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RESEARCH PAPER · Nature Reviews Chemistry · 2024

A US perspective on closing the carbon cycle to defossilize difficult-to-electrify segments of our economy

Wendy J. Shaw, Michelle K. Kidder, Simon R. Bare, Massimiliano Delferro, James Robert Morris, Francesca Maria Toma, Sanjaya D. Senanayake, Tom S. Autrey, Elizabeth J. Biddinger, Shannon Wachter Boettcher, Mark Bowden, Phillip F. Britt, Robert C. Brown, R. Morris Bullock, Jingguang G. Chen, Claus Daniel, Peter K. Dorhout, Rebecca Ann Efroymson, Kelly J. Gaffney, Laura Gagliardi, Aaron S. Harper, David J. Heldebrant, Oana R. Luca, Maxim Lyubovsky, Jonathan L. Male, Daniel J. Miller, Tanya Prozorov, Robert Ralló, Rachita Rana, Robert M. Rioux, Aaron David Sadow, Joshua A. Schaidle, Lisa A. Schulte, William Abraham Tarpeh, Dionisios G. Vlachos, Bryan D. Vogt, Robert S. Weber, Jenny Y. Yang, Elke Arenholz, Brett A. Helms, Wenyu Huang, J.L. Jordahl, Canan Karakaya, Kourosh Kian, Jotheeswari Kothandaraman, Johannes A. Lercher, Ping Liu, Deepika Malhotra, Karl Todd Mueller, Casey P. O’Brien, Robert M. Palomino, Long Qi, José A. Rodríguez, Roger J. Rousseau, Jake C. Russell, Michele L. Sarazen, David S. Sholl, Emily A. Smith, Michaela Burke Stevens, Yogesh Surendranath, Christopher J. Tassone, Ba L. Tran, William Tumas, Krista S. Walton

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A US perspective on closing the carbon cycle to defossilize difficult-to-electrify segments of our economyOriginalReactive direct air capture of CO 2 to C–C coupled products using multifunctional materials19Synthesis of Cerium Doped Zirconium-Based Metal-Organic Framework Nanoparticles and Their Photocatalytic Performance for Carbon Dioxide Cycloaddition1A speedy but thorough interrogation1Harnessing AI for Sustainable Shipping and Green Ports: Challenges and Opportunities73Formulation of N-doped carbon with meso/microporous structure for supercapacitors through biotemplates20From Methane to Methanol: Pd-iC-CeO 2 Catalysts Engineered for High Selectivity via Mechanochemical Synthesis32High‐Entropy Metal‐Organic Frameworks (HEMOFs): A New Frontier in Materials Design for CO 2 Utilization29Enzyme Catalysis for Sustainable Value Creation Using Renewable Biobased Resources7Induction Heating for the Electrification of Catalytic Processes51Insights into catalyst degradation during alkaline water electrolysis under variable operation75Chloride Treatments Improve Zinc Telluride Absorbers for Photoelectrochemical Carbon Dioxide Reduction5Sequential catalysis enables efficient pyrolysis of food waste for syngas production10Bridging the gap between defossilization and decarbonization to achieve net-zero industry17Biogas sequestration to carbon nanofibers via tandem catalytic strategies20High-Temperature Growth of CeOx on Au(111) and Behavior under Reducing and Oxidizing Conditions7Investigating the Electric Double-Layer Structures between a Pt Electrode and Water/Acetonitrile Hybrid Electrolytes4Synthetic transitions: the political economy of fossil fuel as feedstock29Inhibition of polymeric densification at platinum/ionomer interface via enlarging tetrafluoroethylene spacing in perfluorinated sulfonic-acid ionomer0Supercritical water gasification and subsequent steam reforming of the product gas under elevated temperature and pressure6The XPS of pyridine: A combined theoretical and experimental analysis8To convert or not to convert: A comparative techno-economic analysis on CO2-to-methanol and CO2-EOR23A real-time distributed solid oxide electrolysis cell (SOEC) model for cyber-physical simulation15Will biohybrid or tandem CO2 electrolysis prevail?2Sustainable mining – unlocking resources towards circular economy to meet energy transition through electrochemistry26Experimental research on the countercurrent fixed-bed combustion of biomass9Investigation of Moisture Swing Adsorbents for Direct Air Capture by Dynamic Breakthrough Studies41Function–Structure–Synthesis: Machine Learning Enabled Closed-Loop Design of Biomass-Derived Porous Carbon Materials14Unlocking the potential of MXenes in electrocatalysis: A review from fundamentals to applications14Optimizing Olefin Production in Microwave Slurry Catalytic Pyrolysis of Low-Density Polyethylene4Atomic Insights into Pt‐Confined FeO Model Catalyst: Surface Structure and NH 3 Adsorption3Siting bioenergy facilities in the United States: Measuring participation in decisions and distribution of effects4Toward data-driven predictive modeling of electrocatalyst stability and surface reconstruction24Hydrogen Atom Transfer-Mediated N -Heterocycles Dehydrogenation Coupled with the CO 2 Photoreduction to Syngas10Furfural from lignocellulose biomass a comprehensive review of hydrolysis methods production technologies and integration into the circular economy14Optimizing CO 2 -Loaded Aqueous Amine Solutions for Higher Electrocatalytic CO 2 Reduction Activity12Integrated CO 2 Capture and Conversion to Formate with a Molecular Platinum Bis(diphosphine) Electrocatalyst1Reassessment of the energetic value of lignocellulosic biomass in closed carbon cycles1Catalytic Synthesis of Acetic Acid from Methanol Using Formic Acid as a Renewable CO Source5Challenges and Opportunities of Intermediate-Temperature (100–350 °C) Electrocatalysis2Electrification of catalytic processes with induction heating: The possible hidden role of non-thermal magnetic fields8Metal hydrides: a historical perspective10Catalytic CO 2 hydrogenation toward net-zero fuels and chemicals1Multiscale-particle organic hybrid materials as electrolyte additives for electrocatalytic reactive carbon capture0Selective and Stable Pt Catalysts for the Catalytic Conversion of Captured CO 2 to Methanol in an Advanced Water-Lean Postcombustion Solvent5Electrochemical Ocean-Based Carbon Capture: Roadblocks to Scale-Up6Toward Sustainable Electrochemical CO 2 Valorization0Tandem catalysis for carbon circularity3Investigation of CO 2 -to-CO Conversion by Cocatalyst-Free Epitaxial ZnTe Photocathodes0A Novel Adaptive Electrical Equivalent Circuit Model for Accurate Representation of Electrolyzer Dynamics0Scalable Cu-CoOx Electrode for 5-Hydroxymethylfurfural Electrooxidation to 2,5-Furandicarboxylic Acid at >100 A2Enhancing Poly(4-vinylpyridine)-Based Catalysts for CO 2 Conversion via Quaternization1Atomistic Insights into Aqueous Phase Carbonyl Hydrogenation over Ru Catalysts from a Hybrid Quantum Mechanical/Molecular Mechanical/Machine Learning Potential0Artificial intelligence-driven design and optimization opportunities in bio-electrocatalytic CO2 conversion systems0Unraveling in-situ electrochemical reconstruction of indium oxide catalysts with oxygen vacancy for enhanced electrocatalytic CO2-to-formate conversion0Carbon‐Free Energy Carriers and Circular Feedstocks: Bridging CO 2 Valorization with Hydrogen and Ammonia Economies1Macro–micro seepage interaction mechanism in coal treated by a high-temperature CO2–H2O system0From Precatalysts to Real Active Phases: Dynamic Reconstruction of CO2 Reduction Electrocatalysts0Decoupling Mechanical Performance and Macrophase Morphology in Compatibilized Polymer Blends0Exploring oxygen depolarized cathodes for zero-gap CO2 electrolysis0The fossilized pathways of novel technologies: how carbon capture, conversion, and utilization is poised to reinforce carbon lock-in0

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