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RESEARCH PAPER · Macromolecules · 2023

Mechanistic Insights into Processive Polyethylene Hydrogenolysis throughIn SituNMR

Yunpu Zhao, Max Meirow, Akalanka Tennakoon, Xun Wei Wu, Alexander L. Paterson, Long Hao Qi, Anne M. LaPointe, Jessica V. Lamb, Takeshi Kobayashi, Massimiliano Delferro, Aaron David Sadow, Wenyu Huang, Erik Luijten, Frédéric A. Perras

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42 direct citing works

Mechanistic Insights into Processive Polyethylene Hydrogenolysis throughIn SituNMROriginalTwo Mesoporous Domains Are Better Than One for Catalytic Deconstruction of Polyolefins62Entropy Confinement Promotes Hydrogenolysis Activity for Polyethylene Upcycling72Entropy Confinement Promotes Hydrogenolysis Activity for Polyethylene Upcycling8Influence of Pore Length on Hydrogenolysis of Polyethylene within a Mesoporous Support Architecture17Review on Catalytic Depolymerization of Polyolefin Waste by Hydrogenolysis: State-of-the-Art and Outlook57Artificial Processive Catalytic Systems3Size and Structure Effects of Carbon-Supported Ruthenium Nanoparticles on Waste Polypropylene Hydrogenolysis Activity, Selectivity, and Product Microstructure40The Overlooked Potential of Sulfated Zirconia: Reexamining Solid Superacidity Toward the Controlled Depolymerization of Polyolefins11Chemical Upcycling of Polyolefin Plastics Using Structurally Well-defined Catalysts35Insight into the Competitive Adsorption Behavior of Polymer Chains in Silica Nanopores by Small-Angle Neutron Scattering3Catalytic Upcycling of Polyolefins316Modulating the Contact Angle between Nonpolar Polymers and SiO2 Nanoparticles4Tandem Catalysis for Plastic Depolymerization: In Situ Hydrogen Generation via Methanol Aqueous Phase Reforming for Sustainable Polyethylene Hydrogenolysis2Tandem Catalysis for Plastic Depolymerization: In Situ Hydrogen Generation via Methanol Aqueous Phase Reforming for Sustainable Polyethylene Hydrogenolysis27Recent Advances and Applications of NMR Techniques in Plastic Characterizations19Reductive Upcycling of Polyolefins, Polyesters and Mixed Plastic Wastes to Valuable Chemicals: Bridging Chemical Catalysis With Plastic Waste Management35Population Balance Models for Catalytic Depolymerization: From Elementary Steps to Multiphase Reactors8Polymer Upcycling by Catalytic Hydrogenolysis: The Role of Polyolefin Short-Chain Branching3Research progress of high value utilization of waste polyethylene plastics6Recent advancements in catalytic processes for plastic upcycling into fuels: a major step in sustainable waste management and energy production3One-pot co-upcycling of mixed polyolefin waste6Polymer Deconstruction and Redesign Strategies for Plastics Recycling0A Mesopore-Confined and Graphene Oxide-Localized Ruthenium Catalyst Increases Rates of Mid-Chain Polyolefin Hydrogenolysis0Comprehensive quantitative analysis of polyolefin hydrogenolysis toward plastic waste management0Upcycling of polymer waste into high value energy products0

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  1. Two Mesoporous Domains Are Better Than One for Catalytic Deconstruction of Polyolefins

    Journal of the American Chemical Society · 2023-08-04

    Akalanka Tennakoon, Xun Wei Wu, Max Meirow, Daniel Howell, Jarod Willmon, Jiaqi Yu, Jessica V. Lamb, Massimiliano Delferro, Erik Luijten, Wenyu Huang, Aaron David Sadow

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  2. Entropy Confinement Promotes Hydrogenolysis Activity for Polyethylene Upcycling

    Angewandte Chemie International Edition · 2023-10-06

    Qingyun Kang, Mingyu Chu, Panpan Xu, Xuchun Wang, Shiqi Wang, Muhan Cao, Oleksandr Ivasenko, Tsun‐Kong Sham, Qiao Zhang, Qiming Sun, Jinxing Chen

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  3. Entropy Confinement Promotes Hydrogenolysis Activity for Polyethylene Upcycling

    Angewandte Chemie · 2023-10-06

    Qingyun Kang, Mingyu Chu, Panpan Xu, Xuchun Wang, Shiqi Wang, Muhan Cao, Oleksandr Ivasenko, Tsun‐Kong Sham, Qiao Zhang, Qiming Sun, Jinxing Chen

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  4. Influence of Pore Length on Hydrogenolysis of Polyethylene within a Mesoporous Support Architecture

    The Journal of Physical Chemistry C · 2023-12-01

    Max Meirow, Akalanka Tennakoon, Xun Wei Wu, Jarod Willmon, Daniel Howell, Wenyu Huang, Aaron David Sadow, Erik Luijten

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  5. Review on Catalytic Depolymerization of Polyolefin Waste by Hydrogenolysis: State-of-the-Art and Outlook

    Energy & Fuels · 2024-01-22

    Abdulrahman Musa, E. A. Jaseer, Samir Barman, Néstor Garcı́a

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  6. Artificial Processive Catalytic Systems

    Chemistry - A European Journal · 2024-02-07

    Roeland J. M. Nolte, Johannes A. A. W. Elemans

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  7. Size and Structure Effects of Carbon-Supported Ruthenium Nanoparticles on Waste Polypropylene Hydrogenolysis Activity, Selectivity, and Product Microstructure

    ACS Catalysis · 2024-02-15

    Jessie A. Sun, Pavel A. Kots, Zachary R. Hinton, Nebojša Marinković, Lu Ma, Steven N. Ehrlich, Weiqing Zheng, Thomas H. III Epps, LaShanda T. J. Korley, Dionisios G. Vlachos

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  8. The Overlooked Potential of Sulfated Zirconia: Reexamining Solid Superacidity Toward the Controlled Depolymerization of Polyolefins

    Langmuir · 2024-03-21

    Scott R. Cleary, Anne K. Starace, Caleb C. Curran-Velasco, Daniel A. Ruddy, C. Michael McGuirk

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  9. Chemical Upcycling of Polyolefin Plastics Using Structurally Well-defined Catalysts

    JACS Au · 2024-06-04

    Simin Sun, Wenyu Huang

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  10. Insight into the Competitive Adsorption Behavior of Polymer Chains in Silica Nanopores by Small-Angle Neutron Scattering

    Macromolecules · 2024-08-13

    Xuchun Wang, Xingyi Lyu, Xun Wei Wu, Lilin He, Jessica V. Lamb, Alexander S. Filatov, Massimiliano Delferro, Wenyu Huang, Byeongdu Lee

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  11. Catalytic Upcycling of Polyolefins

    Chemical Reviews · 2024-08-16

    Jia‐Kai Sun, Jinhu Dong, Lijun Gao, Yu‐Quan Zhao, Hyunjin Moon, Susannah L. Scott

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  12. Modulating the Contact Angle between Nonpolar Polymers and SiO2 Nanoparticles

    Macromolecules · 2024-08-20

    Anirban Majumder, Anne N. Radzanowski, Ching-Yu Wang, Yijiang Mu, Edward Bryan Coughlin, Raymond J. Gorte, John M. Vohs, Daeyeon Lee

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  13. Tandem Catalysis for Plastic Depolymerization: In Situ Hydrogen Generation via Methanol Aqueous Phase Reforming for Sustainable Polyethylene Hydrogenolysis

    Angewandte Chemie · 2025-01-22

    Junsung Lee, Taeeun Kwon, Ki Hyuk Kang, Wangyun Won, Insoo Ro

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  14. Tandem Catalysis for Plastic Depolymerization: In Situ Hydrogen Generation via Methanol Aqueous Phase Reforming for Sustainable Polyethylene Hydrogenolysis

    Angewandte Chemie International Edition · 2025-01-22

    Junsung Lee, Taeeun Kwon, Ki Hyuk Kang, Wangyun Won, Insoo Ro

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  15. Recent Advances and Applications of NMR Techniques in Plastic Characterizations

    Analytical Chemistry · 2025-03-03

    Zhe Zhou, Xuelei Duan, Yue Yu, Linge Ma, Aitor Moreno, Youlin Xia, Linfeng Chen, Shan Ye, Rongjuan Cong

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  16. Reductive Upcycling of Polyolefins, Polyesters and Mixed Plastic Wastes to Valuable Chemicals: Bridging Chemical Catalysis With Plastic Waste Management

    Advanced Sustainable Systems · 2025-03-20

    Sahil Kumar, Devanshu Sajwan, Devendra Sharma, Venkata Krishnan

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  17. Population Balance Models for Catalytic Depolymerization: From Elementary Steps to Multiphase Reactors

    Accounts of Chemical Research · 2025-05-16

    Lela K. Manis, Jiankai Ge, Changhae Andrew Kim, Emmanuel Ejiogu, Ziqiu Chen, Ryan D. Yappert, Baron Peters

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  18. Polymer Upcycling by Catalytic Hydrogenolysis: The Role of Polyolefin Short-Chain Branching

    ACS Catalysis · 2025-09-23

    Zachary M. Gdowski, Rishi Raj, Aditya Bhan, K. Andre Mkhoyan, Mahesh K. Mahanthappa, Frank S. Bates

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  19. Research progress of high value utilization of waste polyethylene plastics

    Green Chemistry · 2025-12-30

    Mingjun Xiao, Xihang Dai

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  20. Recent advancements in catalytic processes for plastic upcycling into fuels: a major step in sustainable waste management and energy production

    Fuel · 2026-02-26

    Sudipta Nayak, Rajat Singhal, S. M. A. Hakim Siddiki, Ken Motokura, Navya Subray Bhat, Navneet Kumar Gupta

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  21. One-pot co-upcycling of mixed polyolefin waste

    Nature Communications · 2026-03-02

    Weilin Tu, Mingyu Chu, Tianran Yan, Qingqing Zhang, Xianpeng Wang, Liang Zhang, Muhan Cao, Qiao Zhang, Mingshan Zhu, Minzhi Zhan, Jinxing Chen

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  22. Polymer Deconstruction and Redesign Strategies for Plastics Recycling

    Advanced Materials Technologies · 2026-03-16

    Anjani K. Maurya, Arun S. Asundi, Özge Deniz Bozkurt, Katrina M. Knauer, Simon R. Bare, Christopher J. Tassone

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  23. A Mesopore-Confined and Graphene Oxide-Localized Ruthenium Catalyst Increases Rates of Mid-Chain Polyolefin Hydrogenolysis

    Journal of the American Chemical Society · 2026-06-26

    Kajol Tonk, Simin Sun, Olajide H. Bamidele, Minghui Niu, Xiaobing Zuo, Jessica V. Lamb, Arthur Jeremy Kropf, Massimiliano Delferro, Byeongdu Lee, Andreas Heyden, Wenyu Huang, Aaron David Sadow

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  24. Comprehensive quantitative analysis of polyolefin hydrogenolysis toward plastic waste management

    Nature Protocols · 2026-07-24

    Chao Meng, Yue Wang, Xun Wu, Akalanka Tennakoon, Anne M. LaPointe, Frédéric A. Perras, Long Qi, Baron Peters, Aaron David Sadow, Wenyu Huang

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  25. Upcycling of polymer waste into high value energy products

    Elsevier eBooks · 2026-09-25

    Betül Aksoy, Yasemin Ozliman, Melih Soner Çeliktaş

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