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RESEARCH PAPER · Angewandte Chemie International Edition · 2024

Chloride and Hydride Transfer as Keys to Catalytic Upcycling of Polyethylene into Liquid Alkanes

Wei Zhang, Hai Yao, Rachit Khare, Peiran Zhang, Boda Yang, Wenda Hu, Debmalya Ray, Jian Zhi Hu, Donald M. Camaioni, Huamin Wang, Sung Min Kim, Mal‐Soon Lee, Michele L. Sarazen, Jingguang G. Chen, Johannes A. Lercher

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Chloride and Hydride Transfer as Keys to Catalytic Upcycling of Polyethylene into Liquid AlkanesOriginalGraphical Abstract: Angew. Chem. Int. Ed. 17/20240Catalytic chemical recycling and upcycling of polyolefin plastics27Room-Temperature Upcycling of Mixed PVC and Polyolefin Waste1Active species in chloroaluminate ionic liquids catalyzing low-temperature polyolefin deconstruction22Catalytic Upcycling of Polyolefins316Shape selective cracking of polypropylene on an H- MFI type zeolite catalyst with recovery of cyclooctane solvent4Room-temperature co-upcycling of polyvinyl chloride and polypropylene50Induction Heating for the Electrification of Catalytic Processes51Transforming polystyrene wastes into aromatic products near ambient temperature with aluminium chloride6Conversion of Polypropylene to Light Olefins by HMFI Catalysts below Pyrolytic Temperature: Catalytic, Spectroscopic, and Theoretical Studies3Strategies and technologies for sustainable plastic waste treatment and recycling17Advances and Challenges in Low‐Temperature Upcycling of Waste Polyolefins via Tandem Catalysis25Advances and Challenges in Low‐Temperature Upcycling of Waste Polyolefins via Tandem Catalysis2Polyethylene Upcycling to Liquid Alkanes in Molten Salts under Neat and External Hydrogen Source-Free Conditions17Pilot-scale rotor device with low acid-site zeolite for rapid adsorption–desorption of polymerizable VOCs9Synergistic Catalysis for Recycling and Upcycling of Plastics35Integrated low-temperature PVC and polyolefin upgrading38A review of recent advances in thermal-catalytic cracking of plastic waste8Solar-driven upcycling of plastic waste using plasmonic black gold4Catalytic valorization of polyolefins: from catalysts and processes to reactors0Current perspective on heterogeneous thermal catalytic approaches for closed-loop polyolefin plastic recycling1Cleavage Alkylation Coupling with Versatile Amide-Based Eutectic Catalytic Systems0Isopentane Disproportionation in Lewis Acidic Chloroaluminate Ionic Liquid0Efficient Conversion of All- E -Lutein Esters to Z -Lutein Esters and Physiological Activities and Physicochemical Properties of Free and Esterified Lutein Isomers0Solvent-free chemical recycling of polyolefins and polystyrene under mild conditions via GaCl3-based molten catalysts0Waste PVC upcycling enables oxidant-free C-H and C-C bond editing0Microplastic degradation and organic acids recovery via homogeneous catalytic wet air oxidation: Role of redox and Lewis acidity of metal ions0Challenges in polyolefin re/upcycling catalysis specific to polymer feedstock0

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  1. Graphical Abstract: Angew. Chem. Int. Ed. 17/2024

    Angewandte Chemie International Edition · 2024-04-15

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  2. Catalytic chemical recycling and upcycling of polyolefin plastics

    Giant · 2024-06-14

    Yingzi Tan, Yidan Cheng, Jiaming Xu, Haobing Wang

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  3. Room-Temperature Upcycling of Mixed PVC and Polyolefin Waste

    Research Square · 2024-06-19

    Johannes A. Lercher, Wei Zhang, Boda Yang, Benjamin A. Jackson, Junbo Zhang, Donald M. Camaioni, Sung Min Kim, Huamin Wang, János Szanyi, Jingguang G. Chen, Mal‐Soon Lee

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  4. Active species in chloroaluminate ionic liquids catalyzing low-temperature polyolefin deconstruction

    Nature Communications · 2024-07-10

    Wei Zhang, Rachit Khare, Sung Min Kim, Lillian Hale, Wenda Hu, Chun-lin Yuan, Yaoci Sheng, Peiran Zhang, Lennart Wahl, Jiande Mai, Boda Yang, Oliver Y. Gutiérrez, Debmalya Ray, John L. Fulton, Donald M. Camaioni, Jian Zhi Hu, Huamin Wang, Mal‐Soon Lee, Johannes A. Lercher

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  5. Catalytic Upcycling of Polyolefins

    Chemical Reviews · 2024-08-16

    Jia‐Kai Sun, Jinhu Dong, Lijun Gao, Yu‐Quan Zhao, Hyunjin Moon, Susannah L. Scott

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  6. Shape selective cracking of polypropylene on an H- MFI type zeolite catalyst with recovery of cyclooctane solvent

    RSC Sustainability · 2024-11-20

    Tomohiro Fukumasa, Yuya Kawatani, Hiroki Masuda, Ikuto Nakashita, Ryusei Hashiguchi, Masanori Takemoto, Satoshi Suganuma, Etsushi Tsuji, Toru Wakihara, Naonobu Katada

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  7. Room-temperature co-upcycling of polyvinyl chloride and polypropylene

    Nature Sustainability · 2024-11-22

    Zhiwen Gao, Yu Wang, Lei Yuan, Xinrui Shi, Yihao Shang, Jinpeng Jiang, Min Zhang, Shuhui Fang, Wei Zhang, Yue Liu

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  8. Induction Heating for the Electrification of Catalytic Processes

    ChemSusChem · 2024-12-23

    Lai Truong‐Phuoc, Cuong Duong‐Viet, Jean‐Mario Nhut, Anastasia Pappa, Spyridon Zafeiratos, Cuong Pham‐Huu, Cuong Pham‐Huu

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  9. Transforming polystyrene wastes into aromatic products near ambient temperature with aluminium chloride

    Green Chemistry · 2025-01-01

    Shuying Tian, Jing Dai, Zheng Jian Li, Qiqi Wu, Guangxu Chen

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  10. Conversion of Polypropylene to Light Olefins by HMFI Catalysts below Pyrolytic Temperature: Catalytic, Spectroscopic, and Theoretical Studies

    The Journal of Physical Chemistry C · 2025-01-10

    Yuriko Ando, Takumi Miyakage, Akihiko Anzai, Mengwen Huang, Abdellah Ait El Fakir, Takashi Toyao, Yuta Nakasaka, Alisa Phuekphong, Makoto Ogawa, Alexander A. Kolganov, Evgeny A. Pidko, Ken‐ichi Shimizu

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  11. Strategies and technologies for sustainable plastic waste treatment and recycling

    Environmental Functional Materials · 2025-01-19

    Qian Kai, Lu Wang, Jie Teng, Guoshuai Liu

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  12. Advances and Challenges in Low‐Temperature Upcycling of Waste Polyolefins via Tandem Catalysis

    Angewandte Chemie International Edition · 2025-03-13

    Wei Zhang, Sung Min Kim, Michele L. Sarazen, Mingyuan He, Jingguang G. Chen, Johannes A. Lercher

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  13. Advances and Challenges in Low‐Temperature Upcycling of Waste Polyolefins via Tandem Catalysis

    Angewandte Chemie · 2025-03-13

    Wei Zhang, Sung Min Kim, Michele L. Sarazen, Mingyuan He, Jingguang G. Chen, Johannes A. Lercher

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  14. Polyethylene Upcycling to Liquid Alkanes in Molten Salts under Neat and External Hydrogen Source-Free Conditions

    Journal of the American Chemical Society · 2025-04-07

    Liqi Qiu, Felipe Polo‐Garzon, Luke L. Daemen, Min-Jae Kim, Jinghua Guo, Bobby G. Sumpter, Michael Köehler, Carlos Alberto Steren, Tao Wang, Logan T. Kearney, Tomonori Saito, Zhenzhen Yang, Sheng Dai

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  15. Pilot-scale rotor device with low acid-site zeolite for rapid adsorption–desorption of polymerizable VOCs

    Chemical Engineering Journal · 2025-04-21

    Huifang Wu, Wenjing Zhang, Lisha Miao, Kan Li, Haoxuan Liu, Weili Zhu, Zeyao An, Yanfeng Tang, Lizhong Liu, Jinping Jia

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  16. Synergistic Catalysis for Recycling and Upcycling of Plastics

    ACS Catalysis · 2025-05-07

    Hongshun Ran, Xinyang Sun, Mengying Zheng, Yaxuan Jing

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  17. Integrated low-temperature PVC and polyolefin upgrading

    Science · 2025-08-14

    Wei Zhang, Boda Yang, Benjamin A. Jackson, Junbo Zhao, Honghong Shi, Donald M. Camaioni, Sung Min Kim, Huamin Wang, János Szanyi, Mal‐Soon Lee, Jingguang G. Chen, Johannes A. Lercher

    Read original paper ↗ ·

  18. A review of recent advances in thermal-catalytic cracking of plastic waste

    Catalysis Science & Technology · 2025-11-27

    Zhongxu Wang, Jiahui Zhang, Qihao Wu, Quanhua Wang, Yi Liu, Jiajun Zheng, Yan Wang, Weijiong Dai, Ruifeng Li

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  19. Solar-driven upcycling of plastic waste using plasmonic black gold

    Chemical Science · 2025-12-23

    Saideep Singh, Gunjan Sharma, Mamata V. Joshi, Vivek Polshettiwar

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  20. Catalytic valorization of polyolefins: from catalysts and processes to reactors

    Chemical Society Reviews · 2026-01-01

    Cuncun Wu, Chaojie Guo, Xinquan Xu, Kun Liu, Lu Bai, Nan Yang, Donglong Fu, Jinlong Gong

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  21. Current perspective on heterogeneous thermal catalytic approaches for closed-loop polyolefin plastic recycling

    Discover Chemistry. · 2026-01-20

    Haokun Wang, Dermot O’Hare

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  22. Cleavage Alkylation Coupling with Versatile Amide-Based Eutectic Catalytic Systems

    Journal of the American Chemical Society · 2026-03-04

    Jisheng Yu, Di Zhu, Jianguo Zhuang, Y. Hugh Guan, Yuxin Qiu, Xue Wang, Xin Gao, G. Chen, Zhen Song, Xuedong Zhu, D. Chen

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  23. Isopentane Disproportionation in Lewis Acidic Chloroaluminate Ionic Liquid

    Journal of the American Chemical Society · 2026-06-17

    Jiande Mai, David E. Ryan, Wei Zhang, Benjamin A. Jackson, Kiyoung Jo, János Szanyi, Oliver Y. Gutiérrez, Honghong Shi, Donald M. Camaioni, Rachit Khare, Mal‐Soon Lee, Huamin Wang, Sung Min Kim, Johannes A. Lercher

    Read original paper ↗ ·

  24. Efficient Conversion of All- E -Lutein Esters to Z -Lutein Esters and Physiological Activities and Physicochemical Properties of Free and Esterified Lutein Isomers

    Journal of Agricultural and Food Chemistry · 2026-06-24

    Liangman Shi, Lijie Zhu, Jialing Cao, X Xu, Xiaoshu Tang, Shuang Zhang, Li Zhang, Cheng Yang

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  25. Solvent-free chemical recycling of polyolefins and polystyrene under mild conditions via GaCl3-based molten catalysts

    CHINESE JOURNAL OF CATALYSIS (CHINESE VERSION) · 2026-07-01

    Lei Yuan, Zhiwen Gao, Libin Shi, Cuishi Guan, Dongyue Peng, Shuhui Fang, Wei Zhang, Y Liu

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  26. Waste PVC upcycling enables oxidant-free C-H and C-C bond editing

    Research Square · 2026-09-10

    Ning Jiao, Yichen Sun, Hongwei Shi, Yichi Chen, Zengrui Cheng, Xi Wang, Junhong Meng, Yilei Huang, Huizhen Liu, Buxing Han

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  27. Microplastic degradation and organic acids recovery via homogeneous catalytic wet air oxidation: Role of redox and Lewis acidity of metal ions

    Journal of Hazardous Materials · 2026-09-28

    Xing Luo, Chenchen Zhao, Yanchanjuan Yang, Yuanyuan Liu, Shuaiqi Zhao, Wei Huangzhao, Xu Aihua, Xiaoxia Li, Xiuying Liu

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  28. Challenges in polyolefin re/upcycling catalysis specific to polymer feedstock

    Royal Society of Chemistry eBooks · 2026-09-30

    Linxiao Chen, Lucas D. Ellis

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