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RESEARCH PAPER · Nature Communications · 2024

Polyethylene hydrogenolysis by dilute RuPt alloy to achieve H2-pressure-independent low methane selectivity

Qikun Hu, Shuairen Qian, Yuqi Wang, Jiayang Zhao, Meng Jiang, Mingze Sun, Helai Huang, Tao Gan, Jun Ma, Jing Zhang, Yi Cheng, Zhiqiang Niu

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Polyethylene hydrogenolysis by dilute RuPt alloy to achieve H2-pressure-independent low methane selectivityOriginalHighly energy-efficient hydrogenolysis of high-density polyethylene via hydrogen nonthermal plasma reaction engineering4Recent developments in recycling of post-consumer polyethylene waste33Synergistic effect of acidic sites and mesoporous confinement in Ce-doped Ru/SBA-15 catalysts for efficient hydrogenolysis of low-density polyethylene to liquid fuels7Insights into Chemical Recycling and Upgrading Strategies for Polyolefin-Based Plastics15Hydrocracking of Polyethylene to Gasoline-Range Hydrocarbons over a Ruthenium-Zeolite Bifunctional Catalyst System with Optimal Synergy of Metal and Acid Sites9Exploring novel strategies and integrated systems for photothermal catalytic hydrogen production14Enhancing Waste Plastic Hydrogenolysis on Ru/CeO 2 Through Concurrent Incorporation of Fe Single Atoms and FeO x Nanoclusters27Enhancing Waste Plastic Hydrogenolysis on Ru/CeO 2 Through Concurrent Incorporation of Fe Single Atoms and FeO x Nanoclusters4Synergistic Catalysis for Recycling and Upcycling of Plastics35A Minimalist Design for a Dual-Catalyst System for High-Efficiency Conversion of Waste Plastics into Liquid Fuel Products27Hydrogenolysis of LDPE over Ni-catalyst promoted by n-hexane solvent7Tandem Catalysis to Mitigate Coke Formation in the Upcycling of Mixed Polyolefin Wastes11CO-promoted polyethylene hydrogenolysis with renewable formic acid as hydrogen donor20Catalytic Depolymerization of Plastics to Valuable Products7AI-accelerated innovations in photodegradation and depolymerization of waste plastics: a critical review on mechanistic insights, environmental impact, and future perspectives6Chemical recycling of polyethylenes with low gas products by catalytic hydrogenolysis with heterogeneous CeO2-supported Cu-doped Ru catalyst5Advancing chemical recycling for waste plastic conversion1Dual-control strategy for selective upgrading of polyethylene waste into jet fuel-range alkanes2Plasma Catalysis for Plastic Waste Conversion into Value‐Added Products: Advancements and Perspectives11Polyethylene hydrogenolysis to liquid products over bimetallic catalysts with favorable environmental footprint and economics17Recent advances in catalytic hydrogenolysis of polycarbonate, polyurethane and polyurea0Microwave-assisted catalytic upcycling of polyolefin wastes into hydrogen and carbon nanotubes over Pt-promoted Fe/Ni bimetallic catalysts10Tandem depolymerization-electrocatalysis for plastic waste upcycling6Advances of rare earth-based catalysts for recycling CO 2 and plastic waste17Surface and Interface Properties of Metal Species for Waste Plastic Hydroconversion6Mechanistic insights into plastic degradation via catalytic bond breaking: a comprehensive review1Tuning hydroconversion performance of n-hexadecane over Ni/silica-alumina catalysts: Role of Si/Al ratio and nickel loading2Catalytic valorization of polyolefins: from catalysts and processes to reactors0Direct upcycling of mixed plastic waste into liquid alkanes3Electronegativity-driven d-band center shifts in Ru–Ni alloys for low methane hydrogenolysis of polyolefin plastics2Highly selective hydrocracking of polypropylene to gasoline-range fuels over the Pt/MCM-22 catalyst0Enhancing Hydrogen Spillover via Crystalline-Phase Engineering of Ru/ZrO 2 for Selective Liquid Alkane Production in Polyethylene Hydrogenolysis6Current perspective on heterogeneous thermal catalytic approaches for closed-loop polyolefin plastic recycling1PtRu nanoparticle catalysts with adjustable electronic environments for efficient low-temperature dehydrogenation of cycloalkanes0Ecological distribution and functional characterization of polyethylene-degrading enzymes from diverse metagenomes1Mechanistic pathways and influencing factors in the liquefaction of single and mixed plastics toward waste-to-energy conversion: A structured and critical review1Recent advancements in catalytic processes for plastic upcycling into fuels: a major step in sustainable waste management and energy production3Thermo-chemical upgrading of waste polyethylene and polypropylene plastics0Hydrogenolysis Versus Hydrocracking for Polyolefin Upcycling0Structure–performance relationships in heterogeneous catalysts for polyolefin plastic hydroconversion1Preparing methane‐resistant Ru catalysts via moderate metal‐support interactions for polyethylene hydrogenolysis0Techno-economic analysis and life cycle assessment for the catalytic hydrogenolysis and hydrocracking of polyethylene6Catalytic Upcycling of Polyolefins and Polystyrene: Integrating Active Site Design With Mass Transfer Considerations4Enhancing C-O Bond Cleavage in 2,6-Dimethoxy-4-methylphenol Hydrodeoxygenation via Oxygen Vacancy Engineering in Pd-Pt/NiO-FeOx Nanosheets2Highly Selective Gasoline Production by Polyethylene Hydrogenolysis Using Ternary RuNiPt Nanoalloy Catalyst1NiW alloy catalyst for methane suppression in polyethylene hydrogenolysis to enhance liquid hydrocarbon yields1Oxygen vacancy promoted C–H activation enhancing hydrogenolysis of polyethylene plastics over Ru/CeO2 catalyst0Single-Atom Nickel Dispersed on Mo 2 TiC 2 T x MXene for Upcycling of Polyolefins via Catalytic Hydropyrolysis for Fuels and Lubricants0Well‐Defined Heterocatalysts for Plastic Upcycling: From Design to Applications3From waste to wealth: Advanced strategies and mechanisms for chemical recycling and upcycling of polymeric materials1Advances in Catalytic Hydrogenolysis of Waste Plastics to Value-Added Products0Collaborative Pt–Ni Sites Enable CO-Tolerant Hydrocracking for Upcycling Polyolefin Waste1A Mesopore-Confined and Graphene Oxide-Localized Ruthenium Catalyst Increases Rates of Mid-Chain Polyolefin Hydrogenolysis0From Poisoning to Signal Transduction: d-Band Modulated Au@RuPt Nanozyme for Oxygen Reduction Reaction Inhibition-Based Detection of Organophosphates1Solvent-free chemical recycling of polyolefins and polystyrene under mild conditions via GaCl3-based molten catalysts0Catalytic Hydrogenolysis of Polyethylene-Based Plastics into Fuels Using Ruthenium Catalysts Supported on Micro/Mesoporous Carbons0Reductive catalytic upcycling of polyethylene using 2-propanol as transfer hydrogen-donor source1Ultra‐High‐Molecular‐Weight Polyolefins: Advances in Catalytic Synthesis, Entanglement Regulation, Interfacial Chain Diffusion, and Processing0Comprehensive quantitative analysis of polyolefin hydrogenolysis toward plastic waste management0Bifunctional RhRu Dual-Atom Catalyst Drives the Tandem Degradation of Polystyrene for Highly Selective Production of Toluene0Highly Selective Conversion of Polyolefins to Methane via Mechanochemical Hydrogenolysis0FeOx–Au Supported WO3-x for Selective Photocatalytic Methane Conversion to Methanol under Visible Light0Implementable and Sustainable Upcycling of Medical Plastic Waste to Liquid Highly Branched Alkanes via Tandem Catalytic Cracking-Hydrogenation Strategy0Short-Range Order Stabilized Ultrafine Pd on Carbon-Supported Medium-Entropy Mesoporous Interfaces for Plastic Upcycling0Synergetic effect of Ru-Pt bimetallic catalyst for the synthesis of quinazolinones via additive-free acceptorless dehydrogenative coupling of alcohols0Ambient‐Pressure Polyolefin Upcycling With Earth‐Abundant Catalyst0Ambient‐Pressure Polyolefin Upcycling With Earth‐Abundant Catalyst0Internal transport modulates catalytic hydrogenolysis of polyolefins0Homogeneous Ru/La2O2CO3 Catalyst for Efficient Thermal Cracking of Crosslinked Polyethylene0

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  13. CO-promoted polyethylene hydrogenolysis with renewable formic acid as hydrogen donor

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