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RESEARCH PAPER · Chemical Engineering Journal · 2020

Site-selective occupation of Eu2+ activators toward full-visible-spectrum emission in well-designed borophosphate phosphors

xingxing sheng, Pengpeng Dai, Zhiyi Sun, Dawei Wen

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Site-selective occupation of Eu2+ activators toward full-visible-spectrum emission in well-designed borophosphate phosphorsOriginalPreparation of CaAlSiN3:Eu2+ red-emitting phosphor by a two-step method for solid-state lighting applications32Highly Robust Oxynitride Phosphor against Thermal Oxidization and Hydrolysis36Cation sites modification enhanced luminescence and thermal quenching characteristic in the blue light-emitting Na3Sc2-xZnx(PO4)3:0.03Eu2+ phosphors10Mn2+ doping enabled efficient high-color-rendering single-phase white-emitting lead halide perovskites13Discovery of a new phosphor via aliovalent cation substitution: DFT predictions, phase transition and luminescence properties for lighting and anti-counterfeiting applications22Complex crystal structure and photoluminescence of Bi 3+ -doped and Bi 3+ /Eu 3+ co-doped Ca 7 Mg 2 Ga 6 O 1819Controllable crystal form transformation and luminescence properties of up-conversion luminescent material K 3 Sc 0.5 Lu 0.5 F 6 : Er 3+ , Yb 3+ with cryolite structure3Site engineering strategy toward enhanced luminescence thermostability of a Cr 3+ -doped broadband NIR phosphor and its application107Improving the thermal stability and luminescent efficiency of (Ba,Sr)3SiO5:Eu2+ phosphors by structure, bandgap engineering and soft chemistry synthesis method98Spontaneous-reduction and photoluminescence tuning in singly-doped Ba5-Ca (PO4)3Cl:Eu2+/Eu3+ phosphors23Pink-emitting RbBaBP2O8:Sm phosphor with diamondoid structure and high thermostability47Li + Ion Induced Full Visible Emission in Single Eu 2+ ‐Doped White Emitting Phosphor: Eu 2+ Site Preference Analysis, Luminescence Properties, and WLED Applications93Site occupancy and photoluminescence properties of cyan-emitting K2Ca2Si2O7:Bi3+ phosphor for white light emitting diodes44Thermally stable orange-red luminescence of samarium (Ⅲ)-activated KSrBP2O8 borophosphate13Extension of Spectral Shift Controls from Equivalent Substitution to an Energy Migration Model Based on Eu2+/Tb3+-Activated Ba4–xSrxGd3–xLuxNa3(PO4)6F2 Phosphors11Full-visible-spectrum lighting enabled by site-selective occupation in the high efficient and thermal stable (Rb, K)2CaPO4F: Eu2+ solid-solution phosphors58A review and outlook of ratiometric optical thermometer based on thermally coupled levels and non-thermally coupled levels232Bifunctional samarium activated red-emitting and thermal resistant phosphor for simultaneous field emission displays and white light-emitting diodes32Tuning crystal structure and luminescence of Eu 2+ -activated LiSr 1– x Ba x PO 4 solid solution for white light-emitting diodes5Multifunctional Ca9NaZn1-Mg (PO4)7:Eu2+ phosphor for full-spectrum lighting, optical thermometry and pressure sensor applications112A single-component white-light-emitting fluorescent material with high color rendering index based on resonance energy transfer11Luminescence enhancement of single-component Ca19Zn2(PO4)14:Dy3+ white-emitting phosphor powders through partial substitution of PO43− with SiO44− and BO33-19Single Bi3+ Ultrabroadband White Luminescence in Double Perovskite via Crystal Lattice Engineering toward Light‐Emitting Diode Applications86Pressure-triggered enormous redshift and enhanced emission in Ca2Gd8Si6O26:Ce3+ phosphors: Ultrasensitive, thermally-stable and ultrafast response pressure monitoring128Disorder–Order Conversion‐Induced Enhancement of Thermal Stability of Pyroxene Near‐Infrared Phosphors for Light‐Emitting Diodes140Disorder–Order Conversion‐Induced Enhancement of Thermal Stability of Pyroxene Near‐Infrared Phosphors for Light‐Emitting Diodes50Design of luminescence in (Sr,Gd)Li(Al,Mg)3N4:Eu2+ deep red phosphors via crystal field engineering for full-spectrum WLEDs29Manipulating concentration quenching and thermal stability of Eu3+-activated NaYbF4 nanoparticles via phase transition strategy toward diversified applications25Towards single broadband white emission in Rb0.5K1.5CaPO4(F, Cl): Eu2+ via selective site occupancy engineering for solid-state lighting applications42Ultra‐Broadband Green‐Emitting Phosphors without Cyan Gap Based on Double‐Heterovalent Substitution Strategy for Full‐Spectrum WLED Lighting89Environment-Dependent Eu2+-Activated Ba3CaK(PO4)3 toward White-Light Emission by Chemical Cosubstitution of the (BO3)3– Anion Group19Design of K2SrCa(PO4)2-x(BO3)x:Eu2+ phosphors with full-visible spectrum by crystal structure modification12Thermal stable cyan-emitting Ba9(Lu1.5Ga0.5)Si6O24:Ce3+ for high color-rendering white LEDs7Effect of Si4+/Gd3+ doping on luminescence properties of orangish-red light-emitting phosphors of KBaBP2O8:Eu3+4Investigation into the photoluminescence and energy levels in bismuth-doped Sr3MgSi2O8 through first principles calculations1Investigation into the Eu2+ ions occupations and the coordination environments in components modulated Sr3MgSi2O81A single-phase white-emitting La(BO3,PO4):Dy3+ phosphor with high thermostability35Site-Selective Occupancy Control of Cr Ions toward Ultrabroad-Band Infrared Luminescence with a Spectral Width up to 419 nm79Ba5GeO4Br6:Bi3+, a promising cyan phosphor for high-quality full-spectrum white light illumination34Super Broadband Near‐Infrared Solid Solution Phosphors with Adjustable Peak Wavelengths from 1165 to 875 nm for NIR Spectroscopy Applications41A broadband yellow-green emitting mixed orthoborate–pyroborate phosphor, Ba 2 Sc 2 B 4 O 11 :Ce 3+ , for white light emitting diodes23A novel bright cyan emitting phosphor of Eu 2+ activated Ba 6 BO 3 Cl 9 with robust thermal stability for full-spectrum WLED applications65Breakthrough Boost of Stokes Fluorescence from Er3+ in Perovskites for Flexible Temperature Sensing8Site Occupation Regulation of Eu2+ by the Introduction of (Bo3)3- Group Towards Full-Visible-Spectrum Emission in a Singly Doped K2basr(Po4)2:Eu2+ Phosphor0A narrow-band RbBaBP2O8:Tb3+ green phosphor with high thermal stability for backlighting display application34Site‐Engineering for Controlling Multiple‐Excitation and Emission in Eu2+‐Activated CaSrSiO4 Phosphors in Marine Fisheries21Anionic Regulation toward Bi3+ Selective Occupation for Full-Spectrum White Light Emission33Ultra-narrow-band luminescence with spectral width down to 32 nm in bismuth-activated phosphate phosphors with superior thermal stability11Structure and photoluminescence studies of Rb3GdSi2O7: Eu2+ phosphor used for NUV converted white LEDs10Enhancing thermal degradation stability of BaSi2O2N2:Eu2+ for white light-emitting diodes by ultra-thin Al2O3 layer via atomic layer deposition11Hydrothermal synthesis and tunable luminescence of YPO4:Eu2+/Eu3+, Tb3+ nanocrystals17Highly bright broadband cyan-emitting CaLu2HfGaAl3O12:Ce3+ garnet phosphors for high-color-quality white light-emitting diodes15Surface Coating of Lead-free Perovskites to Break the Luminescence Threshold for Fluorescent Information Recognition12Broadband emission characteristics and WLED application of self-activated YMZn3AlO7 (M=Ca, Sr, Ba) phosphors5A highly thermal-stable red-emitting tantalate phosphor for WLED and multiple-mode optical temperature sensor dual-applications25Ultra-broadband emission up to 181 nm of VO4-activated yellow phosphor for white light-emitting diodes with high color rendering index5Achieving white emission by site-selective occupation of Eu 2+ in K 2 BaSr(PO 4 ) 2− x (BO 3 ) x :Eu 2+12Crystal-Site Engineering of Novel Na3kmg7(Po4)6-X(Bo3)X: Eu2+ Phosphor for Full-Spectrum Lighting0Designing of Eu2+-Activated Single-Phase White-Emitting Phosphor Through Modifying Cationic Sites for High Color Rendering Full-Spectrum Illumination0Progress of Ce 3+ /Eu 2+ doped phosphors for violet chip based full-spectra lighting42Structure modification and luminescence regulation in new violet light excitable Sr (2− y ) Ba y Y 4 La 4 (SiO 4 ) 6 O 2 : x Eu 2+ phosphors via cation substitution6Unlocking color-tunable emission of Eu 2+ -activated phosphors through doping-free exploration of hidden sites3Tunable emission of Ce 3+ in (K, Rb) 3 GdSi 2 O 7 phosphors toward broadband cyan luminescence5High quantum efficiency blue phosphor K2SrCa(PO4)2: Eu2+ for plant growth32Study on a Highly Thermostable Dy 3+ -Activated Borophosphate Phosphor71Crystal-Site Engineering of Novel Na3KMg7(PO4)6–x(BO3)x:Eu2+ Phosphors for Full-Spectrum Lighting10Heterostructure anion-groups guided design enabling customizable Eu2+ spectrum behavior in borophosphate7A Brief Synthesis Methods and Luminescence Development of Rare Earth Activated Borophosphate Phosphor Materials0Two substitution strategies realize single-phase full-spectrum emission in Ca10Na(PO4)7:Eu2+ phosphors for WLED17Ca9–yMgyNaGd0.667(PO4)7:Eu2+: A Single Eu2+-Doped Full-Spectrum White Light Emission Phosphor with High Color Rendering Index20Color‐Tunable Emission via Site‐Selective Occupation of Eu2+ Activators in Silicate Phosphors17Cation substitution strategy realizing controllable spectral shape and multiple applications in a novel blue-cyan emitting KBaScSi2O7:Bi3+ phosphor4Designing of Eu2+-activated single-phase white-emitting phosphor through modifying cationic sites for high color rendering full-spectrum illumination3Color tunable emission and scintillation properties of Eu-doped lanthanum alumino-silicate glasses9Structural regulation and properties of Ca8.96Li Na1-Al0.667(PO4)7:0.04Eu2 + full spectrum phosphor9Recent progress of inorganic phosphors in artificial plant cultivation LEDs46A narrow band blue phosphor NaBa 4 Al 2 B 8 O 18 Cl 3 :Eu 2+ for white light emitting diodes5Violet light excitable K x Na 5 −x B 2 P 3 O 13 :Eu ( x = 0, 1, 2) borophosphates as novel phosphors for multifunctional applications2Well-designed sunlight-like Bi 3+ -activated white-light phosphor for general lighting6Preparation and properties of Tm3+/Eu3+/Tb3+ co-doped La2(PO4)1.5(BO3)0.5 phosphors3Ca9-zMzCsLu0.667(PO4)7:Eu2+ (M = Mg2+, Sr2+): β-Ca3(PO4)2-based LED phosphors with improved thermal stability and standard white light3Single‐Grain High‐Efficiency Full‐Visible‐Spectrum White Emitters17Single‐Grain High‐Efficiency Full‐Visible‐Spectrum White Emitters3Tunable photoluminescence in Eu2+-activated KCaLa(PO4)2 phosphor through structural disorder3Multiple site occupancy induced a novel broadband Ca8(Al12O24)(WO4)2: Eu2+ blue phosphor for pc-WLEDs0Understanding the charge state of the Eu ion in anti-perovskites: the role of intrinsic defects0Enhanced and Tunable Luminescent Properties of KSrBP 2 O 8:Eu 3+ Red-Emitting Phosphors Mediated by Si 4+ /Gd 3+ Co-Doping and Charge Compensation0High-efficiency full-spectrum emitters realized through structural evolution0Emission spectrum Matched-degree approaching 99.4 % sunlight-like full-spectrum white-light phosphors3Tunable Broadband Red-To-Near-Infrared Emission in Eu 2+ -Activated Sr 1– x Ba x La 2 Sc 2 O 7 Phosphors via Site-Selective Occupation and Cation Substitution3Eu3+-activated La7O6(BO3)(PO4)2 phosphors for display lighting, anti-counterfeiting patterning, fingerprint visualization and data storage0Boosting red-emitting 5D0→7F2 transition in KSrBP2O8:Eu3+ phosphors via Si4+/Gd3+ Co-doping and charge compensation0Giant luminescence enhancement in Li2MSiO4:Eu2+ (M = Sr, Ba) via two-step synthesis and charge compensation0Single‐Phase White‐Light Emission in Eu 2+ ‐Activated UCr 4 C 4 ‐Type Phosphors via Crystallographic Site Engineering0Multifunctional Ca9Na 1-y Li y Y2/3(PO4)7-Based Phosphors: Li+/Na+ Substitution-Regulated Site-Related Eu2+ Emission and Eu2+→Mn2+ Energy Transfer0

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  2. Highly Robust Oxynitride Phosphor against Thermal Oxidization and Hydrolysis

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  4. Mn2+ doping enabled efficient high-color-rendering single-phase white-emitting lead halide perovskites

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  5. Discovery of a new phosphor via aliovalent cation substitution: DFT predictions, phase transition and luminescence properties for lighting and anti-counterfeiting applications

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  6. Complex crystal structure and photoluminescence of Bi 3+ -doped and Bi 3+ /Eu 3+ co-doped Ca 7 Mg 2 Ga 6 O 18

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  7. Controllable crystal form transformation and luminescence properties of up-conversion luminescent material K 3 Sc 0.5 Lu 0.5 F 6 : Er 3+ , Yb 3+ with cryolite structure

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  8. Site engineering strategy toward enhanced luminescence thermostability of a Cr 3+ -doped broadband NIR phosphor and its application

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  9. Improving the thermal stability and luminescent efficiency of (Ba,Sr)3SiO5:Eu2+ phosphors by structure, bandgap engineering and soft chemistry synthesis method

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  10. Spontaneous-reduction and photoluminescence tuning in singly-doped Ba5-Ca (PO4)3Cl:Eu2+/Eu3+ phosphors

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  11. Pink-emitting RbBaBP2O8:Sm phosphor with diamondoid structure and high thermostability

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  12. Li + Ion Induced Full Visible Emission in Single Eu 2+ ‐Doped White Emitting Phosphor: Eu 2+ Site Preference Analysis, Luminescence Properties, and WLED Applications

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  13. Site occupancy and photoluminescence properties of cyan-emitting K2Ca2Si2O7:Bi3+ phosphor for white light emitting diodes

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  14. Thermally stable orange-red luminescence of samarium (Ⅲ)-activated KSrBP2O8 borophosphate

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  15. Extension of Spectral Shift Controls from Equivalent Substitution to an Energy Migration Model Based on Eu2+/Tb3+-Activated Ba4–xSrxGd3–xLuxNa3(PO4)6F2 Phosphors

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  16. Full-visible-spectrum lighting enabled by site-selective occupation in the high efficient and thermal stable (Rb, K)2CaPO4F: Eu2+ solid-solution phosphors

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  17. A review and outlook of ratiometric optical thermometer based on thermally coupled levels and non-thermally coupled levels

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  18. Bifunctional samarium activated red-emitting and thermal resistant phosphor for simultaneous field emission displays and white light-emitting diodes

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  19. Tuning crystal structure and luminescence of Eu 2+ -activated LiSr 1– x Ba x PO 4 solid solution for white light-emitting diodes

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  20. Multifunctional Ca9NaZn1-Mg (PO4)7:Eu2+ phosphor for full-spectrum lighting, optical thermometry and pressure sensor applications

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  24. Pressure-triggered enormous redshift and enhanced emission in Ca2Gd8Si6O26:Ce3+ phosphors: Ultrasensitive, thermally-stable and ultrafast response pressure monitoring

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  29. Towards single broadband white emission in Rb0.5K1.5CaPO4(F, Cl): Eu2+ via selective site occupancy engineering for solid-state lighting applications

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  30. Ultra‐Broadband Green‐Emitting Phosphors without Cyan Gap Based on Double‐Heterovalent Substitution Strategy for Full‐Spectrum WLED Lighting

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  31. Environment-Dependent Eu2+-Activated Ba3CaK(PO4)3 toward White-Light Emission by Chemical Cosubstitution of the (BO3)3– Anion Group

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  32. Design of K2SrCa(PO4)2-x(BO3)x:Eu2+ phosphors with full-visible spectrum by crystal structure modification

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  33. Thermal stable cyan-emitting Ba9(Lu1.5Ga0.5)Si6O24:Ce3+ for high color-rendering white LEDs

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  34. Effect of Si4+/Gd3+ doping on luminescence properties of orangish-red light-emitting phosphors of KBaBP2O8:Eu3+

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  35. Investigation into the photoluminescence and energy levels in bismuth-doped Sr3MgSi2O8 through first principles calculations

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  36. Investigation into the Eu2+ ions occupations and the coordination environments in components modulated Sr3MgSi2O8

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  37. A single-phase white-emitting La(BO3,PO4):Dy3+ phosphor with high thermostability

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  38. Site-Selective Occupancy Control of Cr Ions toward Ultrabroad-Band Infrared Luminescence with a Spectral Width up to 419 nm

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  39. Ba5GeO4Br6:Bi3+, a promising cyan phosphor for high-quality full-spectrum white light illumination

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  40. Super Broadband Near‐Infrared Solid Solution Phosphors with Adjustable Peak Wavelengths from 1165 to 875 nm for NIR Spectroscopy Applications

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  41. A broadband yellow-green emitting mixed orthoborate–pyroborate phosphor, Ba 2 Sc 2 B 4 O 11 :Ce 3+ , for white light emitting diodes

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  42. A novel bright cyan emitting phosphor of Eu 2+ activated Ba 6 BO 3 Cl 9 with robust thermal stability for full-spectrum WLED applications

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  43. Breakthrough Boost of Stokes Fluorescence from Er3+ in Perovskites for Flexible Temperature Sensing

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  44. Site Occupation Regulation of Eu2+ by the Introduction of (Bo3)3- Group Towards Full-Visible-Spectrum Emission in a Singly Doped K2basr(Po4)2:Eu2+ Phosphor

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  45. A narrow-band RbBaBP2O8:Tb3+ green phosphor with high thermal stability for backlighting display application

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  46. Site‐Engineering for Controlling Multiple‐Excitation and Emission in Eu2+‐Activated CaSrSiO4 Phosphors in Marine Fisheries

    Advanced Optical Materials · 2023-03-12

    Shuifu Liu, Dawei Wen, Rongkai Du, Chunyan Jiang, Jun Chen, Junhao Li, Lei Zhou, Мaxim S. Моlokeev, Mingmei M. Wu

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  47. Anionic Regulation toward Bi3+ Selective Occupation for Full-Spectrum White Light Emission

    Inorganic Chemistry · 2023-03-14

    Sheng Wu, Puxian Xiong, Dongliang Jiang, Quan Liu, Ke Zhang, Binli Xiao, Yan Chen, Yinzhen Wang

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  48. Ultra-narrow-band luminescence with spectral width down to 32 nm in bismuth-activated phosphate phosphors with superior thermal stability

    Materials Today Chemistry · 2023-04-01

    L. Liu, Pengpeng Dai, Dawei Wen

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  49. Structure and photoluminescence studies of Rb3GdSi2O7: Eu2+ phosphor used for NUV converted white LEDs

    Journal of Luminescence · 2023-05-24

    Jiawen Li, Jiawen Wang, Feifei Huang, Youjie Hua, Shiqing Xu, Ruoshan Lei

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  50. Enhancing thermal degradation stability of BaSi2O2N2:Eu2+ for white light-emitting diodes by ultra-thin Al2O3 layer via atomic layer deposition

    Ceramics International · 2023-06-05

    Yujie Zhao, Xiao Lu Wang, Quanan Li, Xinyu Zhang, Ye Li, Rong‐Jun Xie, J. Ruud van Ommen, Hubertus T. Hintzen

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