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RESEARCH PAPER · Chemical Reviews · 2024

Catalytic Upcycling of Polyolefins

Jia‐Kai Sun, Jinhu Dong, Lijun Gao, Yu‐Quan Zhao, Hyunjin Moon, Susannah L. Scott

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Catalytic Upcycling of PolyolefinsOriginalTheoretical determination of a model molecule for the catalytic upcycling of polyolefins1Stirring up success5Functionalized Quasi‐Solid‐State Electrolytes in Aqueous Zn‐Ion Batteries for Flexible Devices: Challenges and Strategies34Recent advances in ring-opening (co)Polymerization of O-carboxyanhydrides4A better fate for PVC2Photochemical upcycling of polymers via visible light-driven C–H bond activation23Heterogeneous catalysis strategies for polyolefin plastic upcycling: co-reactant-assisted and direct transformation under mild conditions15The tandem cracking-oxidation of phthalate esters with high CO2 selectivity and reduced energy cost8C−H Bond Activation by Sulfated Zirconium Oxide is Mediated by a Sulfur‐Centered Lewis Superacid8C−H Bond Activation by Sulfated Zirconium Oxide is Mediated by a Sulfur‐Centered Lewis Superacid2Upcycling of waste plastics: strategies, status-quo, and prospects3Advances in heterogeneous catalysts for sustainable PET upcycling: from mechanistic understanding to catalyst design6Can mixed plastics be recycled and upcycled without separation?11Complementary acid site mechanisms in hydrogen-free polyethylene upcycling: elucidating the distinct roles of Brønsted and Lewis sites in Ce-modified zeolites14Electrothermal upcycling of plastic waste18Exposing active sites in zeolites with fluoropyridines as NMR probe molecules1Highly adaptable oxidative upcycling of polyolefins to multifunctional chemicals containing oxygen and nitrogen9Hydrocracking of polyolefins over ceria-promoted Ni/BEA catalysts23Influence of functional additives, fillers, and pigments on thermal and catalytic pyrolysis of polyethylene for waste plastic upcycling61Metal–organic framework applications for microplastic remediation: exploring pathways and future potential28Renewable aromatic production from waste: exploring pathways, source materials, and catalysts24Theoretical determination of a model molecule for the catalytic upcycling of polyethylene and polypropylene0Tuning cluster size down to single atoms on Pt/γ-Al 2 O 3 catalysts via surface organometallic chemistry5Understanding the competition between hydrodechlorination and Friedel–Crafts alkylation in PVC dechlorination with silylium ions7Ruthenium‐Catalyzed Deconstruction of Polyolefins: A Strategy to Up‐cycle Waste Polyethylene to Value‐Added Alkene1Ruthenium‐Catalyzed Deconstruction of Polyolefins: A Strategy to Up‐cycle Waste Polyethylene to Value‐Added Alkene20Recent advancements in upcycling of polyolefins by hydrocracking: Effect of various heterogeneous catalysts and reaction parameters8Enhancing Rate and Selectivity for Hydrodechlorination of Poly(Vinyl Chloride) with Rh Catalysts9High Carbon Recovery in Photocatalytic Degradation of High-Density Polyethylene (HDPE): Blend with Stearic Acid as a Radical Source2Optimization of pore structure and mechanical properties of ultra-high molecular weight polypropylene porous membranes2Investigating the Role of Acid Sites in the Hydrocracking of Polyethylene-EVOH Multilayer Film Waste over Pt/BEA Catalyst7Activation of Molecular Oxygen and Selective Oxidation with Metal Complexes65Recent advances in synergistic catalytic valorization of CO2 and hydrocarbons by heterogeneous catalysis7Insights into Chemical Recycling and Upgrading Strategies for Polyolefin-Based Plastics15Hydrocarbon Deposition during Polyolefin Upcycling: Irreversible Adsorption and Surface Reactions of Polyethylene and Ethylene Oligomers on Silica Supports2Cold plasma-assisted co-conversion of polyolefin wastes and CO2 into aromatics over hierarchical Ga/ZSM-5 catalyst24Upgrading polyolefin plastics: experiences from petroleum refining and distinct characteristics19Reductive Upcycling of Polyolefins, Polyesters and Mixed Plastic Wastes to Valuable Chemicals: Bridging Chemical Catalysis With Plastic Waste Management35Upcycling of Waste Plastics into Value-Added Chemicals6Catalytic Strategies for the Production of Alkane‐Based Lubricant Base Oils from Biomass and Plastic Wastes11Polyethylene Upcycling to Liquid Alkanes in Molten Salts under Neat and External Hydrogen Source-Free Conditions17Engineering porous Beta zeolite-encapsulated nickel catalyst for waste polyolefins upcycling26Electrochemical Commodity Polymer Up‐ and Re‐Cycling: Toward Sustainable and Circular Plastic Treatment14Iron(III)‐Catalyzed C─H Hydroxylation of Low‐Density Polyethylene Coupled with Short Chain Branching Growth5Iron(III)‐Catalyzed C─H Hydroxylation of Low‐Density Polyethylene Coupled with Short Chain Branching Growth2Reprocessable Polypropylene Covalent Adaptable Networks via Free-Radical Reactive Processing with Vinyl Aromatic Additives15Co-recycling of plastics and other waste materials70Hydrogen Spillover‐Induced Brønsted Acidity Enables Controllable Hydrocracking of Polyolefin Waste to Liquid Fuels32Hydrogen Spillover‐Induced Brønsted Acidity Enables Controllable Hydrocracking of Polyolefin Waste to Liquid Fuels4MOF Catalysts for Plastic Depolymerization4MOF Catalysts for Plastic Depolymerization52Synergistic Catalysis for Recycling and Upcycling of Plastics35Chemical recycling of waste polyester plastics1A Broad-Spectrum Catalyst for Aliphatic Polymer Breakdown4Population Balance Models for Catalytic Depolymerization: From Elementary Steps to Multiphase Reactors8Blocky Selective Postpolymerization C–H Functionalization of Polyolefins14Blocky Selective Postpolymerization C–H Functionalization of Polyolefins2Consequences on Acidity and Reactivity of Inhomogeneous Sodium Exchange in the Shaping of ZSM‐5 with Silica Binders2Uncovering strategies for quantifying thermo-kinetics, reaction heat, and synergistic rates of heat transfer-degradation in the chemical upcycling of polyolefins5Oxidation of n-alkanes using TS-1 and H2O2: Effects of chain length and solvents2Al-Modified Dendritic Fibrous Nanosilica Catalyst: Accurately Regulated Acidity for Tunable Product Distribution in 1-Decene Oligomerization1Recent Advances in the Thermo-Catalytic Upcycling of Polyethylene Waste13Unlocking the Potential of Mn‐based Catalyst for Durable Two‐electron Oxygen Reduction in Acid at High Current Densities17Unlocking the Potential of Mn‐based Catalyst for Durable Two‐electron Oxygen Reduction in Acid at High Current Densities5Gradient Modulation of Ansa‐Metallocenes for Syndiotactic Propylene Polymerization: Multi‐Stage Remote Substituent Effects1Rational design of zeolite-based composite catalysts in catalytic cracking of polyethylene6Syngas from waste plastics and water using Joule heating19Synergistic and antagonistic effects of ZnO/Zn2+ species and Brønsted/Lewis acid sites variations on the catalytic conversion of polyethylene to aromatics7On-Demand Nonalternating Copolymerization Enables Upcycling of Mixed Polyethylene and Nylon Plastics14Methods for Carbon Mass Closure in Polyolefin Hydrocracking6Photocatalytic Waste Polystyrene Plastic Conversion: Reaction Mechanism and Catalyst Design38Continuous Lumped Hydrocracking Kinetics of Plastic (Polyethylene) Pyrolysis Oil Blended with Gas Oil1High-Temperature Size Exclusion Chromatography for Advanced Recycling: Systematic Errors in Analysis of Polyethylene─Alkane Mixtures0Poisoning effects of impurities on hydrogenolysis of polyethylenes over supported Ru catalysts3Engineering functional nanocomposites for enhanced AOP-mediated microplastic mineralization: From mechanistic insights to water remediation strategies3Regulation of Co-Ni/ MIL-101-C MOF reconstruction for enhanced deoxygenation reaction2Valorization of Tetra Pak Waste in a Conical Spouted Bed: Predicting the Polyethylene/Aluminum Mixing Index Using CFD Designs2High-Efficiency Hydrocracking of Polyolefin Plastics by Controlling Intimacy between Pt Clusters and Zeolite Acid Sites65Integrated low-temperature PVC and polyolefin upgrading38Tandem Catalysis to Mitigate Coke Formation in the Upcycling of Mixed Polyolefin Wastes11Understanding the Surface Acidity Mediated Reaction Pathway in CO 2 Assisted Aromatization of Polyolefin Waste8Dual-catalyst system without supported metals toward polyethylene waste upcycling3Kinetic regulation of Brønsted and Lewis acidity in FAU-type zeolites for olefin-selective plastic waste cracking12Modulating Poly(oligocyclobutane) Properties Through Backbone Modifications1The silent partner in catalysis: How support architectures dictate efficiency in polyolefin hydrogenolysis1Efficient conversion of polyethylene to light olefins by self-confined cracking and reforming22Circular economy strategies for converting waste plastics into surfactants6Tandem catalytic cracking of LDPE to C2-C4 olefins over interconnected NZ@Al-meso-SiO2: Role of hierarchical porosity and acidity4Catalytic Depolymerization of Plastics to Valuable Products7Long-lived metal-zeolite catalysts for polyolefin aromatization via synergistic tandem dehydroaromatization and hydrogenolysis12Recyclable Biomass-Derived Polyethylene-like Plastics6A comprehensive review on the sustainable approach of fossil-based polymers toward bio-based polymers9Net-Zero Upcycling of Mixed Polyolefins by Spatially Homogeneous Joule Heating7Waste plastic upcycling via homogeneous catalytic hydrogenation/dehydrogenation/transfer hydrogenation4Upcycling of Polystyrene to 1,2‐Disubstituted Oxygenated Aromatics Through Backbone Rearrangement and Oxidation Reactions1Upcycling of Polystyrene to 1,2‐Disubstituted Oxygenated Aromatics Through Backbone Rearrangement and Oxidation Reactions7Lanthanide contraction effect of PdPr nanosheets boosting PET electrocatalytic value‐added conversion3Effect of Regioregularity on the Solution Behavior of Polyoctenamer‐ graft ‐poly(ethylene glycols)0Functionalizations of C─H and C═C Bonds in Polyolefins Catalyzed by Transition‐Metal Complexes14Main-Chain Ketone Installation in Polyethylene Chains: A Metal-Free Strategy toward Photodegradable Plastics18Molar-Mass-Dependent Partitioning of Polyethylene in Nanopores of Model Catalyst Supports from Small-Angle Neutron Scattering2Closed-loop recycling of polyethylene to ethylene and propylene via a kinetic decoupling–recoupling strategy32Metal–Organic Framework for Plastic Depolymerization and Upcycling5Organic Fluorescent Labeling and Sorting for Plastic Recycling4Monitoring Depolymerization in Mesopores Using Dynamic Properties of Polymeric Melt Accessed via Dielectric Spectroscopy0Precision Oligomeric Building Blocks toward Chemically Recyclable Polyolefin-like Materials4Sustainable polymers for battery applications7Hydrogen-Free Catalytic Strategies for the Upcycling of Polyolefin Plastics3Graph theory-based exploration of structure and dynamics of surface organometallic catalysis2Novel methods for recycling PET plastic bottle waste: Progressing membrane engineering using environmentally friendly solutions10On-Demand Recycling of Polylactic Acid–Based Blends into Upgraded Materials with Customizable Compositions1Mechanically Accelerated Depolymerization of Entangled Linear Polymer Melts2One-Step Compatibilization and Upcycling of Mixed Polyolefins Using a Dynamic Disulfide-Linked Bismaleimide Cross-Linker7Plasma Catalysis for Plastic Waste Conversion into Value‐Added Products: Advancements and Perspectives11Polyethylene hydrogenolysis to liquid products over bimetallic catalysts with favorable environmental footprint and economics17Large-Mesopore Catalysts Synthesized via Calcination and Hydrothermal Treatment of Zinc-Meso-Y Zeolite Composites0Resource-Efficient Upgrading of Plastic Pyrolysis Oil: Nickel-Loaded Kaolin for Enhancing Light Oil Yield at Lower Temperatures1Selective, Oxygen‐Tunable, and Metal‐Free Functionalization of Polyethylene Through Dual‐Mode Nitrosation and Carbonylation1Selective, Oxygen‐Tunable, and Metal‐Free Functionalization of Polyethylene Through Dual‐Mode Nitrosation and Carbonylation7Recent advances in chemical upcycling of plastic waste: microwave-assisted heating and heterogeneous catalysis11Recent advances in plastic upcycling enabled by dynamic covalent cross-linking strategies0Microwave-assisted catalytic upcycling of polyolefin wastes into hydrogen and carbon nanotubes over Pt-promoted Fe/Ni bimetallic catalysts10Valorization of plastic waste into drop-in fuels: Economic and environmental perspectives16When waste plastics meet with MOF: Upcycling waste polypropylene separator into carbon nanotube for efficient freshwater and hydroelectricity co-generation1Advances of rare earth-based catalysts for recycling CO 2 and plastic waste17Surface and Interface Properties of Metal Species for Waste Plastic Hydroconversion6Leveraging and understanding exotherms in tandem catalysts with in situ luminescence thermometry4Research progress in metal-zeolite bifunctional systems for upcycling of waste polyolefins3Upcycling Polyethylene into Separable Aromatics Through Tandem Catalysis with CO2 at Atmospheric Pressure2Polyolefins pyrolysis: quantitative structure-thermal-reactivity relationships for selective high-value fuels and chemicals production5Data-Driven Discovery of Bimetallic Nanoparticles Catalysts for the Hydrogenolysis of Polyethylene3Entropy Engineering for the Efficient Hydrogenolysis of Waste Polyolefins1Heterogeneous catalysis for the production of LOHCs from plastic Waste: Enabling circular hydrogen solutions2Single-Atom Ni on Tungsten Oxides Drives Hydrogen Spillover for Efficient Plastic Waste Upcycling13Thermochemical upcycling of plastic waste: A comprehensive view from technology to commercialization2Comparative study of hierarchical and nanosized SAPO-34 catalysts in methanol to olefins1Photothermal Revolution in Plastic Upcycling24Biorefinery-based production of biodegradable bioplastics: advances and challenges in circular bioeconomy11Decoupling Acidity from Micropore Confinement in an Amorphous–Crystalline Composite for Selective Polyolefin Waste Cracking14Recent developments in recycling technologies for polymeric plastics8Research progress of high value utilization of waste polyethylene plastics6A chemically recyclable thermosetting elastomer via ring-opening metathesis polymerization0Advanced catalyst design and mechanistic insights in electrocatalytic upcycling of PET-derived ethylene glycol and coupled electrolysis systems4Benchmarking electro-Fenton-driven decomposition of synthetic polymers0Can recycled e-waste polymers power the future of sensors?2Carbon–carbon bond cleavage for lignin and plastics deconstruction0Catalytic valorization of polyolefins: from catalysts and processes to reactors0Contaminant-Tolerant Conversion of Polyethylene Waste to α-Olefins6Dual advantages of rapid zeolite channel diffusion and Ni sites: 1Ni/L-DAl zeolite enables efficient polyolefin hydrocracking to liquid fuel1Efficient oxidative upcycling of waste polyolefins into functional carboxylic acid additives over non-noble-metal catalysts1

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  6. Photochemical upcycling of polymers via visible light-driven C–H bond activation

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  18. Hydrocracking of polyolefins over ceria-promoted Ni/BEA catalysts

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  36. Cold plasma-assisted co-conversion of polyolefin wastes and CO2 into aromatics over hierarchical Ga/ZSM-5 catalyst

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  37. Upgrading polyolefin plastics: experiences from petroleum refining and distinct characteristics

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  39. Upcycling of Waste Plastics into Value-Added Chemicals

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  41. Polyethylene Upcycling to Liquid Alkanes in Molten Salts under Neat and External Hydrogen Source-Free Conditions

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  42. Engineering porous Beta zeolite-encapsulated nickel catalyst for waste polyolefins upcycling

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  44. Iron(III)‐Catalyzed C─H Hydroxylation of Low‐Density Polyethylene Coupled with Short Chain Branching Growth

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  45. Iron(III)‐Catalyzed C─H Hydroxylation of Low‐Density Polyethylene Coupled with Short Chain Branching Growth

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  46. Reprocessable Polypropylene Covalent Adaptable Networks via Free-Radical Reactive Processing with Vinyl Aromatic Additives

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  47. Co-recycling of plastics and other waste materials

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  48. Hydrogen Spillover‐Induced Brønsted Acidity Enables Controllable Hydrocracking of Polyolefin Waste to Liquid Fuels

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  49. Hydrogen Spillover‐Induced Brønsted Acidity Enables Controllable Hydrocracking of Polyolefin Waste to Liquid Fuels

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  50. MOF Catalysts for Plastic Depolymerization

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