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RESEARCH PAPER · Chemical Engineering Journal · 2023

Investigating the influence of Ru structures and supports on hydrogenolysis of polyethylene plastic waste

Huy Nguyen‐Phu, Taeeun Kwon, Taehyup Kim, Lien Thi Do, Ki Hyuk Kang, Insoo Ro

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Investigating the influence of Ru structures and supports on hydrogenolysis of polyethylene plastic wasteOriginalSize and Structure Effects of Carbon-Supported Ruthenium Nanoparticles on Waste Polypropylene Hydrogenolysis Activity, Selectivity, and Product Microstructure40Polyethylene hydrogenolysis over bimetallic catalyst with suppression of methane formation15Catalytic Approaches to Tackle Mixed Plastic Waste Challenges: A Review27Catalytic Upcycling of Polyolefins316The role of size and structure of catalytic active sites in polyolefin hydrogenolysis12Green synthesis of Bio-CuS quantum dots by sulfate reducing bacteria for solid-phase photocatalytic degradation of polyethylene film12Unraveling the role of water in mechanism changes for economically viable catalytic plastic upcycling43Reaction engineering of the hydrogenolysis of liquid n-Alkanes: Comparison of flow and batch reaction systems2Complementary acid site mechanisms in hydrogen-free polyethylene upcycling: elucidating the distinct roles of Brønsted and Lewis sites in Ce-modified zeolites14Synergistic effect of acidic sites and mesoporous confinement in Ce-doped Ru/SBA-15 catalysts for efficient hydrogenolysis of low-density polyethylene to liquid fuels7Mechanistic Insights into Polypropylene Hydrogenolysis Using Ni/Al2O3 Catalysts17Crucial role of pre-treatment in plastic photoreforming for precision upcycling11Tandem Catalysis for Plastic Depolymerization: In Situ Hydrogen Generation via Methanol Aqueous Phase Reforming for Sustainable Polyethylene Hydrogenolysis2Tandem Catalysis for Plastic Depolymerization: In Situ Hydrogen Generation via Methanol Aqueous Phase Reforming for Sustainable Polyethylene Hydrogenolysis27Reductive Upcycling of Polyolefins, Polyesters and Mixed Plastic Wastes to Valuable Chemicals: Bridging Chemical Catalysis With Plastic Waste Management35The role of the Pt-group dehydrogenation catalyst in alkane metathesis for polyolefin deconstruction9Tailored Ru Catalysts on Gamma Alumina: Enhancing Polyethylene Hydrogenolysis for High-Value Liquid Fuel Production10Hydrocracking of Polyethylene to Gasoline-Range Hydrocarbons over a Ruthenium-Zeolite Bifunctional Catalyst System with Optimal Synergy of Metal and Acid Sites9Ru-Catalyzed Polyethylene Hydrogenolysis under Quasi-Supercritical Conditions25Predicting a generalized mechanism of branched alkane hydrogenolysis on Ru, Ir, and Pt surfaces relevant to polymer upcycling applications3Plastic-waste hydrogenolysis over two-dimensional MXene-supported ruthenium catalysts with tunable interlayer spacing3The silent partner in catalysis: How support architectures dictate efficiency in polyolefin hydrogenolysis1Chemical recycling of polyethylenes with low gas products by catalytic hydrogenolysis with heterogeneous CeO2-supported Cu-doped Ru catalyst5Polymer Upcycling by Catalytic Hydrogenolysis: The Role of Polyolefin Short-Chain Branching3Surface-doped Ru over WO3 nanocubes for highly selective and ppb-concentration 1-octen-3-ol sensing3Hydrogen-Free Catalytic Strategies for the Upcycling of Polyolefin Plastics3Synergy Effects in a Bimetallic Ru ─ Pt Alloy Catalyst for Low‐H 2 ‐Pressure Hydrogenolysis of Low‐Density Polyethylene3Synergistically photothermocatalytic hydrogenolysis of waste plastics over the robust ultrafine Ru cluster catalysts3Surface and Interface Properties of Metal Species for Waste Plastic Hydroconversion6Sustainable polyolefin upcycling using liquid organic hydrogen carrier based hydrogen delivery and hydrocracking11Enhancing selectivity and yield in polyethylene hydrogenolysis using goal-aware Bayesian algorithm execution0Dehydrogenation of 5-hydroxymethylfurfural to 2,5-diformylfuran over Ru nanoparticles anchored on functionalized UiO-663Preparing methane‐resistant Ru catalysts via moderate metal‐support interactions for polyethylene hydrogenolysis0Catalytic Upcycling of Polyolefins and Polystyrene: Integrating Active Site Design With Mass Transfer Considerations4NiW alloy catalyst for methane suppression in polyethylene hydrogenolysis to enhance liquid hydrocarbon yields1Precision bond cleavage in waste plastics: Directed catalytic upcycling1A Review on Catalyst Chemical Recycling Technologies for Production of Light Gaseous Compounds from Polyolefin Waste1Catalytic Hydrogenolysis of Polyethylene-Based Plastics into Fuels Using Ruthenium Catalysts Supported on Micro/Mesoporous Carbons0Highly active and selective heterogeneous Ru/La2O3-CeO2 catalyst for hydrogenolysis of LDPE to valuable chemicals0

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  1. Size and Structure Effects of Carbon-Supported Ruthenium Nanoparticles on Waste Polypropylene Hydrogenolysis Activity, Selectivity, and Product Microstructure

    ACS Catalysis · 2024-02-15

    Jessie A. Sun, Pavel A. Kots, Zachary R. Hinton, Nebojša Marinković, Lu Ma, Steven N. Ehrlich, Weiqing Zheng, Thomas H. III Epps, LaShanda T. J. Korley, Dionisios G. Vlachos

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  2. Polyethylene hydrogenolysis over bimetallic catalyst with suppression of methane formation

    Frontiers of Chemical Science and Engineering · 2024-06-24

    Xiangkun Zhang, Bingyan Sun, Zhigang Zhao, Tan Li, Marc Mate, Kaige Wang

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  3. Catalytic Approaches to Tackle Mixed Plastic Waste Challenges: A Review

    Langmuir · 2024-08-07

    Taeeun Kwon, Huijeong Jeong, M.J. Kim, Sungyup Jung, Insoo Ro

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  4. Catalytic Upcycling of Polyolefins

    Chemical Reviews · 2024-08-16

    Jia‐Kai Sun, Jinhu Dong, Lijun Gao, Yu‐Quan Zhao, Hyunjin Moon, Susannah L. Scott

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  5. The role of size and structure of catalytic active sites in polyolefin hydrogenolysis

    Chem Catalysis · 2024-08-20

    Jueun Kim, Simin Sun, Donghyeon Kim, Byung Gwan Park, Hojeong Lee, Wenyu Huang, Kwangjin An

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  6. Green synthesis of Bio-CuS quantum dots by sulfate reducing bacteria for solid-phase photocatalytic degradation of polyethylene film

    Separation and Purification Technology · 2024-08-25

    Jian Cheng, Xu Wang, Gongchu Shi, Shihao Zhang, Yanyu Zhou, Yanchao Cui, Jia Wang, Baoping Xin

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  7. Unraveling the role of water in mechanism changes for economically viable catalytic plastic upcycling

    Nature Communications · 2024-11-29

    Taeeun Kwon, Byeongchan Ahn, Ki Hyuk Kang, Wangyun Won, Insoo Ro

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  8. Reaction engineering of the hydrogenolysis of liquid n-Alkanes: Comparison of flow and batch reaction systems

    Chemical Engineering Journal Advances · 2024-12-28

    Zhuoming Feng, Siwon Lee, Raymond J. Gorte, John M. Vohs

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  9. Complementary acid site mechanisms in hydrogen-free polyethylene upcycling: elucidating the distinct roles of Brønsted and Lewis sites in Ce-modified zeolites

    Green Chemistry · 2025-01-01

    Taeeun Kwon, J. S. PARK, Ki Hyuk Kang, Dae-Sung Jung, Wangyun Won, Insoo Ro

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  10. Synergistic effect of acidic sites and mesoporous confinement in Ce-doped Ru/SBA-15 catalysts for efficient hydrogenolysis of low-density polyethylene to liquid fuels

    Catalysis Science & Technology · 2025-01-01

    Zhibin Ren, Zhicheng Luo, Huiyan Zhang

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  11. Mechanistic Insights into Polypropylene Hydrogenolysis Using Ni/Al2O3 Catalysts

    Energy & Fuels · 2025-01-10

    Xiyan Huang, Weixin Meng, Diego A. Acevedo–Guzmán, Hongqi Wang, Balaji Sridharan, Petra Rudolf, Hero Jan Heeres, Jingxiu Xie

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  12. Crucial role of pre-treatment in plastic photoreforming for precision upcycling

    npj Materials Sustainability · 2025-01-16

    Xiandi Zhang, Wenhan Zu, Lawrence Yoon Suk Lee

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  13. Tandem Catalysis for Plastic Depolymerization: In Situ Hydrogen Generation via Methanol Aqueous Phase Reforming for Sustainable Polyethylene Hydrogenolysis

    Angewandte Chemie · 2025-01-22

    Junsung Lee, Taeeun Kwon, Ki Hyuk Kang, Wangyun Won, Insoo Ro

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  14. Tandem Catalysis for Plastic Depolymerization: In Situ Hydrogen Generation via Methanol Aqueous Phase Reforming for Sustainable Polyethylene Hydrogenolysis

    Angewandte Chemie International Edition · 2025-01-22

    Junsung Lee, Taeeun Kwon, Ki Hyuk Kang, Wangyun Won, Insoo Ro

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  15. Reductive Upcycling of Polyolefins, Polyesters and Mixed Plastic Wastes to Valuable Chemicals: Bridging Chemical Catalysis With Plastic Waste Management

    Advanced Sustainable Systems · 2025-03-20

    Sahil Kumar, Devanshu Sajwan, Devendra Sharma, Venkata Krishnan

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  16. The role of the Pt-group dehydrogenation catalyst in alkane metathesis for polyolefin deconstruction

    Journal of Catalysis · 2025-03-21

    Selena Moore, Andrew Tran, Andreas Palmateer, Jose Naranjo Mendez, Dimitri Gatzios, Peter A. Eschbach, Joel Miscall, Lucas D. Ellis

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  17. Tailored Ru Catalysts on Gamma Alumina: Enhancing Polyethylene Hydrogenolysis for High-Value Liquid Fuel Production

    ACS Sustainable Chemistry & Engineering · 2025-03-26

    Yumeng Zhang, Li Gao, Ying Zhang, Xia Zhong, Zhuangzhi Zhi, Bingsen Zhang

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  18. Hydrocracking of Polyethylene to Gasoline-Range Hydrocarbons over a Ruthenium-Zeolite Bifunctional Catalyst System with Optimal Synergy of Metal and Acid Sites

    Catalysts · 2025-03-31

    Qing Bo Du, Xin Chun Shang, Yangyang Yuan, Xiong Su, Yanqiang Huang

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  19. Ru-Catalyzed Polyethylene Hydrogenolysis under Quasi-Supercritical Conditions

    JACS Au · 2025-04-16

    Sung Min Kim, Boda Yang, Oliver Y. Gutiérrez, Wei Zhang, Carlos Lizandara‐Pueyo, Piyush Ingale, Ivana Jevtovikj, Reni Grauke, János Szanyi, Huamin Wang, Stephan A. Schunk, Johannes A. Lercher

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  20. Predicting a generalized mechanism of branched alkane hydrogenolysis on Ru, Ir, and Pt surfaces relevant to polymer upcycling applications

    Journal of Catalysis · 2025-05-08

    Andy Simonson, Lydia Thies, David D. Hibbitts

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  21. Plastic-waste hydrogenolysis over two-dimensional MXene-supported ruthenium catalysts with tunable interlayer spacing

    Chem Catalysis · 2025-07-16

    Ali Kamali, Joshua M. Little, Song Luo, Amy Y. Chen, Akash Warty, Antara Bhowmick, Jorge Moncada, Evan P. Jahrman, Brandon C. Vance, Jong Kahk Keum, Taylor J. Woehl, Po‐Yen Chen, Dionisios G. Vlachos, Dongxia Liu

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  22. The silent partner in catalysis: How support architectures dictate efficiency in polyolefin hydrogenolysis

    Nano Research · 2025-08-22

    Xueping Zhang, Wenli Wang, Mei Hong, Yamei Lin, Guoping Lu

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  23. Chemical recycling of polyethylenes with low gas products by catalytic hydrogenolysis with heterogeneous CeO2-supported Cu-doped Ru catalyst

    Journal of Catalysis · 2025-09-11

    Masazumi Tamura, Yuna Sasano, SMA Hakim Siddiki, Masato Akatsuka, Pengru Chen, Yusuke Kita

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  24. Polymer Upcycling by Catalytic Hydrogenolysis: The Role of Polyolefin Short-Chain Branching

    ACS Catalysis · 2025-09-23

    Zachary M. Gdowski, Rishi Raj, Aditya Bhan, K. Andre Mkhoyan, Mahesh K. Mahanthappa, Frank S. Bates

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  25. Surface-doped Ru over WO3 nanocubes for highly selective and ppb-concentration 1-octen-3-ol sensing

    Talanta · 2025-10-01

    Tingting Wang, Xinhua Zhao, Zhenxu Li, Yi Zhang, Zhu Zhang, Dachi Yang

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  26. Hydrogen-Free Catalytic Strategies for the Upcycling of Polyolefin Plastics

    Korean Journal of Chemical Engineering · 2025-10-20

    Taeeun Kwon, Jae Woo Kim, Insoo Ro

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  27. Synergy Effects in a Bimetallic Ru ─ Pt Alloy Catalyst for Low‐H 2 ‐Pressure Hydrogenolysis of Low‐Density Polyethylene

    Chemistry - A European Journal · 2025-11-02

    Yukari Yamazaki, Xiongjie Jin, Weihan Sun, Satoshi Yamamoto, Katsutoshi Nomoto, Kohei Takahashi, Hiroki Miura, Tetsuya Shishido, Akira Nakayama, Kyoko Nozaki

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  28. Synergistically photothermocatalytic hydrogenolysis of waste plastics over the robust ultrafine Ru cluster catalysts

    Chemical Engineering Journal · 2025-11-24

    Xin Zhou, Shule Zhang, Zhixing Hao, Zeya Li, Zhiquan Hou, Zhiwei Wang, Lu Wei, Jiguang Deng, Hongxing Dai, Yuxi Liu

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  29. Surface and Interface Properties of Metal Species for Waste Plastic Hydroconversion

    ACS Catalysis · 2025-12-10

    Fan Yuan, Hongshun Ran, Tingxi Chen, Yaxuan Jing

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  30. Sustainable polyolefin upcycling using liquid organic hydrogen carrier based hydrogen delivery and hydrocracking

    Nature Communications · 2025-12-24

    Taeeun Kwon, Seoyoung Ahn, Taehyup Kim, Jong Hun Kang, Soo-Hwa Jeong, Ki Hyuk Kang, Wangyun Won, Insoo Ro

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  31. Enhancing selectivity and yield in polyethylene hydrogenolysis using goal-aware Bayesian algorithm execution

    Digital Discovery · 2026-01-01

    Makenna L. Pennel, Akash Ramdas, Sean Gasiorowski, Sathya R. Chitturi, Willie Neiswanger, Nicholas Broadbent, Mike Dunne, Felipe H. da Jornada, Daniel Ratner, Christopher J. Tassone, Matteo Cargnello

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  32. Dehydrogenation of 5-hydroxymethylfurfural to 2,5-diformylfuran over Ru nanoparticles anchored on functionalized UiO-66

    Applied Catalysis A General · 2026-02-17

    Rui Zhu, yuxuan Zhou, Fang Gao, Fujun Yu, LIANG ZHANG

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  33. Preparing methane‐resistant Ru catalysts via moderate metal‐support interactions for polyethylene hydrogenolysis

    AIChE Journal · 2026-03-16

    Yiwei Fang, Yundao Jing, Jinquan Ming, Wenjie Wang, Weixiao Sun, Xiaohu Ge, Wenyao Chen, Gang Qian, Yueqiang Cao, Xuezhi Duan, Xinggui Zhou, Jing Zhang

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  34. Catalytic Upcycling of Polyolefins and Polystyrene: Integrating Active Site Design With Mass Transfer Considerations

    ChemSusChem · 2026-03-29

    Xinlei Han, Jie Sun, Jiuxuan Zhang, Zhengyan Qu, Hong Jiang, Zhenchen Tang, Rui Chen

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  35. NiW alloy catalyst for methane suppression in polyethylene hydrogenolysis to enhance liquid hydrocarbon yields

    Fuel · 2026-04-17

    Bingyan Sun, Zhigang Zhao, Marc Mate, Jing Su, Linjia Yin, Kaige Wang

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  36. Precision bond cleavage in waste plastics: Directed catalytic upcycling

    Renewable and Sustainable Energy Reviews · 2026-04-25

    Yusong Zhang, Yinxiang Wang, Aimin Li

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  37. A Review on Catalyst Chemical Recycling Technologies for Production of Light Gaseous Compounds from Polyolefin Waste

    Processes · 2026-06-09

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  38. Catalytic Hydrogenolysis of Polyethylene-Based Plastics into Fuels Using Ruthenium Catalysts Supported on Micro/Mesoporous Carbons

    Energy & Fuels · 2026-07-07

    Antigoni G. Margellou, Eleftherios Tosounidis, Kyriazis C. Rekos, Konstantinos S. Triantafyllidis

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  39. Highly active and selective heterogeneous Ru/La2O3-CeO2 catalyst for hydrogenolysis of LDPE to valuable chemicals

    Chemical Engineering Journal · 2026-09-18

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