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RESEARCH PAPER · Journal of the American Chemical Society · 2023

Cationic Tantalum Hydrides Catalyze Hydrogenolysis and Alkane Metathesis Reactions of Paraffins and Polyethylene

Jiaxin Gao, Lingchao Zhu, Matthew P. Conley

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Cationic Tantalum Hydrides Catalyze Hydrogenolysis and Alkane Metathesis Reactions of Paraffins and PolyethyleneOriginalEffects of surface acidity on the structure of organometallics supported on oxide surfaces21Upcycling of polyethylenes by catalysis0Polypropylene Degradation Catalyzed by Tantalum Hydrides Supported on Sulfated Alumina23Treasuring trash: Pt/SrTiO3 catalysts process plastic waste into high-value materials25Solar-driven photocatalysis for recycling and upcycling plastics122Current Advances and Challenges in Chemical Recycling of Polymeric Materials5A Supported Ziegler-Type Organohafnium Site Metabolizes Polypropylene8Rapid Polyolefin Hydrogenolysis by a Single‐Site Organo‐Tantalum Catalyst on a Super‐Acidic Support: Structure and Mechanism14Rapid Polyolefin Hydrogenolysis by a Single‐Site Organo‐Tantalum Catalyst on a Super‐Acidic Support: Structure and Mechanism5Rapid Polyolefin Plastic Hydrogenolysis Mediated by Single-Site Heterogeneous Electrophilic/Cationic Organo-group IV Catalysts19Highly Selective and Efficient Perdeuteration of n‐Pentane via H/D Exchange Catalyzed by a Silica‐Supported Hafnium‐Iridium Bimetallic Complex12Highly Selective and Efficient Perdeuteration of n‐Pentane via H/D Exchange Catalyzed by a Silica‐Supported Hafnium‐Iridium Bimetallic Complex3Alkene Isomerization Using a Heterogeneous Nickel-Hydride Catalyst27Demystifying group-4 polyolefin hydrogenolysis catalysis: Gaseous propane hydrogenolysis mechanism over the same catalysts5Mild Catalytic Degradation of Crystalline Polyethylene Units in a Solid State Assisted by Carboxylic Acid Groups23Active species in chloroaluminate ionic liquids catalyzing low-temperature polyolefin deconstruction22Catalytic Upcycling of Polyolefins316The role of size and structure of catalytic active sites in polyolefin hydrogenolysis12Selective Hydrogenolysis Conversion of Polyethylene into Alkyl Oil Over Iridium‐based Catalyst9Influence of Trace Metal in Plastics on Catalyst Activity and Reusability during Polyolefins Upcycling with Polyoxometalates2C−H Bond Activation by Sulfated Zirconium Oxide is Mediated by a Sulfur‐Centered Lewis Superacid8C−H Bond Activation by Sulfated Zirconium Oxide is Mediated by a Sulfur‐Centered Lewis Superacid2Optimization of nickel-based catalysts for hydrogenolysis of light paraffins using machine learning5Photothermocatalytic Wet Reforming of Waste Plastics to Syngas45Trimethylaluminum Activates Zeolite-Confined Lanthanum Borohydrides to Enhance Catalytic C–H Borylation5A Broad-Spectrum Catalyst for Aliphatic Polymer Breakdown4Mechanistic alteration of polyethylene oxidation via heterogenous catalysis for enhanced fatty di-carboxylic acid yields6Upgrading Natural Ores for Efficient Photothermal Polyester Recycling21Stable single-site organonickel catalyst preferentially hydrogenolyses branched polyolefin C–C bonds12Polymer Upcycling by Catalytic Hydrogenolysis: The Role of Polyolefin Short-Chain Branching3Synthesis of Perdeuterated Pentane and THF Under Mild Conditions by Silica‐Supported Ta/M (M = Co, Ir) Heterobimetallic Catalysts0Synthesis of Perdeuterated Pentane and THF Under Mild Conditions by Silica‐Supported Ta/M (M = Co, Ir) Heterobimetallic Catalysts4Facile C–N bond construction from a molecular model of iron on silica0Recent advancements in catalytic processes for plastic upcycling into fuels: a major step in sustainable waste management and energy production3Chemical recycling via precision depolymerization: fundamentals, design principles, and emerging frontiers for circular polymer systems3Selective depolymerization and upcycling of thermoset polyurethane: From waste foam to easily-degradable flame-retardant film3Oxygen vacancy promoted C–H activation enhancing hydrogenolysis of polyethylene plastics over Ru/CeO2 catalyst0Challenges in polyolefin re/upcycling catalysis specific to polymer feedstock0

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  1. Effects of surface acidity on the structure of organometallics supported on oxide surfaces

    Chemical Communications · 2023-01-01

    Kavyasripriya K. Samudrala, Matthew P. Conley

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  2. Upcycling of polyethylenes by catalysis

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  3. Polypropylene Degradation Catalyzed by Tantalum Hydrides Supported on Sulfated Alumina

    ACS Catalysis · 2023-08-01

    Jiaxin Gao, Lingchao Zhu, Matthew P. Conley

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  4. Treasuring trash: Pt/SrTiO3 catalysts process plastic waste into high-value materials

    Matter · 2023-08-08

    Ian L. Peczak, Robert M. Kennedy, Ryan A. Hackler, Byeongdu Lee, Max Meirow, Erik Luijten, Kenneth Reinhard Poeppelmeier, Massimiliano Delferro

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  5. Solar-driven photocatalysis for recycling and upcycling plastics

    Applied Catalysis B: Environmental · 2023-09-30

    Ruochen Cao, Dequan Xiao, Meng Wang, Gao Y, Ding Ma

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  6. Current Advances and Challenges in Chemical Recycling of Polymeric Materials

    Preprints.org · 2023-10-08

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  7. A Supported Ziegler-Type Organohafnium Site Metabolizes Polypropylene

    Journal of the American Chemical Society · 2023-11-03

    Kavyasripriya K. Samudrala, Matthew P. Conley

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  8. Rapid Polyolefin Hydrogenolysis by a Single‐Site Organo‐Tantalum Catalyst on a Super‐Acidic Support: Structure and Mechanism

    Angewandte Chemie International Edition · 2023-11-10

    Qingheng Lai, Alexander H. Mason, Amol Agarwal, Wilson C. Edenfield, Xinrui Zhang, Takeshi Kobayashi, Yosi Kratish, Tobin Jay Marks

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  9. Rapid Polyolefin Hydrogenolysis by a Single‐Site Organo‐Tantalum Catalyst on a Super‐Acidic Support: Structure and Mechanism

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    Qingheng Lai, Alexander H. Mason, Amol Agarwal, Wilson C. Edenfield, Xinrui Zhang, Takeshi Kobayashi, Yosi Kratish, Tobin Jay Marks

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  10. Rapid Polyolefin Plastic Hydrogenolysis Mediated by Single-Site Heterogeneous Electrophilic/Cationic Organo-group IV Catalysts

    ACS Catalysis · 2023-12-26

    Wilson C. Edenfield, Alexander H. Mason, Qingheng Lai, Amol Agarwal, Takeshi Kobayashi, Yosi Kratish, Tobin Jay Marks

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  11. Highly Selective and Efficient Perdeuteration of n‐Pentane via H/D Exchange Catalyzed by a Silica‐Supported Hafnium‐Iridium Bimetallic Complex

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  12. Highly Selective and Efficient Perdeuteration of n‐Pentane via H/D Exchange Catalyzed by a Silica‐Supported Hafnium‐Iridium Bimetallic Complex

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    Andrey V. Pichugov, Léon Escomel, Sébastien Lassalle, Julien Petit, Ribal Jabbour, David Gajan, Laurent Veyre, Emiliano Fonda, Anne S. J. Lesage, Chloé Thieuleux, Clément Camp

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  13. Alkene Isomerization Using a Heterogeneous Nickel-Hydride Catalyst

    Journal of the American Chemical Society · 2024-05-21

    Alison Sy-min Chang, Melanie A. Kascoutas, Quinn P. Valentine, Kiera How, Rachel Thomas, Amanda K. Cook

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  14. Demystifying group-4 polyolefin hydrogenolysis catalysis: Gaseous propane hydrogenolysis mechanism over the same catalysts

    Proceedings of the National Academy of Sciences · 2024-06-23

    Alexander H. Mason, Alessandro Motta, Yosi Kratish, Tobin Jay Marks

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  15. Mild Catalytic Degradation of Crystalline Polyethylene Units in a Solid State Assisted by Carboxylic Acid Groups

    Journal of the American Chemical Society · 2024-07-02

    Bin Lü, Kohei Takahashi, Jian Xin Zhou, Shintaro Nakagawa, Yuta Yamamoto, Takuya Katashima, Naoko Yoshie, Kyoko Nozaki

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  16. Active species in chloroaluminate ionic liquids catalyzing low-temperature polyolefin deconstruction

    Nature Communications · 2024-07-10

    Wei Zhang, Rachit Khare, Sung Min Kim, Lillian Hale, Wenda Hu, Chun-lin Yuan, Yaoci Sheng, Peiran Zhang, Lennart Wahl, Jiande Mai, Boda Yang, Oliver Y. Gutiérrez, Debmalya Ray, John L. Fulton, Donald M. Camaioni, Jian Zhi Hu, Huamin Wang, Mal‐Soon Lee, Johannes A. Lercher

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  17. Catalytic Upcycling of Polyolefins

    Chemical Reviews · 2024-08-16

    Jia‐Kai Sun, Jinhu Dong, Lijun Gao, Yu‐Quan Zhao, Hyunjin Moon, Susannah L. Scott

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  18. The role of size and structure of catalytic active sites in polyolefin hydrogenolysis

    Chem Catalysis · 2024-08-20

    Jueun Kim, Simin Sun, Donghyeon Kim, Byung Gwan Park, Hojeong Lee, Wenyu Huang, Kwangjin An

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  19. Selective Hydrogenolysis Conversion of Polyethylene into Alkyl Oil Over Iridium‐based Catalyst

    ChemSusChem · 2024-08-22

    Jieqi Cao, Xiao Ting Feng, Yinwei Wang, Xinbin Gong, Xiaoxia Zheng, Jin Gao, Jin Gao, Song Shi

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  20. Influence of Trace Metal in Plastics on Catalyst Activity and Reusability during Polyolefins Upcycling with Polyoxometalates

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  21. C−H Bond Activation by Sulfated Zirconium Oxide is Mediated by a Sulfur‐Centered Lewis Superacid

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  22. C−H Bond Activation by Sulfated Zirconium Oxide is Mediated by a Sulfur‐Centered Lewis Superacid

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  23. Optimization of nickel-based catalysts for hydrogenolysis of light paraffins using machine learning

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  25. Trimethylaluminum Activates Zeolite-Confined Lanthanum Borohydrides to Enhance Catalytic C–H Borylation

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  30. Polymer Upcycling by Catalytic Hydrogenolysis: The Role of Polyolefin Short-Chain Branching

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  31. Synthesis of Perdeuterated Pentane and THF Under Mild Conditions by Silica‐Supported Ta/M (M = Co, Ir) Heterobimetallic Catalysts

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