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RESEARCH PAPER · Chemistry of Materials · 2019

Engineering of K3YSi2O7To Tune Photoluminescence with Selected Activators and Site Occupancy

Jianwei Qiao, Mahdi Amachraa, Мaxim S. Моlokeev, Yu‐Chun Chuang, Shyue Ping Ong, Qinyuan Zhang, Zhiguo Xia

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Engineering of K3YSi2O7To Tune Photoluminescence with Selected Activators and Site OccupancyOriginalPhotoluminescence Control of UCr 4 C 4 -Type Phosphors with Superior Luminous Efficiency and High Color Purity via Controlling Site Selection of Eu 2+ Activators112Unified Theory of Thermal Quenching in Inorganic Phosphors0Divalent europium-doped near-infrared-emitting phosphor for light-emitting diodes660A K 3 ScSi 2 O 7 :Eu 2+ based phosphor with broad-band NIR emission and robust thermal stability for NIR pc-LEDs109Crystal structure, theoretical studies and luminescent properties of a new borate Na 3 GdB 8 O 15 with one-dimensional broad-banded anionic framework13Discovery of a Ce 3+ -activated red nitride phosphor for high-brightness solid-state lighting39Full-visible-spectrum lighting realized by a novel Eu 2+ -doped cyan-emitting borosilicate phosphor25Tunable thermal quenching properties of Na 3 Sc 2 (PO 4 ) 3 :Eu 2+ phosphors tailored by phase transformation details37Highly Efficient Green‐to‐Yellowish‐Orange Emitting Eu2+‐Doped Pyrophosphate Phosphors with Superior Thermal Quenching Resistance for w‐LEDs99Multisite-Occupancy-Driven Intense Narrow-Band Blue Emission from Sr 5 SiO 4 Cl 6 :Eu 2+ Phosphor with Excellent Stability and Color Performance69Site-selective occupation of Eu2+ activators toward full-visible-spectrum emission in well-designed borophosphate phosphors96Cation-Deficiency-Induced Crystal-Site Engineering for ZnGa2O4:Mn2+ Thin Film29Thermally Stable Phosphor KBa2(PO3)5:Eu2+ with Broad-Band Cyan Emission Caused by Multisite Occupancy of Eu2+57A dual-excited emission phosphor Eu3+/Eu2+ co-doped Ca4Si2O7F2: Lattice occupancy and luminescence characterization15Data-Driven Photoluminescence Tuning in Eu2+-Doped Phosphors76Predicting Thermal Quenching in Inorganic Phosphors149Identification of Dy 3 + / Dy 2 + as Electron Trap in Persistent Phosphors100Two targets with one strategy: Insights into the role of aluminum atoms on the luminescence properties and thermal stability in Mn4+-doped calcium aluminozincate phosphor16Great emission enhancement of high-efficient broadband K3YSi2O7: Eu red phosphor via enhancing crystallinity43Structural Engineering of Eu2+-Doped Silicates Phosphors for LED Applications242Hetero-valent substitution strategy toward orange-red luminescence in Bi3+ doped layered perovskite oxide phosphors for high color rendering index white light-emitting diodes105A novel Eu2+-activated calcium zirconium silicate phosphor: Ca3ZrSi2O9:Eu2+23Complex crystal structure and photoluminescence of Bi 3+ -doped and Bi 3+ /Eu 3+ co-doped Ca 7 Mg 2 Ga 6 O 1819Site engineering strategy toward enhanced luminescence thermostability of a Cr 3+ -doped broadband NIR phosphor and its application107Very stable and high-quantum-yield phosphor Na 2 BaSr(PO 4 ) 2 :Eu 2+ for plant growth LEDs42Design of Novel Highly Efficient Yellow-Orange Color-Tunable Luminescence in Rb2Sr1–yCayP2O7:xEu2+ Solid Solutions for White Light-Emitting Diodes24Thermally stable and highly efficient red-emitting Eu3+-doped Cs3GdGe3O9 phosphors for WLEDs: non-concentration quenching and negative thermal expansion480Learning from Mineral Structures toward New Luminescence Materials for Light-Emitting Diode Applications146Charge transfer from Eu2+ to trivalent lanthanide co-dopants: Systematic behavior across the series27Eu 2+ Stabilized at Octahedrally Coordinated Ln 3+ Site Enabling Red Emission in Sr 3 LnAl 2 O 7.5 (Ln = Y or Lu) Phosphors61Effect of the anion on the luminescence properties of Bi3+-doped X-mayenite (X=O, F, Cl) phosphors8Full-visible-spectrum emission with high color rendering index and low correlated color temperature enabled by a single-phased phosphor of α-Sr2V1.98P0.02O7: 0.5% Eu3+19Lattices selective occupation, optical spectra regulation, and photoluminescence properties of Eu2+ activated Ca9La(PO4)7 phosphor19Rapid Synthesis of Red‐Emitting Sr2Sc0.5Ga1.5O5:Eu2+ Phosphors and the Tunable Photoluminescence Via Sr/Ba Substitution90Design principles for achieving red emission in Eu2+/Eu3+ doped inorganic solids83Photoluminescence tuning in Ba3ScB3O9:Eu2+ phosphor by crystal-site engineering17Broadband excited Na 3 Tb(PO 4 ) 2 :Ce 3+ /Eu 2+ green/yellow‐emitting phosphors with high color purity for LED‐based application15Warm white light emission, thermochromic property and long persistent luminescence derived from multi-sites of Eu2+/Eu3+ in host lattice71Design of a broadband cyan-emitting phosphor with robust thermal stability for high-power WLED application52Tunable Luminescence of Ce 3 +/Eu 2 + Activated in Single-Phase Li 2 BaSiO 4 Phosphor via Energy Transfer3Exploration of the structural, spectroscopic and thermal properties of double sulfate monohydrate NaSm(SO4)2·H2O and its thermal decomposition product NaSm(SO4)220Giant Red‐Shifted Emission in (Sr,Ba)Y 2 O 4 :Eu 2+ Phosphor Toward Broadband Near‐Infrared Luminescence230Achievement of high-efficiency sunlight-like emission in Rb2CaP2O7: Ce3+, Eu2+ phosphors16Achieving zero-thermal quenching luminescence in ZnGa2O4: 0.02Eu3+ red phosphor47A new type of phosphate-based phosphor Na 3 CsMg 7 (PO 4 ) 6 :Eu 2+ /Mn 2+ with high quantum efficiency and high thermostability24Achieving highly thermostable red emission in singly Mn 2+ -doped BaXP 2 O 7 (X = Mg/Zn) via self-reduction36Dual-Site Occupancy Induced Blue Emission in Both Eu2+ and Ce3+ Doped Naba3si2o7f0Self-reduction-induced BaMgP 2 O 7 :Eu 2+/3+ : a multi-stimuli-responsive phosphor for X-ray detection, anti-counterfeiting and optical thermometry36Tunable concentration/excitation-dependent deep-red and white light emission in single-phase Eu 2+ -activated Sc-based oxide phosphors for blue/UV-LEDs32Sn4+ induced Bi3+ multi-lattice selective occupation and its color-tunable emission of La2MgZrO6: Bi3+, Sn4+ double perovskite phosphors24Tendentious multiple sites occupation towards white light emission in single-phase Ba2(1-/3)Ca(1-/3)Sr B2Si4O14:Eu2+ phosphors16Competitive Site Occupation toward Improved Quantum Efficiency of SrLaScO 4 :Eu Red Phosphors for Warm White LEDs103Eu2+ Doping Concentration-Induced Site-Selective Occupation and Photoluminescence Tuning in KSrScSi2O7:Eu2+ Phosphor77Near‐Infrared Light‐Emitting Diodes utilizing a Europium‐Activated Calcium Oxide Phosphor with External Quantum Efficiency of up to 54.7%320Multiple Charge Transfer Bands Induced Broad Excitation Eu3+ Red Emission in a Vanadium Phosphate System for White Light-Emitting Diodes22Dual-mode optical thermometry design in K 3 YSi 2 O 7 :Eu multi-site phosphor8A novel sulfide phosphor, BaNaAlS3:Eu2+, discovered via particle swarm optimization24Low-concentration Ce3+-activated ScCaO(BO3) blue-cyan phosphor with high efficiency toward full-spectrum white LED applications58Luminescence Enhancement of Red‐Emitting Sr9MnK(PO4)7 Phosphor via Energy Transfer and Charge Compensation3A new optical temperature sensor based on the fluorescence intensity ratio of Mn 2+ and Mn 4+19Exploring the structural stability and optical properties of rare-earth doped K3LuSi2O7 phosphor from first-principles calculations4Ultra‐Broadband Green‐Emitting Phosphors without Cyan Gap Based on Double‐Heterovalent Substitution Strategy for Full‐Spectrum WLED Lighting89A novel Cr3+-doped stannate far red phosphor for plant lighting: structure evolution, broad-narrow spectrum tuning and application prospect39Environmentally-friendly and low-cost Fe3+-doped broadband NIR light-emitting phosphors54Ultra-broad NIR emission from two-site Cr3+ occupation in fluoride phosphor via composition-driven structural transformation41Multichannel Control of PersL/Upconversion/Down-Shifting Luminescence in a Single Core–Shell Nanoparticle for Information Encryption32Design of novel cyan phosphor Ca7NaLu(PO4)6:Eu2+ for full-visible-spectrum white LED: enhanced thermal stability and tuned emission by neighbor cation effect30Study on luminescence properties of Bi3+ doped Ba2YAlO5：A wide-band yellow emitting phosphor with excellent thermal stability20Ceramics phosphor powders4Dysprosium site occupancy in SrZnO 2 nanophosphors probed through XANES0Red Emitting Phosphors for Display and Lighting Applications1Simultaneous realization of tunable luminescence and enhanced thermal stability in Eu2+-based blue-green phosphors for multifunctional applications16Enhancement on Tb3+ luminescence in CaScBO4-based ceramic phosphors by Ce3+-induced resonance energy transfer and the generation of white light emission collaborated with Mn2+10A self-referenced fluorescence intensity ratio optical temperature sensing materials K3YSi2O7:Bi3+/Sm3+based on multi-strategy combination32Efficient, stable, broadband cyan‐emitting Ca‐substituted Ba 9 Lu 2 Si 6 O 24 :Eu 2+ with multisite luminescence for NUV‐wLEDs7Structure and photoluminescence studies of Rb3GdSi2O7: Eu2+ phosphor used for NUV converted white LEDs10Color-tunable persistent luminescence phosphor for multimode dynamic anti-counterfeiting22A novel K3(Y0.88Yb0.10Er0.02)Si2O7 silicate phosphor for multi-mode thermometry of high sensitivity through up-conversion luminescence20The Broadband Emitting and Lattice Occupation Analysis of Eu2+, Eu3+ and Ce3+ co-doped K3YSi2O7 Phosphors0Developing a new persistent luminescence material by introducing cation defects8A Novel Cyan Phosphor (K,Rb) 3 GdSi 2 O 7 :Ce 3+ for Full‐Spectrum Lighting through Local Structure Tailoring48Highly efficient blue‐emitting phosphor via charge compensation strategy and its application for white LED lighting10Highly Efficient Narrow-Band Green-Emitting Na 3 K 5 (Li 3 SiO 4 ) 8 :Eu 2+ Phosphor with Low Thermal Quenching49Effect of lanthanide doping on the optical properties of Barium Yttrium Borate2A polymorphic SrGa 2 O 4 :Eu 2+ red phosphor for warm illumination and operando visualization of H 2 O 2 catalytic reaction4Preparation of a novel violet-excitable Na 3 YSi 2 O 7 :Eu 2+ green phosphor via salt-flux assistance and its luminescence properties15High moisture resistant and thermal stable NaYSiO4:Eu3+ red phosphor with activator protected by cyclic silicon-oxygen tetrahedra13Tunable emission of Ce 3+ in (K, Rb) 3 GdSi 2 O 7 phosphors toward broadband cyan luminescence5Deep‐Red (Sr,Ba)Lu2O4: Eu2+ Phosphor for Full‐Spectrum Lighting7Lattice occupation and luminous properties of the K3YSi2O7:Tm3+,Dy3+ phosphor for NUV-excited white LEDs1A highly sensitive multiple-mode optical thermometer designed in Eu 2+/3+ and Li + co-doped polymorphism compound LaSc 3 (BO 3 ) 432High‐Efficiency Cyan–Green‐Emitting Y 3 Sc 2 Ga 3 O 12 :Ce Phosphor for Microcrystals and Ultrathin Phosphor‐Glass Composite for Light‐Emitting Diode26Efficient violet-light-excitable blue-cyan-emitting Ca2YHf2GaAl2O12:Ce3+ garnet phosphors enable high-color-rendering full-spectrum warm-white LEDs44A yellow-green-emitting phosphor K3LaSi2O7:Eu2+ with superior thermal stability for solid-state lighting9Structure–Photoluminescence Relationship in Ce3+-Doped K5Y(P2O7)2 and Its Sensitization to Dy3+ with Enhanced White Light Emission7A novel red emitting phosphor CaSc2O4:Eu2+ for the warm white LEDs8Achieving successful reduction of Eu3 + to Eu2+ in NaYSiO4 lattice towards lighting & display applications by a two-pronged approach6A Novel Anti-Thermal Quenching Ca9znk(Vo4)7:Sm3+ Phosphor for Highly Sensitive Dual-Modal Optical Thermometer1A novel negative-thermal quenching Ca 9 ZnK(VO 4 ) 7 :Sm 3+ phosphor for a sensitive optical thermometer2Remarkable Thermal Stability of Ca9mgk(Vo4)7:Sm3+ Phosphor for Sensitive Optical Thermometry and Plant-Growth Lighting0Remarkable Thermal Stability of Ca9mgk(Vo4)7:Sm3+ Phosphor For Sensitive Optical Thermometry and Plant-Growth Lighting0Color-Tunable Photoluminescence via Site-Selective Occupancy of Bi3+/Eu3+ and Chemical Composition Modulation in Stable K3YSi2O7 toward wLED and Optical Temperature-Sensing Applications19Achievement of an ultra-broadband deep red phosphor K3Ca0.3Y0.7Si2O7:Eu2+ (phase 1) for phytochrome matching plant-lighting12Novel phosphor K3YSi2O7:Bi3+/ Eu3+ for dual-mode optical thermometry and multicolor anti-counterfeiting13Europium(II) Activated Blue–Cyan Aluminosilicate Phosphors with Zero Thermal Quenching3Remarkable thermal stability of Ca9MgK(VO4)7:Sm3+ phosphor for sensitive optical thermometry and plant-growth lighting4Recent progress in Eu2+ activated red phosphors for white LEDs and laser displays: focusing on efficient host screening and innovative structural design20A Novel Cyan‐Emitting Phosphor K 3 Ca 0.3 Y 0.7 Si 2 O 7 :Ce 3+ Enables Full‐Spectrum Lighting and Fingerprint Detection via Phase‐Structure Alteration9Differential Optical Responses of Robustly Single-Phased K 3 YSi 2 O 7 :Ce/Tb/Gd under Diverse Stimulations toward Optical Thermometry, Dynamic Anticounterfeiting, Optical Storage, and Encryption Applications5A novel narrow-band red-emitting phosphor for lighting and backlight display1Highly thermally stable Ce 3+ /Tb 3+ -activated Ba 2 MgY 2 (BO 3 ) 4 phosphors prepared by a one-step reductive solid-state reaction0Tunable Broadband Red-To-Near-Infrared Emission in Eu 2+ -Activated Sr 1– x Ba x La 2 Sc 2 O 7 Phosphors via Site-Selective Occupation and Cation Substitution3Li+-induced preferential site occupancy and enhanced Eu2+ reduction toward highly efficient blue-emitting Na3RbMg7(PO4)6:Eu2+3Ce 3+ -Sensitized Single-Phase White Emission from Dy 3+ in LiSrY 2 (BO 3 ) 3 with High Thermal Stability under Near-UV Excitation1Highly efficient adjustable photoluminescence with negative thermal expansion/quenching of SrGa2B2O7: Bi/Na/Tb/Eu for LEDs via synergistic alkali metal ions and Sr/O vacancies regulations0Synthesis and luminescence properties of Ba3Y2B6O15: Ce3 +, Eu3+/Eu2+ phosphors with Ca2+-induced auto-reduction for high-performance pc-wLEDs0Sunlight‐Excitable K 3 YSi 2 O 7 : Ce 3+ Green Persistent Luminescence Material for Anti‐Counterfeiting and pc‐WLEDs0

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  3. Divalent europium-doped near-infrared-emitting phosphor for light-emitting diodes

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  10. Multisite-Occupancy-Driven Intense Narrow-Band Blue Emission from Sr 5 SiO 4 Cl 6 :Eu 2+ Phosphor with Excellent Stability and Color Performance

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  14. A dual-excited emission phosphor Eu3+/Eu2+ co-doped Ca4Si2O7F2: Lattice occupancy and luminescence characterization

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  17. Identification of Dy 3 + / Dy 2 + as Electron Trap in Persistent Phosphors

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  19. Great emission enhancement of high-efficient broadband K3YSi2O7: Eu red phosphor via enhancing crystallinity

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  32. Full-visible-spectrum emission with high color rendering index and low correlated color temperature enabled by a single-phased phosphor of α-Sr2V1.98P0.02O7: 0.5% Eu3+

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  33. Lattices selective occupation, optical spectra regulation, and photoluminescence properties of Eu2+ activated Ca9La(PO4)7 phosphor

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  34. Rapid Synthesis of Red‐Emitting Sr2Sc0.5Ga1.5O5:Eu2+ Phosphors and the Tunable Photoluminescence Via Sr/Ba Substitution

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  35. Design principles for achieving red emission in Eu2+/Eu3+ doped inorganic solids

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  36. Photoluminescence tuning in Ba3ScB3O9:Eu2+ phosphor by crystal-site engineering

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  37. Broadband excited Na 3 Tb(PO 4 ) 2 :Ce 3+ /Eu 2+ green/yellow‐emitting phosphors with high color purity for LED‐based application

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  38. Warm white light emission, thermochromic property and long persistent luminescence derived from multi-sites of Eu2+/Eu3+ in host lattice

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  39. Design of a broadband cyan-emitting phosphor with robust thermal stability for high-power WLED application

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  40. Tunable Luminescence of Ce 3 +/Eu 2 + Activated in Single-Phase Li 2 BaSiO 4 Phosphor via Energy Transfer

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  42. Giant Red‐Shifted Emission in (Sr,Ba)Y 2 O 4 :Eu 2+ Phosphor Toward Broadband Near‐Infrared Luminescence

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  43. Achievement of high-efficiency sunlight-like emission in Rb2CaP2O7: Ce3+, Eu2+ phosphors

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  44. Achieving zero-thermal quenching luminescence in ZnGa2O4: 0.02Eu3+ red phosphor

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  48. Self-reduction-induced BaMgP 2 O 7 :Eu 2+/3+ : a multi-stimuli-responsive phosphor for X-ray detection, anti-counterfeiting and optical thermometry

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  49. Tunable concentration/excitation-dependent deep-red and white light emission in single-phase Eu 2+ -activated Sc-based oxide phosphors for blue/UV-LEDs

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  50. Sn4+ induced Bi3+ multi-lattice selective occupation and its color-tunable emission of La2MgZrO6: Bi3+, Sn4+ double perovskite phosphors

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