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RESEARCH PAPER · Accounts of Materials Research · 2020

Structural Engineering of Eu2+-Doped Silicates Phosphors for LED Applications

Ming Zhao, Qinyuan Zhang, Zhiguo Xia

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Structural Engineering of Eu2+-Doped Silicates Phosphors for LED ApplicationsOriginalA solid-solution modulation strategy in trivalent bismuth-doped gallate phosphors for single substrate tunable emission5CaY 2 Al 4 SiO 12 :Ce 3+ ,Mn 2+ : a single component phosphor to produce high color rendering index WLEDs with a blue chip53Complex crystal structure and photoluminescence of Bi 3+ -doped and Bi 3+ /Eu 3+ co-doped Ca 7 Mg 2 Ga 6 O 1819Crystal phase transition and polyhedron transformation towards the evolution of photoluminescence and the improvement of thermal stability in efficient blue-emitting Ba 0.47− x Sr 0.50+ x Al 2 Si 2 O 8 :Eu 2+10Efficient energy transfer from Bi 3+ to Mn 2+ in CaZnOS for WLED application28Novel ultrabright luminescent copper nanoclusters and application in light-emitting devices17Optical and structural properties of the Fe 3+ -doped Lu 3 Al 5 O 12 :Ce 3+ garnet phosphor16Recent progress of effect of crystal structure on luminescence properties of Ce 3+ –Eu 2+ Co-doped phosphors14Recomposition and storage of sunlight with intelligent phosphors for enhanced photosynthesis4Very stable and high-quantum-yield phosphor Na 2 BaSr(PO 4 ) 2 :Eu 2+ for plant growth LEDs42Site-selective excitation and photoluminescence properties of a cyan-emitting NaGd9(SiO4)6O2: Bi3+ phosphor for potential application in white light-emitting diodes32Learning from Mineral Structures toward New Luminescence Materials for Light-Emitting Diode Applications146Eu 2+ Stabilized at Octahedrally Coordinated Ln 3+ Site Enabling Red Emission in Sr 3 LnAl 2 O 7.5 (Ln = Y or Lu) Phosphors61Solution growth of millimeter‐scale Na 2 SiF 6 single crystals for Mn 4+ ‐doping as red phosphor28Role of the Eu3+ Distribution on the Properties of β-Ca3(PO4)2 Phosphors: Structural, Luminescent, and 151Eu Mössbauer Spectroscopy Study of Ca9.5–1.5xMgEux(PO4)733High Quantum Yield Gd4.67Si3O13:Eu3+ Red-Emitting Phosphor for Tunable White Light-Emitting Devices Driven by UV or Blue LED87Synthesis and photoluminescence of high color purity red-emitting BaLaLiTeO6:Eu3+ phosphors24A new solid solution Bi1.48Eu0.52Pb0·5Sr0·5B2O7 and luminescent properties of the Bi2-xPb0.5Sr0·5B2O7:xEu3+ phosphors7Rapid Synthesis of Red‐Emitting Sr2Sc0.5Ga1.5O5:Eu2+ Phosphors and the Tunable Photoluminescence Via Sr/Ba Substitution90Design principles for achieving red emission in Eu2+/Eu3+ doped inorganic solids83Ultra-Broad-Band-Excitable Cu(I)-Based Organometallic Halide with Near-Unity Emission for Light-Emitting Diode Applications168Tailoring of White Luminescence in a NaLi 3 SiO 4 :Eu 2+ Phosphor Containing Broad‐Band Defect‐Induced Charge‐Transfer Emission183Controllable structural ordering via chemical substitution to the efficient and thermally stable luminescence in NASICON-type phosphor Series: Na1+Hf2−Sc (PO4)3:Eu12Li + Ion Induced Full Visible Emission in Single Eu 2+ ‐Doped White Emitting Phosphor: Eu 2+ Site Preference Analysis, Luminescence Properties, and WLED Applications93Bismuth activated blue phosphor with high absorption efficiency for white LEDs55Efficient and Tunable Luminescence in Ga 2– x In x O 3 :Cr 3+ for Near-Infrared Imaging172Realization of non-rare earth doped blue-emitting phosphor Ba2Y5B5O17: Sb by selective site excitation, and its application in n-UV excited wLEDs3Preparation and photoluminescence properties of transparent suspensions of Ca(Y1−Eu )2(MoO4)4 nanophosphors3Synthesis and luminescence performance of Tb3+/Eu3+ codoped SrLaGa3O7 phosphors15Ca[B 8 O 11 (OH) 4 ] : Eu 2+ – A Highly Efficient Deep Blue‐Emitting Phosphor Prepared by Low‐Temperature Self‐reduction12Investigation of luminescence properties of Eu-doped Si-Al-O-N glasses synthesized via sol-gel process14Low Dimensional, Broadband, Luminescent Organic‐Inorganic Hybrid Materials for Lighting Applications57Giant Red‐Shifted Emission in (Sr,Ba)Y 2 O 4 :Eu 2+ Phosphor Toward Broadband Near‐Infrared Luminescence230Chasing Down the Eu2+ Ions: The Delicate Structure−Property Relationships in the Ultra‐Narrow Band Phosphor K1.6Na2.1Li0.3[Li3SiO4]4:Eu2+35Ce3+ luminescence, near-UV excitation enhancement of Tb3+ emission via energy transfer in Y4Zn4(SiO4)5:Ce3+,Tb3+ phosphor for white LED application6Tuning crystal structure and luminescence of Eu 2+ -activated LiSr 1– x Ba x PO 4 solid solution for white light-emitting diodes5Composition and Antithermal Quenching of Noninteger Stoichiometric Eu2+-Doped Na-β-Alumina with Cyan Emission for Near-UV WLEDs37Concentration palette enabling temperature-responsive luminescence co-modulations of inorganic phosphors for a thermally triggered security tag0Governing the crystallographic sites for tuning Eu 2+ emission in an apatite oxyfluoride host to be applied for superior white light emitting diodes14High efficiency near-infrared light emission and ultra-high stability of the lead-free double perovskite Cs 2 Na 1− x Ag x Bi 1− y Al y Cl 617Local environment rigidity and the evolution of optical properties in the green-emitting phosphor Ba 1− x Sr x ScO 2 F:Eu 2+12Luminescent MOFs (LMOFs): recent advancement towards a greener WLED technology72Manipulating trap distribution and density by chemical unit cosubstitution for near-infrared persistent luminescent Zn 1−2 x Li x Ga 2+ x O 4 :Cr 3+ solid solutions22Regulation of Local Site Structures to Stabilize Mixed-Valence Eu2+/3+ under a Reducing Atmosphere for Multicolor Photoluminescence23Inverse‐Tunable Red Luminescence and Electronic Properties of Nitridoberylloaluminates Sr2−xBax[BeAl3N5]:Eu2+ (x=0–2)3Structural Changes from Conventional SrSnO3 to Ruddlesden–Popper Sr2SnO4 Perovskites and Its Implication on Photoluminescence and Optoelectronic Properties18High-performance narrow-band green-emitting phosphor enabled by substituting Na with Rb6Simultaneous Spectral Tuning and Thermal Stability Adjustment in Ca8ZnGa(1–x)Lax(PO4)7:Eu2+ Phosphors23Competitive Site Occupation toward Improved Quantum Efficiency of SrLaScO 4 :Eu Red Phosphors for Warm White LEDs103Effect of ionic couple substitution on the enhanced photoluminescence properties of (BaMg)1-x(KxAl10+x)O17:Eu2+ phosphor for white LEDs application7Novel one-dimensional Ga2O3:Cr3+ nanofibers with broadband emission for near infrared LED sources13Controlled Modulation of the Structure and Luminescence Properties of Zero-Dimensional Manganese Halide Hybrids through Structure-Directing Metal-Ion (Cd 2+ and Zn 2+ ) Centers29Pressure-driven configurational crossover between 4f7 and 4f65d1 States – Giant enhancement of narrow Eu2+ UV-Emission lines in SrB4O7 for luminescence manometry30K replaces Rb towards cyan to red ultra-wideband perovskite-type phosphors for full-spectrum lighting8A novel cyan-emitting phosphor Ba2La8(SiO4)6O2:Eu2+ for full-spectrum white light-emitting diodes22Carbon dots embedded in lead-free luminescent metal halide crystals toward single-component white emitters32Highly Efficient Broad-Band Green-Emitting Cerium(III)-Activated Garnet Phosphor Allows the Fabrication of Blue-Chip-Based Warm-White LED Device with a Superior Color Rendering Index69Investigation on Ba2(Y1-x, Lux)5B5O17: y at.% Bi as a new type of N-UV excited high efficient blue phosphor for wLED6Towards single broadband white emission in Rb0.5K1.5CaPO4(F, Cl): Eu2+ via selective site occupancy engineering for solid-state lighting applications42Study the effect of Zn2+ co-doping on the structural and optical properties of CdSiO3:Eu3+ phosphor1Manipulating Upconversion Emission and Thermochromic Properties of Ho3+/Yb3+-Codoped Al2Mo3O12 Microparticles by Negative Lattice Expansion for Multimode Visual Optical Thermometry79Sr-substitution-guided Eu2+ site engineering of Ca9Nd(PO4)7:Eu2+ for high-efficiency white light-emitting diodes9Exploring the structural stability and optical properties of rare-earth doped K3LuSi2O7 phosphor from first-principles calculations4Ostensibly perpetual optical data storage in glass with ultra-high stability and tailored photoluminescence37Environment-Dependent Eu2+-Activated Ba3CaK(PO4)3 toward White-Light Emission by Chemical Cosubstitution of the (BO3)3– Anion Group19Photochromic, down-conversion nano bismuth chloride layered material: Latent fingerprint visualization and data security applications36Shining Transparent Displays with Stable Narrow‐Band Blue‐Emitting Phosphor in Layered Film50Tuning emission color of Eu2+-activated phosphor through phase segregation22Luminescence in the solid state7Blue-light-excited red emission in a CaO:Eu phosphor17Recent progress in Ce 3+ /Eu 2+ -activated LEDs and persistent phosphors: focusing on the local structure and the electronic structure137Sr2BN2Cl:Eu2+-Based Narrow-Band Blue-Emitting Phosphor: A Potential Color Converter for Illumination and Displays10Improvement the near-infrared luminescence properties of double perovskite phosphor La(Mg0.5Sn0.5In0.5Sc0.5)0.5O3:Cr3+ via co-doping Yb3+8Novel Sm3+-activated YCa4O(BO3)3 phosphors with high quantum efficiency and thermal stability for red-backlight display and indoor illumination27Laser Phosphors for Next-Generation Lighting Applications152Comparison of luminescence between Eu2+-activated Na2CaPO4F and NaCaPO4 green-emitting phosphors for pc-wLEDs17Fluorescence modulation in Pr3+-doped MGd2O4 (M = Sr, Ba) by the site engineering strategy4Achievement of broadband NIR emission in double perovskite NaLaMgWO6 via non-equivalent substitution of Cr3+17Stabilization of Eu 2+ in Li 2 B 4 O 7 with the BO 3 network through U 6+ co-doping and defect engineering8Study on luminescence properties of Bi3+ doped Ba2YAlO5：A wide-band yellow emitting phosphor with excellent thermal stability20Designing stimuli-responsive and color-tunable indicators via the coexistence of dual emitting centers7Ceramics phosphor powders4Eu 2+ luminescence in CaYGaO 4 olivine: a new efficient red phosphor for warm illumination47Highly-efficient Eu 2+ -activated Sr 8 Si 4 O 12 Cl 8 cyan-emitting phosphors with zero-thermal quenching luminescence for versatile applications16Introduction to properties of aluminates and its scope0Investigation of the luminescence properties and energy transfer mechanisms in Gd 3 TaO 7 :Bi 3+ ,Eu 3+ phosphors for their potential application in full-spectrum WLEDs10Research progress on surface modifications for phosphors used in light-emitting diodes (LEDs)27Synthesis and photoluminescence properties of Eu2+-doped olivine Mg2SiO4 blue-emitting phosphor for plant growth5Structure and Luminescence Studies of a Ce3+-Activated Ba5La3MgAl3O15 Green-Emitting Phosphor31Engineering charge-transfer interactions for red-emitting SrLa(Sc,Ga)O4:Ce3+ phosphor with improved thermal stability22Regulating Eu 2+ Multisite Occupation through Structural Disorder toward Broadband Near-Infrared Emission91Abnormal Eu3+ → Eu2+ Reduction in Ca9−xMnxEu(PO4)7 Phosphors: Structure and Luminescent Properties19Infrared to Short-Wave Infrared-Emitting Phosphors for Light-Emitting Diode Applications23Mixed Microscopic Eu 2+ Occupancies in the Next‐Generation Red LED Phosphor Sr[Li 2 Al 2 O 2 N 2 ]:Eu 2+ (SALON:Eu 2+ )37Eu 2+ -Doped Ca 4 Y 3 Si 7 O 15 N 5 Phosphor with High Thermal Stability and Pressure Sensitivity for Dual-Functional Applications in W-LEDs and Pressure Sensors32Chemical Group Substitution Enables Highly Efficient Mn4+ Luminescence in Heterovalent Systems27Simultaneous realization of tunable luminescence and enhanced thermal stability in Eu2+-based blue-green phosphors for multifunctional applications16Site‐Engineering for Controlling Multiple‐Excitation and Emission in Eu2+‐Activated CaSrSiO4 Phosphors in Marine Fisheries21Deep‐Red Ca3Al2Ge3O12:Eu3+ Garnet Phosphor with Near‐Unity Internal Quantum Efficiency and High Thermal Stability for Plant Growth Application67A novel reddish-orange-emitting phosphor Ca3Gd7(PO4)(SiO4)5O2: Sm3+ for white light-emitting diodes13Cold Sintering of Highly Transparent Calcium Fluoride Nanoceramic as a Universal Platform for High‐Power Lighting64Green synthesis of calcium magnesium silicate using industrial waste material3Synthesis of Eu3+-Doped NaGd9Si6O26 Sub-Microcrystals from a NaGdF4@SiO2 Structure2A new Milarite type KMLS:Eu3+ orange-red-emitting phosphor for pc-white LEDs and Forensic applications23Recent Advances in Light-Conversion Phosphors for Plant Growth and Strategies for the Modulation of Photoluminescence Properties47Cyan-to-yellow color tunable NaAlSiO4:Eu2+ with high quantum efficiency and thermal stability for white light-emitting diodes14Broadband near infrared luminescent properties of Cr3+ activated SrGa2Si2O8 phosphor18Near-Infrared LuCa 2 ScZrGa 2 GeO 12 :Cr 3+ Garnet Phosphor with Ultra-broadband Emission for NIR LED Applications60Development of a novel Eu3+-doped tantalate red-emitting phosphor for w-LEDs application17Photoluminescence of Mn2+ in the Borosulfate Zn[B2(SO4)4] : Mn2+—A Tool to Detect Weak Coordination Behavior of Ligands18Photolumineszenz von Mn2+ in dem Borosulfat Zn[B2(SO4)4] : Mn2+ – Eine Möglichkeit zum Nachweis schwach koordinierender Liganden0Luminescent properties of the Sr8−Ba MgY(PO4)7:Eu2+ solid solution0Structural and luminescence studies of Eu3+ doped K2BaSr(PO4)2 phosphor0STRUCTURAL DESIGN OF Eu2+-CONTAINING GLASS AND GLASS-CERAMICS BASED ON THE SYSTEM BaO–ZrO2–SiO2–MgF2 FOR LED APPLICATION0Highly efficient blue‐emitting phosphor via charge compensation strategy and its application for white LED lighting10Structural Design of Eu2+-Containing Glasses and Glass-Ceramics Based on the BaO–ZrO2–SiO2–MgF2 System for LED Application2Regulation of Anti‐Thermal Quenching and Emission Color in Eu 2+ ‐Activated Na‐Beta‐Alumina Phosphors for Full‐Spectrum Illumination11A potential cyan phosphor for full spectrum light-emitting diodes: Bi3+ activated SrBaGdGaO5 phosphor20Efficient broadband yellow-emitting Mg2.5Lu1.5Al1.5Si2.5O12:Ce3+ garnet phosphors for blue-light-pumped white light-emitting diodes21Isolated Coordination Polyhedron Confinement in ABP2O7:Mn2+ (A = Ba/Sr; B = Mg/Zn)5Design the green emitting phosphor Ca9La(PO4)7:Eu2+ by the structural modulation and its application to white LEDs5Bluish-green emission of novel BaAl2Ge2O8:Eu2+ phosphors under near-ultraviolet excitation20Elucidating photoluminescent properties of Eu‐doped Ca–Al–Si–O(–N) glasses and the local structures of Eu ions7Temperature/electric field induced photoluminescence-modulation effect in dysprosium-doped barium titanate ferroelectric ceramics16Achieving the performance luminescence of LaMg0.5Sn0.5O3:Cr3+ by [In3+-Sc3+] co-substitution [Mg2+-Sn4+] and its application to the biodetection and night vision lighting4Achieving a Eu 2+ -doped NIR phosphor via ionic modulation and its multifunctional applications4Barium molybdate up-conversion nanoscale particles with IR-LED chip, temperature sensing, and anti-counterfeiting applications11Effect of Rare-Earth Doping on Upconversion Luminescence of CaF2 Glass–Ceramic Nanoparticles1High-performance green-emitting Ca 2 YScAl 2 Si 2 O 12 :Ce 3+ garnet phosphors and their applications in high-quality blue-chip-pumped white LEDs48Highly efficient and thermally stable broadband green-emitting BaY 2 Sc 2 Al 2 SiO 12 :Ce 3+ phosphors enabling warm-white LEDs with high luminous efficacy and high color rendering index44Structure modification and luminescence regulation in new violet light excitable Sr (2− y ) Ba y Y 4 La 4 (SiO 4 ) 6 O 2 : x Eu 2+ phosphors via cation substitution6An efficient and thermally stable red emitting Eu2+ doped oxide for rechargeable portable flashlight62Multicolor regulation of trivalent lanthanide ions-codoped boggildite-type phosphor toward superb warm white luminescence for white light-emitting diodes13Deep‐Red (Sr,Ba)Lu2O4: Eu2+ Phosphor for Full‐Spectrum Lighting7Ce 3+ -Activated SrLu 2 Al 3 ScSiO 12 Cyan-Green-Emitting Garnet-Structured Inorganic Phosphor Materials toward Application in Blue-Chip-Based Phosphor-Converted Solid-State White Lighting68Pure-red phosphor Ca3Si2O7:Eu2+ obtained by the CO reduction strategy13Investigating the use of Er3+ doped β-Ca2SiO4 phosphors derived from agricultural waste for thermal sensing and forensic applications5Highly efficient broadband near-infrared luminescence phosphors Ca3MgSn0.5Zr0.5Ge3O12:Pr3+,Cr3+ for multifunctional applications in pc-LEDs field19Study of Charge Transfer Green Luminescence in Tb3+ Activated BaSrLa4O8 Nanophosphor for Advanced Indoor Lighting Applications1Bandgap Narrowing in Europium(II)-Based Bromide Hybrids toward Improved X-ray Scintillation and Imaging32Luminescence properties of complex fluoride Na3CaMg3AlF14 phosphors doped with cerium and europium ions2Delineating Dy3+ and Sm3+ in thermally stable strontium silicate apatites for multifunctional applications11Multi-sites induced ultra-broadband luminescence based on Eu2+ doped whitlockite-type phosphor for full-spectrum WLEDs9Highly efficient blue-light-excitable ultra-broadband orange-emitting Mg2.5Y1.5Al1.5Si2.5O12:Ce3+ garnet phosphors for solid-state lighting24Luminescent properties of Y2LaCaGa3ZrO12: Bi3+, Al3+ cyan phosphors for application in white light emitting diodes11A novel green phosphor Ba2Sc2((BO3)2B2O5):Ce3+ for high color rendering index full-spectrum lighting and low-temperature sensors21Synthesis and characterization of eco-friendly, stable green-emitting Tb3+-doped borosilicate glasses using waste silica gel7Ultra‐Broadband Near‐Infrared Luminescence from a Vanadium‐Activated Phosphate Glass12Synergetic manipulation of components and multiple activator sites towards full-spectrum lighting in Eu2+-doped whitlockite phosphors for high color-rendering WLED4Effect of copper addition on lithium zinc borosilicate glass containing terbium oxide3

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    Advanced Optical Materials · 2021-10-08

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  36. Tuning crystal structure and luminescence of Eu 2+ -activated LiSr 1– x Ba x PO 4 solid solution for white light-emitting diodes

    Materials Advances · 2021-11-23

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  37. Composition and Antithermal Quenching of Noninteger Stoichiometric Eu2+-Doped Na-β-Alumina with Cyan Emission for Near-UV WLEDs

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  39. Governing the crystallographic sites for tuning Eu 2+ emission in an apatite oxyfluoride host to be applied for superior white light emitting diodes

    Dalton Transactions · 2022-01-01

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  40. High efficiency near-infrared light emission and ultra-high stability of the lead-free double perovskite Cs 2 Na 1− x Ag x Bi 1− y Al y Cl 6

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  41. Local environment rigidity and the evolution of optical properties in the green-emitting phosphor Ba 1− x Sr x ScO 2 F:Eu 2+

    Journal of Materials Chemistry C · 2022-01-01

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  42. Luminescent MOFs (LMOFs): recent advancement towards a greener WLED technology

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  43. Manipulating trap distribution and density by chemical unit cosubstitution for near-infrared persistent luminescent Zn 1−2 x Li x Ga 2+ x O 4 :Cr 3+ solid solutions

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  44. Regulation of Local Site Structures to Stabilize Mixed-Valence Eu2+/3+ under a Reducing Atmosphere for Multicolor Photoluminescence

    Inorganic Chemistry · 2022-01-10

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  45. Inverse‐Tunable Red Luminescence and Electronic Properties of Nitridoberylloaluminates Sr2−xBax[BeAl3N5]:Eu2+ (x=0–2)

    Chemistry - A European Journal · 2022-01-12

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  46. Structural Changes from Conventional SrSnO3 to Ruddlesden–Popper Sr2SnO4 Perovskites and Its Implication on Photoluminescence and Optoelectronic Properties

    ACS Applied Electronic Materials · 2022-02-04

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  47. High-performance narrow-band green-emitting phosphor enabled by substituting Na with Rb

    Journal of Luminescence · 2022-02-05

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  48. Simultaneous Spectral Tuning and Thermal Stability Adjustment in Ca8ZnGa(1–x)Lax(PO4)7:Eu2+ Phosphors

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  49. Competitive Site Occupation toward Improved Quantum Efficiency of SrLaScO 4 :Eu Red Phosphors for Warm White LEDs

    Advanced Optical Materials · 2022-02-20

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  50. Effect of ionic couple substitution on the enhanced photoluminescence properties of (BaMg)1-x(KxAl10+x)O17:Eu2+ phosphor for white LEDs application

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