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RESEARCH PAPER · Journal of the American Chemical Society · 2024

Stable Interfacial Ruthenium Species for Highly Efficient Polyolefin Upcycling

Ping Hu, Congyang Zhang, Mingyu Chu, Xianpeng Wang, Lu Wang, Youyong Li, Tianran Yan, Liang Zhang, Zhifeng Ding, Muhan Cao, Panpan Xu, Yifan Li, Yi Cui, Qiao Zhang, Jinxing Chen, Lifeng Chi

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Stable Interfacial Ruthenium Species for Highly Efficient Polyolefin UpcyclingOriginalShell biorefineries: mixed biofuel production from chitin5Mechanistic Insight into Heteroatom Removal from Vacuum Gas Oil Blended with PMMA or PET Waste4Catalytic chemical recycling and upcycling of polyolefin plastics27Recent advances in polyolefin plastic waste upcycling via mild heterogeneous catalysis route from catalyst development to process design25Unlocking opportunities: Supported metal catalysts for the chemical upcycling of waste plastics26Industrial and Laboratory Technologies for the Chemical Recycling of Plastic Waste70Catalytic Upcycling of Polyolefins316The role of size and structure of catalytic active sites in polyolefin hydrogenolysis12Interfacial Reactions in Chemical Recycling and Upcycling of Plastics18Ultra‐Narrow Alkane Product Distribution in Polyethylene Waste Hydrocracking by Zeolite Micro‐Mesopore Diffusion Optimization12Ultra‐Narrow Alkane Product Distribution in Polyethylene Waste Hydrocracking by Zeolite Micro‐Mesopore Diffusion Optimization66Hydroconversion of waste polyethylene plastics under mild conditions using mechanically mixed bifunctional catalysts: Impact of metal-acid balance and proximity9Production of Branched Alkanes by Upcycling of Waste Polyethylene over Controlled Acid Sites of SO 4 /ZrO 2 ‐Al 2 O 3 Catalyst27Production of Branched Alkanes by Upcycling of Waste Polyethylene over Controlled Acid Sites of SO 4 /ZrO 2 ‐Al 2 O 3 Catalyst6Efficient Hydrogenolysis of Consumer-Grade High-Density Polyethylene Wastes over MgAl-Layered Double Oxide-Supported Ru Catalysts11Enhancing the Conversion Efficiency of Polyethylene to Methane through Codoping of Mn Atoms into Ru Centers and CeO2 Supports37Polyethylene hydrogenolysis by dilute RuPt alloy to achieve H2-pressure-independent low methane selectivity70Recent Progress for Designing of Catalysts for Photothermal Conversion of Plastic Wastes48Highly Selective, Catalyst‐Free, and Low Temperature Depolymerizable Styrene Copolymer With Incorporated α‐Methylstyrene Structural Units3Co-upcycling of mixed polypropylene and polyesters5Effective production of liquid/wax fuels from polyethylene plastics using Ru/Al 2 O 3 catalysts10Selective hydrocracking of polyolefin waste into branched liquid fuels over a non-noble metal bifunctional Ni–W/ZrO 2 catalyst4Upgrading of waste polyolefins with non-noble metal catalysts21Mechanistic Insights into Polypropylene Hydrogenolysis Using Ni/Al2O3 Catalysts17Ruthenium‐Catalyzed Deconstruction of Polyolefins: A Strategy to Up‐cycle Waste Polyethylene to Value‐Added Alkene1Ruthenium‐Catalyzed Deconstruction of Polyolefins: A Strategy to Up‐cycle Waste Polyethylene to Value‐Added Alkene20Tandem Catalysis for Plastic Depolymerization: In Situ Hydrogen Generation via Methanol Aqueous Phase Reforming for Sustainable Polyethylene Hydrogenolysis2Tandem Catalysis for Plastic Depolymerization: In Situ Hydrogen Generation via Methanol Aqueous Phase Reforming for Sustainable Polyethylene Hydrogenolysis27Soluble polymer microenvironments promote photocatalytic hydrogen peroxide production and self-Fenton reactions9Highly selective upcycling of plastic mixture waste by microwave-assisted catalysis over Zn/b-ZnO68Hydrocarbon Deposition during Polyolefin Upcycling: Irreversible Adsorption and Surface Reactions of Polyethylene and Ethylene Oligomers on Silica Supports2Advances and Challenges in Low‐Temperature Upcycling of Waste Polyolefins via Tandem Catalysis25Advances and Challenges in Low‐Temperature Upcycling of Waste Polyolefins via Tandem Catalysis2Upgrading polyolefin plastics: experiences from petroleum refining and distinct characteristics19Reductive Upcycling of Polyolefins, Polyesters and Mixed Plastic Wastes to Valuable Chemicals: Bridging Chemical Catalysis With Plastic Waste Management35Polyolefin Recycling with Binary Cobalt–Nickel Nanosheets6Synergistic Co‐Recycling: Selective Oxidation of Polyethylene to Dicarboxylic Acids over Spent LiCoO 2 Cathodes22Synergistic Co‐Recycling: Selective Oxidation of Polyethylene to Dicarboxylic Acids over Spent LiCoO 2 Cathodes3Metal Synergistic Dual Activation Enables Efficient Transesterification by Multinuclear Titanium Catalyst: Recycling and Upcycling of Polyester Waste25Metal Synergistic Dual Activation Enables Efficient Transesterification by Multinuclear Titanium Catalyst: Recycling and Upcycling of Polyester Waste7Enhancing Waste Plastic Hydrogenolysis on Ru/CeO 2 Through Concurrent Incorporation of Fe Single Atoms and FeO x Nanoclusters27Enhancing Waste Plastic Hydrogenolysis on Ru/CeO 2 Through Concurrent Incorporation of Fe Single Atoms and FeO x Nanoclusters4Co-recycling of plastics and other waste materials70Synergistic Catalysis for Recycling and Upcycling of Plastics35Sustainable catalytic upcycling of medical face mask wastes into hydrocarbon-rich gases for potential carbonaceous nanomaterial production4Intentional corrosion-induced asymmetric charge on Ru/nZVI-Ni for efficient atomic hydrogen-mediated dechlorination: Microsolvation effects5Mechanistic alteration of polyethylene oxidation via heterogenous catalysis for enhanced fatty di-carboxylic acid yields6Methods for Carbon Mass Closure in Polyolefin Hydrocracking6Low‐temperature hydrodeoxygenation of fatty acids to biodiesel via Ru–Mo strong metal‐support interaction7Tandem Catalysis to Mitigate Coke Formation in the Upcycling of Mixed Polyolefin Wastes11CO-promoted polyethylene hydrogenolysis with renewable formic acid as hydrogen donor20The silent partner in catalysis: How support architectures dictate efficiency in polyolefin hydrogenolysis1Stable single-site organonickel catalyst preferentially hydrogenolyses branched polyolefin C–C bonds12Chemical recycling of polyethylenes with low gas products by catalytic hydrogenolysis with heterogeneous CeO2-supported Cu-doped Ru catalyst5Orchestrating catalytic hotspots and macromolecular architectures: molecular engineering toward zero-waste polymer circularity4Closed-loop recycling of polyethylene to ethylene and propylene via a kinetic decoupling–recoupling strategy32Fine regulation of Ru species improved the polyethylene hydrogenolysis performance over Ru/Al 2 O 3 catalyst5Synergy Effects in a Bimetallic Ru ─ Pt Alloy Catalyst for Low‐H 2 ‐Pressure Hydrogenolysis of Low‐Density Polyethylene3Water-Modulated Ru Catalysis: Overcoming the Activity-Selectivity Trade-Off in C–O Bond Cleavage1Plasma Catalysis for Plastic Waste Conversion into Value‐Added Products: Advancements and Perspectives11Polyethylene hydrogenolysis to liquid products over bimetallic catalysts with favorable environmental footprint and economics17Oriented Mechanism in Ru-Catalyzed Hydro-Dehalogenation: Synergistic Effect of Electron-Rich Microenvironment and Lewis Acid1Tandem depolymerization-electrocatalysis for plastic waste upcycling6Surface and Interface Properties of Metal Species for Waste Plastic Hydroconversion6Electrocatalytic dechlorination of polyvinylidene chloride for tandem dual radical-driven synthesis of β-chloroalcohols0Entropy Engineering for the Efficient Hydrogenolysis of Waste Polyolefins1Mechanistic insights into plastic degradation via catalytic bond breaking: a comprehensive review1Recycling of Polyvinyl Chloride with Polypropylene Derivative0Electronegativity-driven d-band center shifts in Ru–Ni alloys for low methane hydrogenolysis of polyolefin plastics2Influence of chlorine impurities on chemical recycling of plastic waste and adsorptive dechlorination0The effect of organic additives on catalyst structure and performance for the hydrogenation of CO bonds0Tuning ruthenium states for enhanced polyethylene hydroconversion over HZSM-5 catalysts0Acid sites in hydrogen-involved polyolefin upcycling: mechanistic insights and design principles0Hydrocracking Polyolefins to Jet Fuel over a NiW/WO x Catalyst2Rational design of bifunctional catalysts for hydrocracking of polyethylene waste plastics to narrow-distributed liquid fuels4Hydrogenolysis Versus Hydrocracking for Polyolefin Upcycling0One-pot co-upcycling of mixed polyolefin waste6Tailoring the polyolefin hydrogenolysis performance of Ru/TiO2 through TiO2 support facet engineering1Structure–performance relationships in heterogeneous catalysts for polyolefin plastic hydroconversion1Interfacial configurational entropy tuning strategy enabling liquid alloys for efficient depolymerization of polyolefin waste2Preparing methane‐resistant Ru catalysts via moderate metal‐support interactions for polyethylene hydrogenolysis0Catalytic Upcycling of Polyolefins and Polystyrene: Integrating Active Site Design With Mass Transfer Considerations4Highly Selective Gasoline Production by Polyethylene Hydrogenolysis Using Ternary RuNiPt Nanoalloy Catalyst1Engineering Interfacial Compatibility and Dynamic Active Hydrogen Pools to Accelerate Polyolefin Hydrogenolysis0Manipulation of the microenvironment of Pt nanoparticles via surface molecular design strategy encapsulated in metal-organic frameworks for enhanced photocatalytic performance0Ni Supported on Urea‐Modified LaFeO 3 Perovskite for Efficient Hydrogenolysis of Polyethylene Plastics2A Panoramic View on Plastic Waste Recycling and Upcycling: Heterogeneous Catalytic Strategies for Diverse Plastics and Multiple Pathways6Well‐Defined Heterocatalysts for Plastic Upcycling: From Design to Applications3Atomically precise catalysts design toward efficient waste plastic hydrogenolysis2Advances in Catalytic Hydrogenolysis of Waste Plastics to Value-Added Products0Unlocking sustainable potential of photo-aged polyolefins in land and sea: An urchin-like Ru/CeO2 catalytic strategy for production of hydrocarbon fuels and waxes0Tailored CuPd nanoclusters with stabilized Cu+: synergistic catalysis for furfural hydrogenation0A Mesopore-Confined and Graphene Oxide-Localized Ruthenium Catalyst Increases Rates of Mid-Chain Polyolefin Hydrogenolysis0Design and analysis of a new Ru-Cu/ZSM-5 bimetallic catalyst for hydrogenolysis of polyolefin waste0Comprehensive quantitative analysis of polyolefin hydrogenolysis toward plastic waste management0Upgrading Polyolefin Plastics Into Ethanol Using an Integrated Hydrothermal‐Photoelectrocatalytic Strategy0Ambient‐Pressure Polyolefin Upcycling With Earth‐Abundant Catalyst0Ambient‐Pressure Polyolefin Upcycling With Earth‐Abundant Catalyst0Ru Single‐Atom Anchored Zeolite for Selective Upcycling of Polyolefins Into Butanes0Ru Single‐Atom Anchored Zeolite for Selective Upcycling of Polyolefins Into Butanes0Efficient and Selective Low-Temperature Polypropylene Hydrogenolysis Using Zr-Doped Mixed Metal Oxides Catalysts0Hierarchical Accessibility and Framework‐Al Organization in Ultra‐High‐Silica ZSM‐5 Enable Efficient Cracking of Polyolefin Waste to Light Olefins0Hierarchical Accessibility and Framework‐Al Organization in Ultra‐High‐Silica ZSM‐5 Enable Efficient Cracking of Polyolefin Waste to Light Olefins0Defect-Engineered Pd/ZSM-5 for Hydroconversion of LDPE to Light Alkanes0

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