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RESEARCH PAPER · Nature Communications · 2024

Circular olefin copolymers made de novo from ethylene and α-olefins

Xing‐Wang Han, Xun Zhang, You‐Yun Zhou, Aizezi Maimaitiming, Xiu‐Li Sun, Yanshan Gao, Peizhi Li, Boyu Zhu, Eugene Y.‐X. Chen, Xiaokang Kuang, Yong Jin Tang

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Circular olefin copolymers made de novo from ethylene and α-olefinsOriginalHydrocracking of a HDPE/VGO Blend: Influence of Catalyst-to-Feed Ratio on Fuel Yield and Composition6Polyethylene to gasoline via a self-supplied hydrogen strategy0Catalytic chemical recycling and upcycling of polyolefin plastics27Et3Al and Et2Zn cooperatively enhanced Ti catalyzed ethylene coordinative chain transfer polymerization3New sustainable polymers with on-demand depolymerization property88Tailoring the Properties of Chemically Recyclable Polyethylene‐Like Multiblock Polymers by Modulating the Branch Structure32Tailoring the Properties of Chemically Recyclable Polyethylene‐Like Multiblock Polymers by Modulating the Branch Structure9Installing a Trigger to Upcycle High-Density Polyethylene42Biorenewable and circular polyolefin thermoplastic elastomers51Chemically recyclable polyvinyl chloride-like plastics24Alkyl polyglycosides derived from α-olefins via Fisher glycosidation and their adsorption and aggregation behavior in aqueous solution6Electrical and Dielectrical Properties of Composites Based on Alumina and Cyclic Olefin Copolymers3Preparation of bimodal polyethylene with different branching densities by a co-anchoring strategy4Synthesis and self-assembly of a diblock copolymer consisting of a cyclic olefin copolymer and polycaprolactone0Functional Polyolefins and Composites76Functional Polyolefins and Composites3Upcycling Polynorbornene Derivatives into Chemically Recyclable Multiblock Linear and Thermoset Plastics8Upcycling Polynorbornene Derivatives into Chemically Recyclable Multiblock Linear and Thermoset Plastics6Circularity in polydiketoenamine thermoplastics via control over reactive chain conformation4Monomer Design Enables Mechanistic Mapping of Anionic Ring‐Opening Polymerization of Aromatic Thionolactones9Monomer Design Enables Mechanistic Mapping of Anionic Ring‐Opening Polymerization of Aromatic Thionolactones2Synthesis of Telechelic Isotactic Polypropylenes for Circular Polypropylene-like Materials via Chain Transfer Polymerization32Well‐Controlled Block‐Type Cyclic Olefin Copolymers with High Heat Resistance, Outstanding Strength and Low‐Temperature Toughness14Tough and Closed‐Loop Recyclable Thermoplastic Elastomers From Sequential Ring‐Opening Copolymerization of Bio‐Renewable β‐Methyl‐δ‐Valerolactone and δ‐Valerolactone12Enhanced hydrodeoxygenation of biomass-derived polyols to light alkanes over boron oxide modified nickel silicate catalysts3Catalytic closed-loop recycling of polyethylene-like materials produced by acceptorless dehydrogenative polymerization of bio-derived diols45Accessing Degradable Polyethylene Materials with In-chain Ester Units via Mechanochemical Backbone Editing9Repurposing Post‐Consumer Polyethylene to Access Cross‐Linked Polyethylene with Reprocessability, Recyclability, and Tunable Properties18Repurposing Post‐Consumer Polyethylene to Access Cross‐Linked Polyethylene with Reprocessability, Recyclability, and Tunable Properties2Tailored synthesis of circular polyolefins27High Molecular Weight Biobased Long-Chain Aliphatic Polyesters with Degradability: Insights into Mimicking Polyethylene24Synthesis of Graft‐Modified Polyolefin Compatibilizers for Compatibilizing Mixed Plastics8Lewis Acid Promoted Radical Alternating Polymerization of Simple and Higher α-Olefins with Maleic Anhydride1Polar Functionalization of Polyalphaolefin Lubricants and Polyisobutylenes by Cationic Copolymerization from Ionic Cluster-Type Polar Monomers1Performance-Guided Design of Chemically Recyclable Polymeric Materials: A Case Study on Thermoplastic Elastomers9Recyclable Cross-Linked Polyethylene from Self-Condensing Telechelic Polyethylene by Combining Olefin Metathesis, Hydrogenation, and Transesterification4Sustainable and Orthogonally Closed-Loop Recyclable Acetal-Based Long-Chain Polyesters19Facile Synthesis of Polyhydroperoxides from Ethylene and Carbon Monoxide10Polyethylene-like Polyesters: Strategies for Tailoring Mechanical Properties and Adhesion Performance6High-Molecular-Weight Polyesters Mimicking Linear Low-Density Polyethylene: Mechanistic Insight and Structure–Property Relationship1High‐Density Polyethylenes with Dual Degradability Enabled by In‐Chain Photolyzable and Mechanoresponsive Units6Sulfur Treatment of Coordinative Chain Transfer Polymerization Products for Extending Polyolefin Chains with Polysulfide Linkages3Chemically Recyclable and Tunable Polyolefin‐Like Multiblock Copolymer Adhesives2Chemically Recyclable and Tunable Polyolefin‐Like Multiblock Copolymer Adhesives13Recyclable Biomass-Derived Polyethylene-like Plastics6Precision Oligomeric Building Blocks toward Chemically Recyclable Polyolefin-like Materials4Advances in sustainable polyolefins: synthesis, chemical transformation and recycling23Chemically recyclable, fully biobased polyolefins with performance parity to low-density polyethylene11A Constrained Structural Symmetry Strategy for Nickel-Catalyzed Olefin Polymerization and Copolymerization with Polar Monomers19Efficient Product Regulation of CO 2 Hydrogenation over an Intelligent Dual-Zeolite System6Research progress on polyester chemical recycling and industrialization0Synthesis of linear multi-block copolymers and their application in plastic recycling and modification0From inert carbon chains to closed-loop recycling: emerging polyolefin chemistry enabled by telechelic (macro)monomers0Vinylsilanes as Chain-Transfer Agents in Ethylene Polymerization: Direct Synthesis of Heterotelechelic Polyolefins3Incorporating Carbamate Groups into Polyolefin Elastomers for High Performance and Closed-Loop Recyclability5Degradable polyethylene-like materials1Dual-functional upgrading of high-molecular-weight random styrene–butadiene rubber (rSBR): cyclic optical films and degradable adhesives0Selectively controlled ring-opening copolymerization to chemically recyclable thermoplastic elastomers1Synthesis of discrete oligoethylenes towards chemically recyclable polyolefins3Alkyl Alcohol Chain-length Mediated Steric Hindrance at Support Surface in Heterogeneous α-Diimine Ni Catalysts for Modulating Ethylene Polymerization2Super-Tough and Resilient Recyclable Polyester Elastomers Enabled by Dynamic Cross-Linking3Mechanically driven hybrid recycling of polyolefin elastomer glass–glass photovoltaic module for targeted material recovery2All-Hydrocarbon Polymers with Chemical Recyclability via a Catalyst-Free and Solvent-Free Method1High-Performance and Closed-Loop Recyclable Thermoplastic Elastomers from Sequential Ring-Opening Copolymerization of Biobased β-Methyl-δ-valerolactone and p -Dioxanone1Thermo-chemical upgrading of waste polyethylene and polypropylene plastics0Upcycling and Redesigning of Polyolefins3Chemically Recyclable Thermoplastic Elastomers: Preparation, Properties, and On-Demand Depolymerization0Precise Structural Design for Chemically Recyclable Polymers1Bimodal Polyethylenes Synthesized by Flexible Fluorinated “Sandwich” α‐Diimine Nickel( II ) Catalysts0Chemically Recyclable Polyester Miscible with HDPE Transforms Contamination into Functional Enhancement0Accessing Degradable Polyethylenes via Catalytic Ethylene Copolymerization1A tutorial review on designing pluripotent olefinic hybrids via covalent adaptable networks: integrating dynamic chemistry with machine‑learning0From Molecular Defect to Macroscopic Performance: Manipulating Dichroism and Mechanics in Iodine-doped Poly(vinyl alcohol) via Ethylene Incorporation1Mechanistic Insights into Comonomer Effects on Propylene Polymerization over TiCl3 Catalysts0Repetitive Ethylene Insertion into the Pd–OAc Bond: Synthesis of Heterotelechelic Polyethylene and Effective Copolymerization of Ethylene with Vinyl or Allyl Acetate0Enhancing asphalt performance through chemical crosslinking of olefin block copolymers0Synergistic d-π Conjugation and Thermal Stability Enable Efficient High-Temperature Photoinduced Olefin Polymerization in Metallocene–Organic Semiconductor Hybrids0Facile Synthesis of α,ω‐Dihydroxy Telechelic Macromonomers From Ethylene and α‐Olefins for Recyclable Alternating Block Copolymers0Facile Synthesis of α,ω‐Dihydroxy Telechelic Macromonomers From Ethylene and α‐Olefins for Recyclable Alternating Block Copolymers0Mapping the multidimensional structure–property landscape of polyolefin elastomers with interpretable machine learning0Characterisation of the mechanical performance of a novel thermoplastic film adhesive0

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  3. Catalytic chemical recycling and upcycling of polyolefin plastics

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  8. Installing a Trigger to Upcycle High-Density Polyethylene

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  19. Circularity in polydiketoenamine thermoplastics via control over reactive chain conformation

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  22. Synthesis of Telechelic Isotactic Polypropylenes for Circular Polypropylene-like Materials via Chain Transfer Polymerization

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  23. Well‐Controlled Block‐Type Cyclic Olefin Copolymers with High Heat Resistance, Outstanding Strength and Low‐Temperature Toughness

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