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RESEARCH PAPER · Chemistry of Materials · 2019

Photoluminescence Control of UCr 4 C 4 -Type Phosphors with Superior Luminous Efficiency and High Color Purity via Controlling Site Selection of Eu 2+ Activators

Wei Wang, Mengxuan Tao, Yixin Liu, Yi Wei, Gongcheng Xing, Peipei Dang, Jun Lin, Guogang Li

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Photoluminescence Control of UCr 4 C 4 -Type Phosphors with Superior Luminous Efficiency and High Color Purity via Controlling Site Selection of Eu 2+ ActivatorsOriginalAchieving high thermal stability of different rare-earth ions in a single matrix host via the manipulation of the local structure by a solid solution13Novel narrow-band blue-emitting Cs 3 Zn 6 B 9 O 21 :Bi 3+ phosphor with superior thermal stability33A novel tunable extra-broad yellow-emitting nitride phosphor with zero-thermal-quenching property106Cuboid-Size-Controlled Color-Tunable Eu-Doped Alkali–Lithosilicate Phosphors85Site-selective occupation of Eu2+ activators toward full-visible-spectrum emission in well-designed borophosphate phosphors96Dual‐Shelled RbLi(Li 3 SiO 4 ) 2 :Eu 2+ @Al 2 O 3 @ODTMS Phosphor as a Stable Green Emitter for High‐Power LED Backlights90Dual‐Shelled RbLi(Li3SiO4)2:Eu2+@Al2O3@ODTMS Phosphor as a Stable Green Emitter for High‐Power LED Backlights8A novel Mn4+-activated Li3CsGe8O18 red phosphor and cation substitution induced photoluminescence improvement11Narrow-band emitters in LED backlights for liquid-crystal displays217Broadband NaK2Li[Li3SiO4]4:Ce Alkali Lithosilicate Blue Phosphors19Broad-Band Excited and Tunable Luminescence of CaTbAl3O7:RE3+ (RE3+ = Ce3+ and/or Eu3+) Nanocrystalline Phosphors for Near-UV WLEDs24Highly thermal stable phosphor LiSrPO4:Eu2+ with a new crystal structure15Broadband Near-Infrared Emitting Ca2LuScGa2Ge2O12:Cr3+ Phosphors: Luminescence Properties and Application in Light-Emitting Diodes202Manipulating the redistribution of single dopant via crystal-site engineering approach in Ba4Gd3(K1-xNax)3(PO4)6F2:Eu2+ phosphors for warm white light emitting diodes45Zero-thermal-quenching and improved chemical stability of a UCr4C4-type phosphor via crystal site engineering42Adjustable photoluminescence of Bi3+ and Eu3+ in solid solution constructed by isostructural end components through composition and excitation-driven strategy90Red-tunable LuAG garnet phosphors via Eu 3+ →Mn 4+ energy transfer for optical thermometry sensor application72Near‐Unity Cyan‐Green Emitting Lead‐Free All‐Inorganic Cesium Copper Chloride Phosphors for Full‐Spectrum White Light‐Emitting Diodes25Two-Site Occupancy Induced a Broad-Band Emission in Phosphor K2YZr(PO4)3:Eu2+ for White-Light-Emitting Diode Applications47A zero-thermal-quenching perovskite-like phosphor with an ultra-narrow-band blue-emission for wide color gamut backlight display applications67Complex crystal structure and photoluminescence of Bi 3+ -doped and Bi 3+ /Eu 3+ co-doped Ca 7 Mg 2 Ga 6 O 1819Crystal phase transition and polyhedron transformation towards the evolution of photoluminescence and the improvement of thermal stability in efficient blue-emitting Ba 0.47− x Sr 0.50+ x Al 2 Si 2 O 8 :Eu 2+10Design of broadband near-infrared Y 0.57 La 0.72 Sc 2.71 (BO 3 ) 4 :Cr 3+ phosphors based on one-site occupation and their application in NIR light-emitting diodes71Enhanced luminescence and tunable color in [Eu 2+ , Si 4+ ]/Mn 2+ doped K 2 BaCa(PO 4 ) 2 based on charge compensation and energy transfer5Highly efficient green-emitting phosphor Sr 4 Al 14 O 25 :Ce,Tb with low thermal quenching and wide color gamut upon UV-light excitation for backlighting display applications56Learning from Mineral Structures toward New Luminescence Materials for Light-Emitting Diode Applications146Superior thermally-stable narrow-band green emitter from Mn2+-doped zero thermal expansion (ZTE) material78Spontaneous-reduction and photoluminescence tuning in singly-doped Ba5-Ca (PO4)3Cl:Eu2+/Eu3+ phosphors23High-Performance NaK2Li[Li3SiO4]4:Eu Green Phosphor for Backlighting Light-Emitting Diodes52The Phase Transition and Photoluminescence Properties of (Ca9−x Sr x )Mg1.5(PO4)7:Eu2+ Solid-Solution Phosphors3Near-ultraviolet excited broadband orange-yellow emitting Sr8MgIn(PO4)7:Eu2+ phosphors for WLEDs with high color rendering index10Simultaneous Broadening and Enhancement of Cr 3+ Photoluminescence in LiIn 2 SbO 6 by Chemical Unit Cosubstitution: Night‐Vision and Near‐Infrared Spectroscopy Detection Applications325Simultaneous Broadening and Enhancement of Cr3+Photoluminescence in LiIn2SbO6by Chemical Unit Cosubstitution: Night‐Vision and Near‐Infrared Spectroscopy Detection Applications5A broadband emitting Sr8MgGa(PO4)7:Eu2+ phosphor for application in white light-emitting diodes with excellent color rendering index6Tailoring of White Luminescence in a NaLi 3 SiO 4 :Eu 2+ Phosphor Containing Broad‐Band Defect‐Induced Charge‐Transfer Emission183Na Replaces Rb towards High‐Performance Narrow‐Band Green Phosphors for Backlight Display Applications53Ca[B 8 O 11 (OH) 4 ] : Eu 2+ – A Highly Efficient Deep Blue‐Emitting Phosphor Prepared by Low‐Temperature Self‐reduction12Optical properties of double-perovskite Sr3TeO6:Sm3+ reddish-orange emitting phosphors for w-LEDs19Linking Macro- and Micro-structural Analysis with Luminescence Control in Oxynitride Phosphors for Light-Emitting Diodes13Highly Efficient Green‐Emitting Phosphor BaZnAl 10 O 17 :Mn 2+ with Ultra‐Narrow Band and Extremely Low Thermal Quenching for Wide Color Gamut LCD Backlights59Chasing Down the Eu2+ Ions: The Delicate Structure−Property Relationships in the Ultra‐Narrow Band Phosphor K1.6Na2.1Li0.3[Li3SiO4]4:Eu2+35Narrow Bandwidth Luminescence in Sr2Li(Al,Ga)O4:Eu2+ by Selective Site Occupancy Engineering for High Definition Displays52Suppression of Eu2+ Luminescence Loss14Full-visible-spectrum lighting enabled by site-selective occupation in the high efficient and thermal stable (Rb, K)2CaPO4F: Eu2+ solid-solution phosphors58Anti-thermal-quenching red-emitting phosphors based on lanthanide doped negative-thermal-expansion (NTE) hosts46Tuning crystal structure and luminescence of Eu 2+ -activated LiSr 1– x Ba x PO 4 solid solution for white light-emitting diodes5Development of narrow band emitting phosphors for backlighting displays and solid state lighting using a clean and green energy technology22Multifunctional Ca9NaZn1-Mg (PO4)7:Eu2+ phosphor for full-spectrum lighting, optical thermometry and pressure sensor applications112(INVITED)Narrow-band violet and blue emission of Bi3+ in M10P6O25 (M = Ca, Sr) based on highly symmetric crystal structure10High thermal stability phosphors with a rigid structure similar to the benzene ring and application in plant growth21Novel ultra-high-temperature zero-thermal quenching plant-protecting type blue-green dual-emission KAl 11 O 17 :Eu 2+ ,Mn 2+ phosphors for urban ecological lighting39Tunable emission of Li 4 SrCaSi 2 O 4− y N 2 y / 3 :Eu 2+ phosphors based on anion substitution induction for WLEDs and optical thermometry12Tuning of the thermal quenching performance of Bi 3+ -doped scheelite Ca(Mo/W)O 4 solid solution phosphors13How to Obtain Anti‐Thermal‐Quenching Inorganic Luminescent Materials for Light‐Emitting Diode Applications252Optical thermometry based on europium doped self-activated dual-emitting LiCa3ZnV3O12 phosphor27High-performance narrow-band green-emitting phosphor enabled by substituting Na with Rb6Microscopic Mechanism of the Heat‐Induced Blueshift in Phosphors and a Logarithmic Energy Dependence on the Nearest Dopant–Vacancy Distance24Microscopic Mechanism of the Heat‐Induced Blueshift in Phosphors and a Logarithmic Energy Dependence on the Nearest Dopant–Vacancy Distance1Narrow-band phosphor K2ZnP2O7:Eu2+ discovered using local structure similarity19Structural induced tunable NIR luminescence of (Y,Lu)3(Mg,Al)2(Al,Si)3O12: Cr3+ phosphors37Electronic and Optical Properties of Eu2+-Activated Narrow-Band Phosphors for Phosphor-Converted Light-Emitting Diode Applications: Insights from a Theoretical Spectroscopy Perspective70Highly Efficient Broad-Band Green-Emitting Cerium(III)-Activated Garnet Phosphor Allows the Fabrication of Blue-Chip-Based Warm-White LED Device with a Superior Color Rendering Index69Evolutionary Generation of Phosphor Materials and Their Progress in Future Applications for Light-Emitting Diodes563Facile Microwave Synthesis of a Narrow-Band Green-Emitting Phosphor Cs3MnBr5 and the Effect of Anion Substitution on Its Luminescence Properties17Towards single broadband white emission in Rb0.5K1.5CaPO4(F, Cl): Eu2+ via selective site occupancy engineering for solid-state lighting applications42A novel sulfide phosphor, BaNaAlS3:Eu2+, discovered via particle swarm optimization24Photoluminescence of Bi3+ in LiCaY5(BO3)6 and color-tunable emission through energy transfer to Eu3+/Tb3+11Defect and energy transfer induced abnormal thermally stable and highly efficient narrow-band green emission19Novel near-ultraviolet-excited and thermally-stable blue-emitting phosphor for healthy WLED lighting30Prediction of formation energies of UCr4C4-type compounds from Magpie feature descriptor-based machine learning approaches9Shining Transparent Displays with Stable Narrow‐Band Blue‐Emitting Phosphor in Layered Film50Accurately Controlling the Occupation of Eu2+ in Cs(K, Na)3(Li3SiO4)4 to Achieve Narrow-Band Green Emission for Wide Color Gamut Displays29Luminescence in the solid state7Tuning the thermal quenching properties of Ga3+-modified LiTaO3:Bi3+ phosphor through defect engineering strategy12Narrow-Band Emitting Phosphor Na2Cs2Sr(B9O15)2:Eu2+ Discovered from Local Structure Similarity with Sulfate Phosphor8A novel bright cyan emitting phosphor of Eu 2+ activated Ba 6 BO 3 Cl 9 with robust thermal stability for full-spectrum WLED applications65A novel narrow-band blue-emitting phosphor with high efficiency and thermal stability for WLEDs and FEDs31Local Structure and Self‐Defect Evolution under Nonstoichiometric Effect Unlock Zero‐Thermal‐Quenching15Site‐Engineering for Controlling Multiple‐Excitation and Emission in Eu2+‐Activated CaSrSiO4 Phosphors in Marine Fisheries21Ultra-narrow-band luminescence with spectral width down to 32 nm in bismuth-activated phosphate phosphors with superior thermal stability11Site regulation and luminescence properties of Eu3+, Eu2+ in (La, Mg):SrAl12O19 matrix6Thiogallate phosphor for white LEDs with water-resistance and green light-emitting capability7The developments of cyan emitting phosphors to fulfill the cyan emission gap of white-LEDs9Highly Efficient Narrow-Band Green-Emitting Na 3 K 5 (Li 3 SiO 4 ) 8 :Eu 2+ Phosphor with Low Thermal Quenching49Unusual red luminescence and super thermal stability of a new narrow-band emission phosphor for backlight display application21A novel reddish‐orange emitting NaSrBiTeO 6 :Sm 3+ phosphor with high moisture resistance and thermostability for horticultural light emitting diode applications17Narrow-band green phosphor RbK 2 Na(Li 3 SiO 4 ) 4 :Eu 2+ with excellent thermal stability and high efficiency for wide color gamut displays8Progress of Ce 3+ /Eu 2+ doped phosphors for violet chip based full-spectra lighting42BaLiZn 3 (PO 4 ) 3 :Eu 2+ : Ultranarrow-Band Violet Emission in a Highly Symmetric Crystal Structure24Mn–Mn Magnetic Coupling Interaction-Induced Red Emission in a Tetra-Coordinated Lattice23Acid Post-Treatment Triggered High-Efficiency Blue-Emitting LiNa2Sr8B12O24F6Cl:Eu2+ Phosphors toward Multipurpose LED Applications0Broadband spectral cyan emission phosphor for full-spectrum LED caused by interstitial site occupation2Phosphor-converted light-emitting diodes in the marine environment: current status and future trends40Discovering a Novel Cyan‐Light‐Emitting Thiosilicate Phosphor, Li 2 BaSiS 4 :Eu 2+ , via Experimental Active Learning4Designing Ultra‐Narrow‐Band Red Phosphor via Oxygen Vacancy Engineering for Transparent Display Application14Narrow-band green nitride phosphor for wide color gamut backlighting11Ca9-zMzCsLu0.667(PO4)7:Eu2+ (M = Mg2+, Sr2+): β-Ca3(PO4)2-based LED phosphors with improved thermal stability and standard white light3Novel ultra-broadband cyan phosphor with excellent thermal stability for full-spectrum WLED7Development of Eu 2+ ‐Doped UCr 4 C 4 ‐Type Phosphors Toward Advanced Display Applications22Narrow‐Band Green Phosphors for Advanced Display Technologies: Material Design, Performance Optimization, and Future Prospects6From Model to Material: Machine Learning Enabled Discovery of LED‐Compatible Phosphors4Modulation of Lattice Strain‐Induced Eu 2+ Single Lattice Site Emission for Narrow‐Band Green Phosphors in High‐Performance Laser Displays2Manipulating Persistent Luminescence via Chemical Unit Cosubstitution in Gallate Spinel Li 1– x Mg 2 x Ga 5– x O 8 :Cr 3+ Solid Solution2Defect and crystal field engineering enables high efficiency and anti-thermal quenching in Cr3+ doped rigid garnet phosphors for multifunctional optoelectronics2A Non‐Stoichiometric Thioaluminate Phosphor with Severe Stacking Faults, Na 0.9 AlS 2 :Eu 2+1Narrow‐Band Green‐Emitting β‐SiAlON:Eu 2+ for Wide‐Color‐Gamut Laser‐Driven Projection Displays1Heavy-element substitution simultaneously boosts comprehensive photoluminescence performance of Ce3+-activated garnets toward multifunctional optical applications0Site-selective Eu2+ occupation in multi-polyhedral Ca3Al2O6 for tunable high-color-purity blue and red emission0Blue-light-excitable Y2W3O12:Eu phosphor enabling efficient high-temperature photothermal feedback0Cation‐Engineered Narrow‐Band Green Emitting Phosphor Toward High‐Performance Laser‐Driven Displays0

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  5. Site-selective occupation of Eu2+ activators toward full-visible-spectrum emission in well-designed borophosphate phosphors

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  11. Broad-Band Excited and Tunable Luminescence of CaTbAl3O7:RE3+ (RE3+ = Ce3+ and/or Eu3+) Nanocrystalline Phosphors for Near-UV WLEDs

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