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RESEARCH PAPER · Nature Chemical Engineering · 2024

Assessment of transport phenomena in catalyst effectiveness for chemical polyolefin recycling

Shibashish D. Jaydev, Antonio José Martín, David Garcia, Katia Chikri, Javier Pérez‐Ramírez

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Assessment of transport phenomena in catalyst effectiveness for chemical polyolefin recyclingOriginalAdvances in catalytic chemical recycling of synthetic textiles43Sustainable catalysts for propylene synthesis3Stirring up success5A better fate for PVC2Heterogeneous catalysis strategies for polyolefin plastic upcycling: co-reactant-assisted and direct transformation under mild conditions15Intensification & Scale-up of Waste Plastic Upcycling to Lubricants Conversion0Self-cleaning catalysts enable recycling of multilayered plastic films4One year of Nature Chemical Engineering1Supercritical Fluids for Enhanced Chemical Transformation of Postconsumer Plastics: A Review4Hydrocarbon Deposition during Polyolefin Upcycling: Irreversible Adsorption and Surface Reactions of Polyethylene and Ethylene Oligomers on Silica Supports2A rapid-heating copper block reactor system for improved isothermal kinetics of polyethylene pyrolysis3Population Balance Models for Catalytic Depolymerization: From Elementary Steps to Multiphase Reactors8Mechanistic alteration of polyethylene oxidation via heterogenous catalysis for enhanced fatty di-carboxylic acid yields6Methods for Carbon Mass Closure in Polyolefin Hydrocracking6Residual Faraday Efficiency Enabling Interpretable Data-Driven Optimization of Mass Transport for CO 2 Electroreduction4High-Efficiency Hydrocracking of Polyolefin Plastics by Controlling Intimacy between Pt Clusters and Zeolite Acid Sites65Efficient conversion of polyethylene to light olefins by self-confined cracking and reforming22Efficient chemical recycling of mixed plastics by intramolecular glycolysis13Enhanced hydrocracking of oleic acid to sustainable biofuel over Ni–Cu/mesoporous silica catalyst: Effects of reaction conditions, kinetic modelling, and mechanistic insights2Mechanically Accelerated Depolymerization of Entangled Linear Polymer Melts2On the Influence of Catalyst Mesopore Structure in the Catalytic Cracking of Polypropylene1Selective polyethylene hydrocracking to liquid and gaseous hydrocarbons over Co–Ni catalysts supported on H-BEA zeolite10Intrinsically Bifunctional and Tunable Tungsten Carbide Catalysts Enable Efficient PVC-Compatible Polyolefin Hydrocracking8Data-Driven Discovery of Bimetallic Nanoparticles Catalysts for the Hydrogenolysis of Polyethylene3Biomass pyrolysis with a Fe-Ni-CaO char-based catalyst for efficient green hydrogen generation and bio-oil upgrading via coupled –H/O–H activation4Catalytic valorization of polyolefins: from catalysts and processes to reactors0Direct upcycling of mixed plastic waste into liquid alkanes3Plastics recycling and valorization: Focus on polyethylene terephthalate waste and beyond0Illuminating the Effects of Interchain Interactions on the Catalytic Amidation of C–H Bonds in Polyethylenes4Hydrogenolysis Versus Hydrocracking for Polyolefin Upcycling0Shape-Selective Conversion of High-Density Polyethylene into Benzene with Zeolite-Encapsulated Subnanometer Pt Catalysts6Techno-economic analysis and life cycle assessment for the catalytic hydrogenolysis and hydrocracking of polyethylene6Towards Sustainable Plastics Management: Value Chain Assessment of Pyrolysis Oil Integration in the Petrochemical Industry0Catalytic Upcycling of Polyolefins and Polystyrene: Integrating Active Site Design With Mass Transfer Considerations4Impact of Small-Alkane Solvents on Polyolefin Hydrogenolysis over a Ruthenium Catalyst0Construction of Tunable Degradable Polydicyclopentadiene: Regulating the Performance–Environment Trade-off through Phosphoester Bonds0Bifunctional nanocatalyst design for polyolefin hydrocracking2Reductive catalytic upcycling of polyethylene using 2-propanol as transfer hydrogen-donor source1Enabling Refinery Integration for Plastic Waste Recycling: A Probabilistic Techno-economic Analysis and Carbon Footprint Assessment of Poly-Crude Production0Comprehensive quantitative analysis of polyolefin hydrogenolysis toward plastic waste management0Insights into mixing of non-isothermal multi-polymer melts for complex plastics recycling0Methodological Landscape of Acid Catalyst Screening for In Situ Plastic Pyrolysis: A Critical Review0Internal transport modulates catalytic hydrogenolysis of polyolefins0Challenges in polyolefin re/upcycling catalysis specific to polymer feedstock0Adsorption of Polyolefins from Alkanes on Alumina and Silica0

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  1. Advances in catalytic chemical recycling of synthetic textiles

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  2. Sustainable catalysts for propylene synthesis

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  3. Stirring up success

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  4. A better fate for PVC

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  5. Heterogeneous catalysis strategies for polyolefin plastic upcycling: co-reactant-assisted and direct transformation under mild conditions

    Chemical Communications · 2024-12-18

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  6. Intensification & Scale-up of Waste Plastic Upcycling to Lubricants Conversion

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  7. Self-cleaning catalysts enable recycling of multilayered plastic films

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    Dai‐Phat Bui, Shuheng Wang, Laura A. Gomez, Tahmid Ul Karim, Thomas Salas, Samira Abdolbaghi, Kevin Nelson, Lance L. Lobban, Christos T. Maravelias, Steven P. Crossley

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  8. One year of Nature Chemical Engineering

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  9. Supercritical Fluids for Enhanced Chemical Transformation of Postconsumer Plastics: A Review

    ChemCatChem · 2025-02-05

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  10. Hydrocarbon Deposition during Polyolefin Upcycling: Irreversible Adsorption and Surface Reactions of Polyethylene and Ethylene Oligomers on Silica Supports

    Industrial & Engineering Chemistry Research · 2025-03-12

    Fawaz Motolani, Rebekah J. Snellings, Sogand Aghamohammadi, Hee Jeung Oh, Gina A. Noh, Bert D. Chandler, Bryan D. Vogt

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  11. A rapid-heating copper block reactor system for improved isothermal kinetics of polyethylene pyrolysis

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  12. Population Balance Models for Catalytic Depolymerization: From Elementary Steps to Multiphase Reactors

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  13. Mechanistic alteration of polyethylene oxidation via heterogenous catalysis for enhanced fatty di-carboxylic acid yields

    Science China Chemistry · 2025-07-10

    Huidong Lv, Yi Ji, Wenjun Chen, Yuan Xiang, Yue Liu, Jianrong Zeng, Fei Huang, Fan Zhang

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  14. Methods for Carbon Mass Closure in Polyolefin Hydrocracking

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  15. Residual Faraday Efficiency Enabling Interpretable Data-Driven Optimization of Mass Transport for CO 2 Electroreduction

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  16. High-Efficiency Hydrocracking of Polyolefin Plastics by Controlling Intimacy between Pt Clusters and Zeolite Acid Sites

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  17. Efficient conversion of polyethylene to light olefins by self-confined cracking and reforming

    Nature Communications · 2025-08-26

    Zhongwen Dong, Bo Peng, Nantian Xiao, Wenjun Chen, Tingyu Lei, Meng Wang, Cheng Li, Rongxin Zhang, Zhengxing Qin, Xingchen Liu, Xiaodong Wen, Mingfeng Li, Ding Ma, Fan Zhang

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  18. Efficient chemical recycling of mixed plastics by intramolecular glycolysis

    AIChE Journal · 2025-09-03

    Yanfen Wu, Xin Zi Tang, Shuairen Qian, Helai Huang, Yizhen Che, Qikun Hu, Mingze Sun, Yi Lung Cheng, Zhiqiang Niu

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  19. Enhanced hydrocracking of oleic acid to sustainable biofuel over Ni–Cu/mesoporous silica catalyst: Effects of reaction conditions, kinetic modelling, and mechanistic insights

    Next Materials · 2025-10-01

    Ahmad Suseno, Gunawan Gunawan, Eli Dwi Astuti, Roni Adi Wijaya

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  20. Mechanically Accelerated Depolymerization of Entangled Linear Polymer Melts

    Macromolecules · 2025-11-05

    Junghyun Ahn, Jon M. Bingaman, Rachel A. Segalman, Susannah L. Scott, Lynn M. Walker

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  21. On the Influence of Catalyst Mesopore Structure in the Catalytic Cracking of Polypropylene

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    Sebastian Rejman, Tim Meijer, Hamid Seyed Khabbaz, Ali Gooneie, Adriaan J. A. Duijndam, Johan H. van de Minkelis, Ina Vollmer, Bert Marc Weckhuysen

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  22. Selective polyethylene hydrocracking to liquid and gaseous hydrocarbons over Co–Ni catalysts supported on H-BEA zeolite

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  23. Intrinsically Bifunctional and Tunable Tungsten Carbide Catalysts Enable Efficient PVC-Compatible Polyolefin Hydrocracking

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  24. Data-Driven Discovery of Bimetallic Nanoparticles Catalysts for the Hydrogenolysis of Polyethylene

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  25. Biomass pyrolysis with a Fe-Ni-CaO char-based catalyst for efficient green hydrogen generation and bio-oil upgrading via coupled –H/O–H activation

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  26. Catalytic valorization of polyolefins: from catalysts and processes to reactors

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  28. Plastics recycling and valorization: Focus on polyethylene terephthalate waste and beyond

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  29. Illuminating the Effects of Interchain Interactions on the Catalytic Amidation of C–H Bonds in Polyethylenes

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  30. Hydrogenolysis Versus Hydrocracking for Polyolefin Upcycling

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  31. Shape-Selective Conversion of High-Density Polyethylene into Benzene with Zeolite-Encapsulated Subnanometer Pt Catalysts

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  32. Techno-economic analysis and life cycle assessment for the catalytic hydrogenolysis and hydrocracking of polyethylene

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  33. Towards Sustainable Plastics Management: Value Chain Assessment of Pyrolysis Oil Integration in the Petrochemical Industry

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  34. Catalytic Upcycling of Polyolefins and Polystyrene: Integrating Active Site Design With Mass Transfer Considerations

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  35. Impact of Small-Alkane Solvents on Polyolefin Hydrogenolysis over a Ruthenium Catalyst

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  36. Construction of Tunable Degradable Polydicyclopentadiene: Regulating the Performance–Environment Trade-off through Phosphoester Bonds

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  37. Bifunctional nanocatalyst design for polyolefin hydrocracking

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  38. Reductive catalytic upcycling of polyethylene using 2-propanol as transfer hydrogen-donor source

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  39. Enabling Refinery Integration for Plastic Waste Recycling: A Probabilistic Techno-economic Analysis and Carbon Footprint Assessment of Poly-Crude Production

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  40. Comprehensive quantitative analysis of polyolefin hydrogenolysis toward plastic waste management

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  41. Insights into mixing of non-isothermal multi-polymer melts for complex plastics recycling

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  43. Internal transport modulates catalytic hydrogenolysis of polyolefins

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  44. Challenges in polyolefin re/upcycling catalysis specific to polymer feedstock

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  45. Adsorption of Polyolefins from Alkanes on Alumina and Silica

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