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RESEARCH PAPER · Science · 2022

Catalytic deconstruction of waste polyethylene with ethylene to form propylene

Richard J. Conk, Steven Hanna, Jake X. Shi, Ji Yang, Nicodemo R. Ciccia, Liang Qi, Brandon J. Bloomer, Steffen Heuvel, Tyler Wills, Ji Su, Alexis T. Bell, John F. Hartwig

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Catalytic deconstruction of waste polyethylene with ethylene to form propyleneOriginalMicroplastic materials in the environment: Problem and strategical solutions201Unraveling the potential human health risks from used disposable face mask-derived micro/nanoplastics during the COVID-19 pandemic scenario: A critical review46Understanding the Structure–Activity Relationships in Catalytic Conversion of Polyolefin Plastics by Zeolite-Based Catalysts: A Critical Review269Towards a Cradle‐to‐Cradle Polyolefin Lifecycle11Towards a Cradle‐to‐Cradle Polyolefin Lifecycle1Catalytic hydroconversion processes for upcycling plastic waste to fuels and chemicals94Catalytic Chemical Recycling of Post-Consumer Polyethylene188Chemical Structures, Properties, and Applications of Selected Crude Oil-Based and Bio-Based Polymers29Bis(pentafluorophenyl)borane-catalyzed E -selective isomerization of terminal alkenes to internal alkenes10Controllable carbonyl-assisted C(sp 3 )–C(sp 3 ) bond reduction and reorganization6Heterogeneous Pt-catalyzed transfer dehydrogenation of long-chain alkanes with ethylene7Selective oxidative upgrade of waste polystyrene plastics by nitric acid to produce benzoic acid43Tandem oxidative and thermal cracking of polypropylene at low temperatures21The E factor at 30: a passion for pollution prevention339Thiol–ene Click Chemistry Incorporates Hydroxyl Functionality on Polycyclooctene to Tune Properties30Constructing stable “bridge” structures with compatibilizer POE‐g‐GMA to improve the compatibility of starch‐based composites12Trendbericht Anorganische Chemie 2023: Nebengruppen, Bioanorganik und Koordinationschemie0Cationic Tantalum Hydrides Catalyze Hydrogenolysis and Alkane Metathesis Reactions of Paraffins and Polyethylene38A highly ionic reaction environment achieving low-temperature polyethylene upcycling3Repeatedly Recyclable 3D Printing Catalyst‐Free Dynamic Thermosetting Photopolymers75Multicatalysis enables turning plastic waste into chemical commodities2Catalytic upcycling of waste polypropylene for gram-scale production of FeCo@N-doped carbon nanotubes toward efficient oxygen reduction electrocatalysis26Metal-catalyzed plastic depolymerization79Recent Advances in Catalytic Chemical Recycling of Polyolefins104Catalytic Biorefining of Natural Oils to Basic Olefinic Building Blocks of Proven Chemical Valorization Schemes10Catalytic Biorefining of Natural Oils to Basic Olefinic Building Blocks of Proven Chemical Valorization Schemes1Hybrid Monomer Design Synergizing Property Trade‐offs in Developing Polymers for Circularity and Performance63Hybrid Monomer Design Synergizing Property Trade‐offs in Developing Polymers for Circularity and Performance4Making Persistent Plastics Degradable14Degradation of Polyacrylates by One-Pot Sequential Dehydrodecarboxylation and Ozonolysis82Low-Temperature Dehydrogenation of Cyclooctane by Using Pincer Iridium Complexes Bearing an N,N′-Diarylated PNCNP Ligand7A Review on the Microwave-Assisted Pyrolysis of Waste Plastics62Zeolite Supported Pt for Depolymerization of Polyethylene by Induction Heating18Boosting the aqueous-phase production of lactic acid via dual-site activation of carbohydrates2Catalytic recycling of polyesters via a binuclear catalyst6Bifunctional tandem catalytic upcycling of polyethylene to surfactant-range alkylaromatics101Deconvoluting the roles of polyolefin branching and unsaturation on depolymerization reactions over acid catalysts34Upcycling contaminated plastics21An atomic insight into reaction pathways and temperature effects in the degradation of polyethylene, polypropylene and polystyrene21Sustainable developments in polyolefin chemistry: Progress, challenges, and outlook204Efficient solvent- and hydrogen-free upcycling of high-density polyethylene into separable cyclic hydrocarbons171α,ω-Diene Generation from Ethylene and Butadiene by Copolymer Upcycling6Direct catalytic plastics waste upcycling7Hydrogen-free catalytic depolymerization of waste polyolefins at mild temperatures43Efficient upcycling of high-density polyethylene into separable cyclic hydrocarbons1Upcycling of polyethylenes by catalysis0Chemical recycling of polyolefins: a closed-loop cycle of waste to olefins126Chemical Upcycling of Polyolefins through C−H Functionalization50Chemical upcycling of polyethylene, polypropylene, and mixtures to high-value surfactants349Hydroformylation of pyrolysis oils to aldehydes and alcohols from polyolefin waste195Steric modulation of CAACs controls orientation and ethenolysis performance1Plastics upcycling made more sustainable and practical21Waste PET Derived Beetle-like Membrane with High Mechanical Robustness for Regenerable Emulsion Separation10Quantifying synergy for mixed end-scission and random-scission catalysts in polymer upcycling12Solvent‐Free Depolymerization of Plastic Waste Enabled by Plastic‐Catalyst Interfacial Engineering55Solvent‐Free Depolymerization of Plastic Waste Enabled by Plastic‐Catalyst Interfacial Engineering3Homogeneous Catalysis in Plastic Waste Upcycling: A DFT Study on the Role of Imperfections in Polymer Chains15Stapler Strategies for Upcycling Mixed Plastics0Entropy Confinement Promotes Hydrogenolysis Activity for Polyethylene Upcycling72Entropy Confinement Promotes Hydrogenolysis Activity for Polyethylene Upcycling8Co-upcycling of polyvinyl chloride and polyesters199Recent Advances in the Functionalized Poly(α-Hydroxy Acids) Synthesized fromO-Carboxyanhydrides4Chemically recyclable polyolefin-like multiblock polymers201O-Methyl-N-nitroisourea as a NCO Surrogate in Cu-Catalyzed Alkane C–H Amidination. A Masked Isocyanate Strategy9Thermally Robust yet Deconstructable and Chemically Recyclable High‐Density Polyethylene (HDPE)‐Like Materials Based on Si−O Bonds55Thermally Robust yet Deconstructable and Chemically Recyclable High‐Density Polyethylene (HDPE)‐Like Materials Based on Si−O Bonds17A hybrid chemical-biological approach can upcycle mixed plastic waste with reduced cost and carbon footprint48Rapid Polyolefin Hydrogenolysis by a Single‐Site Organo‐Tantalum Catalyst on a Super‐Acidic Support: Structure and Mechanism14Rapid Polyolefin Hydrogenolysis by a Single‐Site Organo‐Tantalum Catalyst on a Super‐Acidic Support: Structure and Mechanism5High-performance chlorinated polyvinyl chloride/polyurea nanocomposite foam with excellent solvent resistance, flame-triggered shape memory effect and its upcycling14Selective Electrocatalytic Degradation of Ether‐Containing Polymers31Selective Electrocatalytic Degradation of Ether‐Containing Polymers1The thermodynamics and kinetics of depolymerization: what makes vinyl monomer regeneration feasible?98Precise activation of C–C bonds for recycling and upcycling of plastics81Direct-writing assembly of high-strength hierarchical porous mullite-based lattices with a multiscale reinforcing strategy3A butadiene-derived semicrystalline polyolefin with two-tiered chemical recyclability23Numerical study on waste polyethylene pyrolysis driven by self-sustaining smoldering9Rapid Polyolefin Plastic Hydrogenolysis Mediated by Single-Site Heterogeneous Electrophilic/Cationic Organo-group IV Catalysts19Thiol-ene click chemistry incorporates carboxylic acid-terminated alkane pendants on polycyclooctene to tune properties14A facile methodology for side- and upcycling of HDPE waste via partial creation of unsaturated double bonds12Closed-loop recyclable polymers: from monomer and polymer design to the polymerization–depolymerization cycle106Computational Insights into Catalysis: Evaluating Alternative Metal Potentials in Mgcl2-Supported Ziegler-Natta Catalysts0Controlled degradation of chemically stable poly(aryl ethers) via directing group-assisted catalysis6Depolymerization of waste polyethylene to linear alkenes via sequential dehydrogenation and metathesis19Design of depolymerizable polymers toward a circular economy69Efficient Degradation of Oxidized Polyethylene Containing Ester Bonds by Cutinase or Lipase in Aqueous Phase0Heterogeneous catalysis for the environment92Isomer-driven polymerization, depolymerization, and reconstruction3Modern mechanistic approaches for the depolymerization of commodity plastics via organometallic catalysis0Ruthenium-catalyzed “open-loop” recycling of polyethylene via tandem isomerization-metathesis (ISOMET)12Sustainable high-density polyethylene via chemical recycling: From modification to polymerization methods45Photo- and electrochemical processes to convert plastic waste into fuels and high-value chemicals45Recycled polymer: Green roads for polyester plastics65Highly Selective Upgrading of Polyethylene into Light Aromatics via a Low-Temperature Melting-Catalysis Strategy55Catalytic conversion of mixed polyolefins under mild atmospheric pressure48Microwave-intensified catalytic upcycling of plastic waste into hydrogen and carbon nanotubes over self-dispersing bimetallic catalysts80Chemically Recyclable Linear and Branched Polyethylenes Synthesized from Stoichiometrically Self-Balanced Telechelic Polyethylenes82Population Balance Equations for Reactive Separation in Polymer Upcycling20Upcycling Waste Plastics with a C–C Backbone by Heterogeneous Catalysis45Circular olefin copolymers made de novo from ethylene and α-olefins83Ring-Opening Polymerization of Lactones to Prepare Closed-Loop Recyclable Polyesters116Upgrading waste plastics to value-added aromatics30Tandem catalysis enables chlorine-containing waste as chlorination reagents48Synthesis and Deconstruction of Polyethylene-type Materials194Catalytic upcycling plastics with CO2: A novel strategy for carbon waste valorization0Paths to circularity for plastics in the United States27Chloride and Hydride Transfer as Keys to Catalytic Upcycling of Polyethylene into Liquid Alkanes3Chloride and Hydride Transfer as Keys to Catalytic Upcycling of Polyethylene into Liquid Alkanes29Sustainable ultra-strong polyesteramide elastomers with rapid degradation and high resilience8“Inverted” Cyclic(Alkyl)(Amino)Carbene (CAAC) Ruthenium Complex Catalyzed Isomerization Metathesis (ISOMET) of Long Chain Olefins to Propylene at Low Ethylene Pressure15Searching for bacterial plastitrophs in modified Winogradsky columns3The Overlooked Potential of Sulfated Zirconia: Reexamining Solid Superacidity Toward the Controlled Depolymerization of Polyolefins11Organoaluminum complexes containing a pyrrolylaldiminate pincer ligand1Upcycling of polyethylene to gasoline through a self-supplied hydrogen strategy in a layered self-pillared zeolite166A Microkinetic Model for Isomerizing Ethenolysis8Complete hydrogenolysis of mixed plastic wastes101Review of the Potential Effects and Remediation Strategies of Microplastic Pollutants in Drinking Water Sources63Influence of pyrolysis temperature on carbon deposition from the perspective of volatile evolution during the ex-situ pyrolysis-catalysis of plastic17Selective Photoreforming of Waste Plastics into Diesel Olefins via Single Reactive Oxygen Species51Selective Photoreforming of Waste Plastics into Diesel Olefins via Single Reactive Oxygen Species8Architectural Editing of Polyesters and Polyurethanes via Palladium(II)-Catalyzed [3,3]-Sigmatropic Oxo-Rearrangements18Oxidative Upcycling of Polyethylene to Long Chain Diacid over Co‐MCM‐41 Catalyst12Oxidative Upcycling of Polyethylene to Long Chain Diacid over Co‐MCM‐41 Catalyst58Deconstruction of Polymers through Olefin Metathesis101A Merger of Relay Catalysis with Dynamic Kinetic Resolution Enables Enantioselective β‐C(sp3)−H Arylation of Alcohols0A Merger of Relay Catalysis with Dynamic Kinetic Resolution Enables Enantioselective β‐C(sp3)−H Arylation of Alcohols11Recent progress of waste plastic upcycling based on multifunctional zeolite catalysts13Closed‐Loop Recycling of Mixed Plastics of Polyester and CO2‐Based Polycarbonate to a Single Monomer33Closed‐Loop Recycling of Mixed Plastics of Polyester and CO2‐Based Polycarbonate to a Single Monomer3Hydrocarboxylation of C═C Bonds in Polycyclooctene: Progress Toward Valorization of Waste Polyolefins8A Mechanistic Understanding of the Activity-Stability Trade-off in PETase2Indolo[3,2-b]carbazole-based Hyper-Crosslinked organic polymers for adsorptive separation of C3H6/C2H412Lifecycle Management for Sustainable Plastics: Recent Progress from Synthesis, Processing to Upcycling87Catalytic chemical recycling and upcycling of polyolefin plastics27Mechanochemical Recycling of Highly Cross‐Linked Thermosets: Economic‐Friendly and Pollution‐Free15Room-Temperature Upcycling of Mixed PVC and Polyolefin Waste1Recent advances in polyolefin plastic waste upcycling via mild heterogeneous catalysis route from catalyst development to process design25Mild Catalytic Degradation of Crystalline Polyethylene Units in a Solid State Assisted by Carboxylic Acid Groups23Stapler Strategies for Upcycling Mixed Plastics49Recycling polyolefin plastic waste at short contact times via rapid joule heating93Active species in chloroaluminate ionic liquids catalyzing low-temperature polyolefin deconstruction22Deconstruction of unsaturated polymers through photo-mediated oxidation under O27Copolymerization of Olefins and Conjugated Dienes: A Promising Approach to Produce Recyclable Polyolefins14PP upcycling employing FCC spent catalyst: The role of contaminants, atmosphere and pressure5Polyoxymethylene Upcycling into Methanol and Methyl Groups Catalyzed by a Manganese Pincer Complex18Advances in Nonreactive Polymer Compatibilizers for Commodity Polyolefin Blends102Circular Melt-Spun Textile Fibers from Polyethylene-like Long-Chain Polyesters7Chemical recycling of post-consumer polyester wastes using a tertiary amine organocatalyst9Industrial and Laboratory Technologies for the Chemical Recycling of Plastic Waste70Catalytic Upcycling of Polyolefins316

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