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RESEARCH PAPER · Angewandte Chemie · 2019

Site‐Selective Occupancy of Eu2+Toward Blue‐Light‐Excited Red Emission in a Rb3YSi2O7:Eu Phosphor

Jianwei Qiao, Lixin Ning, Мaxim S. Моlokeev, Yu‐Chun Chuang, Qinyuan Zhang, Kenneth Reinhard Poeppelmeier, Zhiguo Xia

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Site‐Selective Occupancy of Eu2+Toward Blue‐Light‐Excited Red Emission in a Rb3YSi2O7:Eu PhosphorOriginalEngineering of K3YSi2O7To Tune Photoluminescence with Selected Activators and Site Occupancy118Synthesis and investigation of orange-emitting Eu2+ doped Ba4Li2B10O20 phosphor5The photoluminescence properties and latent photocatalytic hydrogen evolution application of AlN:Eu3+27Concentration quenching and thermal stability of Eu2+ emission in green emitting phosphor Li2BaSiO4: Eu2+31A Double‐Band Emitter with Ultranarrow‐Band Blue and Narrow‐Band Green Luminescence15Designing High‐Performance LED Phosphors by Controlling the Phase Stability via a Heterovalent Substitution Strategy76Photoluminescence control and abnormal Eu 3+ orange emission in Ln 3+ (Ln 3+ = Ce 3+ , Eu 3+ )-doped oxyapatite-type phosphors17Crystal structure refinement, photoluminescence properties and energy transfer of multicolor tunable Ca2Al2SiO7:Tm3+, Dy3+ for NUV white-light-emitting diodes20Evaluating Thermal Quenching Temperature in Eu 3+ -Substituted Oxide Phosphors via Machine Learning81Luminescence and energy transfer of color-tunable Lu2MgAl4SiO12:Eu2+,Ce3+,Mn2+ phosphors43A K 3 ScSi 2 O 7 :Eu 2+ based phosphor with broad-band NIR emission and robust thermal stability for NIR pc-LEDs111Full-visible-spectrum lighting realized by a novel Eu 2+ -doped cyan-emitting borosilicate phosphor26Multi-peaked broad-band red phosphor Y 3 Si 6 N 11 :Pr 3+ for white LEDs and temperature sensing21Novel narrow-band blue-emitting Cs 3 Zn 6 B 9 O 21 :Bi 3+ phosphor with superior thermal stability33Phase stabilization of red-emitting olivine-type NaMgPO 4 :Eu 2+ phosphors via molten-phase quenching29Multi-site occupancies and photoluminescence characteristics in developed Eu2+-activated Ba5SiO4Cl6 bifunctional platform: Towards manufacturable optical thermometer and indoor illumination32Eu3+-activated Ca3Mo0.2W0.8O6 red-emitting phosphors: A near-ultraviolet and blue light excitable platform for solid-state lighting and thermometer33Self-activated luminescence in AZn4(BO3)3 (A = K, Rb, Cs) and oxygen-defects-related photoluminescence tuning28Cation-Deficiency-Induced Crystal-Site Engineering for ZnGa2O4:Mn2+ Thin Film29Thermally Stable Phosphor KBa2(PO3)5:Eu2+ with Broad-Band Cyan Emission Caused by Multisite Occupancy of Eu2+58Borate Hydrides as a New Material Class: Structure, Computational Studies, and Spectroscopic Investigations on Sr5(BO3)3H and Sr5(11BO3)3D19Energy transfer and photo/cathodoluminescence performances investigation of a luminescent material Ce3+/Tb3+ co-doped Na2Ca2Si2O7 for multifunctional applications15A novel green‐emitting luminescent materials with broad‐band emission for high‐quality warm white LED indoor lighting20Two targets with one strategy: Insights into the role of aluminum atoms on the luminescence properties and thermal stability in Mn4+-doped calcium aluminozincate phosphor16Great emission enhancement of high-efficient broadband K3YSi2O7: Eu red phosphor via enhancing crystallinity44Exploiting the diverse photoluminescence behaviors of NaLuF4:xEu3+ nanoparticles and g-C3N4 to realize versatile applications in white light-emitting diode and optical thermometer163Ba 3 YB 3 O 9 based phosphor ceramic plates with excellent thermal stability for wLED applications18Single phase white LED phosphor Ca3YAl3B4O15:Ce3+,Tb3+,Sm3+ with superior performance: Color-tunable and energy transfer study184A Study on the Anti-thermal Dy3+/Eu3+ Co-doped BaLa4Si3O13 Red Phosphors for White-Light-Emitting Diodes and Optical Thermometry Applications41Eu 2+ Stabilized at Octahedrally Coordinated Ln 3+ Site Enabling Red Emission in Sr 3 LnAl 2 O 7.5 (Ln = Y or Lu) Phosphors61Spontaneous-reduction and photoluminescence tuning in singly-doped Ba5-Ca (PO4)3Cl:Eu2+/Eu3+ phosphors23Synthesis red-emitting Ca2LaNbO6:xSm3+ phosphors for good color-rendering-index white-LED devices19Research on Molecular Structure and Electronic Properties of Ln3+ (Ce3+, Tb3+, Pr3+)/Li+ and Eu2+ Co-Doped Sr2Si5N8 via DFT Calculation5Preparation and photoluminescent property of blue-emitting phosphors Sr5Al2F16:Eu2+6Creating a Green-Emitting Phosphor through Selective Rare-Earth Site Preference in NaBaB 9 O 15 :Eu 2+69Designing a Thermally Robust Green-Emitting Phosphor Rb2HfSi2O7: Eu2+ by an Atomic Chain Vibration Model and Its White Light-Emitting Diode Application16Warm white light emission, thermochromic property and long persistent luminescence derived from multi-sites of Eu2+/Eu3+ in host lattice71A Novel Ba 2 LuNbO 6 :Mn 4+ Double-Perovskite Far-Red Phosphor for Indoor Plant Cultivation8Bright Red-Emitting Ca3LuAl3B4O15:Ce3+,Sm3+ Phosphors with High Thermal Stability for Elevating the Color Rendering of Near-Ultraviolet-Based White-Light-Emitting Diodes21Structure tailoring and defect engineering of LED phosphors with enhanced thermal stability and superior quantum efficiency44Molten-salt synthesis and spectral characteristics of perovskite KCa2Nb3O10:Sm3+ phosphors31A novel single-phased white light emitting phosphor with single Eu2+ doped whitlockite structure25A new type of phosphate-based phosphor Na 3 CsMg 7 (PO 4 ) 6 :Eu 2+ /Mn 2+ with high quantum efficiency and high thermostability24Simultaneous construction of impermeable dual-shell stabilizing fluoride phosphors for white light-emitting diodes24Ultra‐Broadband Green‐Emitting Phosphors without Cyan Gap Based on Double‐Heterovalent Substitution Strategy for Full‐Spectrum WLED Lighting92Basic crystal field theory—A simple and useful tool to understand the structure–property relationship in luminescent materials9Recent progress in Ce 3+ /Eu 2+ -activated LEDs and persistent phosphors: focusing on the local structure and the electronic structure140Enhanced cyan emission via competitive site occupancy engineering in Sr2SiO4:Eu2+ phosphor for achieving full-spectrum LED lighting20Cationic composition engineering in double perovskite XLaLiTeO 6 :Eu 3+ (X = Ba, Sr, Ca, and Mg) toward efficient and thermally stable red luminescence for domestic white-LEDs35Eu 2+ luminescence in CaYGaO 4 olivine: a new efficient red phosphor for warm illumination48White electroluminescence of diamond/ZnSe composite film1Synthesis and luminescence properties of Ca3Ga4O9:Eu3+: An efficient red-emitter for WLEDs39Blue-red dual color emitting phosphor Cs2NaLuCl6: Sb3+, Ho3+ for plant growth LEDs66Optical temperature-sensing properties in La1.55SiO4.33:Yb3+,Ho3+ phosphors affected by Ho3+-doping concentration12Effect of Eu3+ doping on structural and optical properties of zirconium titanate19Efficient deep-red luminescence with high colour purity from Mn4+-doped ZnAl2O4 nanophosphor19Upconversion luminescence and optical thermometry behaviors of Yb3+ and Ho3+ co-doped GYTO crystal16Expanding the Emission of CsPbBr3 Nanocrystals in the Blue Region21Bluish-green emission of novel BaAl2Ge2O8:Eu2+ phosphors under near-ultraviolet excitation20Development of thermally stable red-emitting lead-free double-perovskite phosphors with an internal PLQY approaching 100%18Unusual red luminescence and super thermal stability of a new narrow-band emission phosphor for backlight display application21A Novel Multi-Color Tunable of Linbo3:Re3+ (Re3+=Tm3+, Eu3+, Tm3+/Eu3+) Phosphors0A polymorphic SrGa 2 O 4 :Eu 2+ red phosphor for warm illumination and operando visualization of H 2 O 2 catalytic reaction4Manipulating Cationic Ordering Toward Highly Efficient and Zero-Thermal-Quenching Cyan Photoluminescence0Preparation of a novel violet-excitable Na 3 YSi 2 O 7 :Eu 2+ green phosphor via salt-flux assistance and its luminescence properties15The Luminescent Behaviors and J-O Theory Analysis of Red Phosphor Ca1-Xgeo3:Xeu3+0An efficient and thermally stable red emitting Eu2+ doped oxide for rechargeable portable flashlight62Pure-red phosphor Ca3Si2O7:Eu2+ obtained by the CO reduction strategy13Manipulating cationic ordering toward highly efficient and zero-thermal-quenching cyan photoluminescence35Modulation of components toward blue light emission and scintillation properties of Eu2+ activated Sr1-xLaxMgxAl12-xO19 crystal1Achieving zero-thermal quenching of Al2(WO4)3:Eu,Tb red phosphors with low thermal expansion for LEDs21Tailoring traps in Eu2+ activated persistent phosphors for multilevel information storage and encryption23Achieving the Anomalous Far‐Red Emission of Eu3+ by Tailoring Distorted Square Antiprism Symmetry in Potassium‐Bismuth‐Phosphates47A novel white Y2(Ti0.8Hf0.2)2O7: Eu phosphors regulated by HfO2 exhibiting low color shifting for high temperature2Highly Efficient and Stable Narrow Band Green Emitting Phosphor of Sb 3+ /Ce 3+ Sensitized Cs 2 NaTbCl 6 for WLED35Wide Range Near‐Zero Thermal Quenching of Orange–Yellow Phosphor via Impeding Self‐Oxidation of Eu 2+ for Versatile Optoelectronic Applications20The luminescent behaviors and J-O theory analysis of red phosphor Ca1-xGeO3:xEu3+17Thermal enhancing luminescence and thermal quenching luminescence of Sc2(MoO4)3: X mol% Eu3+9Air and Thermally Stable Fluoride Bridged Rare‐Earth Clusters Showing Intense Photoluminescence and Potential LED Application44Broadband red emission in disordered Sr2LaGaO5:Eu2+ phosphors7Enhanced Stability and Brightness through Co‐Substitution: Promoting Plant Growth with Green‐Excited Deep Red Phosphor Ca1‐zSrzLi1‐xMg2xAl3‐xN4:yEu2+13KBaScSi3O9:Eu2+ Glass‐Ceramics as Single‐Phase High‐Power White Emitters49Recent progress of inorganic phosphors in artificial plant cultivation LEDs46Energy transfer and charge compensation of Ba 2 ZnGe 2 O 7 :Tb 3+ ,Eu 3+ phosphors for white LEDs14Near-infrared luminescent materials: a review of their practical applications and prospective advancements48Violet light excitable K x Na 5 −x B 2 P 3 O 13 :Eu ( x = 0, 1, 2) borophosphates as novel phosphors for multifunctional applications2Theoretically Guided Development of Excitation-Wavelength-Dependent Multifunctional Phosphor Based on Gallium Vacancy Perturbation10Investigation into the great enhancement of luminescence intensity through K/Na substitution in Nepheline structure for WLED1Highly efficient Eu3+→Tb3+ energy transfer and colour tunable Y4Al2O9: Eu3+, Tb3+ nanophosphors: A promising material for concealed fingerprint analysis and solid-state lighting15Tunable photoluminescence in Eu2+-activated KCaLa(PO4)2 phosphor through structural disorder3Luminescent properties and structure of Pr3+ - doped multi-component transparent lead zinc borate glasses for red LEDs7Activator – host structure relations of applied optical materials: a review7Recent progress in Eu2+ activated red phosphors for white LEDs and laser displays: focusing on efficient host screening and innovative structural design20Ultrawideband Emission of Bi 3+ Ions Spanning Visible to Near‐Infrared Spectral Regions (400 nm–1700 nm)0A novel deep-blue emitting BaSr2(PO4)2: Eu2+ phosphor with excellent thermostability for advanced anti-counterfeiting and white light-emitting diodes1Site-selective luminescence in Ca-doped Sr2YNbO6:Eu3+ phosphors for high-color-purity red emission13Crystal structure elucidation and luminescence properties of a blue-emitting BaMgSi 3 O 8 :Eu 2+ phosphor with an alkali feldspar structure0High-temperature-stable Sr3GaAlO6: Eu2+ broadband red phosphor: Dual applications from LED lighting to fingerprint development0Efficient and thermally stable red-emitting Eu3+-activated Ca9Y(PO4)7 for high-energy excitation0A Non‐Stoichiometric Thioaluminate Phosphor with Severe Stacking Faults, Na 0.9 AlS 2 :Eu 2+1Amorphous Structure Engineering for Fabricating Highly Efficient Eu 2+ ‐Doped Red‐Emitting Luminescent Glass Ceramics2Surface modification of Ba1.53Sr0.37SiO4:0.1Eu2+ green emitting phosphors with theobromine (3,7-dimethylxanthine)0Ce3+ sensitized Tb3+ delayed emission and short persistent luminescence in NaBa3Y3Si6O20 silicate phosphors for time-resolved anticounterfeiting0

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  3. The photoluminescence properties and latent photocatalytic hydrogen evolution application of AlN:Eu3+

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  6. Designing High‐Performance LED Phosphors by Controlling the Phase Stability via a Heterovalent Substitution Strategy

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  7. Photoluminescence control and abnormal Eu 3+ orange emission in Ln 3+ (Ln 3+ = Ce 3+ , Eu 3+ )-doped oxyapatite-type phosphors

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  8. Crystal structure refinement, photoluminescence properties and energy transfer of multicolor tunable Ca2Al2SiO7:Tm3+, Dy3+ for NUV white-light-emitting diodes

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  9. Evaluating Thermal Quenching Temperature in Eu 3+ -Substituted Oxide Phosphors via Machine Learning

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  10. Luminescence and energy transfer of color-tunable Lu2MgAl4SiO12:Eu2+,Ce3+,Mn2+ phosphors

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  12. Full-visible-spectrum lighting realized by a novel Eu 2+ -doped cyan-emitting borosilicate phosphor

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  13. Multi-peaked broad-band red phosphor Y 3 Si 6 N 11 :Pr 3+ for white LEDs and temperature sensing

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  15. Phase stabilization of red-emitting olivine-type NaMgPO 4 :Eu 2+ phosphors via molten-phase quenching

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  16. Multi-site occupancies and photoluminescence characteristics in developed Eu2+-activated Ba5SiO4Cl6 bifunctional platform: Towards manufacturable optical thermometer and indoor illumination

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  17. Eu3+-activated Ca3Mo0.2W0.8O6 red-emitting phosphors: A near-ultraviolet and blue light excitable platform for solid-state lighting and thermometer

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  19. Cation-Deficiency-Induced Crystal-Site Engineering for ZnGa2O4:Mn2+ Thin Film

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  20. Thermally Stable Phosphor KBa2(PO3)5:Eu2+ with Broad-Band Cyan Emission Caused by Multisite Occupancy of Eu2+

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  21. Borate Hydrides as a New Material Class: Structure, Computational Studies, and Spectroscopic Investigations on Sr5(BO3)3H and Sr5(11BO3)3D

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  33. Research on Molecular Structure and Electronic Properties of Ln3+ (Ce3+, Tb3+, Pr3+)/Li+ and Eu2+ Co-Doped Sr2Si5N8 via DFT Calculation

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  34. Preparation and photoluminescent property of blue-emitting phosphors Sr5Al2F16:Eu2+

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  35. Creating a Green-Emitting Phosphor through Selective Rare-Earth Site Preference in NaBaB 9 O 15 :Eu 2+

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  36. Designing a Thermally Robust Green-Emitting Phosphor Rb2HfSi2O7: Eu2+ by an Atomic Chain Vibration Model and Its White Light-Emitting Diode Application

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  37. Warm white light emission, thermochromic property and long persistent luminescence derived from multi-sites of Eu2+/Eu3+ in host lattice

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  39. Bright Red-Emitting Ca3LuAl3B4O15:Ce3+,Sm3+ Phosphors with High Thermal Stability for Elevating the Color Rendering of Near-Ultraviolet-Based White-Light-Emitting Diodes

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  40. Structure tailoring and defect engineering of LED phosphors with enhanced thermal stability and superior quantum efficiency

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  41. Molten-salt synthesis and spectral characteristics of perovskite KCa2Nb3O10:Sm3+ phosphors

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  44. Simultaneous construction of impermeable dual-shell stabilizing fluoride phosphors for white light-emitting diodes

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  45. Ultra‐Broadband Green‐Emitting Phosphors without Cyan Gap Based on Double‐Heterovalent Substitution Strategy for Full‐Spectrum WLED Lighting

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  46. Basic crystal field theory—A simple and useful tool to understand the structure–property relationship in luminescent materials

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  47. Recent progress in Ce 3+ /Eu 2+ -activated LEDs and persistent phosphors: focusing on the local structure and the electronic structure

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  48. Enhanced cyan emission via competitive site occupancy engineering in Sr2SiO4:Eu2+ phosphor for achieving full-spectrum LED lighting

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    Jun Long Wang, Tianchun Lang, Mingsheng Cai, Xiaolong Jing, Lingling Peng, Qinping Qiang, Nikolaevich Yakovlev, Tao Han, Bitao Liu

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  49. Cationic composition engineering in double perovskite XLaLiTeO 6 :Eu 3+ (X = Ba, Sr, Ca, and Mg) toward efficient and thermally stable red luminescence for domestic white-LEDs

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    Jing Zhu, Tongsheng Yang, Hong Li, Yuefei Xiang, Ruitong Song, Hongzhi Zhang

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  50. Eu 2+ luminescence in CaYGaO 4 olivine: a new efficient red phosphor for warm illumination

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    Tao Hu, Zelong Jiang, Bo Wang, Ting Yu, Dawei Wen, Qinguang Zeng, Yan Na Gao

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