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RESEARCH PAPER · Journal of the American Chemical Society · 2018

Eu 2+ Site Preferences in the Mixed Cation K 2 BaCa(PO 4 ) 2 and Thermally Stable Luminescence

Jianwei Qiao, Lixin Ning, Мaxim S. Моlokeev, Yu‐Chun Chuang, Quanlin Liu, Zhiguo Xia

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Eu 2+ Site Preferences in the Mixed Cation K 2 BaCa(PO 4 ) 2 and Thermally Stable LuminescenceOriginalA far-red emission (Ca,Sr)14Zn6Ga10O35:Mn4+ phosphor for potential application in plant-growth LEDs57Far-red-emitting double-perovskite CaLaMgSbO 6 :Mn 4+ phosphors with high photoluminescence efficiency and thermal stability for indoor plant cultivation LEDs76Multiple anti-counterfeiting realized in NaBaScSi 2 O 7 with a single activator of Eu 2+57Novel SrMg 2 La 2 W 2 O 12 :Mn 4+ far-red phosphors with high quantum efficiency and thermal stability towards applications in indoor plant cultivation LEDs89Photoluminescence tuning in a novel Bi 3+ /Mn 4+ co-doped La 2 ATiO 6 :(A = Mg, Zn) double perovskite structure: phase transition and energy transfer78Structural Confinement toward Giant Enhancement of Red Emission in Mn2+‐Based Phosphors165Rb3SiF7:Mn4+ and Rb2CsSiF7:Mn4+ Red-Emitting Phosphors with a Faster Decay Rate90Persistent luminescence instead of phosphorescence: History, mechanism, and perspective680Importance of Evaluating the Intensity Dependency of the Quantum Efficiency: Impact on LEDs and Persistent Phosphors66Highly Efficient and Thermally Stable Blue-Green (Ba0.8Eu0.2O)(Al2O3)4.575×(1+x) Phosphor through Structural Modification55Layered Structure Produced Nonconcentration Quenching in a Novel Eu3+-Doped Phosphor185Luminescence of Ca3ZrSi2O9: Ce3+ blue phosphor with good thermal stability44Understanding the blue-emitting orthoborate phosphor NaBaBO 3 :Ce 3+ through experiment and computation49Warm White Light with a High Color-Rendering Index from a Single Gd3Al4GaO12:Ce3+ Transparent Ceramic for High-Power LEDs and LDs165Aliovalent substitution toward reinforced structural rigidity in Ce 3+ -doped garnet phosphors featuring improved performance44Dopant preferential site occupation and high efficiency white emission in K 2 BaCa(PO 4 ) 2 :Eu 2+ ,Mn 2+ phosphors for high quality white LED applications87Enhanced photoluminescence and thermal stability in solid solution Ca 1−x Sr x Sc 2 O 4 :Ce 3+ ( x = 0–1) via crystal field regulation and site-preferential occupation49Epitaxial growth via anti-solvent-induced deposition towards a highly efficient and stable Mn 4+ doped fluoride red phosphor for application in warm WLEDs73Highly efficient and thermally stable single-activator white-emitting phosphor K 2 Ca(PO 4 )F:Eu 2+ for white light-emitting diodes71Multichannel photoluminescence tuning in Eu-doped apatite phosphors via coexisting cation substitution, energy transfer and valence mixing54Non-concentration quenching, good thermal stability and high quantum efficiency of K 5 Y(P 2 O 7 ) 2 :Eu 3+ /Tb 3+ phosphors with a novel two-dimensional layer structure78Non-stoichiometric defect-controlled reduction toward mixed-valence Mn-doped hexaaluminates and their optical applications47Realizing emission color tuning, ratiometric optical thermometry and temperature-induced redshift investigation in novel Eu 3+ -doped Ba 3 La(VO 4 ) 3 phosphors81Thermal enhancement and quenching of upconversion emission in nanocrystals109Li substituent tuning of LED phosphors with enhanced efficiency, tunable photoluminescence, and improved thermal stability205Recent advances in solid-state LED phosphors with thermally stable luminescence325Structural Micromodulation on Bi3+-Doped Ba2Ga2GeO7 Phosphor with Considerable Tunability of the Defect-Oriented Optical Properties93Li4SrCa(SiO4)2:Eu2+: A Potential Temperature Sensor with Unique Optical Thermometric Properties111Enhanced narrow green emission and thermal stability in γ-AlON: Mn2+, Mg2+ phosphor via charge compensation56Luminescence of K2BaCa(PO4)2: Ce3+, Tb3+ dual-emitting phosphor and its application as ratiometric optical thermometer73Tuning of the Compositions and Multiple Activator Sites toward Single-Phased White Emission in (Ca 9– x Sr x )MgK(PO 4 ) 7 :Eu 2+ Phosphors for Solid-State Lighting115Unraveling the Mechanisms of Thermal Quenching of Luminescence in Ce3+-Doped Garnet Phosphors238Controllable Eu 2+ -Doped Orthophosphate Blue-/Red-Emitting Phosphors: Charge Compensation and Lattice-Strain Control49Application of thermally coupled energy levels in Er3+ doped CdMoO4 phosphors: Enhanced solid-state lighting and non-contact thermometry48Polyhedron Transformation toward Stable Narrow‐Band Green Phosphors for Wide‐Color‐Gamut Liquid Crystal Display201Eu3+-Activated NaGdF4 Nanorods for Near-Ultraviolet Light-Triggered Indoor Illumination89Novel cyan‐emitting KBaScSi 2 O 7 :Eu 2+ phosphors with ultrahigh quantum efficiency and excellent thermal stability for WLEDs57Energy transfer and cross-relaxation induced multicolor upconversion emissions in Er3+/Tm3+/Yb3+ doped double perovskite La2ZnTiO6 phosphors42Engineering of K3YSi2O7To Tune Photoluminescence with Selected Activators and Site Occupancy117Trap distribution and photo‐stimulated luminescence in LaSrAl 3 O 7 :Eu 2+ long‐lasting phosphors for optical data storage43Promotion of efficiency and thermal stability by restraining dynamic energy migration based on the highly symmetric rigid structure in the n-UV excitation green emission garnet phosphors62High-efficient and thermal-stable Ca19Zn2(PO4)14: Eu2+, Mn2+ blue-red dual-emitting phosphor for plant cultivation LEDs57Constructing new thermally coupled levels based on different emitting centers for high sensitive optical thermometer83Zero‐Thermal Quenching of Mn2+ Red Luminescence via Efficient Energy Transfer from Eu2+ in BaMgP2O7113Optical temperature sensing of up-conversion luminescent materials: Fundamentals and progress380A warm white emission of Bi3+-Eu3+ and Bi3+-Sm3+ codoping Lu2Ge2O7 phosphors by energy transfer of Bi3+-sensitized Eu3+/Sm3+73Realizing an impressive red-emitting Ca 9 MnNa(PO 4 ) 7 phosphor through a dual function based on disturbing structural confinement and energy transfer52Divalent europium-doped near-infrared-emitting phosphor for light-emitting diodes660Designing High‐Performance LED Phosphors by Controlling the Phase Stability via a Heterovalent Substitution Strategy76The structures and luminescence properties of Sr 4 Gd 3 Na 3 (PO 4 ) 6 F 2 :Ce 3+ ,Tb 3+ green phosphors with zero-thermal quenching of Tb 3+ for WLEDs49Ultra-broadband cyan-to-orange emitting Ba 1+x Sr 1−x Ga 4 O 8 :Bi 3+ phosphors: luminescence control and optical temperature sensing95Single‐Crystal Red Phosphors: Enhanced Optical Efficiency and Improved Chemical Stability for wLEDs74Tuning of Emission by Eu3+ Concentration in a Pyrophosphate: the Effect of Local Symmetry121Dual-site occupancy induced broadband cyan emission in Ba 2 CaB 2 Si 4 O 14 :Ce 3+79Strategies for Designing Antithermal‐Quenching Red Phosphors216Tb3+/Mn2+ singly/doubly doped Sr3Ce(PO4)3 for multi-color luminescence, excellent thermal stability and high-performance optical thermometry55Broad-band emission in metal halide perovskites: Mechanism, materials, and applications288Highly Efficient Cyan-Green Emission in Self-Activated Rb3RV2O8 (R = Y, Lu) Vanadate Phosphors for Full-Spectrum White Light-Emitting Diodes (LEDs)87Site-selective occupation of Eu2+ activators toward full-visible-spectrum emission in well-designed borophosphate phosphors96Eu3+, Sm3+ Deep‐Red Phosphors as Novel Materials for White Light‐Emitting Diodes and Simultaneous Performance Enhancement of Organic–Inorganic Perovskite Solar Cells84Recent Advances in Bismuth Ion‐Doped Phosphor Materials: Structure Design, Tunable Photoluminescence Properties, and Application in White LEDs363Thermally Stable Phosphor KBa2(PO3)5:Eu2+ with Broad-Band Cyan Emission Caused by Multisite Occupancy of Eu2+57A red phosphor LaSc3(BO3)4:Eu3+ with zero-thermal-quenching and high quantum efficiency for LEDs251Long persistent luminescence properties of NaBaScSi2O7: Tb3+ and it’s applications above room temperature53Narrow-band emitters in LED backlights for liquid-crystal displays217Ternary solid solution phosphors Ca1--Li Al1--Si1++N3-O :Ce3+ with enhanced thermal stability for high-power laser lighting67A novel single-phase Na3.6Y1.8(PO4)3:Bi3+,Eu3+ phosphor for tunable and white light emission42Thermally Robust and Color-Tunable Blue-Green-Emitting BaMgSi 4 O 10 :Eu 2+ ,Mn 2+ Phosphor for Warm-White LEDs44A novel thermally stable eulytite-type NaBaBi2(PO4)3:Eu3+ red-emitting phosphor for pc-WLEDs104Wide range zero-thermal-quenching ultralong phosphorescence from zero-dimensional metal halide hybrids289Enhanced Cyan Emission and Optical Tuning of Ca 3 Ga 4 O 9 :Bi 3+ for High‐Quality Full‐Spectrum White Light‐Emitting Diodes139Manipulating the redistribution of single dopant via crystal-site engineering approach in Ba4Gd3(K1-xNax)3(PO4)6F2:Eu2+ phosphors for warm white light emitting diodes45Efficient Energy Transfer from Trap Levels to Eu3+ Leads to Antithermal Quenching Effect in High-Power White Light-Emitting Diodes46Anti‐Thermal‐Quenching Bi 3+ Luminescence in a Cyan‐Emitting Ba 2 ZnGe 2 O 7 :Bi Phosphor Based on Zinc Vacancy162Thermal enhancement of upconversion emission in nanocrystals: a comprehensive summary75Two-Site Occupancy Induced a Broad-Band Emission in Phosphor K2YZr(PO4)3:Eu2+ for White-Light-Emitting Diode Applications47A broadband near-infrared phosphor BaZrGe 3 O 9 :Cr 3+ : luminescence and application for light-emitting diodes73Garnet phosphors for white-light-emitting diodes: modification and calculation63Overcoming thermal quenching in upconversion nanoparticles93Recent advances on metal oxide-based luminescence thermometry118Recent progress of zero-dimensional luminescent metal halides873Site engineering strategy toward enhanced luminescence thermostability of a Cr 3+ -doped broadband NIR phosphor and its application107Sodium difluorophosphate: facile synthesis, structure, and electrochemical behavior as an additive for sodium-ion batteries49Thermal stability of nitride phosphors for light-emitting diodes66Improving the thermal stability and luminescent efficiency of (Ba,Sr)3SiO5:Eu2+ phosphors by structure, bandgap engineering and soft chemistry synthesis method98Single phase white LED phosphor Ca3YAl3B4O15:Ce3+,Tb3+,Sm3+ with superior performance: Color-tunable and energy transfer study183Superior thermally-stable narrow-band green emitter from Mn2+-doped zero thermal expansion (ZTE) material78Glass crystallization making red phosphor for high-power warm white lighting236Advancing Human-Centric LED Lighting Using Na2MgPO4F:Eu2+101Robust thermal performance of red-emitting phosphor composites for white light-emitting diodes: Energy transfer and oxygen-vacancy induced electronic localization43Design principles for achieving red emission in Eu2+/Eu3+ doped inorganic solids83Combinations of Superior Inorganic Phosphors for Level‐Tunable Information Hiding and Encoding61Tunable emission, energy transfer and thermal stability of Ce3+, Tb3+ co-doped Na2BaCa(PO4)2 phosphors52Defect Engineering in a Eu2+-Doped β-Al2O3 Structure Blue Phosphor and Its Controllable Zero-Thermal Quenching Luminescence97Defect‐Induced Self‐Reduction and Anti‐Thermal Quenching in NaZn(PO3)3:Mn2+ Red Phosphor135Bismuth activated blue phosphor with high absorption efficiency for white LEDs55Advances in Near-Infrared Luminescent Materials without Cr3+: Crystal Structure Design, Luminescence Properties, and Applications171Influence of Dy3+ ion concentration on photoluminescence and energy transfer mechanism of promising KBaScSi3O9 phosphors for warm white LEDs57Highly efficient and zero-thermal-quenching blue-emitting Eu2+-activated K-beta-alumina phosphors72Exploring Intrinsic Electron-Trapping Centers for Persistent Luminescence in Bi3+-Doped LiREGeO4 (RE = Y, Sc, Lu): Mechanistic Origin from First-Principles Calculations46Structural Confinement toward Controlling Energy Transfer Path for Enhancing Near-Infrared Luminescence77A review and outlook of ratiometric optical thermometer based on thermally coupled levels and non-thermally coupled levels232Anti-thermal-quenching red-emitting phosphors based on lanthanide doped negative-thermal-expansion (NTE) hosts46Achieving zero-thermal quenching luminescence in ZnGa2O4: 0.02Eu3+ red phosphor47Structure tailoring and defect engineering of LED phosphors with enhanced thermal stability and superior quantum efficiency44Variation from Zero to Negative Thermal Quenching of Phosphor with Assistance of Defect States45Anti-thermal-quenching, color-tunable and ultra-narrow-band cyan green-emitting phosphor for w-LEDs with enhanced color rendering85A highly efficient narrow-band blue phosphor of Bi3+-activated cubic borate Ba3Lu2B6O15 towards backlight display applications85Eu2+‐Doped Layered Double Borate Phosphor with Ultrawide Near‐Infrared Spectral Distribution in Response to Ultraviolet–Blue Light Excitation110How to Obtain Anti‐Thermal‐Quenching Inorganic Luminescent Materials for Light‐Emitting Diode Applications252Crystal‐Field Engineering Control of an Ultraviolet–Visible‐Responsive Near‐Infrared‐Emitting Phosphor and Its Applications in Plant Growth, Night Vision, and NIR Spectroscopy Detection123Metal To Metal Charge Transfer Induced Efficient Yellow/Far‐Red Luminescence in Na2Ca3(Nb, Ta)2O9:Bi3+ toward the Applications of White‐LEDs and Plant Growth Light48Near‐Infrared Light‐Emitting Diodes utilizing a Europium‐Activated Calcium Oxide Phosphor with External Quantum Efficiency of up to 54.7%320Broadband Near-Infrared-Emitting Phosphors with Suppressed Concentration Quenching in a Two-Dimensional Structure47Challenges and Strategies to Design Phosphors for Future White Light Emitting Diodes104Zero-Thermal-Quenching Layered Metal Halide Perovskite44Organo-Metal Halide Scintillator with Weak Thermal Quenching Up to 200 °C46Enhancement of Near‐Infrared Phosphor Luminescence Properties via Construction of Stable and Compact Energy Transfer Paths54Delayed stress memory by CaAl2O4:Eu2+ mechanoluminescent phosphor with defect engineering regulation57Low-concentration Ce3+-activated ScCaO(BO3) blue-cyan phosphor with high efficiency toward full-spectrum white LED applications58Highly Efficient and Ultralong Afterglow Emission with Anti‐Thermal Quenching from CsCdCl 3 : Mn Perovskite Single Crystals125Realizing High‐Power Laser Lighting: Artfully Importing Micrometer BN into Ce: GdYAG Phosphor‐in‐Glass Film43Exploiting Desired Phosphor‐In‐Glass for All‐Inorganic Solid‐State White Illumination47A novel bright cyan emitting phosphor of Eu 2+ activated Ba 6 BO 3 Cl 9 with robust thermal stability for full-spectrum WLED applications65Facile Synthesis of Highly Efficient and Thermally Stable BaAl 4 Sb 2 O 12 :Eu 2+ Phosphor in Air72Energy‐Trapping Management in X‐Ray Storage Phosphors for Flexible 3D Imaging222Ab Initio Site‐Selective Occupancy and Luminescence Enhancement in Broadband NIR Emitting Phosphor Mg 7 Ga 2 GeO 12 :Cr 3+150Improved Thermal and Chemical Stability of Oxynitride Phosphor from Facile Chemical Synthesis for Vehicle Cornering Lights50Colossal Chromatic Shift in the Ba 2 Ca 2 B 4 O 10 :Ce 3+ Phosphor45Moderate Trap Engineering for Enhanced Thermal Stability and High Efficiency in a Bi3+-Doped Phosphor45High thermal stability of warm white emitting single phase GdPO4: Dy3+/ Sm3+ phosphor for UV excited wLEDs45Site Occupation Engineering toward Giant Red-Shifted Photoluminescence in (Ba,Sr)2LaGaO5:Eu2+ Phosphors63Red‐Emitting Cordierite Ceramic Enabling General Healthy Warm White Laser Lighting55Cr 3+ ↔Fe 3+ Energy Transfer Offset Enabling Anti‐Thermal Quenching Near‐Infrared Emission for Coded Wireless‐Communication Applications43Highly Efficient Narrow-Band Green-Emitting Na 3 K 5 (Li 3 SiO 4 ) 8 :Eu 2+ Phosphor with Low Thermal Quenching49Zero-thermal-quenching and charge compensation for efficient luminescence in Ca9ZnK(PO4)7:Sm3+: Optimizing defect engineering47Recent progress on modulating luminescence thermal quenching properties of Bi 3+ -activated phosphors77Bright Circularly Polarized Mechanoluminescence from 0D Hybrid Manganese Halides99Achieving High‐Temperature Phosphorescence by Organic Cocrystal Engineering110A Robust Anti-Thermal-Quenching Phosphor Based on Zero-Dimensional Metal Halide Rb3InCl6:xSb3+80LaMg6Ga6S16: a chemical stable divalent lanthanide chalcogenide70Dynamic multicolor emissions of multimodal phosphors by Mn2+ trace doping in self-activated CaGa4O7154High‐Capacity Photochromic Rotary Encoder for Information Encryption and Storage66Suppressing Self‐Oxidation of Eu 2+ in Li 2 CaSiO 4 for Full‐Spectrum Lighting and Accurate Temperature Sensing65Blue‐Light‐Excitable Broadband Ca 3 Ga 2 Ge 3 O 12 :Cr 3+ ,Ni 2+ Phosphor for the Applications in NIR‐II Window82Unlocking Chlorine Oxide‐Based Ultra‐Wideband Near‐Infrared Phosphor and Advancing Spectral Performance via Lattice Engineering43A novel High-Efficiency cyan phosphor for Human-Centric lighting with 410 nm excited white LEDs49Air and Thermally Stable Fluoride Bridged Rare‐Earth Clusters Showing Intense Photoluminescence and Potential LED Application44Compositional engineering of phase-stable and highly efficient deep-red emitting phosphor for advanced plant lighting systems94A review of recent advances in Ce3+-activated garnet phosphors for blue-chip-pumped pc-WLEDs81

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  9. Structural Confinement toward Giant Enhancement of Red Emission in Mn2+‐Based Phosphors

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  36. Epitaxial growth via anti-solvent-induced deposition towards a highly efficient and stable Mn 4+ doped fluoride red phosphor for application in warm WLEDs

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  37. Highly efficient and thermally stable single-activator white-emitting phosphor K 2 Ca(PO 4 )F:Eu 2+ for white light-emitting diodes

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  38. Investigation of local structure distortion and electron cloud interaction on emission-band broadening induced by the concentration perturbation effect of cation substitution in BaY 2 Si 3 O 10 :Eu phosphors

    CrystEngComm · 2019-01-01

    Haoran Li, Yujun Liang, Yingli Zhu, Shiqi Liu, Jiahui Chen, Hang Zhang, Yongjun Chen

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  39. Lithium ion doping triggered splendid quantum efficiency and thermal stability in Li 2 SrSiO 4 : x Eu 2+ phosphors for optical thermometry and high luminous efficiency white-LED

    New Journal of Chemistry · 2019-01-01

    Luhui Zhou, Peng Du, Weiping Li, Laihui Luo

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  40. Mixing the valence control of Eu 2+ /Eu 3+ and energy transfer construction of Eu 2+ /Mn 2+ in the solid solution (1 − x )Ca 3 (PO 4 ) 2 – x Ca 9 Y(PO 4 ) 7 for multichannel photoluminescence tuning

    Inorganic Chemistry Frontiers · 2019-01-01

    Peipei Dang, Dongjie� Liu, Guogang Li, Sisi Liang, Hongzhou Lian, Mengmeng Shang, Jun Lin

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  41. Multichannel photoluminescence tuning in Eu-doped apatite phosphors via coexisting cation substitution, energy transfer and valence mixing

    Journal of Materials Chemistry C · 2019-01-01

    Peipei Dang, Guogang Li, Sisi Liang, Hongzhou Lian, Jun Lin

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  42. Multicolor properties and applications of Ln 3+ doped hierarchical NaY(WO 4 ) 2 via a facile solvothermal process

    CrystEngComm · 2019-01-01

    Ming Zeng, Jie Liu, Yang Ding, Wen He, Ranran Lan, Yuxin Tang, Mengyang Zhou, Xibin Yu

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  43. Non-concentration quenching, good thermal stability and high quantum efficiency of K 5 Y(P 2 O 7 ) 2 :Eu 3+ /Tb 3+ phosphors with a novel two-dimensional layer structure

    Journal of Materials Chemistry C · 2019-01-01

    Dan Zhao, Ya-Li Xue, Shirui Zhang, Lin‐Ying Shi, Baozhong Liu, Yan-Ping Fan, Qingxia Yao, Shao-Jie Dai

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  44. Non-stoichiometric defect-controlled reduction toward mixed-valence Mn-doped hexaaluminates and their optical applications

    Journal of Materials Chemistry C · 2019-01-01

    Jieqi Hu, Enhai Song, Yayun Zhou, Shaolin Zhang, Shi Ye, Zhiguo Xia, Qinyuan Zhang

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  45. Realizing emission color tuning, ratiometric optical thermometry and temperature-induced redshift investigation in novel Eu 3+ -doped Ba 3 La(VO 4 ) 3 phosphors

    Dalton Transactions · 2019-01-01

    Peixin Yang, Li Li, Yongsen Deng, Yongjie Wang, Sha Jiang, Xiaobing Luo, Guotao Xiang, Yi Chun Lu, Xianju Zhou

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  46. Sensitivity improvement induced by thermal response behavior for temperature sensing applications

    Physical Chemistry Chemical Physics · 2019-01-01

    Youfusheng Wu, Fengqin Lai, Bin Liu, Jianhui Huang, Xinyu Ye, Weixiong You

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  47. The first lithium difluorophosphate LiPO 2 F 2 with a neutral polytetrahedral microporous architecture

    Chemical Communications · 2019-01-01

    Guopeng Han, Ying Wang, Hao Li, Zhihua Yang, Shilie Pan

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  48. Thermal enhancement and quenching of upconversion emission in nanocrystals

    Nanoscale · 2019-01-01

    Zijun Wang, Jeppe Christiansen, Dennie F. L. Wezendonk, Xiaobin Xie, Marijn A. van Huis, Andries Meijerink

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  49. Two-dimensional CdX (X = Se, Te) nanosheets: controlled synthesis and their photoluminescence properties

    Journal of Materials Chemistry C · 2019-01-01

    Yasir A. Haleem, Qiumei Di, Bing Bai, Meng Kai Xu, Wenxing Chen, Jiajia Liu, Jia Liu, Hongpan Rong, Jiatao Zhang

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  50. Vibrationally induced color shift tuning of photoluminescence in Ce 3+ -doped garnet phosphors

    Journal of Materials Chemistry C · 2019-01-01

    Yuan-Chih Lin, Paul Erhart, Maths Karlsson

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