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RESEARCH PAPER · Chemical Communications · 2020

A K 3 ScSi 2 O 7 :Eu 2+ based phosphor with broad-band NIR emission and robust thermal stability for NIR pc-LEDs

Qiang Zhang, Xicheng Wang, Zuobin Tang, Yuhua Wang

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A K 3 ScSi 2 O 7 :Eu 2+ based phosphor with broad-band NIR emission and robust thermal stability for NIR pc-LEDsOriginalFull-visible-spectrum lighting realized by a novel Eu 2+ -doped cyan-emitting borosilicate phosphor25A review on fluorescence intensity ratio thermometer based on rare-earth and transition metal ions doped inorganic luminescent materials440Abnormal Bi3+-Activated NIR Emission in Highly Symmetric XAl12O19 (X = Ba, Sr, Ca) by Selective Sites Occupation106The photoluminescence, thermal properties and tunable color of bright green-emitting Ba3Sc(BO3)3:Ce3+/Tb3+ phosphors via efficient energy transfer41A near infrared-II broad emission material with multi-spectral excitation and long persistent luminescence properties21A single luminescence center ultra-broadband near-infrared LiScGeO 4 :Cr phosphor for biological tissue penetration49Energy transfer enhanced broadband near-infrared phosphors: Cr 3+ /Ni 2+ activated ZnGa 2 O 4 –Zn 2 SnO 4 solid solutions for the second NIR window imaging114Multi-site Cr 3+ occupation-related broadband NIR luminescence in Cr 3+ -doped Li 3 Mg 2 NbO 634Recent progress of effect of crystal structure on luminescence properties of Ce 3+ –Eu 2+ Co-doped phosphors14A broadband near-infrared phosphor Ca3Y2Ge3O12:Cr3+ with garnet structure136Design of Novel Highly Efficient Yellow-Orange Color-Tunable Luminescence in Rb2Sr1–yCayP2O7:xEu2+ Solid Solutions for White Light-Emitting Diodes24Structural and spectroscopic investigation of an efficient and broadband NIR phosphor InBO3: Cr3+ and its application in NIR pc-LEDs106Learning from Mineral Structures toward New Luminescence Materials for Light-Emitting Diode Applications146Simultaneous Broadening and Enhancement of Cr 3+ Photoluminescence in LiIn 2 SbO 6 by Chemical Unit Cosubstitution: Night‐Vision and Near‐Infrared Spectroscopy Detection Applications325Simultaneous Broadening and Enhancement of Cr3+Photoluminescence in LiIn2SbO6by Chemical Unit Cosubstitution: Night‐Vision and Near‐Infrared Spectroscopy Detection Applications5Advances in Near-Infrared Luminescent Materials without Cr3+: Crystal Structure Design, Luminescence Properties, and Applications171Design of a broadband cyan-emitting phosphor with robust thermal stability for high-power WLED application52Ca[B 8 O 11 (OH) 4 ] : Eu 2+ – A Highly Efficient Deep Blue‐Emitting Phosphor Prepared by Low‐Temperature Self‐reduction12Multi spectral responsive near infrared-II broad emission material and its LED device and imaging research12Giant Red‐Shifted Emission in (Sr,Ba)Y 2 O 4 :Eu 2+ Phosphor Toward Broadband Near‐Infrared Luminescence230Spectrally tunable and thermally stable near-infrared luminescence in Na 3 Sc 2 (PO 4 ) 3 :Cr 3+ phosphors by Ga 3+ co-doping for light-emitting diodes62Crystallographic control for Cr 4+ activators toward efficient NIR-II luminescence91Deep-red to near-infrared luminescence from Eu 2+ -trapped exciton states in YSiO 2 N9Dual-Site Occupancy Induced Blue Emission in Both Eu2+ and Ce3+ Doped Naba3si2o7f0Investigation on the Luminescent Property and Application of In2BP3O12:Cr3+ Broadband Near-Infrared Phosphor※8Ni 2+ -activated MgTi 2 O 5 with broadband emission beyond 1200 nm for NIR-II light source applications49Tunable concentration/excitation-dependent deep-red and white light emission in single-phase Eu 2+ -activated Sc-based oxide phosphors for blue/UV-LEDs32Eu2+‐Doped Layered Double Borate Phosphor with Ultrawide Near‐Infrared Spectral Distribution in Response to Ultraviolet–Blue Light Excitation110Charge compensating effect of rare earth ions Ln3+ (Ln =Y, La) on the photoluminescence improvement of Sr9MgK(PO4)7:Eu2+ phosphor5MgGd 4 Si 3 O 13 :Ce 3+ , Mn 2+ : A Dual-Excitation Temperature Sensor13Broadband near-infrared emitting Sr3Sc4O9: Cr3+ phosphors: Luminescence properties and application in light-emitting diodes46K replaces Rb towards cyan to red ultra-wideband perovskite-type phosphors for full-spectrum lighting8Highly efficient Fe3+-doped A2BB′O6 (A = Sr2+, Ca2+; B, B′ = In3+, Sb5+, Sn4+) broadband near-infrared-emitting phosphors for spectroscopic analysis251Efficient near-infrared phosphors discovered by parametrizing the Eu(II) 5d-to-4f energy gap92Dual-mode optical thermometry design in K 3 YSi 2 O 7 :Eu multi-site phosphor8A Zero-Thermal-Quenching Blue Phosphor for Sustainable and Human-Centric WLED Lighting130Exploring the structural stability and optical properties of rare-earth doped K3LuSi2O7 phosphor from first-principles calculations4Ultra‐Broadband Green‐Emitting Phosphors without Cyan Gap Based on Double‐Heterovalent Substitution Strategy for Full‐Spectrum WLED Lighting89Achieving the ultra-broadband near-infrared La3SnGa5O14:Cr3+ phosphor via multiple lattice sites occupation for biological nondestructive detection and night-vision technology45A novel far-red phosphors Li2ZnTi3O8:Cr3+ for indoor plant cultivation:Synthesis and luminescence properties55Recent Advances in Chromium‐Doped Near‐Infrared Luminescent Materials: Fundamentals, Optimization Strategies, and Applications252Near-infrared emission in perovskite oxides MZrO3:Bi (M = Ba, Sr) by dopants’ selective site occupancy19The Separation of Europium/Americium from High-Acidity Solutions Using a Manufactured Resin Material0Single‐Site Occupancy of Eu 2+ in Multiple Cations Enables Efficient Ultra‐Broadband Visible to Near‐Infrared Luminescence83Synthesis, luminescence and photometric investigation of Sr2B2O5:Dy3+ phosphor for UV-based white LEDs15A novel Mn 4+ ‐activated far‐red Sr 2 MgWO 6 phosphor: synthesis, luminescence enhancement, and application prospect13Structure and photoluminescence studies of Rb3GdSi2O7: Eu2+ phosphor used for NUV converted white LEDs10A novel K3(Y0.88Yb0.10Er0.02)Si2O7 silicate phosphor for multi-mode thermometry of high sensitivity through up-conversion luminescence20Tetracoordinate Fe 3+ Activated Li 2 ZnAO 4 (A = Si, Ge) Near-Infrared Luminescent Phosphors65A novel broad-band red K2MgSiO4:Eu2+ phosphor and defect-induced tunable emission from red to yellow20Multifunctional near-infrared Zn2TiO4:Cr3+ phosphors for luminescence, thermometry, and plant cultivation24Engineering deep-red Al20B4O36:Cr3+ phosphors for photomorphogenesis9Compositional modulation induced broadband NIR luminescence enhancement in A2ScNbO6:Cr3+ (A = Ba, Sr)12Achieving a Eu 2+ -doped NIR phosphor via ionic modulation and its multifunctional applications4Enhanced NIR emission and thermal stability of La 2 MgSnO 6 :Mn 4+ ,Ni 2+ via energy transfer15Preparation of a novel violet-excitable Na 3 YSi 2 O 7 :Eu 2+ green phosphor via salt-flux assistance and its luminescence properties15Realizing efficient broadband near-infrared emission and multimode photoluminescence switching via coordination structure modulation in Sb 3+ -doped 0D organic metal chlorides50Research progress on Fe 3+ -activated near-infrared phosphor18Structure tailoring and defect engineering of a highly thermally stable red emitting phosphor22Tailoring Emission Characteristics of Na-Sc Co-Substituted Camgge2o6:Cr3+ Phosphors for Iris Acquisition0Thermal activation induced charge transfer state absorption redshift realizes strong anti-thermal quenching in Pr 3+ -activated phosphor10绿色合成Li3Na3Ga2F12∶Cr3+氟化物宽带近红外荧光材料（特邀）0Luminescence improvement of Gd3Ga5O12:Cr3+,Bi3+ NIR phosphor with superior thermal stability for plant cultivation24Separation of europium as a homologue of americium from high acidity solutions using a manufactured resin material7Thermally Stable Red-Emitting Ca18K3Sc(PO4)14:Mn2+ Phosphor and Enhanced Luminescence by Energy Transfer Between Ce3+-Eu2+-Mn2+22Pure-red phosphor Ca3Si2O7:Eu2+ obtained by the CO reduction strategy13A new yellowish‐green‐emitting phosphor: Eu 2+ ‐doped Ba 3 YAl 2 O 7.55Dual substitution of host lattice ions to enhance the luminescence properties of Zn2TiO4:Cr3+ phosphor3Comprehensive Review on Downconversion/Downshifting Silicate-Based Phosphors for Solar Cell Applications21Highly Efficient and Thermally Stable Broadband NIR Phosphors with Superlong Afterglow Performance and their Multifunctional Applications53Europium Ions Self‐Reduction Benefiting from AlO4/Si(Al)O4 Network Structure for Multimode Optical Thermometry Manometry27Co-precipitation synthesis and thermally enhanced upconversion luminescence properties of ScPO4:Yb3+/Er3+ phosphors for temperature sensing4Unlocking Chlorine Oxide‐Based Ultra‐Wideband Near‐Infrared Phosphor and Advancing Spectral Performance via Lattice Engineering43Regulating the broadband near-infrared emission of Eu2+-doped Ca3Sc2Si3O12 phosphors through constructing defect for diversified applications56Tailoring emission characteristics of Na+-Sc3+ co-substituted CaMgGe2O6:Cr3+ phosphors for iris acquisition7Sunlight‐Activated Eu2+‐Doped Red Persistent Luminescence Material for Night‐Vision Signage, Anti‐Counterfeiting and Location Detection30Structure regulation and luminescence improvement of Gd3Ga5O12:Cr3+: An anti-thermal quenching NIR phosphor for multifunctional applications15A yellow-green-emitting phosphor K3LaSi2O7:Eu2+ with superior thermal stability for solid-state lighting9Enhanced thermal stability of broadband NIR phosphors Ca3.3Mg0.7ZrGe3O12:Cr3+ for pc-LEDs8A high-efficiency blue-LED-excitable broadband Cr 3+ /Ni 2+ co-doped garnet phosphor toward next-generation spectroscopy applications19Near-infrared luminescent materials: a review of their practical applications and prospective advancements47Synthesis and Luminescent Properties of Novel Narrow-Band Green-Emitting Phosphors Na3ysi2o7: Eu2+ for Full-Spectrum Lighting0Achievement of an ultra-broadband deep red phosphor K3Ca0.3Y0.7Si2O7:Eu2+ (phase 1) for phytochrome matching plant-lighting12Site occupation engineering induced red-shifted luminescence in (Ca, Sr)Sc2O4:Eu2+ phosphor20Neighboring‐Cation Substitution Engineering Strategy toward High Performance in Near‐Infrared Light Source for Multifunctional Applications13Near-infrared emission of Eu2+ in M4Li(BN2)3 (M = Ca, Sr, Ba)1Broad-Band Near-Infrared Emission with High External Quantum Efficiency from Molybdenum-Doped Vacancy-Ordered Double Perovskites for Spectroscopic Analysis23Dual mode luminescence and abnormal thermal quenching of Ho3+ activated Ca2SnO4 phosphors3Structural, luminescent, and temperature-dependent luminescence of Tb3+-doped silicate phosphors for non-contact thermometry applications5Synthesis, conductivity and anti-counterfeiting applications of neodymium doped LiAlSiO4 nanopowders3Broadband Near‐Infrared Emitting Lead‐Free Perovskites with High Internal Quantum Efficiency and Small Stokes Shift for Versatile Spectroscopy Applications13Wavelength-Tunable of Broad Red to Near-Infrared Emission in (Sr,Ba)3Sc4O9 :Eu2+ Phosphors: Crystal Field Effects and Thermal Stability6Synthesis and luminescent properties of novel cyan-green-emitting phosphors Na3YSi2O7: Eu2+ for full-spectrum lighting0A Novel Cyan‐Emitting Phosphor K 3 Ca 0.3 Y 0.7 Si 2 O 7 :Ce 3+ Enables Full‐Spectrum Lighting and Fingerprint Detection via Phase‐Structure Alteration9Effects of Al/Ga ratio and Ce3+/Cr3+ Co-doping on the structural and luminescent properties of Z(A,G)GO:Ce3+,Cr3+ phosphors1Synthesis and luminescent properties of novel red-emitting K3GdSi2O7: Eu2+ phosphors for warm white leds0Revolutionary near-infrared phosphors with emerging structures and mechanisms driving next-generation applications32High efficiency near-infrared emission from Fe3+-doped NaAl11O17 phosphors for plant lighting8Waste to wealth: transforming Eu2+/Eu3+ co-activation from weak link to strength for advanced multifunctional lighting3A novel narrow-band red-emitting phosphor for lighting and backlight display1Tailoring intervalence charge transfer band position to suppress thermal quenching in Mg1-xCaxNb2O6:Pr3+ phosphors1White light emission regulation of Eu2+/Bi3+/Sm3+ Co-doped Ca4MgAl2Si3O14 phosphors under near-ultraviolet excitation3Recent developments in near-infrared phosphors for broad-band light-emitting diodes light sources9Tunable Broadband Red-To-Near-Infrared Emission in Eu 2+ -Activated Sr 1– x Ba x La 2 Sc 2 O 7 Phosphors via Site-Selective Occupation and Cation Substitution3The luminescence aging and mitigation strategies of Cr3+-Activated deep-red and near-infrared phosphors1Enhancing near‑infrared luminescence in Fe3+‑doped Na‑β‑Al2O3 phosphors via cation substitution for LED application0Self‐Recoverable Near‐Infrared Mechanoluminescence in Fe 3+ ‐Activated Garnet via Trap‐Engineered Multimodal Excitation0Broadband near-infrared emission in double perovskite phosphor BaLaMgTaO6:Cr3+ for organic compound detection, night vision and biological imaging0Energy Transfer Engineering Enables Efficient Near‐Infrared Luminescence and Zero‐Thermal‐Quenching in GAGG: Fe 3+ , Yb 3+ Phosphors0

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  3. Abnormal Bi3+-Activated NIR Emission in Highly Symmetric XAl12O19 (X = Ba, Sr, Ca) by Selective Sites Occupation

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  4. The photoluminescence, thermal properties and tunable color of bright green-emitting Ba3Sc(BO3)3:Ce3+/Tb3+ phosphors via efficient energy transfer

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  6. A single luminescence center ultra-broadband near-infrared LiScGeO 4 :Cr phosphor for biological tissue penetration

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  8. Multi-site Cr 3+ occupation-related broadband NIR luminescence in Cr 3+ -doped Li 3 Mg 2 NbO 6

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  9. Recent progress of effect of crystal structure on luminescence properties of Ce 3+ –Eu 2+ Co-doped phosphors

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  11. Design of Novel Highly Efficient Yellow-Orange Color-Tunable Luminescence in Rb2Sr1–yCayP2O7:xEu2+ Solid Solutions for White Light-Emitting Diodes

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  12. Structural and spectroscopic investigation of an efficient and broadband NIR phosphor InBO3: Cr3+ and its application in NIR pc-LEDs

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  14. Simultaneous Broadening and Enhancement of Cr 3+ Photoluminescence in LiIn 2 SbO 6 by Chemical Unit Cosubstitution: Night‐Vision and Near‐Infrared Spectroscopy Detection Applications

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  16. Advances in Near-Infrared Luminescent Materials without Cr3+: Crystal Structure Design, Luminescence Properties, and Applications

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  17. Design of a broadband cyan-emitting phosphor with robust thermal stability for high-power WLED application

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  18. Ca[B 8 O 11 (OH) 4 ] : Eu 2+ – A Highly Efficient Deep Blue‐Emitting Phosphor Prepared by Low‐Temperature Self‐reduction

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  33. Highly efficient Fe3+-doped A2BB′O6 (A = Sr2+, Ca2+; B, B′ = In3+, Sb5+, Sn4+) broadband near-infrared-emitting phosphors for spectroscopic analysis

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  34. Efficient near-infrared phosphors discovered by parametrizing the Eu(II) 5d-to-4f energy gap

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  35. Dual-mode optical thermometry design in K 3 YSi 2 O 7 :Eu multi-site phosphor

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  37. Exploring the structural stability and optical properties of rare-earth doped K3LuSi2O7 phosphor from first-principles calculations

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  39. Achieving the ultra-broadband near-infrared La3SnGa5O14:Cr3+ phosphor via multiple lattice sites occupation for biological nondestructive detection and night-vision technology

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  40. A novel far-red phosphors Li2ZnTi3O8:Cr3+ for indoor plant cultivation:Synthesis and luminescence properties

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  42. Near-infrared emission in perovskite oxides MZrO3:Bi (M = Ba, Sr) by dopants’ selective site occupancy

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  43. The Separation of Europium/Americium from High-Acidity Solutions Using a Manufactured Resin Material

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  44. Single‐Site Occupancy of Eu 2+ in Multiple Cations Enables Efficient Ultra‐Broadband Visible to Near‐Infrared Luminescence

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  45. Synthesis, luminescence and photometric investigation of Sr2B2O5:Dy3+ phosphor for UV-based white LEDs

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  46. A novel Mn 4+ ‐activated far‐red Sr 2 MgWO 6 phosphor: synthesis, luminescence enhancement, and application prospect

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  47. Structure and photoluminescence studies of Rb3GdSi2O7: Eu2+ phosphor used for NUV converted white LEDs

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  48. A novel K3(Y0.88Yb0.10Er0.02)Si2O7 silicate phosphor for multi-mode thermometry of high sensitivity through up-conversion luminescence

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    Jiantong Wang, Bowen Wang, Bowen Wang, Bowen Wang, Yuhan Teng, Changshuai Gong, Xuyan Xue, Xuejiao Wang, Ji‐Guang Li

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