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RESEARCH PAPER · Advanced Functional Materials · 2021

Giant Red‐Shifted Emission in (Sr,Ba)Y 2 O 4 :Eu 2+ Phosphor Toward Broadband Near‐Infrared Luminescence

Zhiyu Yang, Yifei Zhao, Yayun Zhou, Jianwei Qiao, Yu‐Chun Chuang, Мaxim S. Моlokeev, Zhiguo Xia

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Giant Red‐Shifted Emission in (Sr,Ba)Y 2 O 4 :Eu 2+ Phosphor Toward Broadband Near‐Infrared LuminescenceOriginalAccessing High-Power Near-Infrared Spectroscopy Using Cr3+-Substituted Metal Phosphate Phosphors114Deep-red to near-infrared emission of binuclear platinum( ii ) complexes by breaking hydrogen bonds3Design of a nitridoalumosilicate red phosphor synthesized under mild conditions5Efficient broadband near-infrared emission induced by Nb 5+ substitution for Ta 5+ in GaTa 1− y Nb y O 4 :Cr 3+ phosphor50Local environment rigidity and the evolution of optical properties in the green-emitting phosphor Ba 1− x Sr x ScO 2 F:Eu 2+12Manipulating trap distribution and density by chemical unit cosubstitution for near-infrared persistent luminescent Zn 1−2 x Li x Ga 2+ x O 4 :Cr 3+ solid solutions22Optical fiber temperature sensor of Er 3+ /Yb 3+ codoped LaGaO 3 microcrystals with high reliability and stability40Reducing the cyan-cavity: Lu 2 MAl 4 SiO 12 :Ce 3+ (M = Mg, Ca, Sr and Ba) phosphor-in-glass film towards full-spectrum laser-driven lighting24Tunable concentration/excitation-dependent deep-red and white light emission in single-phase Eu 2+ -activated Sc-based oxide phosphors for blue/UV-LEDs32Utilizing the energy transfer mechanism to realize color tunable luminescence14Stable Tunable Luminescence of Hetero-valent Eu Ion Activated Ba2InTaO6 Phosphors Synthesized by Defect-Induced Self-Reduction in the Molten-Salt Method16Photoluminescence Properties of AScSi 2 O 6 :Cr 3+ (A = Na and Li) Phosphors with High Efficiency and Thermal Stability for Near-Infrared Phosphor-Converted Light-Emitting Diode Light Sources175Efficient and Thermally Stable Broad-Band Near-Infrared Emission in a KAlP 2 O 7 :Cr 3+ Phosphor for Nondestructive Examination191A novel Cr3+-activated far-red titanate phosphor: synthesis, luminescence enhancement and application prospect59Design of a Novel Near-Infrared Luminescence Material Li2Mg3TiO6:Cr3+ with an Ultrawide Tuning Range Applied to Near-Infrared Light-Emitting Diodes111Novel one-dimensional Ga2O3:Cr3+ nanofibers with broadband emission for near infrared LED sources13Near-Infrared-to-Near-Infrared Optical Thermometer BaY 2 O 4 : Yb 3+ /Nd 3+ Assembled with Photothermal Conversion Performance72Broadband near-infrared emission in the NaInP2O7:Cr3+ phosphor for light-emitting-diode applications50Near‐Infrared Light‐Emitting Diodes utilizing a Europium‐Activated Calcium Oxide Phosphor with External Quantum Efficiency of up to 54.7%320Broadband Near-Infrared-Emitting Phosphors with Suppressed Concentration Quenching in a Two-Dimensional Structure47Luminescence characteristics of Bi3+, Cr3+ and Bi3+/Cr3+ activated Sr3Y2Ge3O12 phosphors27Synthesis of the Red-Emitting (Ba, Ca)2ScAlO5:Eu3+ Phosphors with Photoluminescence Properties30Modulation of Thermally Stable Photoluminescence in Cr 3+ -Based Near-Infrared Phosphors201Blue LED‐Pumped Broadband Short‐Wave Infrared Emitter Based on LiMgPO4:Cr3+,Ni2+ Phosphor97Towards single broadband white emission in Rb0.5K1.5CaPO4(F, Cl): Eu2+ via selective site occupancy engineering for solid-state lighting applications42A super stable Near-Infrared garnet phosphor resistant to thermal Quenching, thermal degradation and hydrolysis57Interstitial Li + Occupancy Enabling Radiative/Nonradiative Transition Control toward Highly Efficient Cr 3+ -Based Near-Infrared Luminescence83Efficient near-infrared broadband garnet phosphor for pc-LED and its application to vascular visualization and night vision13Low-concentration Ce3+-activated ScCaO(BO3) blue-cyan phosphor with high efficiency toward full-spectrum white LED applications58A novel blue-emitting Tm3+ and Tb3+ co-doped Ca9Nd(PO4)7 phosphor for white light-emitting diodes1Enhanced Thermal Stability and Energy Transfer by Crystal‐Field Engineering in a Garnet Phosphor for Thermometry and NIR‐LED48Ultra‐Broadband Green‐Emitting Phosphors without Cyan Gap Based on Double‐Heterovalent Substitution Strategy for Full‐Spectrum WLED Lighting89Environment-Dependent Eu2+-Activated Ba3CaK(PO4)3 toward White-Light Emission by Chemical Cosubstitution of the (BO3)3– Anion Group19High-Efficiency and Wavelength-Tunable Near-Infrared Emission of Lanthanide Ions Doped Lead-Free Halide Double Perovskite Nanocrystals toward Fluorescence Imaging70Light-Induced Charge Transfer to Achieve Deep-Red Emission in SrSc2O4:Bi toward Multiple Optical Applications17Investigation into the Eu2+ ions occupations and the coordination environments in components modulated Sr3MgSi2O81Structure and Upconversion Luminescence Properties of Pr3+-Doped Y2SiO5 Phosphor24Compositional tuning and site engineering of Sr-alloyed Ca3(PO4)2:Mn2+, Eu2+ towards multicenter-activated single-component white light emitter6Synthesis and luminescent properties of red-emitting Li2CaSnO4: xEu3+ phosphors0Broadband NIR Phosphor Ca2LuScAl2Si2O12:Cr3+ for NIR LED Applications151Recent Developments of Microscopic Study for Lanthanide and Manganese Doped Luminescent Materials8Recent progress in Ce 3+ /Eu 2+ -activated LEDs and persistent phosphors: focusing on the local structure and the electronic structure137Single-Site Mn2+-Activated and Sr-Alloyed Ca3(PO4)2 Red Phosphors and Their Lighting Applications1Site-Selective Occupancy Control of Cr Ions toward Ultrabroad-Band Infrared Luminescence with a Spectral Width up to 419 nm79Highly efficient Mn–Mn dimer activated phosphors for high-power near-infrared LED application27Recent Advances in Chromium‐Doped Near‐Infrared Luminescent Materials: Fundamentals, Optimization Strategies, and Applications252Thermally stable and tunable broadband near-infrared emission from NIR-I to NIR-II in Bi-doped germanate glass for smart light sources19Designing stimuli-responsive and color-tunable indicators via the coexistence of dual emitting centers7A broadband near-infrared Cr 3+ -doped phosphor applied to near-infrared light-emitting diodes: enhanced luminescence and thermal stability by annealing20Achieving excellent thermostable red emission in singly Mn 2+ -doped near-zero thermal expansion (NZTE) material Li 2 Zn 3 (P 2 O 7 ) 26An efficient and thermally stable Cr 3+ -activated Y 2 GdSc 2 Al 2 GaO 12 garnet phosphor for NIR spectroscopy applications14High performance of broad excitation and narrow emission green phosphor NaAl 11 O 17 :Eu 2+ , Mn 2+ for backlight displays20Highly efficient and thermally stable broadband near-infrared emitting garnet Ca 3 Sc 2 Ge 3 O 12 :Cr 3+ ,Ce 3+ phosphors for multiple pc-LED applications33Multiple site occupancy induced yellow-orange emission in an Eu 2+ -doped KSr 6 Sc(SiO 4 ) 4 phosphor towards optical temperature sensors13Oxynitride K 2 Ba 6.72 Si 16 O 40−1.5 y N y :0.28Eu 2+ phosphor with high thermal stability realized by crystal field engineering1Site-selective occupation, optical spectrum regulation and photoluminescence property investigation of Eu 2+ -activated blue light-excited yellow-orange emitting phosphors5The broadband emission of Cr 3+ -doped CaY 2 Mg 2 Ge 3 O 12 and its applications for NIR detectors17Achievement of full-visible-spectrum lighting in Bi3+-activated strontium gallates via lattice site occupancy engineering toward WLEDs applications32LaMgGa11O19:Cr3+,Ni2+ as Blue‐Light Excitable Near‐Infrared Luminescent Materials with Ultra‐Wide Emission and High External Quantum Efficiency111Solid solution of Cr3+ doped ZnGa2O4 and Zn2SnO4 to create cation inversion and its role on persistent deep red emission19Engineering charge-transfer interactions for red-emitting SrLa(Sc,Ga)O4:Ce3+ phosphor with improved thermal stability22Broadband and Multimode Near‐Infrared Emitter Based on Cr3+‐Activated Stannate for Multifunctional Applications75Synthesis and luminescence properties of Eu3+, Dy3+ co-doped Ca3Bi(PO4)3 single-phase phosphor64Single‐Site Occupancy of Eu 2+ in Multiple Cations Enables Efficient Ultra‐Broadband Visible to Near‐Infrared Luminescence83Ingredient regulation engineering of samarium(III)-activated double-perovskite niobate matrices12Facile Synthesis of Highly Efficient and Thermally Stable BaAl 4 Sb 2 O 12 :Eu 2+ Phosphor in Air72Infrared to Short-Wave Infrared-Emitting Phosphors for Light-Emitting Diode Applications23An efficient double-perovskite CaLaLiTeO6:Mn4+ far-red phosphor towards indoor plant lighting application57Achieving High Quantum Efficiency Broadband NIR Mg4Ta2O9:Cr3+ Phosphor Through Lithium‐Ion Compensation189Near‐Infrared Persistent Phosphor‐Mediated Smart Sensing Light‐Emitting Diodes for Advanced Driver Assistance Systems11Deep‐Red Ca3Al2Ge3O12:Eu3+ Garnet Phosphor with Near‐Unity Internal Quantum Efficiency and High Thermal Stability for Plant Growth Application67Thermally Stable Red‐Emitting Oxide Ceramics for Laser Lighting153Developing Broadband Cr3+-Substituted Phosphor-Converted Near-Infrared Light Sources38Near-Infrared LuCa 2 ScZrGa 2 GeO 12 :Cr 3+ Garnet Phosphor with Ultra-broadband Emission for NIR LED Applications60Research progress of rare earth/transition metal ions doped NIR luminescent materials6The ultra-wideband near-infrared luminescence properties and applications of K2SrGe8O18:Cr3+ phosphor26A New Efficient Deep-Red-Emission Phosphor Y3Al4.9Sb0.1O12: Ce3+, Cr3+ with Application Potential in Plant Growth3A novel broad-band red K2MgSiO4:Eu2+ phosphor and defect-induced tunable emission from red to yellow20The development of a new efficient red phosphor based on Eu2+ doped traditional inorganic oxygenate-perovskite compounds7Efficient Ultra‐Broadband Phosphors for High-Power Near-infrared LED and night vision imaging system sources15Developments of Eu2+/Ce3+-activated red luminescence in oxide host matrices with strong crystal field coordination6Highly Quantum Efficient and Thermally Stable Near‐Infrared‐Emitting K‐β‐Al 2 O 3 :Cr 3+ Phosphor56Novel red ZnLaB5O10:Sm3+ phosphor with high thermal stability for application in high CRI w-LEDs9Synthesis, spectral characteristics and energy transfer of SrLa2Al2O7:Mn4+, Dy3+31Optical Thermometer Based on Efficient Near‐Infrared Dual‐Emission of Cr3+ and Ni2+ in Magnetoplumbite Structure53Site Occupation Engineering toward Giant Red-Shifted Photoluminescence in (Ba,Sr)2LaGaO5:Eu2+ Phosphors63Valence conversion and site reconstruction in near-infrared-emitting chromium-activated garnet for simultaneous enhancement of quantum efficiency and thermal stability161Simultaneous enhancement of red luminescence and thermal stability of a novel red phosphor: A Li+-Eu3+ co-occupied site strategy in BaAl2Ge2O8 lattices27SrHfO3:Cr3+ Perovskite Microcubes for Rare-Earth-Free NIR-I Light Emission11Cr 3+ -Doped La 2 MgSnO 6 Double Perovskite Phosphors for Near-Infrared pc-LEDs22High Output Power and High Quantum Efficiency in Novel NIR Phosphor MgAlGa0.7B0.3O4:Cr3+ with Profound FWHM Variation143Near‐Infrared Emission of Sm2+ in Oxynitrides14Broadband emitting Fe 3+ ‐doped double perovskite‐type antimonates phosphors for NIR spectroscopy applications28Regulation of the luminescence of Bi3+-activated Ca5Ga6O14 phosphors by varying doping concentration and composition design5Spectroscopic investigation of K5La(MoO4)4:Sm3+ red phosphor with excellent thermal stability and color purity for white LEDs45Thermally stable broadband near-infrared emitting pyrochlore oxide phosphors codoped with Cr3+ and Yb3+ ions22Small Stokes Shift and Two‐Site Occupation in the ANb2O6:Cr3+ (A = Zn/Mg) Phosphors Toward Highly Efficient Ultra‐Broadband Near‐Infrared Emission for Multifunctional Applications24Abnormal spectral broadening of ordered-structure near-infrared phosphor La 2 CaHfO 6 :Cr 3+15Achieving a Eu 2+ -doped NIR phosphor via ionic modulation and its multifunctional applications4Achieving spectrally tunable and thermally stable near-infrared emission in Fe 3+ -activated spinel phosphors via the cation site modulation strategy34Boosting broadband short-wave infrared emission to achieve near-unity quantum efficiency via bridging Cr 3+ –Ni 2+ in spinel solid-solutions towards light-emitting diode applications31Broadband short-wave near-infrared-emitting phosphor MgNb 2 O 6 :Cr 3+ for pc -LED applications9Highly efficient and thermostable far-red phosphor for promoting root growth in plants11Long wavelength near-infrared II emitting Na3YSi3O9:x Cr3+ silicate and spectral broadening by multi-site occupancy0Research progress on Fe 3+ -activated near-infrared phosphor18Structure modification and luminescence regulation in new violet light excitable Sr (2− y ) Ba y Y 4 La 4 (SiO 4 ) 6 O 2 : x Eu 2+ phosphors via cation substitution6Structure tailoring and defect engineering of a highly thermally stable red emitting phosphor22Synthesis and photoluminescence properties of high-quality reddish-orange emitting Ca 4 Nb 2 O 9 :Eu 3+ phosphors for WLEDs and anti-counterfeiting18Broadband NIR luminescence of Cr3+-doped Mg4Nb2O9 phosphors toward LED light source applications for NIR spectrometry7An efficient and thermally stable red emitting Eu2+ doped oxide for rechargeable portable flashlight62Optical properties of Sr2LuNbO6:Mn4+ deep-red phosphor: crystal-field splitting and multimode vibrational coupling21Directly Identifying Multiple Cr3+ Emitting Centers for Broad Near‐Infrared Emission in an Efficient and Near‐Zero Thermal Quenching Garnet‐Type Phosphor50Thermally Stable Red-Emitting Ca18K3Sc(PO4)14:Mn2+ Phosphor and Enhanced Luminescence by Energy Transfer Between Ce3+-Eu2+-Mn2+22Efficient Near-Infrared Luminescence with Near-Unity Photoluminescence Quantum Yield in Erbium-Doped Double Perovskites Cs 2 NaYCl 6 under Green Light Excitation55Tailoring the Cr3+ Emission via Combinatorial Management of Crystal‐Field and Energy Transfer for Multiple NIR LEDs30Near‐infrared emitting metal halide materials: Luminescence design and applications78Well-Performed Green Phosphor BaY 4 Si 5 O 17 :Ce 3+ ,Tb 3+ with High Quantum Efficiency and Thermal Stability23Deciphering crystal structure of Li 3 Bi 3 Te 2 O 12 :Sm 3+ phosphors with high thermal stability for plant cultivation and white light‐emitting diodes16Ultrahigh Quantum Efficiency Near-Infrared-II Emission Achieved by Cr 3+ Clusters to Ni 2+ Energy Transfer51A highly sensitive multiple-mode optical thermometer designed in Eu 2+/3+ and Li + co-doped polymorphism compound LaSc 3 (BO 3 ) 432Boosting Near‐Infrared Emission in Spinel‐Type Phosphor via Oxygen Vacancy Engineering for Versatile Application121Simultaneous NIR Emission and Thermal Stability Enhancement in Garnet‐Type NIR Phosphors through the Synergistic Effect of Lattice Distortion and Enhanced Rigidity60Achieving broadband NIR-I to NIR-II emission in layer-structured Mg4Nb2O9:Cr3+,Yb3+ phosphor for multifunctional applications12Color-tunable photoluminescence and energy transfer properties of single-phase Sr2MgSi2O7:Eu3+, Dy3+29Mn 2+ –Mn 2+ Dimers Induced Robust Light Absorption in Heavy Mn 2+ Doped ZnAl 2 O 4 Near‐Infrared Phosphor with an Excellent Photoluminescence Quantum Yield and Thermal Stability28Amorphous to Crystalline Phase Transformation Enables Tunable Persistent Luminescence for Multi‐Mode Optical Information Storage53Europium Ions Self‐Reduction Benefiting from AlO4/Si(Al)O4 Network Structure for Multimode Optical Thermometry Manometry27Ultra‐Broadband Near‐Infrared Luminescence from a Vanadium‐Activated Phosphate Glass12Realizing Ultrabroadband NIR-II Emission and Wide-Range Wavelength Tuning in Cr4+-activated ABO2 (A = Li, Na; B = Al, Ga) Phosphors10Crystal Field Engineering Inducing Transformation from Narrow Band of Eu3+ to Broadband of Eu2+2Unlocking Chlorine Oxide‐Based Ultra‐Wideband Near‐Infrared Phosphor and Advancing Spectral Performance via Lattice Engineering43Colour change and long-persistent properties of a new phosphor YBaZn3GaO7:Bi3+/Eu3+6Regulating the broadband near-infrared emission of Eu2+-doped Ca3Sc2Si3O12 phosphors through constructing defect for diversified applications56Thermal Stability Enhancement by a Cationic Substitution Strategy in Red-Emitting Eu2W3–xMoxO12 Solid-Solution Phosphors1CaLu2Mg2Si3O12:Ce3+, Cr3+, Nd3+ Phosphor‐In‐Glass Film for Laser‐Driven Ultra‐Broadband Near‐Infrared Lighting with Watt‐Level Output35Ultrabroadband Long-Wavelength Near-Infrared MgIn2O4:Ni2+ Phosphor Synthesized via Sol–gel Combustion Method as a Light Source for Night Vision Imaging, Nonvisual Detection, and Anticounterfeiting Display38Structural characterization and luminescence properties of Cr3+ activated ZnMgTiO4 far-red emitting phosphor2Wide Range Near‐Zero Thermal Quenching of Orange–Yellow Phosphor via Impeding Self‐Oxidation of Eu 2+ for Versatile Optoelectronic Applications20Achieving a Balance of Good Quantum Efficiency and Thermal Stability in the Y2CaScAl3GeO12:Cr3+ Broadband Phosphor for Multiple NIR Spectroscopy Applications17Local structure engineering of Ba1-K La2Y2(SiO4)2O1-: Eu2+ green phosphors for violet-light-excitable full-spectrum lighting11Color‐Tunable Emission via Site‐Selective Occupation of Eu2+ Activators in Silicate Phosphors17Cr3+-doped Na2CaSn2Ge3O12 garnet showing broadband near-infrared emission at 820 nm with zero thermal quenching and near-unity quantum yield48Color-tunable luminescence and energy transfer of Ba2YZrO6:R (R = Dy3+, Sm3+, Dy3+/Sm3+)10Non‐volatile and Secure Optical Storage Medium with Multilevel Information Encryption18Ultra-broadband emission from Mg7Ga2GeO12:Ni2+,Cr3+ phosphor spanning the NIR I–III regions for spectroscopy applications10Enhanced thermal stability of broadband NIR phosphors Ca3.3Mg0.7ZrGe3O12:Cr3+ for pc-LEDs8Structure–Photoluminescence Relationship in Ce3+-Doped K5Y(P2O7)2 and Its Sensitization to Dy3+ with Enhanced White Light Emission7Customized Cyan Phosphors for Efficient Full‐Spectrum Illumination and Fingerprint Detection22Low‐Coordination Crystallographic Lattice Engineering to Discover Ce 3+ ‐Activated Ultra‐Wide Visible‐to‐Near‐Infrared Luminescent Materials9Enhanced Stability and Brightness through Co‐Substitution: Promoting Plant Growth with Green‐Excited Deep Red Phosphor Ca1‐zSrzLi1‐xMg2xAl3‐xN4:yEu2+13

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  39. Synthesis and luminescent properties of red-emitting Li2CaSnO4: xEu3+ phosphors

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  43. Single-Site Mn2+-Activated and Sr-Alloyed Ca3(PO4)2 Red Phosphors and Their Lighting Applications

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  44. Site-Selective Occupancy Control of Cr Ions toward Ultrabroad-Band Infrared Luminescence with a Spectral Width up to 419 nm

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  45. Highly efficient Mn–Mn dimer activated phosphors for high-power near-infrared LED application

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  47. Thermally stable and tunable broadband near-infrared emission from NIR-I to NIR-II in Bi-doped germanate glass for smart light sources

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  48. Designing stimuli-responsive and color-tunable indicators via the coexistence of dual emitting centers

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  49. A broadband near-infrared Cr 3+ -doped phosphor applied to near-infrared light-emitting diodes: enhanced luminescence and thermal stability by annealing

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