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RESEARCH PAPER · Progress in Polymer Science · 2023

Sustainable developments in polyolefin chemistry: Progress, challenges, and outlook

Xiaoyan Wang, Yanshan Gao, Yong Jin Tang

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Sustainable developments in polyolefin chemistry: Progress, challenges, and outlookOriginalSaBOX/Copper-Catalyzed Synthesis, Degradation, and Upcycling of a PMMA-Based Copolymer10Evolution of the Deformation‐ and Flow‐Induced Crystallization and Characterization of the Microstructure of a Single Spherulite, Lamella, and Chain of Isotactic Polypropylene31Precise activation of C–C bonds for recycling and upcycling of plastics81Polyethylene Materials Bearing In-chain Mechanophores1Achieving high molecular weight alternating copolymers of 1-octene with methyl acrylate via Lewis acid catalyzed copolymerization3Barbier polymerization towards synthesizing polar polyolefin analogues for polyolefin modification1Closed-loop recyclable polymers: from monomer and polymer design to the polymerization–depolymerization cycle106Degradable polyolefins prepared by integration of disulfides into metathesis polymerizations with 3,6-dihydro-1,2-dithiine9Electrochemical recycling of polymeric materials56Modern mechanistic approaches for the depolymerization of commodity plastics via organometallic catalysis0Polypropylene-based transesterification covalent adaptable networks with internal catalysis41Synthesis of ethylene copolymers with 2-allylphenol by using half-titanocene catalysts containing SiEt 3 -, Si i Pr 3 -substituted phenoxide ligands, Cp*TiCl 2 (O-2,6- i Pr 2 -4-SiR 3 -C 6 H 2 ) (R = Et, i Pr)9Transition metal-free decarboxylative olefination of carboxylic acid salts8Recyclable, Reprocessable, Anticorrosive, and Hydrolysis-Resistant Long-Chain Aliphatic Polycarbonates as Polyethylene-like Materials15Sustainable high-density polyethylene via chemical recycling: From modification to polymerization methods45Review on Catalytic Depolymerization of Polyolefin Waste by Hydrogenolysis: State-of-the-Art and Outlook57Sustainable degradation of synthetic plastics: A solution to rising environmental concerns19Circular olefin copolymers made de novo from ethylene and α-olefins83Modulating Thermal Conductivity and Flame Retardancy of Polyolefin Composites via Distributed Structures of Magnesium Hydroxide and Hexagonal Boron Nitride18Recyclable and (Bio)degradable Polyesters in a Circular Plastics Economy400Micelles Cascade Assembly to Tandem Porous Catalyst for Waste Plastics Upcycling3Micelles Cascade Assembly to Tandem Porous Catalyst for Waste Plastics Upcycling50Brønsted-acid sites induced photocatalytic cracking of low-polarity polyethylene plastics17Chemically recyclable rosin-based polymers10The Third Compound Promoted Copolymerization of Ethylene with 4‐Penten‐1‐ol by Using Metallocene Catalyst5Preparation of polyethylene/Siloxene nanocomposites through siloxene‐ MgCl supported Ziegler‐Natta catalyst4The third compound promoted ethylene homopolymerization and copolymerization with 1-octene by using metallocene catalyst3Polyethylene to gasoline via a self-supplied hydrogen strategy0Catalytic chemical recycling and upcycling of polyolefin plastics27Tailoring amino-functionalized cellulose separators for improved lithium-ion battery performance24Chemical upcycling of polyolefins into liquid refinery feedstock from the circularity and chemical engineering aspects11Degradation of a Wholly Aromatic Main-Chain Thermotropic Liquid-Crystalline Polymer Mediated by Superbases9Exploring ethylene insertion reaction mechanism in nickel complexes: a comparative study by the reaction force and reaction electronic flux in molecular and SiO2-supported catalysts1Preparation of High-Performance Polyethylene Nanocomposites with Oleic Acid–Siloxene-Supported Ziegler–Natta Catalysts2Transparent, Self-Healing, and Recyclable Biomass-Based Covalent Adaptable Networks Formed via Magnolol and Dynamic Boronate Ester7Et3Al and Et2Zn cooperatively enhanced Ti catalyzed ethylene coordinative chain transfer polymerization3New sustainable polymers with on-demand depolymerization property88One-Step Upcycling the Engineering Plastic of Polyoxymethylene toward a Flowing Telechelic Polyester: From Poly(A) to Poly(A-alt-B)4Upcycling of polyethylene/polypropylene mixtures promoted by well-controlled multiblock olefin copolymers20Factorial Analysis and Thermal Kinetics of Chemical Recycling of Poly(ethylene terephthalate) Aided by Neoteric Imidazolium-Based Ionic Liquids7Polyolefin vitrimers bearing acetoacetate functionality13Advancing H-Bonding Organocatalysis for Ring-Opening Polymerization: Intramolecular Activation of Initiator/Chain End22N2O deconstruction of polycyclooctene to generate carbonyl-functionalized macromonomers3p-Aryl-Substituted Iminopyridine Chromium Complexes as Precatalysts for Ethylene Polymerization: The Question of the Physical Oxidation State Examined by Experimental and Density Functional Study in the Absence of Structural Data1Cross-Linked Polyolefins: Opportunities for Fostering Circularity Throughout the Materials Lifecycle28Tailoring the Properties of Chemically Recyclable Polyethylene‐Like Multiblock Polymers by Modulating the Branch Structure32Tailoring the Properties of Chemically Recyclable Polyethylene‐Like Multiblock Polymers by Modulating the Branch Structure9Recent Advances in Propylene-Based Elastomers Polymerized by Homogeneous Catalysts6Catalytic Installation of Primary Amines Onto Polyolefins for Oligomer Valorization2Synthesis, Structure, and Actual Applications of Double Metal Cyanide Catalysts5Upcycling polyethylene into closed-loop recyclable polymers through titanosilicate catalyzed C-H oxidation and in-chain heteroatom insertion50Effect of intumescent flame retardants on the properties of poly(ethylene‐ co ‐vinyl acetate)/high‐density polyethylene blends9Photooxidation of Polyolefins to Produce Materials with In‐Chain Ketones and Improved Materials Properties2Photooxidation of Polyolefins to Produce Materials with In‐Chain Ketones and Improved Materials Properties32Heterocene Catalysts for Copolymerization of Hex-1-ene and Polar Vinyl Monomers5Extrudable and Highly Creep-Resistant Covalent Adaptable Networks Made from Polyethylene and Ethylene/1-Octene Copolymers by Reactive Processing with Aromatic Disulfide Cross-Links21Cationic polymerization of vinyl ethers using trifluoromethyl sulfonate/solvent/ligand to access well-controlled poly(vinyl ether)s6Gradient-temperature control enhances oxi-upcycling of polyethylene plastics to dicarboxylic acids over TS-1 zeolite14Recent Advancements in the Synthesis of Functional Polyolefins by Non-Bridged Half-Titanocenes11Binuclear Ni catalyzed ethylene copolymerization with short chain alkenol monomers9Commercially available sustainable additives0Efficient catalytic depolymerization of high-molecular-weight PMMA under low-temperature and high-concentration conditions10Oxidation upcycling of polyethylene into degradable, recyclable and high-performance materials4Recyclable Polypentenamers with Precise Crystallization and Versatile Functionalization15An Review of the Production of Polyolefins1Synthesis of Telechelic Isotactic Polypropylenes for Circular Polypropylene-like Materials via Chain Transfer Polymerization32Recyclable polyolefin-like materials with weakened all-carbon backbones1Mechanical and thermal properties of polylactic acid blended with recycled polymethyl methacrylate12Modulating Polyethylene Mimics with Degradability via Synthesis and Modeling22Self-assembly of phosphorus-containing ionic liquids on black phosphorus nanosheets for enhancing the fire safety of ethylene-vinyl acetate copolymers8Repurposing Post‐Consumer Polyethylene to Access Cross‐Linked Polyethylene with Reprocessability, Recyclability, and Tunable Properties18Repurposing Post‐Consumer Polyethylene to Access Cross‐Linked Polyethylene with Reprocessability, Recyclability, and Tunable Properties2Tailored synthesis of circular polyolefins27Advances in High-Temperature Non-Metallocene Catalysts for Polyolefin Elastomers4Polyolefin based Nano-Objects via ARGET ATRP mediated Polymerization-Induced Self-Assembly process6Crystallization, thermal, and mechanical properties of ethylene-propylene block copolymer/random copolymer blends1Advanced characterization of 3D printed polyolefin elastomer-carbon black composites: cyclic mechanical behavior, thermophysical properties, and morphological analysis3Polymer depolymerization, recycling, and high-value transformation: Charting a sustainable future for polymer science3Recycling reinvented: Converting PET bottle waste into 3D printable PCR polypropylene vitrimers for a sustainable future20Large-Scale Compatibilization of Postconsumer Polyolefins in the Presence of Paraffin Wax as a Rheology Modifier5Synthesis of Graft‐Modified Polyolefin Compatibilizers for Compatibilizing Mixed Plastics8Upcycling of Polyethylene through Sustainable Introduction of In-Chain Amides Using Zeolite Catalysis5Probing the Catalytic Degradation of Unsaturated Polyolefin Materials via Fe‐Based Lewis Acids‐Initiated Carbonyl–Olefin Metathesis18Probing the Catalytic Degradation of Unsaturated Polyolefin Materials via Fe‐Based Lewis Acids‐Initiated Carbonyl–Olefin Metathesis1Iron(III)‐Catalyzed C─H Hydroxylation of Low‐Density Polyethylene Coupled with Short Chain Branching Growth5Iron(III)‐Catalyzed C─H Hydroxylation of Low‐Density Polyethylene Coupled with Short Chain Branching Growth2Enhancing Polylactic Acid Properties by Blending With Recycled Polycarbonate: The Effect of a Bio‐Based Compatibilizer on Properties11Reprocessable Polypropylene Covalent Adaptable Networks via Free-Radical Reactive Processing with Vinyl Aromatic Additives15Synergistic Catalysis for Recycling and Upcycling of Plastics35Polyethyleneketones with Controlled Spacer Units: Synthesis, Characterization, and Photodegradation13A chemical method to upcycle waste polypropylene into bitumen compatible modifier by polyol grafting through reactive extrusion5UV-Induced Aging in Thermochromic Pigment-Integrated Food-Grade Polymers: A Performance Assessment2Compatibilized ternary blends of polypropylene copolymer, polyethylene, and thermoplastic polyurethane for fused deposition modeling three-dimensional printing technology: preparation, printing, and properties0Recent Advances in the Thermo-Catalytic Upcycling of Polyethylene Waste13Morphology‐Controlled Rheological and Non‐Isothermal Crystallization Behaviors in Immiscible Polypropylene/High Density Polyethylene Blends1Gradient Modulation of Ansa‐Metallocenes for Syndiotactic Propylene Polymerization: Multi‐Stage Remote Substituent Effects1Ethylene-propylene block copolymers featuring dual crystalline networks: high-performance elastomers and sustainable high-density polyethylene/isotactic polypropylene blends upcycling10Polyethylene Packaging as a Source of Microplastics: Current Knowledge and Future Directions on Food Contamination29Performance-Guided Design of Chemically Recyclable Polymeric Materials: A Case Study on Thermoplastic Elastomers9Intelligent Self-Healing Design of Conventional Polyolefin Materials8Block copolymer molecular design to address practical limitations to recycling polyolefin blends12Fully Recyclable and Remarkably Robust Cross-Linked Polyethylene Networks via Direct Free-Radical Copolymerization with Disulfide Dynamic Covalent Bonds19Enhancing Mechanical Properties and Crystallization Kinetics of Isotactic Polypropylene by Boronic Acid-Cross-Linked Additives3Synthesis of white carbon quantum dots for the upcycling of highly durable olefin plastics1Synthesis, Properties, and Metathesis Activity of Polyurethane Thermoplastics and Thermosets from a Renewable Polysesquiterpene Diol3Hafnium-Catalyzed Controlled Polymerization of 1,5-Hexadiene toward Polyolefin-Based Graft Copolymers for Poly(lactic Acid) Toughening with High Transparency4Degradable Polyketone Thermoplastic Elastomers with Biomass Sourced Composition3Degradable Polyketone Thermoplastic Elastomers with Biomass Sourced Composition3Propylene–Ethylene Copolymer Covalent Adaptable Networks Synthesized by Resonance‐Stabilized, Radical‐Based Reactive Processing with Excellent Elevated‐Temperature Creep Resistance6Stable single-site organonickel catalyst preferentially hydrogenolyses branched polyolefin C–C bonds12Linear Polyethylene with Ketone Groups for Photodegradability: Higher Efficiency with Side-Chain Carbonyls than In-Chain15Recent advances in transition metal-catalyzed ethylene/polar olefin copolymerization28Development of biodegradable polymer nonwoven using green solvents and their applications: a review6Upcycling Waste Polypropylene into Multifunctional Homogeneous Additives for Simultaneously Enhanced Mechanical Performance and Processability6Recyclable Biomass-Derived Polyethylene-like Plastics6Laser‐Driven Superfast‐Heating and Quenching Approach to Selectively Upcycle Waste Polyolefin into Long‐Chain Terminal Alkenes and Functionalization2Non-isocyanate route of biomimetic hierarchical hydrogen-bonding elastomers with solvent and temperature-assisted healability via structural functional region engineering for electronic skin applications2Main-Chain Ketone Installation in Polyethylene Chains: A Metal-Free Strategy toward Photodegradable Plastics18Sustainable polymers for battery applications7High-value recycling of polyamide 6 via formic acid solution2Compatibilization of Polyethylene and Polypropylene via Dynamic Cross-Linking163D-printed sustainable biocomposites via valorization of biomass: focus on challenges and their future perspectives5Mechanistic insight into Lewis acid coupling weak Brønsted base mediated removal of chlorine/hydrogen ions in polyolefin2Advances in sustainable polyolefins: synthesis, chemical transformation and recycling23Selective, Oxygen‐Tunable, and Metal‐Free Functionalization of Polyethylene Through Dual‐Mode Nitrosation and Carbonylation1Selective, Oxygen‐Tunable, and Metal‐Free Functionalization of Polyethylene Through Dual‐Mode Nitrosation and Carbonylation7Research progress on compatibilizers for physical blending recycling of polyolefins0Chemically recyclable, fully biobased polyolefins with performance parity to low-density polyethylene11Synthesis and Upcycling of All‐Carbon‐Backbone Degradable Polyethylene with Dispersed On‐Chain Ketones5Synthesis and Upcycling of All‐Carbon‐Backbone Degradable Polyethylene with Dispersed On‐Chain Ketones0Laser-induced pyrolysis of waste polyethylene to long-chain terminal alkenes and amphiphilic functionalization for anti-fouling film application0Free-Radical Emulsion Copolymerization of Ethylene and Butyl Acrylate Monomers: Synthesis, Properties, and Application0Thermodynamically driven closed-loop recyclable bridged polymers: from molecular design to high-performance materials0From inert carbon chains to closed-loop recycling: emerging polyolefin chemistry enabled by telechelic (macro)monomers0Efficiency and synergy of bis-urea anions for the polymerization of cyclic esters2Incorporating Carbamate Groups into Polyolefin Elastomers for High Performance and Closed-Loop Recyclability5Recent developments in recycling technologies for polymeric plastics8Nonbridged Half-titanocenes Modified with Anionic Ancillary Donor Ligands as Efficient Catalysts for Olefin Polymerization0A chemically recyclable thermosetting elastomer via ring-opening metathesis polymerization0Binuclear nickel catalysts enable one-step copolymerization of ethylene with 2-allylphenol to phenol-functionalized branched polyethylenes1Creep-resistant, extrudable, and recyclable polyolefin covalent adaptable networks incorporating azine cross-links via reactive processing3Embedding diazirine-based carbene precursors into polyolefins via catalyst-tuned olefin metathesis0Machine learning approaches to predicting metal catalyst performance in olefin polymerization0Recent advances in allylic and vinylic C–H bond functionalization of simple alkenes via visible-light photocatalysis2Recent Advances in Earth-Abundant Metal-Catalyzed Oxidative Degradation of Polyolefins0Selectively controlled ring-opening copolymerization to chemically recyclable thermoplastic elastomers1Synthesis of well-defined polyolefin graft copolymers based on single-site transition metal-mediated olefin polymerization0Synthesis of discrete oligoethylenes towards chemically recyclable polyolefins3Synthesis and characterization of nitrobenzyl carbonate (NBC)-based photodegradable amphiphilic polymers with temperature/pH/light-response2The role of biodegradable plastics in the global plastic future11

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