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RESEARCH PAPER · Joule · 2018

Mining Unexplored Chemistries for Phosphors for High-Color-Quality White-Light-Emitting Diodes

Zhenbin Wang, Jungmin Ha, Yoon Hwa Kim, Won Bin Im, Joanna M. McKittrick, Shyue Ping Ong

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Mining Unexplored Chemistries for Phosphors for High-Color-Quality White-Light-Emitting DiodesOriginalEu 2+ Site Preferences in the Mixed Cation K 2 BaCa(PO 4 ) 2 and Thermally Stable Luminescence577(INVITED) A review on the Eu2+ doped β-Ca3(PO4)2-type phosphors and the sites occupancy for photoluminescence tuning17Aliovalent substitution toward reinforced structural rigidity in Ce 3+ -doped garnet phosphors featuring improved performance44Color tunable single-phase Eu 2+ and Ce 3+ co-activated Sr 2 LiAlO 4 phosphors31Li substituent tuning of LED phosphors with enhanced efficiency, tunable photoluminescence, and improved thermal stability205Accelerating materials science with high-throughput computations and machine learning136Realizing Visible Light Excitation of Tb3+ via Highly Efficient Energy Transfer from Ce3+ for LED‐Based Applications63Graph Networks as a Universal Machine Learning Framework for Molecules and Crystals1525Energy, Phonon, and Dynamic Stability Criteria of Two-Dimensional Materials137Small Alkaline-Earth-based Core/Shell Nanoparticles for Efficient Upconversion86Synthesis of Ba1−Sr YSi2O5N and discussion based on structure analysis and DFT calculation5Computational Discovery and Design of MXenes for Energy Applications: Status, Successes, and Opportunities153Site‐Selective Occupancy of Eu 2+ Toward Blue‐Light‐Excited Red Emission in a Rb 3 YSi 2 O 7 :Eu Phosphor221Site‐Selective Occupancy of Eu2+Toward Blue‐Light‐Excited Red Emission in a Rb3YSi2O7:Eu Phosphor102Data-Driven Discovery of Full-Visible-Spectrum Phosphor133Engineering of K3YSi2O7To Tune Photoluminescence with Selected Activators and Site Occupancy117Polymorphs and derivates of Sr2LiAlO4:Eu2+12Broadband emission of double perovskite Cs2Na04Ag06In0995Bi0005Cl6:Mn2+ for single-phosphor white-light-emitting diodes44Photoluminescence Control of UCr 4 C 4 -Type Phosphors with Superior Luminous Efficiency and High Color Purity via Controlling Site Selection of Eu 2+ Activators112Unified Theory of Thermal Quenching in Inorganic Phosphors0Critical Review—A Promising Cs3CoCl5 Prototype Phosphor toward the Discovery of Next-Generation LED Phosphor3Critical Review—Data-Driven Discovery of Novel Phosphors25Divalent europium-doped near-infrared-emitting phosphor for light-emitting diodes660Designing High‐Performance LED Phosphors by Controlling the Phase Stability via a Heterovalent Substitution Strategy76Photoluminescence control and abnormal Eu 3+ orange emission in Ln 3+ (Ln 3+ = Ce 3+ , Eu 3+ )-doped oxyapatite-type phosphors17Discovery of a Ce 3+ -activated red nitride phosphor for high-brightness solid-state lighting39Novel narrow-band blue-emitting Cs 3 Zn 6 B 9 O 21 :Bi 3+ phosphor with superior thermal stability33Realizing red/orange emission of Eu 2+ /Ce 3+ in La 26−x Sr x Si 41 O x+1 N 80−x ( x = 12.72–12.90) phosphors for high color rendition white LEDs19A deep-learning technique for phase identification in multiphase inorganic compounds using synthetic XRD powder patterns199Highly Efficient Green‐to‐Yellowish‐Orange Emitting Eu2+‐Doped Pyrophosphate Phosphors with Superior Thermal Quenching Resistance for w‐LEDs99Recent progress on discovery of novel phosphors for solid state lighting88Violet-light-excitable super-narrow band green emitting phosphor for high-quality white LEDs9Broadband deep‐red‐to‐near‐infrared emission from Mn 2+ in strong crystal‐field of nitride MgAlSiN 344Preparation, luminescence properties and electronic structure of RE (RE=Eu3+,Sm3+,Dy3+)-doped multi-color silico-phosphate Ca15(PO4)2(SiO4)6 phosphors31Data-Driven Photoluminescence Tuning in Eu2+-Doped Phosphors76Predicting Thermal Quenching in Inorganic Phosphors149Narrow-band emitters in LED backlights for liquid-crystal displays217Energy transfer and photo/cathodoluminescence performances investigation of a luminescent material Ce3+/Tb3+ co-doped Na2Ca2Si2O7 for multifunctional applications15Design Principles for Aqueous Na-Ion Battery Cathodes48Exploring Frontiers in Research and Teaching: NanoEngineering and Chemical Engineering at UC San Diego6Acid-Stable Oxides for Oxygen Electrocatalysis189Anti‐Thermal‐Quenching Bi 3+ Luminescence in a Cyan‐Emitting Ba 2 ZnGe 2 O 7 :Bi Phosphor Based on Zinc Vacancy162Chemist versus Machine: Traditional Knowledge versus Machine Learning Techniques80A data-driven approach to predicting band gap, excitation, and emission energies for Eu 2+ -activated phosphors28Structural design and evolution of a novel Bi 3+ -doped narrow-band emission blue phosphor with excellent photoluminescence performance for wide color gamut wLED29Opportunities for Next-Generation Luminescent Materials through Artificial Intelligence85A single host phosphor Ca3(SiO3)3:Eu2+, Mn2+ with good monodispersity for phosphor-converted white LEDs12Superior thermally-stable narrow-band green emitter from Mn2+-doped zero thermal expansion (ZTE) material78Ternary sulfides ALnS2:Eu2+ (A = Alkaline Metal, Ln = rare-earth element) for lighting: Correlation between the host structure and Eu2+ emission maxima18Screening and discovery of phosphors by the single-particle-diagnosis approach6Deciphering the site occupancy and photoluminescence character of Sm3+ in dense-packed Ca3MgSi2O8 nanocrystals using time-resolved emission spectroscopy20Stable UV-Pumped White Light-Emitting Diodes Based on Anthracene-Coated CsCu2I322Controllable structural ordering via chemical substitution to the efficient and thermally stable luminescence in NASICON-type phosphor Series: Na1+Hf2−Sc (PO4)3:Eu12Bismuth‐activated, narrow‐band, cyan garnet phosphor Ca 3 Y 2 Ge 3 O 12 :Bi 3+ for near‐ultraviolet‐pumped white LED application39Advances in Near-Infrared Luminescent Materials without Cr3+: Crystal Structure Design, Luminescence Properties, and Applications171Metastable materials discovery in the age of large-scale computation53Applied Machine Learning for Developing Next‐Generation Functional Materials72Eu 2+ activated NaBa 3 Si 2 O 7 F: A new efficient blue‐emitting luminescent material for solid‐state lighting and display7Accelerating materials discovery with Bayesian optimization and graph deep learning142Fósforos de impacto ambiental reducido para iluminación artificial0Narrow Bandwidth Luminescence in Sr2Li(Al,Ga)O4:Eu2+ by Selective Site Occupancy Engineering for High Definition Displays52H{[Na(H2O)3]6F}(PO4)2 ⋅ 2(H2O): A New Polycation‐Type Phosphate with Deep Ultraviolet Transparency0Anti-thermal-quenching red-emitting phosphors based on lanthanide doped negative-thermal-expansion (NTE) hosts46Nanophotonics for current and future white light-emitting devices11Structure tailoring and defect engineering of LED phosphors with enhanced thermal stability and superior quantum efficiency44A novel single-phased white light emitting phosphor with single Eu2+ doped whitlockite structure24A highly efficient narrow-band blue phosphor of Bi3+-activated cubic borate Ba3Lu2B6O15 towards backlight display applications85(INVITED)KRbAl2B2O7: Eu2+: A new blue-emitting luminescent material with good thermal stability0An efficient blue phosphor with high thermal stability for lighting and optical pressure sensor applications69Investigations on electron beam irradiated rare-earth doped SrF 2 for application as low fading dosimeter material: evidence for and DFT simulation of a radiation-induced phase8Locally-ordered A-site vacancy assisted photoluminescence enhancement in simply rare-earth doped perovskite oxide13Anti-Defect engineering toward high luminescent efficiency in whitlockite phosphors53Emerging materials and devices for efficient light generation2Broadband Near-Infrared-Emitting Phosphors with Suppressed Concentration Quenching in a Two-Dimensional Structure47Efficient near-infrared phosphors discovered by parametrizing the Eu(II) 5d-to-4f energy gap92A novel Bi3+-Activated garnet phosphor with site-selected excitations and high temperature sensitivity42Challenges and Strategies to Design Phosphors for Future White Light Emitting Diodes104Facile Conjugated‐Polymer‐Based Flexible Lighting Fabrication and Microdeformation Monitoring3Design of a europium‐activated lithium‐silicate cyan phosphor via cation substitution3A tunable blue–cyan dual emission phosphor in Ca 4− x Lu 2 x Hf 1− x Ge 3 O 12 :Bi 3+ via forming segregation structure for WLEDs13Design of K2SrCa(PO4)2-x(BO3)x:Eu2+ phosphors with full-visible spectrum by crystal structure modification12Unraveling the Evolution of Luminescence Center in an Eu‐Doped Orthophosphate: Beyond the Probe Limitation to Trace Activator5Nanoantennas Patterned by Colloidal Lithography for Enhanced Nanophosphor Light Emission7Laser Phosphors for Next-Generation Lighting Applications152Rapid discovery of new Eu 2+ -activated phosphors with a designed luminescence color using a data-driven approach15Ba 4 Al 7 Li 28.08 O 26.92 N 1.08 , the Barium Oxonitridolithoaluminate with a Highly Condensed LiO 4 Tetrahedra Framework3Energy transfer and tunable emission in BaSrGd 4 O 8 :Bi 3+ ,Eu 3+ phosphors for warm WLED9Non-rare-earth-doped submicron-grade narrow-band red phosphors for W-LED as well as FED and enhanced Bi 3+ -doped blue light absorption32Recent progress in trivalent europium (Eu 3+ )-based inorganic phosphors for solid-state lighting: an overview72The Application of Novel Functional Materials to Machine Learning0Photoluminescence properties of novel blue-light excited orange-red phosphors Sr3Al2Si3O12:Eu2+23Facile Synthesis of Highly Efficient and Thermally Stable BaAl 4 Sb 2 O 12 :Eu 2+ Phosphor in Air72Site‐Engineering for Controlling Multiple‐Excitation and Emission in Eu2+‐Activated CaSrSiO4 Phosphors in Marine Fisheries21Cation substitution induced highly symmetric crystal structure in cyan-green-emitting Ca2La1-xLuxHf2Al3O12:Ce3+ solid-solution phosphors with enhanced photoluminescence emission and thermal stability: Toward full-visible-spectrum white LEDs41High-Throughput Screening on Halide Perovskite Derivatives and Rational Design of Cs 3 LuCl 629Moderate Trap Engineering for Enhanced Thermal Stability and High Efficiency in a Bi3+-Doped Phosphor45Crystal structure of the quaternary lithogallate Sr 2 LiGaO 42First principle study to investigate color tunable properties in Bi3+, Tb3+, and Yb3+ doped GdVO4 phosphor13Monoclinic to cubic structural transformation, local electronic structure, and luminescence properties of Eu-doped HfO211Machine-learning assisted high-throughput discovery of solid-state electrolytes for Li-ion batteries80The Luminescent Behaviors and J-O Theory Analysis of Red Phosphor Ca1-Xgeo3:Xeu3+0White light emission and superior color stability in a single-component host with exceptional eminent color rendering and theoretical calculations on D uv for color quality10Disordered enthalpy–entropy descriptor for high-entropy ceramics discovery243Mn–Mn Magnetic Coupling Interaction-Induced Red Emission in a Tetra-Coordinated Lattice23One stone, two birds: Luminescence properties of Ca8ZnY(PO4)7:Eu2+, Mn2+ and multifunctional applications in WLEDs & optical anti-counterfeiting26Achieving Ultra‐Broadband Sunlight‐Like Emission in Single‐Phase Phosphors: The Interplay of Structure and Luminescence44Accelerating Computational Materials Discovery with Machine Learning and Cloud High-Performance Computing: from Large-Scale Screening to Experimental Validation142Isomorphism of Sr[Li3AlO4] and Sr[Li3GaO4] – Syntheses, Crystal Structure, and Europium(II) Luminescence8Robust and orange-yellow-emitting Sr-rich polytypoid α-SiAlON (Sr 3 Si 24 Al 6 N 40 :Eu 2+ ) phosphor for white LEDs3The luminescent behaviors and J-O theory analysis of red phosphor Ca1-xGeO3:xEu3+16Exploring new useful phosphors by combining experiments with machine learning10Preparation, structure and properties of ultra-broadband yellow-emitting CaGd2Sc2Al2SiO12:Ce3+ garnet phosphors for blue-chip-pumped white LEDs18Compositional engineering of phase-stable and highly efficient deep-red emitting phosphor for advanced plant lighting systems94Energy transfer and charge compensation of Ba 2 ZnGe 2 O 7 :Tb 3+ ,Eu 3+ phosphors for white LEDs14Luminescence enhancement and color regulation of Sr2LiAlO4-1.5N : Eu2+ phosphor for high color rendering index white LED applications4A narrow-band Bi³ ⁺-activated blue phosphor with high thermal stability for multiple applications1Accelerated data-driven materials science with the Materials Project296Machine learning-driven discovery of efficient narrow-band green phosphor for wide-color-gamut backlight displays9A review of recent advances in Ce3+-activated garnet phosphors for blue-chip-pumped pc-WLEDs81Narrow‐Band Green Phosphors for Advanced Display Technologies: Material Design, Performance Optimization, and Future Prospects6Unlocks Photoluminescence Quantum Efficiency Enhancement in Eu 2+ ‐Doped Phosphors via Bond Angle Variance Index22Unlocks Photoluminescence Quantum Efficiency Enhancement in Eu2+‐Doped Phosphors via Bond Angle Variance Index6Density functional theory facilitates heterovalent substitution: The multi-functional application of near-infrared emitting phosphors with excellent thermal stability0High Ionic Conductivity and Cost-Effective Halide Solid Electrolyte Enabled by Long-Range Cooperative Transport in Bi-Doped Li 2 ZrCl 610Synthesis of ZnO in PVA media: Expanding the applicability of ZnO toward lighting2From Model to Material: Machine Learning Enabled Discovery of LED‐Compatible Phosphors4The barium oxolithogallate Ba 2 [LiGaO 4 ] as an ordered variant of the BaZnO 2 -type structure0Scalable Synthesis of Highly Efficient and Thermostable Graphitic Carbon Nitride for White Light-Emitting Diodes3Ba 2+ co-doping enhances phase purity and enables narrow–band green emission in a Sr 5/6 Li 17/6 Al 7/6 O 4 :Eu 2+ phosphor for backlight display applications1Data-Driven Advances in Rare-Earth Substituted Inorganic Phosphors for Solid-State Lighting and Display Applications: A 6G Perspective0Resolving energy transfer dynamics in Eu²⁺-activated multi-site phosphors via metaheuristic optimization and physics-informed neural networks1High thermal stability and red emitting phosphor Sr2LiAlO4: Sm3+ for white LED3Thermally Driven Eu 2+ Site‐Selective Occupation Enables Narrow‐Band Green Emission in an Oxolithoaluminate Phosphor for Backlight Display Applications5Multi-site regulation and luminescence enhancement of narrow-band green-emitting Sr2Li(Al,Ga)(O,N)4: Eu2+ phosphors1Cuprous-Hybrid Metal Halides with Multimode Self-Trapped Excitons Enable Full-Spectrum White-Light Emission with Considerable Color Stability0

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  1. Eu 2+ Site Preferences in the Mixed Cation K 2 BaCa(PO 4 ) 2 and Thermally Stable Luminescence

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  2. (INVITED) A review on the Eu2+ doped β-Ca3(PO4)2-type phosphors and the sites occupancy for photoluminescence tuning

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  3. Aliovalent substitution toward reinforced structural rigidity in Ce 3+ -doped garnet phosphors featuring improved performance

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  4. Color tunable single-phase Eu 2+ and Ce 3+ co-activated Sr 2 LiAlO 4 phosphors

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  5. Li substituent tuning of LED phosphors with enhanced efficiency, tunable photoluminescence, and improved thermal stability

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  6. Accelerating materials science with high-throughput computations and machine learning

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  7. Realizing Visible Light Excitation of Tb3+ via Highly Efficient Energy Transfer from Ce3+ for LED‐Based Applications

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  9. Energy, Phonon, and Dynamic Stability Criteria of Two-Dimensional Materials

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  10. Small Alkaline-Earth-based Core/Shell Nanoparticles for Efficient Upconversion

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  11. Synthesis of Ba1−Sr YSi2O5N and discussion based on structure analysis and DFT calculation

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  12. Computational Discovery and Design of MXenes for Energy Applications: Status, Successes, and Opportunities

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  13. Site‐Selective Occupancy of Eu 2+ Toward Blue‐Light‐Excited Red Emission in a Rb 3 YSi 2 O 7 :Eu Phosphor

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  14. Site‐Selective Occupancy of Eu2+Toward Blue‐Light‐Excited Red Emission in a Rb3YSi2O7:Eu Phosphor

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  15. Data-Driven Discovery of Full-Visible-Spectrum Phosphor

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  16. Engineering of K3YSi2O7To Tune Photoluminescence with Selected Activators and Site Occupancy

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  17. Polymorphs and derivates of Sr2LiAlO4:Eu2+

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  18. Broadband emission of double perovskite Cs2Na04Ag06In0995Bi0005Cl6:Mn2+ for single-phosphor white-light-emitting diodes

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  19. Photoluminescence Control of UCr 4 C 4 -Type Phosphors with Superior Luminous Efficiency and High Color Purity via Controlling Site Selection of Eu 2+ Activators

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  20. Unified Theory of Thermal Quenching in Inorganic Phosphors

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  21. Critical Review—A Promising Cs3CoCl5 Prototype Phosphor toward the Discovery of Next-Generation LED Phosphor

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  24. Designing High‐Performance LED Phosphors by Controlling the Phase Stability via a Heterovalent Substitution Strategy

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  25. Photoluminescence control and abnormal Eu 3+ orange emission in Ln 3+ (Ln 3+ = Ce 3+ , Eu 3+ )-doped oxyapatite-type phosphors

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  28. Realizing red/orange emission of Eu 2+ /Ce 3+ in La 26−x Sr x Si 41 O x+1 N 80−x ( x = 12.72–12.90) phosphors for high color rendition white LEDs

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  30. Highly Efficient Green‐to‐Yellowish‐Orange Emitting Eu2+‐Doped Pyrophosphate Phosphors with Superior Thermal Quenching Resistance for w‐LEDs

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  31. Recent progress on discovery of novel phosphors for solid state lighting

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  32. Violet-light-excitable super-narrow band green emitting phosphor for high-quality white LEDs

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  33. Broadband deep‐red‐to‐near‐infrared emission from Mn 2+ in strong crystal‐field of nitride MgAlSiN 3

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  34. Preparation, luminescence properties and electronic structure of RE (RE=Eu3+,Sm3+,Dy3+)-doped multi-color silico-phosphate Ca15(PO4)2(SiO4)6 phosphors

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  35. Data-Driven Photoluminescence Tuning in Eu2+-Doped Phosphors

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  36. Predicting Thermal Quenching in Inorganic Phosphors

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  37. Narrow-band emitters in LED backlights for liquid-crystal displays

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  38. Energy transfer and photo/cathodoluminescence performances investigation of a luminescent material Ce3+/Tb3+ co-doped Na2Ca2Si2O7 for multifunctional applications

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  39. Design Principles for Aqueous Na-Ion Battery Cathodes

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  40. Exploring Frontiers in Research and Teaching: NanoEngineering and Chemical Engineering at UC San Diego

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  41. Acid-Stable Oxides for Oxygen Electrocatalysis

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  42. Anti‐Thermal‐Quenching Bi 3+ Luminescence in a Cyan‐Emitting Ba 2 ZnGe 2 O 7 :Bi Phosphor Based on Zinc Vacancy

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  43. Chemist versus Machine: Traditional Knowledge versus Machine Learning Techniques

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  44. A data-driven approach to predicting band gap, excitation, and emission energies for Eu 2+ -activated phosphors

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  45. Structural design and evolution of a novel Bi 3+ -doped narrow-band emission blue phosphor with excellent photoluminescence performance for wide color gamut wLED

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  46. Opportunities for Next-Generation Luminescent Materials through Artificial Intelligence

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  47. A single host phosphor Ca3(SiO3)3:Eu2+, Mn2+ with good monodispersity for phosphor-converted white LEDs

    Journal of Alloys and Compounds · 2021-02-17

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  48. Superior thermally-stable narrow-band green emitter from Mn2+-doped zero thermal expansion (ZTE) material

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