aerobic Upcycling of Polystyrene Plastics via Synergistic Indirect HAT Catalysis30A General Approach for Photo‐Oxidative Degradation of Various Polymers16Electrocatalytic upcycling of plastic waste: Progress, challenges, and future53Catalytic Upcycling of Polyolefins316Anodic Commodity Polymer Recycling: The Merger of Iron‐Electrocatalysis with Scalable Hydrogen Evolution Reaction25Anodisches Recycling von gängigen Polymeren: Die Kombination von Eisen‐Elektrokatalyse und skalierbarer Wasserstoffentwicklungsreaktion3Recent progress in energy-saving hydrogen production by coupling with value-added anodic reactions164Electrochemical Postpolymerization Modification and Deconstruction of Macromolecules23Reactivity and philicity of phthalimide-N-oxyl and benzotriazol-N-oxyl radicals in addition reactions to vinyl compounds2Low‐Temperature Catalytic Approaches for Upcycling Plastics into Oxygenated Aromatic Compounds14Catalytic materials based on metals (ions) used in the upcycling of plastics and polymers into fuels and valuable chemicals as part of sustainable development23Electrochemical C−H Hydroxylation and Alkoxylation Reactions14Upcycling of Polystyrene to Aromatic Polyacids by Tandem Friedel–Crafts and Oxidation Reactions30Research progress and challenges in the upcycling of polyolefin plastics through chemical oxidation4Electrochemical Deconstruction of Waste Polyvinylidene Chloride (PVDC) to Value‐Added Products in Batch and Flow16Harnessing Non-Thermal External Stimuli for Polymer Recycling23Catalytic conversion of polymer waste into high-value products for advancing circular economy and eco-sustainability11Pure and doped crystalline polyethylene under Earth’s conditions: A density functional theory study0Catalysis for the Upcycling of Polymers1Electrochemical Commodity Polymer Up‐ and Re‐Cycling: Toward Sustainable and Circular Plastic Treatment14Highly selective aerobic oxidation of polystyrene to benzoic acid catalyzed by nitrogen dioxide9Divergent Upcycling of Polystyrene into Phenol and Hydroquinone Derivatives by Photocatalysis and Electrocatalysis20Divergent Upcycling of Polystyrene into Phenol and Hydroquinone Derivatives by Photocatalysis and Electrocatalysis5Recent progress in upcycling of plastic-derived intermediates into value-added chemicals via electrocatalytic strategies – A review1Conversion of Polystyrene to Terephthalic Acid via Sequential Acetylation and Mn/Br-Catalyzed Autoxidation4Tandem depolymerization-electrocatalysis for plastic waste upcycling6Electrochemical depolymerization of polycarbonates under catalyst-free conditions0Highly efficient photoreforming of plastic waste for hydrogen production: recent advances and prospects1Nitroreductases as alkoxyamine-selective triggers0Research Progress in Metal-Free Electrochemical C—H Bond Activation for the Construction of C—N/C—O Bonds1Solar-Driven Upcycling of Polystyrene Enabled by Elemental Sulfur8Transforming plastics at the interface: Electrochemical re- and upcycling strategies5The Role of Free Radicals in the Mimetic Naphthalene Dioxygenase Function of Trametes versicolor Laccase Application for Biosynthesis of Isatin and Indirubin0Automated Microdroplet Reaction Platform for Condition Optimization and Kinetic Investigation of Photocatalytic Benzylic Oxidations0A Cu Single-Atom Catalyst as an Intrinsic Hydrogen Atom Transfer Mediator for Electrooxidation of C(sp3)–H Bonds0Electrochemical Postfunctionalization of Polymers: Versatile Strategies for Macromolecular Transformation0The Accelerated NHPI‐PINO Cycling Mediated by Surface Co‐Superoxo for Efficient Aerobic Oxidation of Alcohols to Acids0Lower-temperature bulk depolymerization of commercial polymethacrylates1Beyond Oxygen Evolution: Anodic High‐Value Conversion for Energy‐Saving Hydrogen and Chemical Co‐Production0Assessing biological degradation of non-hydrolysable synthetic polymers1

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