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RESEARCH PAPER · Angewandte Chemie International Edition · 2025

Advances and Challenges in Low‐Temperature Upcycling of Waste Polyolefins via Tandem Catalysis

Wei Zhang, Sung Min Kim, Michele L. Sarazen, Mingyuan He, Jingguang G. Chen, Johannes A. Lercher

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Advances and Challenges in Low‐Temperature Upcycling of Waste Polyolefins via Tandem CatalysisOriginalSynergistic Catalysis for Recycling and Upcycling of Plastics35Beyond Hydroconversion: A Paradigm Shift for Sustainable Plastic Waste Upcycling9Integrated low-temperature PVC and polyolefin upgrading38One-Step Compatibilization and Upcycling of Mixed Polyolefins Using a Dynamic Disulfide-Linked Bismaleimide Cross-Linker7Plasma Catalysis for Plastic Waste Conversion into Value‐Added Products: Advancements and Perspectives11Catalytic valorization of polyolefins: from catalysts and processes to reactors0Circular economy in polystyrene photodegradation to valuable chemicals0Mild‐Condition Upcycling of Polyolefins Enabled by Micropore Confinement in Zeolites3Mild‐Condition Upcycling of Polyolefins Enabled by Micropore Confinement in Zeolites5Acid sites in hydrogen-involved polyolefin upcycling: mechanistic insights and design principles0Tandem hydropyrolysis–hydrogenolysis of polyolefin wastes over morphology‐tuned Co 3 O 4 for jet‐fuel hydrocarbons0Chemical recycling of polystyrene via pyrolysis and hydrocracking for high-value light aromatics3Catalytic Upcycling of Polyolefins and Polystyrene: Integrating Active Site Design With Mass Transfer Considerations4Valorization of waste polyolefins to butene, unsaturated fatty alcohols, and branched alkenes using CO2 and plasma catalyst2Effect of Radical Initiators on Polypropylene Thermal Deconstruction0Light‐Driven Coupled Upcycling of Polyethylene and CO 2 to Aromatics over Zeolite–Ni/CeO 2 Composite Catalysts0Solvent-free chemical recycling of polyolefins and polystyrene under mild conditions via GaCl3-based molten catalysts0Selective Oxidative Upcycling of Polyethylene Pyrolyzed Wax to High‐Performance Surfactants Using Synthesized Co and Mn–Co Stearate Catalysts0Upgrading Polyolefin Plastics Into Ethanol Using an Integrated Hydrothermal‐Photoelectrocatalytic Strategy0Next-Generation Waste Degradation and Valorization Processes: Engineering Challenges and Process Intensification0Ambient‐Pressure Polyolefin Upcycling With Earth‐Abundant Catalyst0Ambient‐Pressure Polyolefin Upcycling With Earth‐Abundant Catalyst0Mechanochemical AlCl3-Catalyzed Cracking of Waste Polyolefins and Synthetic Rubbers into Liquid Fuel0Hierarchical Accessibility and Framework‐Al Organization in Ultra‐High‐Silica ZSM‐5 Enable Efficient Cracking of Polyolefin Waste to Light Olefins0

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24 direct citing papers saved.

  1. Synergistic Catalysis for Recycling and Upcycling of Plastics

    ACS Catalysis · 2025-05-07

    Hongshun Ran, Xinyang Sun, Mengying Zheng, Yaxuan Jing

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  2. Beyond Hydroconversion: A Paradigm Shift for Sustainable Plastic Waste Upcycling

    ACS Sustainable Chemistry & Engineering · 2025-06-16

    Haokun Wang, Yiyang Li, Shik Chi Edman Tsang

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  3. Integrated low-temperature PVC and polyolefin upgrading

    Science · 2025-08-14

    Wei Zhang, Boda Yang, Benjamin A. Jackson, Junbo Zhao, Honghong Shi, Donald M. Camaioni, Sung Min Kim, Huamin Wang, János Szanyi, Mal‐Soon Lee, Jingguang G. Chen, Johannes A. Lercher

    Read original paper ↗ ·

  4. One-Step Compatibilization and Upcycling of Mixed Polyolefins Using a Dynamic Disulfide-Linked Bismaleimide Cross-Linker

    Industrial & Engineering Chemistry Research · 2025-11-10

    Yongjun Zhu, Ce Wei, Lingyan Kong, Xuhui Zhang, Ting Li, Yang Wang, Jing Huang, Weifu Dong

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  5. Plasma Catalysis for Plastic Waste Conversion into Value‐Added Products: Advancements and Perspectives

    Advanced Functional Materials · 2025-11-10

    Yanan Diao, Xuetao Qin, Chengxin Hou, Bingbing Chen, Tianqi Yun, Xinwen Guo, Ding Ma, Chuan Shi

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  6. Catalytic valorization of polyolefins: from catalysts and processes to reactors

    Chemical Society Reviews · 2026-01-01

    Cuncun Wu, Chaojie Guo, Xinquan Xu, Kun Liu, Lu Bai, Nan Yang, Donglong Fu, Jinlong Gong

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  7. Circular economy in polystyrene photodegradation to valuable chemicals

    Chemical Communications · 2026-01-01

    Chitra Sarkar, Solanki Chowdhury, Ratul Paul, Asim Bhaumik

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  8. Mild‐Condition Upcycling of Polyolefins Enabled by Micropore Confinement in Zeolites

    Angewandte Chemie · 2026-01-21

    Zhuohan Lin, Tingjun Gu, Wenbo Li, Fei Lin, Wang Xu, Lihui Zhou, Sheng Dai, Yan Li

    Read original paper ↗ ·

  9. Mild‐Condition Upcycling of Polyolefins Enabled by Micropore Confinement in Zeolites

    Angewandte Chemie International Edition · 2026-01-21

    Zhuohan Lin, Tingjun Gu, Wenbo Li, Fei Lin, Wang Xu, Lihui Zhou, Sheng Dai, Yan Li

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  10. Acid sites in hydrogen-involved polyolefin upcycling: mechanistic insights and design principles

    Science China Chemistry · 2026-01-27

    Qi Zhang, Xiang Wang

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  11. Tandem hydropyrolysis–hydrogenolysis of polyolefin wastes over morphology‐tuned Co 3 O 4 for jet‐fuel hydrocarbons

    AIChE Journal · 2026-02-05

    Dongxian Li, Xiaocao Shan, Xianzhi Meng, Jia Wang, Jianchun Jiang, Arthur J. Ragauskas

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  12. Chemical recycling of polystyrene via pyrolysis and hydrocracking for high-value light aromatics

    Chemical Engineering Journal · 2026-03-27

    Kyutae Kim, Seoyeong Park, Jaecheol Jeong, Jinho Oh, Jeonghwan Seo, Yong-Kul Lee, Jung Kyoo Lee

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  13. Catalytic Upcycling of Polyolefins and Polystyrene: Integrating Active Site Design With Mass Transfer Considerations

    ChemSusChem · 2026-03-29

    Xinlei Han, Jie Sun, Jiuxuan Zhang, Zhengyan Qu, Hong Jiang, Zhenchen Tang, Rui Chen

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  14. Valorization of waste polyolefins to butene, unsaturated fatty alcohols, and branched alkenes using CO2 and plasma catalyst

    Journal of Cleaner Production · 2026-03-31

    S. Uday, Xianglan Bai

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  15. Effect of Radical Initiators on Polypropylene Thermal Deconstruction

    Industrial & Engineering Chemistry Research · 2026-04-19

    Diana García Pérez, Roshaan Surendhran, Nikolas M. Angyal, Alex H. Balzer, Charles C Fields, Raúl F. Lobo

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  16. Light‐Driven Coupled Upcycling of Polyethylene and CO 2 to Aromatics over Zeolite–Ni/CeO 2 Composite Catalysts

    ChemSusChem · 2026-06-13

    Weiwei Li, Q Feng, Zhiyi Wu, Yuxuan Zhou, Jiahui Shen, Yihe Huang, Xiaohan Jin, Liu Cao, Kai Ming Feng, Xingda An, Ning Zhang, Chaoran Li, Le He

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  17. Solvent-free chemical recycling of polyolefins and polystyrene under mild conditions via GaCl3-based molten catalysts

    CHINESE JOURNAL OF CATALYSIS (CHINESE VERSION) · 2026-07-01

    Lei Yuan, Zhiwen Gao, Libin Shi, Cuishi Guan, Dongyue Peng, Shuhui Fang, Wei Zhang, Y Liu

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  18. Selective Oxidative Upcycling of Polyethylene Pyrolyzed Wax to High‐Performance Surfactants Using Synthesized Co and Mn–Co Stearate Catalysts

    Advanced Sustainable Systems · 2026-08-01

    Abdul Aziz Jallow, Usman Bello, Muhammad Faizan, Roa'a H. Alzoubi, Maryem Ourimi, Abdul Gani Abdul Jameel, Usama Ahmed, Mohammad Nahid Siddiqui

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  19. Upgrading Polyolefin Plastics Into Ethanol Using an Integrated Hydrothermal‐Photoelectrocatalytic Strategy

    ChemCatChem · 2026-08-01

    Xiang Gao, Longfei Hong, Yuting Jiang, Yixuan Li, Lian-Hua Xu, Qingyu Liu, Huiyan Zhang, Sheng Chu

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  20. Next-Generation Waste Degradation and Valorization Processes: Engineering Challenges and Process Intensification

    Processes · 2026-09-02

    Ho‐Shing Wu

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  21. Ambient‐Pressure Polyolefin Upcycling With Earth‐Abundant Catalyst

    Angewandte Chemie · 2026-09-07

    Qianyue Feng, Mingyu Chu, Zhongyu Li, Yeping Xie, Qiao Zhang, Jinxing Chen, Ding Ma

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  22. Ambient‐Pressure Polyolefin Upcycling With Earth‐Abundant Catalyst

    Angewandte Chemie International Edition · 2026-09-07

    Qianyue Feng, Mingyu Chu, Zhongyu Li, Yeping Xie, Qiao Zhang, Jinxing Chen, Ding Ma

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  23. Mechanochemical AlCl3-Catalyzed Cracking of Waste Polyolefins and Synthetic Rubbers into Liquid Fuel

    ACS Sustainable Chemistry & Engineering · 2026-09-07

    Xiaojuan Zhao, Lizheng Chen, Wenjuan Zhang, Gang Liu, Dayang Wang

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  24. Hierarchical Accessibility and Framework‐Al Organization in Ultra‐High‐Silica ZSM‐5 Enable Efficient Cracking of Polyolefin Waste to Light Olefins

    Angewandte Chemie International Edition · 2026-09-23

    Wang Xu, Jingyue Hu, Juan Liu, Zhuohan Lin, Qiaohui Ruan, Xianrui Meng, Yan Li

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