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RESEARCH PAPER · Journal of the American Chemical Society · 2024

Layered Double Hydroxide Derivatives for Polyolefin Upcycling

Mingyu Chu, Xianpeng Wang, Xuchun Wang, Panpan Xu, Zhang Lin, Shengming Li, Kun Feng, Jun Bo Zhong, Lu Wang, Youyong Li, Le He, Muhan Cao, Qiao Zhang, Lifeng Chi, Jinxing Chen

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Layered Double Hydroxide Derivatives for Polyolefin UpcyclingOriginalCatalytic chemical recycling and upcycling of polyolefin plastics27Recent advancement in synthesis and applications of layered double hydroxides (LDHs) composites78Recent advances in polyolefin plastic waste upcycling via mild heterogeneous catalysis route from catalyst development to process design25Economically attractive production of commercial-grade gasoline from waste plastics1Catalytic Upcycling of Polyolefins316The role of size and structure of catalytic active sites in polyolefin hydrogenolysis12Interfacial Reactions in Chemical Recycling and Upcycling of Plastics18Plasmonic Copper‐Ruthenium Superstructure for Efficient Photothermal Conversion and Plastic Recycling39Hydrogen-free upcycling of polyethylene waste to methylated aromatics over Ni/ZSM-5 under mild conditions19Gold Nanoparticles Decorated CoAl LDH Monolayer: A Peroxidase-Like Nanozyme for Sensitive Colorimetric Detection of Acetylcholinesterase and Inhibitors18Elucidating the effect of nanocube support morphology on the hydrogenolysis of polypropylene over Ni/CeO 2 catalysts7Recent Progress for Designing of Catalysts for Photothermal Conversion of Plastic Wastes48Depolymerization of lignin into cycloalkanes over a hydrotalcite-derived NiFe alloy catalyst8Heterogeneous catalysis strategies for polyolefin plastic upcycling: co-reactant-assisted and direct transformation under mild conditions15Gradient-temperature control enhances oxi-upcycling of polyethylene plastics to dicarboxylic acids over TS-1 zeolite14Co-upcycling of mixed polypropylene and polyesters5Selective hydrocracking of polyolefin waste into branched liquid fuels over a non-noble metal bifunctional Ni–W/ZrO 2 catalyst4Unraveling the light-promoted synergy between highly dispersed Ni and Ni nanoparticles for efficient photothermocatalytic cellulose steam reforming to syngas3Upgrading of waste polyolefins with non-noble metal catalysts21Catalytic and engineering strategies for enhanced hydrogenation reactions: A review of heterogeneous catalysts and process optimization15Sustainable production of bio-based pentanediol from ring-opening hydrogenolysis of furan derivative over hydrotalcite-derived mixed metal oxide catalyst8Temperature regulating the directional catalytic transfer hydrogenolysis of lignin over a in situ topologically prepared NiRu/Al2O37Insights into the Light‐Promoted Synergy Among Active Oxygen, Oxygen Vacancies, and H 2 O Adsorption Sites in Ni/La 3+ ‐Doped CeO 2 for Highly Efficient Photothermocatalytic Cellulose Steam Reforming to Syngas10Reductive Upcycling of Polyolefins, Polyesters and Mixed Plastic Wastes to Valuable Chemicals: Bridging Chemical Catalysis With Plastic Waste Management35Hydrodeoxygenation of lignin-derived oxygenated aromatic compounds catalyzed by nano-floral hydrotalcite for the preparation of liquid-phase organic hydrogen carriers20Polyolefin Recycling with Binary Cobalt–Nickel Nanosheets6Zeolites in the epoch of catalytic recycling plastic waste: Toward circular economy and sustainability20Synergistic Co‐Recycling: Selective Oxidation of Polyethylene to Dicarboxylic Acids over Spent LiCoO 2 Cathodes22Synergistic Co‐Recycling: Selective Oxidation of Polyethylene to Dicarboxylic Acids over Spent LiCoO 2 Cathodes3Electrochemically Promoted Activation of Light Alkanes at Ambient Conditions0Electrochemically Promoted Activation of Light Alkanes at Ambient Conditions5Enhancing Waste Plastic Hydrogenolysis on Ru/CeO 2 Through Concurrent Incorporation of Fe Single Atoms and FeO x Nanoclusters27Enhancing Waste Plastic Hydrogenolysis on Ru/CeO 2 Through Concurrent Incorporation of Fe Single Atoms and FeO x Nanoclusters4Synergistic Catalysis for Recycling and Upcycling of Plastics35Overcoming limitations in polyolefins upcycling by codesigning endothermic-exothermic magnetocatalytic system8Recent Advances in the Thermo-Catalytic Upcycling of Polyethylene Waste13Layered double hydroxide embedded in loofah-derived biocarbon composites towards broadband electromagnetic wave absorption and enhanced flame retardancy21In-line NMR guided orthogonal transformation of real-life plastics63Multifunctional Hollow Carbon Microspheres Enable Superior Electromagnetic Wave Response and Corrosion Barrier94Flower-like Ag/MIL-125-Ti/CoAl-LDH S-scheme heterojunctions toward optimized photothermal-photocatalytic performance12Methods for Carbon Mass Closure in Polyolefin Hydrocracking6Nanoarchitectonics of ZnFe‐Layered Double Hydroxide Catalysts for Valorization of Waste Polyethylene Terephthalate Bottles into Value‐Added Products16Fe-induced d-orbital electron redistribution tailoring peroxymonosulfate activation pathway for efficient degradation of various antibiotics7Noble Metal‐Free Low‐Temperature Aromatization of Polyethylene Waste for High‐Quality Fuel Production8Noble Metal‐Free Low‐Temperature Aromatization of Polyethylene Waste for High‐Quality Fuel Production3Solar‐Driven Plastic Upcycling Coupled with Valuable Reduction Reactions3Crystal structure and oxygen vacancy engineering of cobalt-aluminate spinel enhances peroxymonosulfate activation and high-valent cobalt-oxo species formation for wastewater purification12The silent partner in catalysis: How support architectures dictate efficiency in polyolefin hydrogenolysis1Stable single-site organonickel catalyst preferentially hydrogenolyses branched polyolefin C–C bonds12Defect Engineering-Regulated Electron Transfer of NiAl-MMO for Catalyzing Directed Conversion of Lignin into Cyclohexanol-Based Chemicals8Hierarchical porous carbon nanosheets derived from ZIF-on-LDH as coating for solid phase microextraction of polychlorinated biphenyl in beverages9Closed-loop recycling of polyethylene to ethylene and propylene via a kinetic decoupling–recoupling strategy32Fine regulation of Ru species improved the polyethylene hydrogenolysis performance over Ru/Al 2 O 3 catalyst5Plasma Catalysis for Plastic Waste Conversion into Value‐Added Products: Advancements and Perspectives11Microwave-assisted catalytic upcycling of polyolefin wastes into hydrogen and carbon nanotubes over Pt-promoted Fe/Ni bimetallic catalysts10Crucial role of surface hydroxyl in Au/CaCO3-Al2O3-HT catalyst for base-free oxidative esterification of furfural3Highly Efficient Catalyst Derived from Ultrathin Co-Based Layered Double Hydroxide for Catalytic Transfer Hydrogenation of Guaiacol under Mild Conditions1Breaking the yield–selectivity trade-off in polystyrene waste valorization via tandem depolymerization and hydrogenolysis18Surface and Interface Properties of Metal Species for Waste Plastic Hydroconversion6Phase Interface Engineering of Cu 1 Co Single Atom Alloy Catalysts for Enhanced Hydrogen Production from Methanol Decomposition0Entropy Engineering for the Efficient Hydrogenolysis of Waste Polyolefins1Catalytic valorization of polyolefins: from catalysts and processes to reactors0Decoding active sites, mechanisms, and reactivities of layered double hydroxide catalysts for organic transformation reactions0Electronegativity-driven d-band center shifts in Ru–Ni alloys for low methane hydrogenolysis of polyolefin plastics2Enhancing aromatic yield by zeolites in polypropylene hydrocracking to jet fuel over Ru 1 -ZrO 2 without forming CH 40Metal-support interactions and interfacial defect engineering in CuAl catalyst for selective C–O bond cleavage of lignin-derived compounds0Oxygen evolution catalysts by self-assembly of MS 2 (M = Mo, W) and Ni 3 Fe-LDH nanosheets0Versatile synthesis of ultra-high surface area layered double hydroxide nanosheets1Construction of integrated structural-microwave absorbing composites: Layered double hydroxide exfoliation-reassembly strategy5Suppressing Hydrogen Transfer and Aromatization Reactions Enables Efficient Photothermal Recycling of Polyethylene into Platform Olefins5Acid sites in hydrogen-involved polyolefin upcycling: mechanistic insights and design principles0Rational design of bifunctional catalysts for hydrocracking of polyethylene waste plastics to narrow-distributed liquid fuels4Material Engineering of Cu 0 /Cu + Sites and Oxygen Vacancies for Efficient In Situ Hydrodeoxygenation of Lignin‐Based Compounds4Structure–performance relationships in heterogeneous catalysts for polyolefin plastic hydroconversion1Techno-economic analysis and life cycle assessment for the catalytic hydrogenolysis and hydrocracking of polyethylene6Photothermal catalysis for plastic upcycling: a review on material design and reaction mechanisms2Highly Selective Gasoline Production by Polyethylene Hydrogenolysis Using Ternary RuNiPt Nanoalloy Catalyst1Selective Hydrocracking of Polystyrene without Solvent to Alkylbenzenes over a Single-Atom Catalyst Co1-Al2O33NiW alloy catalyst for methane suppression in polyethylene hydrogenolysis to enhance liquid hydrocarbon yields1Engineering Interfacial Compatibility and Dynamic Active Hydrogen Pools to Accelerate Polyolefin Hydrogenolysis0Ni Supported on Urea‐Modified LaFeO 3 Perovskite for Efficient Hydrogenolysis of Polyethylene Plastics2A Panoramic View on Plastic Waste Recycling and Upcycling: Heterogeneous Catalytic Strategies for Diverse Plastics and Multiple Pathways6Structural regulation of CoAl layered double hydroxide–derived catalysts for efficient hydrogenation of N-methylindole in batch and continuous-flow systems0Frustrated Lewis Pairs and Metallic Ni Synergistically Enabled Low‐Temperature Hydrogenolysis of Lignin Models1Mn1Con single-atom alloy Nano-island derived from Mn-doped layered double hydroxides nanosheets triggers efficient non-radical dominated PMS activation: Ultralow Mn doping maximizes tetracycline degradation0Boosting CO oxidation over Ru/MgFe2O4 single-atom catalysts via MnOx-mediated electronic modulation and oxygen activation0Selective hydrogenolysis of waste polyolefins to aviation fuel over a Co‑modified Ni/SiO2 catalyst1Dynamic Self‐Focusing Photothermal Localization Induced Mild Solvent‐Free Upcycling of Polystyrene0Solar‐Driven CO 2 ‐Mediated Upcycling of Waste Plastics Into Value‐Added Syngas and Carbon Nanotubes0Solar‐Driven CO 2 ‐Mediated Upcycling of Waste Plastics Into Value‐Added Syngas and Carbon Nanotubes0Implementable and Sustainable Upcycling of Medical Plastic Waste to Liquid Highly Branched Alkanes via Tandem Catalytic Cracking-Hydrogenation Strategy0Synergistic Role of Co 0 and Lewis Basic Sites for Transfer Hydrogenation of Substituted Nitroarenes by In Situ Hydrogen Generation0Ambient‐Pressure Polyolefin Upcycling With Earth‐Abundant Catalyst0Ambient‐Pressure Polyolefin Upcycling With Earth‐Abundant Catalyst0Role of molybdenum promotion in Ni/SiO2 catalysts for Polyolefins Hydrogenolysis0Efficient and Selective Low-Temperature Polypropylene Hydrogenolysis Using Zr-Doped Mixed Metal Oxides Catalysts0Mechanistic insights into the Cr-Zr/ZSM-5 catalyzed cracking of waste polyethylene: Steering product distribution toward BTX aromatics and sustainable aviation fuel0Near-Ambient-Pressure X-ray Photoelectron Spectroscopy for Mechanistic Insights and Applications in Catalysis0Hierarchical Accessibility and Framework‐Al Organization in Ultra‐High‐Silica ZSM‐5 Enable Efficient Cracking of Polyolefin Waste to Light Olefins0Hierarchical Accessibility and Framework‐Al Organization in Ultra‐High‐Silica ZSM‐5 Enable Efficient Cracking of Polyolefin Waste to Light Olefins0Photo‐Enhanced Electronic Metal–Support Interaction Boosts Low‐Temperature Water–Gas Shift Reaction via Ni δ+ –O V –Ce 3+ Interfacial Redox Cycling0Photo‐Enhanced Electronic Metal–Support Interaction Boosts Low‐Temperature Water–Gas Shift Reaction via Ni δ+ –O V –Ce 3+ Interfacial Redox Cycling0Layered double hydroxides cathode for long-lifespan dual ion batteries0

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