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RESEARCH PAPER · Angewandte Chemie International Edition · 2024

Pyrolytic Depolymerization of Polyolefins Catalysed by Zirconium‐based UiO‐66 Metal–Organic Frameworks

Jerry Zhi Xiong Heng, Tristan Tsai Yuan Tan, Xin Li, Wei Wei Loh, Yuting Chen, Zhenxiang Xing, Zhiyan Lim, Jennet Li Ying Ong, Katherine Shiyun Lin, Yusuke Nishiyama, Takefumi Yoshida, Lili Zhang, Ken‐ichi Otake, Susumu Kitagawa, Xian Jun Loh, Enyi Ye, Jason Y. C. Lim

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Pyrolytic Depolymerization of Polyolefins Catalysed by Zirconium‐based UiO‐66 Metal–Organic FrameworksOriginalHydrogenolysis of Polyethylene by Metal–Organic Framework Confined Single-Site Ruthenium Catalysts16Low‐Temperature Catalytic Approaches for Upcycling Plastics into Oxygenated Aromatic Compounds14Recent Advances in Transition Metal‐Based Metal‐Organic Frameworks for Hydrogen Production25Engineering porous Beta zeolite-encapsulated nickel catalyst for waste polyolefins upcycling26Zero- to One-Dimensional Transformation in a Highly Porous Metal–Organic Framework to Enhance Physicochemical Properties20Mesopore matters: Hierarchically porous metal–organic framework with facilitated redox-hopping and electrochemical behaviors toward the use in supercapacitors11Trace solvents-assisted mechanochemistry of waste poly(ethylene terephthalate) into MIL-53Al for efficient hydroelectricity generation25The Facile Construction of Defect-Engineered and Surface-Modified UiO-66 MOFs for Promising Oxidative Desulfurization Performance5P-modulated NiP active centers and PNC support enabling synergistic H2/H2O activation in cellulose cascade conversion1Catalytic Depolymerization of Plastics to Valuable Products7Acidic Site-Controlled ZSM-5 Catalysts for Fast Molten-Phase Pyrolysis of Plastic Waste with Tunable Product Distribution4Laser‐Driven Superfast‐Heating and Quenching Approach to Selectively Upcycle Waste Polyolefin into Long‐Chain Terminal Alkenes and Functionalization2Plasma Catalysis for Plastic Waste Conversion into Value‐Added Products: Advancements and Perspectives11Solvent swelling-induced microstructural modulation of polypropylene for targeted pyrolysis: Product distribution and pyrolysis mechanisms explored through experimental and DFT investigations2Optimization of Fenton-like-driven waste plastic upgrading processes: Trade-off strategies between environmental and techno-economic benefits1Research progress in metal-zeolite bifunctional systems for upcycling of waste polyolefins3Dual advantages of rapid zeolite channel diffusion and Ni sites: 1Ni/L-DAl zeolite enables efficient polyolefin hydrocracking to liquid fuel1Synergistic defect engineering and interfacial regulation in amphiphilic cerium-based metal–organic frameworks for efficient heavy oil upgrading1Mechanistic Pathways and Product Selectivity in Pyrolysis of PE, PP and PVC: A Foundation for Applied Chemistry in Europe12Current perspective on heterogeneous thermal catalytic approaches for closed-loop polyolefin plastic recycling1Machine‐Learning‐Driven Design of Dynamically Adaptive MOF Catalysts: Structural Evolution Mechanisms and Industrial Translation Pathways in Seawater Electrolysis30Hydrolyzable Graft Copolymers with In-Chain Esters from Polyethylene via Oxidative Chlorination1Cleavage Alkylation Coupling with Versatile Amide-Based Eutectic Catalytic Systems0Surfactant-Directed Synthesis of UiO-66-(OH) 2 Nanosheets for Efficient Phosphatase-like Catalysis1Site-selective dehydrogenation and protonation synergy for efficient polyolefin upcycling into aromatics0Controlled Pyrolysis of Polystyrene Using Metal–Organic Frameworks4Modulation of Ni species distribution and hydrogenation performance of Ni/UiO-66 catalysts0A Panoramic View on Plastic Waste Recycling and Upcycling: Heterogeneous Catalytic Strategies for Diverse Plastics and Multiple Pathways6Low‐Temperature in Situ Upgrading of Ultra‐Deep Heavy Oil Using Ni–Ce/MOF–OTf Superacid Catalysts to Enhance Energy Utilization and Sustainability0Controlling Polyolefin Hydrogenolysis Selectivity by Engineering Single-Site Nickel(II) Hydride Active Catalytic Species0In Situ Grown UiO‐66‐NH 2 on Nanocellulose Aerogels for Gas Capture0Zirconium-Based Metal–Organic Framework Thin Films with Large Mesopores for Amplifying Electrochemical Sensing Response toward Dopamine1Healable and Post‐Programmable Metal–Organic Framework—Vitrimer Composites0Recent advances in catalytic technologies for plastic conversion: a review0Emerging Catalytic Platforms for Plastic Waste Recycling and Upcycling Over MOFs and COFs: Catalyst Engineering and Reaction Mechanisms0Fe3 +-induced interfacial electronic effects in UiO-66 for enhanced electrocatalytic nitrate-to-ammonia conversion0Current Advances and Prospects in Europium Wastewater Treatment: Health-environmental Issues, Innovative Technologies, and Composite-based Solutions0Ru Single‐Atom Anchored Zeolite for Selective Upcycling of Polyolefins Into Butanes0

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  1. Hydrogenolysis of Polyethylene by Metal–Organic Framework Confined Single-Site Ruthenium Catalysts

    Chemistry of Materials · 2024-10-24

    Manav Chauhan, Chhaya Thadhani, Bharti Rana, Poorvi Gupta, Biplab Ghosh, Kuntal Manna

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  2. Low‐Temperature Catalytic Approaches for Upcycling Plastics into Oxygenated Aromatic Compounds

    ChemCatChem · 2024-11-19

    Jason Y. C. Lim

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  3. Recent Advances in Transition Metal‐Based Metal‐Organic Frameworks for Hydrogen Production

    Small Science · 2025-02-17

    Ting Yang, Hua Zhang, Bo Pang, Jonathan W.C. Wong

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  4. Engineering porous Beta zeolite-encapsulated nickel catalyst for waste polyolefins upcycling

    Applied Catalysis B: Environmental · 2025-04-08

    Jiahui Zhan, Lin Li, Ruihong Dai, Baohuan Wei, Hu Luo, Rongfei Cong, Haozhi Zhou, Lin Xia, Xiaofang Liu, Shunan Zhang, Shunan Zhang, Shicheng Zhang, Shicheng Zhang, Hui Wang, Yuhan Sun

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  5. Zero- to One-Dimensional Transformation in a Highly Porous Metal–Organic Framework to Enhance Physicochemical Properties

    Journal of the American Chemical Society · 2025-05-07

    Enhui Jiang, Daisong Chen, Zhuoliang Ying, Jiaming Zhou, Artit Jarusarunchai, Xinyu Zhang, Chenxi Xiong, Keunhong Jeong, Dong‐Myeong Shin, Jin Shang, Seungkyu Lee

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  6. Mesopore matters: Hierarchically porous metal–organic framework with facilitated redox-hopping and electrochemical behaviors toward the use in supercapacitors

    Electrochimica Acta · 2025-05-13

    Tzu-Hsien Yang, Chi-Lun Chuang, Yu-Chi Wang, Ya-Mei Weng, Cheng-Yan Hsieh, Hsin-Ya Tsai, Kuan-Chu Wu, Cheng‐Hui Shen, Chung‐Wei Kung

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  7. Trace solvents-assisted mechanochemistry of waste poly(ethylene terephthalate) into MIL-53Al for efficient hydroelectricity generation

    Chemical Engineering Journal · 2025-05-17

    Yan She, Weikang Han, Huajian Liu, Guixin Hu, Huiyue Wang, Xueying Wen, Lijie Liu, Lingling Feng, Xinyao Zhang, Jiang Gong

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  8. The Facile Construction of Defect-Engineered and Surface-Modified UiO-66 MOFs for Promising Oxidative Desulfurization Performance

    Nanomaterials · 2025-06-15

    Chao Wang, Junchao Ding, Haoyu Wu, Jiaxuan Zhang, Feng Xu, Ying Zhang, Ming Ma, Ming Zhang, Hongping Li

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  9. P-modulated NiP active centers and PNC support enabling synergistic H2/H2O activation in cellulose cascade conversion

    Applied Catalysis B: Environmental · 2025-08-18

    Yixin Luo, Rui Ma, Chengjie Sun, Ting Yu, Haoxuan Yan, Xiaomei Zhou, Qingxin Guan, Mo Qiu, Wei Li

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  10. Catalytic Depolymerization of Plastics to Valuable Products

    ChemCatChem · 2025-09-07

    Li Zhao, Bing Liu, Teng He, Ping Chen

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  11. Acidic Site-Controlled ZSM-5 Catalysts for Fast Molten-Phase Pyrolysis of Plastic Waste with Tunable Product Distribution

    Energy & Fuels · 2025-09-11

    Wei Xiong, Ruilong Zhang, Christina H. M. Tsang, Yuehan Jiang, Xinxin Lu, Yuchao Shao, Jun Liang Zhao

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  12. Laser‐Driven Superfast‐Heating and Quenching Approach to Selectively Upcycle Waste Polyolefin into Long‐Chain Terminal Alkenes and Functionalization

    Advanced Functional Materials · 2025-09-14

    Lun Chen, Fu‐Lu Chang, Guangjian He, Haoqin Zhang, Chunyan Wang, Jinping Qu

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  13. Plasma Catalysis for Plastic Waste Conversion into Value‐Added Products: Advancements and Perspectives

    Advanced Functional Materials · 2025-11-10

    Yanan Diao, Xuetao Qin, Chengxin Hou, Bingbing Chen, Tianqi Yun, Xinwen Guo, Ding Ma, Chuan Shi

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  14. Solvent swelling-induced microstructural modulation of polypropylene for targeted pyrolysis: Product distribution and pyrolysis mechanisms explored through experimental and DFT investigations

    Fuel · 2025-11-20

    Shanglong Zhang, Qiuxiang Yao, Yongliang Wang, Wei Wang, Lei He, Linyang Wang, Ming Sun

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  15. Optimization of Fenton-like-driven waste plastic upgrading processes: Trade-off strategies between environmental and techno-economic benefits

    Chinese Chemical Letters · 2025-12-08

    Guanyi Chen, Xu Chang, Rui Wang, Xiaoming Peng, Zhanjun Cheng, Beibei Yan, Ning Li

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  16. Research progress in metal-zeolite bifunctional systems for upcycling of waste polyolefins

    Journal of Analytical and Applied Pyrolysis · 2025-12-17

    Wei Qiang, Kangzhou Wang, Wenlong Song, Tong Liu, Yongjun Jiang, Weijie Zhang, Chenlong Huang, Xiaowei Li, Jianli Zhang

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  17. Dual advantages of rapid zeolite channel diffusion and Ni sites: 1Ni/L-DAl zeolite enables efficient polyolefin hydrocracking to liquid fuel

    Green Chemistry · 2026-01-01

    Hongyu Fu, Huibin Liu, Abulikemu Abulizi, Kenji Okitsu, Yasuaki Maeda, Tiezhen Ren, Aisha Nulahong, Changhai Liang

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  18. Synergistic defect engineering and interfacial regulation in amphiphilic cerium-based metal–organic frameworks for efficient heavy oil upgrading

    Journal of Materials Chemistry A · 2026-01-01

    Li Wang, Ji-Xiang Guo, Kunpeng Li, Qiming Huang, Chi Li, Yajie Wu

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  19. Mechanistic Pathways and Product Selectivity in Pyrolysis of PE, PP and PVC: A Foundation for Applied Chemistry in Europe

    Molecules · 2026-01-06

    Tim Tetičkovič, Dušan Klinar, Klavdija Rižnar, Darja Pečar

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  20. Current perspective on heterogeneous thermal catalytic approaches for closed-loop polyolefin plastic recycling

    Discover Chemistry. · 2026-01-20

    Haokun Wang, Dermot O’Hare

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  21. Machine‐Learning‐Driven Design of Dynamically Adaptive MOF Catalysts: Structural Evolution Mechanisms and Industrial Translation Pathways in Seawater Electrolysis

    Advanced Energy Materials · 2026-02-18

    Tengyu Gui, Yuchen Wang, Jin Li, Zhongyuan Qiao, Zhu Lian Wu, Yawen Sheng, Longchao Zhuo, Yinghong Wu, Imran Shakir, Xiujuan Wu, Ligang Feng, Xuping Sun, Xijun Liu

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  22. Hydrolyzable Graft Copolymers with In-Chain Esters from Polyethylene via Oxidative Chlorination

    ACS Materials Letters · 2026-03-02

    Jaime J. M. Pang, Albert Ong, Wei Wei Loh, J H S Teo, Debbie Hwee Leng Seng, Lewis Queh, Li Zibiao, Jason Y. C. Lim

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  23. Cleavage Alkylation Coupling with Versatile Amide-Based Eutectic Catalytic Systems

    Journal of the American Chemical Society · 2026-03-04

    Jisheng Yu, Di Zhu, Jianguo Zhuang, Y. Hugh Guan, Yuxin Qiu, Xue Wang, Xin Gao, G. Chen, Zhen Song, Xuedong Zhu, D. Chen

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  24. Surfactant-Directed Synthesis of UiO-66-(OH) 2 Nanosheets for Efficient Phosphatase-like Catalysis

    ACS Applied Nano Materials · 2026-03-18

    Xin Xiang, Jiadong Wang, Dongdong Xu, Zhihui H. Dai

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  25. Site-selective dehydrogenation and protonation synergy for efficient polyolefin upcycling into aromatics

    Chemical Engineering Journal · 2026-04-03

    Yusong Zhang, Yue Ding, Lei Zhang, Guozhao Ji, Yuan Gao, Aimin Li

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  26. Controlled Pyrolysis of Polystyrene Using Metal–Organic Frameworks

    Journal of the American Chemical Society · 2026-04-15

    Haruma Tatsumi, Ami Nishijima, Joseph C. A. Prentice, Takashi Uemura

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  27. Modulation of Ni species distribution and hydrogenation performance of Ni/UiO-66 catalysts

    Microporous and Mesoporous Materials · 2026-05-04

    Gui Li, Ziyun Wang, Hao Wang, Zhaoyuan Hu, Xuecheng Liu, Lidan Deng

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  28. A Panoramic View on Plastic Waste Recycling and Upcycling: Heterogeneous Catalytic Strategies for Diverse Plastics and Multiple Pathways

    Advanced Materials · 2026-05-12

    Chang‐Jie Yang, Xin-Yu Wang, Mei‐Qi Zhu, Tianyou Zhao, Yong-Zhou Pan, Yuhai Dou, Jie Yang, Zechao C. Zhuang, Zhenglong Li, Zhijun Wu, Wen‐Gang Cui, Hongge Pan, Weiwei Li, Dingsheng S. Wang

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  29. Low‐Temperature in Situ Upgrading of Ultra‐Deep Heavy Oil Using Ni–Ce/MOF–OTf Superacid Catalysts to Enhance Energy Utilization and Sustainability

    EcoEnergy · 2026-05-23

    Li Wang, Ji-Xiang Guo, Qiming Huang, Kunpeng Li, Chi Li, Yajie Wu

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  30. Controlling Polyolefin Hydrogenolysis Selectivity by Engineering Single-Site Nickel(II) Hydride Active Catalytic Species

    ACS Catalysis · 2026-06-08

    Bharti Rana, Manav Chauhan, Poorvi Gupta, A Rajendra Kumar, Chhaya Thadhani, Rahul Kalita, Kuntal Manna

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  31. In Situ Grown UiO‐66‐NH 2 on Nanocellulose Aerogels for Gas Capture

    High Voltage · 2026-06-11

    Hongsong Lian, Jin Huang, Yonghua Lai, Huixin Liu, Dongsheng Zheng, Han Dong, W T Zhang, Hongye Yuan

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  32. Zirconium-Based Metal–Organic Framework Thin Films with Large Mesopores for Amplifying Electrochemical Sensing Response toward Dopamine

    ACS Applied Nano Materials · 2026-06-25

    Yin-Chu Tai, Cheng-Yan Hsieh, Hsin-Ya Tsai, Chi-Lun Chuang, Chou-Hung Hsueh, Tsan-Yu Chuang, Tzu-Chi Lin, Jia-Rui Zhang, Chung‐Wei Kung

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  33. Healable and Post‐Programmable Metal–Organic Framework—Vitrimer Composites

    Advanced Materials · 2026-07-25

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  34. Recent advances in catalytic technologies for plastic conversion: a review

    Journal of Materials Science · 2026-08-05

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  35. Emerging Catalytic Platforms for Plastic Waste Recycling and Upcycling Over MOFs and COFs: Catalyst Engineering and Reaction Mechanisms

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  36. Fe3 +-induced interfacial electronic effects in UiO-66 for enhanced electrocatalytic nitrate-to-ammonia conversion

    Applied Catalysis B: Environmental · 2026-09-12

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  37. Current Advances and Prospects in Europium Wastewater Treatment: Health-environmental Issues, Innovative Technologies, and Composite-based Solutions

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  38. Ru Single‐Atom Anchored Zeolite for Selective Upcycling of Polyolefins Into Butanes

    Angewandte Chemie International Edition · 2026-09-15

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