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RESEARCH ARTICLE · JACS Au · 2024

Chemical Upcycling of Polyolefin Plastics Using Structurally Well-defined Catalysts

Simin Sun, Wenyu Huang

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Chemical Upcycling of Polyolefin Plastics Using Structurally Well-defined CatalystsOriginalSelective Upcycling of Polyolefins into High-Value Nitrogenated Chemicals80Hydrogenolysis of Polyethylene by Metal–Organic Framework Confined Single-Site Ruthenium Catalysts16Scalable Synthesis of Degradable Copolymers Containing α-Lipoic Acid via Miniemulsion Polymerization61Chemical Innovations in Polymer Upcycling: Beyond Traditional Recycling1Heterogeneous catalysis strategies for polyolefin plastic upcycling: co-reactant-assisted and direct transformation under mild conditions15Reaction engineering of the hydrogenolysis of liquid n-Alkanes: Comparison of flow and batch reaction systems2Enhancing liquified petroleum gas selectivity through hierarchical porosity in MWW-type MCM-49 zeolite for polyethylene hydrocracking0Techno-economic and life cycle analyses of the synthesis of a platinum–strontium titanate catalyst15Advanced Catalysts for the Chemical Recycling of Plastic Waste90Preparation of peroxide initiator monomer containing degradable disulphide bond0High Molecular Weight Biobased Long-Chain Aliphatic Polyesters with Degradability: Insights into Mimicking Polyethylene24Synergistic Catalysis for Recycling and Upcycling of Plastics35Sustainable and Orthogonally Closed-Loop Recyclable Acetal-Based Long-Chain Polyesters19Upgrading waste LiMn2O4 cathode for efficient photothermal polyester recycling20Metal–Organic Framework for Plastic Depolymerization and Upcycling5Surface and Interface Properties of Metal Species for Waste Plastic Hydroconversion6Selective polyethylene hydrocracking to liquid and gaseous hydrocarbons over Co–Ni catalysts supported on H-BEA zeolite10Solar-driven upcycling of plastic waste using plasmonic black gold4Acidified montmorillonite (MMT)-supported ultrafine Ru nanoparticles for polyethylene plastic upcycling0Electronegativity-driven d-band center shifts in Ru–Ni alloys for low methane hydrogenolysis of polyolefin plastics2Upcycling waste PET into functional multiblock copolymers through controlled macromolecular design1Recent advancements in catalytic processes for plastic upcycling into fuels: a major step in sustainable waste management and energy production3Thermo-chemical upgrading of waste polyethylene and polypropylene plastics0Shape-Selective Conversion of High-Density Polyethylene into Benzene with Zeolite-Encapsulated Subnanometer Pt Catalysts6Spent battery-derived electrocatalysts for circular upcycling of polystyrene waste: Simultaneous generation of aromatic nitriles and green hydrogen0Catalytic Polymerization of the Conjugated Dienes Using Quinolyl-Based NNN -Pincer Rare-Earth Metal Chlorides0Engineering Zeolite Synthesis for the Green Energy Transformation1Controlling Polyolefin Hydrogenolysis Selectivity by Engineering Single-Site Nickel(II) Hydride Active Catalytic Species0A Mesopore-Confined and Graphene Oxide-Localized Ruthenium Catalyst Increases Rates of Mid-Chain Polyolefin Hydrogenolysis0Acyclic Hydrocarbon α , ω ‐Dienes: From Biomass and Plastic Upcycling to Carbocycles, Precision Polymers, and Cross‐Linked Elastomers0A novel cucurbit[6]uril derivative-based integrated SPME–GC analysis system for efficiently determining the migration of multiple classes of plastic additives from food contact materials0Recent advances in catalytic technologies for plastic conversion: a review0Masterbatch-enabled acceleration of polyolefin biodegradation under open air terrestrial environmental conditions0Functionalized and Chemically Recyclable “Polyethylene-like” Polyesters from Selective Ring-Opening Polymerization of Bifunctional Macrocycles0Upcycling of polymer waste into high value energy products0

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  1. Selective Upcycling of Polyolefins into High-Value Nitrogenated Chemicals

    Journal of the American Chemical Society · 2024

    Binzhi Zhao, Zhibin Hu, Yichen Sun, Rehemuhali Hajiayi, Teng Wang, Ning Jiao

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  2. Hydrogenolysis of Polyethylene by Metal–Organic Framework Confined Single-Site Ruthenium Catalysts

    Chemistry of Materials · 2024

    Manav Chauhan, Chhaya Thadhani, Bharti Rana, Poorvi Gupta, Biplab Ghosh, Kuntal Manna

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  3. Scalable Synthesis of Degradable Copolymers Containing α-Lipoic Acid via Miniemulsion Polymerization

    Journal of the American Chemical Society · 2024

    Parker T. Morris, Kodai Watanabe, Kaitlin R. Albanese, Greggory T. Kent, Rohini Gupta, Matthias Gerst, Javier Read de Alaniz, Craig J. Hawker, Christopher M. Bates

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  4. Chemical Innovations in Polymer Upcycling: Beyond Traditional Recycling

    Advances in sustainability science and technology · 2024

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  5. Heterogeneous catalysis strategies for polyolefin plastic upcycling: co-reactant-assisted and direct transformation under mild conditions

    Chemical Communications · 2024

    Haokun Wang, Sijie Huang, Shik Chi Edman Tsang

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  6. Reaction engineering of the hydrogenolysis of liquid n-Alkanes: Comparison of flow and batch reaction systems

    Chemical Engineering Journal Advances · 2024

    Zhuoming Feng, Siwon Lee, Raymond J. Gorte, John M. Vohs

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  7. Enhancing liquified petroleum gas selectivity through hierarchical porosity in MWW-type MCM-49 zeolite for polyethylene hydrocracking

    Catalysis Science & Technology · 2025

    Ruoyan Bai, Juhong Nie, Roudan Lian, Jian Zhang, Maolin Zhang

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  8. Techno-economic and life cycle analyses of the synthesis of a platinum–strontium titanate catalyst

    Catalysis Science & Technology · 2025

    Sultana Ferdous, Ulises R. Gracida-Alvarez, Magali S. Ferrandon, Massimiliano Delferro, Pahola Thathiana Benavides, Meltem Urgun‐Demirtas

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  9. Advanced Catalysts for the Chemical Recycling of Plastic Waste

    Advanced Materials · 2025

    Jibo Qin, Feiyan Wu, Yibo Dou, Dan Zhao, Claus Hélix‐Nielsen, Wenjing Angela Zhang

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  10. Preparation of peroxide initiator monomer containing degradable disulphide bond

    Materials Research Innovations · 2025

    Fang Jiang, Feiyao Huang, Hongjun Yang, Li Jiang, Qimin Jiang, Wenyan Huang, Xiaoqiang Xue, Bibiao Jiang

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  11. High Molecular Weight Biobased Long-Chain Aliphatic Polyesters with Degradability: Insights into Mimicking Polyethylene

    Macromolecules · 2025

    Nagarjuna A. Mahadas, Amir Suhail, M. Taylor Sobczak, Xiaomeng Li, Kezhi Chen, Kenan Song, Guangbin Dong, Olga Kuksenok, Chuanbing Tang

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  12. Synergistic Catalysis for Recycling and Upcycling of Plastics

    ACS Catalysis · 2025

    Hongshun Ran, Xinyang Sun, Mengying Zheng, Yaxuan Jing

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  13. Sustainable and Orthogonally Closed-Loop Recyclable Acetal-Based Long-Chain Polyesters

    Journal of the American Chemical Society · 2025

    Xiaomeng Li, Zhitao Hu, Mengxue Zhang, Morgan Stefik, Colleen N. Scott, Chuanbing Tang

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  14. Upgrading waste LiMn2O4 cathode for efficient photothermal polyester recycling

    中国科学通报：英文版 · 2025

    Xiangxi Lou, Penglei Yan, Qingqing Zhang, Binglei Jiao, Zhongyu Li, Panpan Xu, Muhan Cao, Jinxing Chen, Qiao Zhang

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  15. Metal–Organic Framework for Plastic Depolymerization and Upcycling

    Crystals · 2025

    K.-S. Lee, Sumin Han, Minse Kim, Byoung-su Kim, Jeong‐Ann Park, Kwang Suk Lim, Suk‐Jin Ha, Hyun‐Ouk Kim

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  16. Surface and Interface Properties of Metal Species for Waste Plastic Hydroconversion

    ACS Catalysis · 2025

    Fan Yuan, Hongshun Ran, Tingxi Chen, Yaxuan Jing

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  17. Selective polyethylene hydrocracking to liquid and gaseous hydrocarbons over Co–Ni catalysts supported on H-BEA zeolite

    Green Chemistry · 2025

    Mahdokht Soltani, Julia N. Hancock, Zeno Rizqi Ramadhan, Samuel V. Somerville, Jamie Clark, Richard David Tilley, Julie E. Rorrer

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  18. Solar-driven upcycling of plastic waste using plasmonic black gold

    Chemical Science · 2025

    Saideep Singh, Gunjan Sharma, Mamata V. Joshi, Vivek Polshettiwar

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  19. Acidified montmorillonite (MMT)-supported ultrafine Ru nanoparticles for polyethylene plastic upcycling

    Green Chemistry · 2026

    Ruoyan Bai, Roudan Lian, Jian Zhang, Maolin Zhang

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  20. Electronegativity-driven d-band center shifts in Ru–Ni alloys for low methane hydrogenolysis of polyolefin plastics

    Journal of Materials Chemistry A · 2026

    Qianfeng Zhou, Huijie Li, Shengdong Zhang, Changhu Leng, Chuanya Li, Yongchao Wang, C. Ma, W. J. Wang, Xiaogang Fu, Lei Zhu, Tengshijie Gao, Cheng Wang, Li‐Zhu Wu, Zhi-Jun Li

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  21. Upcycling waste PET into functional multiblock copolymers through controlled macromolecular design

    Green Chemistry · 2026

    Shelby Watson-Sanders, Alison R. Biery, Karina Guerrero, Nicholas J. Galan, Tomonori Saito, Brian K. Long, Mark Dadmun

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  22. Recent advancements in catalytic processes for plastic upcycling into fuels: a major step in sustainable waste management and energy production

    Fuel · 2026

    Sudipta Nayak, Rajat Singhal, S. M. A. Hakim Siddiki, Ken Motokura, Navya Subray Bhat, Navneet Kumar Gupta

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  23. Thermo-chemical upgrading of waste polyethylene and polypropylene plastics

    Scientia Sinica Chimica · 2026

    Wanying Han, Longfei Lin, Buxing Han

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  24. Shape-Selective Conversion of High-Density Polyethylene into Benzene with Zeolite-Encapsulated Subnanometer Pt Catalysts

    Journal of the American Chemical Society · 2026

    Yunchao Feng, Hongtao Wang, Tianxiang Chen, Minghao Gao, Zhe He, Gaoqian Yuan, Lichen Liu

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  25. Spent battery-derived electrocatalysts for circular upcycling of polystyrene waste: Simultaneous generation of aromatic nitriles and green hydrogen

    Applied Catalysis B: Environmental · 2026

    Songan Zhao, YUFENG WU, Weijin Cao, Didier Astruc, Changlong Wang

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  26. Catalytic Polymerization of the Conjugated Dienes Using Quinolyl-Based NNN -Pincer Rare-Earth Metal Chlorides

    Organometallics · 2026

    Li Chen, Rui Pan, Mengmeng Han, Fenhua Wang, Qinghai Li, Shaowu Wang, Zeming Huang

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  27. Engineering Zeolite Synthesis for the Green Energy Transformation

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    Jie Zhu, Koki Muraoka, Toru Wakihara, Tatsuya Okubo

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  28. Controlling Polyolefin Hydrogenolysis Selectivity by Engineering Single-Site Nickel(II) Hydride Active Catalytic Species

    ACS Catalysis · 2026

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  29. A Mesopore-Confined and Graphene Oxide-Localized Ruthenium Catalyst Increases Rates of Mid-Chain Polyolefin Hydrogenolysis

    Journal of the American Chemical Society · 2026

    Kajol Tonk, Simin Sun, Olajide H. Bamidele, Minghui Niu, Xiaobing Zuo, Jessica V. Lamb, Arthur Jeremy Kropf, Massimiliano Delferro, Byeongdu Lee, Andreas Heyden, Wenyu Huang, Aaron David Sadow

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  30. Acyclic Hydrocarbon α , ω ‐Dienes: From Biomass and Plastic Upcycling to Carbocycles, Precision Polymers, and Cross‐Linked Elastomers

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  31. A novel cucurbit[6]uril derivative-based integrated SPME–GC analysis system for efficiently determining the migration of multiple classes of plastic additives from food contact materials

    Food Chemistry X · 2026

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  32. Recent advances in catalytic technologies for plastic conversion: a review

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    邹宝, Jisheng Zhang, Xianghai Song, Pengwei Huo

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  33. Masterbatch-enabled acceleration of polyolefin biodegradation under open air terrestrial environmental conditions

    npj Materials Degradation · 2026

    Ceren Kütahya, Catalina Cruañas Paniker, Faith Ly, Arjun Jerath, Emma Little, Rocio Gali, Muhammad Zuhayr Dzul Haimi, Abdul Hafiz Bin Abd Malek, Karimah Binti Muhamad, Suffeiya Binti Supian, Taylor B. Young, Sally Lawrence, Bell Thomas, Tan Yong Nee, José I. Jiménez, Florence Huynh

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  34. Functionalized and Chemically Recyclable “Polyethylene-like” Polyesters from Selective Ring-Opening Polymerization of Bifunctional Macrocycles

    Precision Chemistry · 2026

    Mingqian Wang, Shiyu Guan, Yujia Cheng, Zhiqiang Ding, Bin Wang

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  35. Upcycling of polymer waste into high value energy products

    Elsevier eBooks · 2026

    Betül Aksoy, Yasemin Ozliman, Melih Soner Çeliktaş

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