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RESEARCH PAPER · Angewandte Chemie International Edition · 2023

Entropy Confinement Promotes Hydrogenolysis Activity for Polyethylene Upcycling

Qingyun Kang, Mingyu Chu, Panpan Xu, Xuchun Wang, Shiqi Wang, Muhan Cao, Oleksandr Ivasenko, Tsun‐Kong Sham, Qiao Zhang, Qiming Sun, Jinxing Chen

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Entropy Confinement Promotes Hydrogenolysis Activity for Polyethylene UpcyclingOriginalConsumer Grade Polyethylene Recycling via Hydrogenolysis on Ultrafine Supported Ruthenium Nanoparticles2Consumer Grade Polyethylene Recycling via Hydrogenolysis on Ultrafine Supported Ruthenium Nanoparticles38Increase in the effective viscosity of polyethylene under extreme nanoconfinement13Review on Catalytic Depolymerization of Polyolefin Waste by Hydrogenolysis: State-of-the-Art and Outlook57Upcycling Waste Plastics with a C–C Backbone by Heterogeneous Catalysis45Hydrogen Bubbles: Harmonizing Local Hydrogen Transfer for Efficient Plastic Hydro-Depolymerization19Recent progress of waste plastic upcycling based on multifunctional zeolite catalysts13Chemical Upcycling of Polyolefin Plastics Using Structurally Well-defined Catalysts35Poisoning effect of polyvinyl chloride on the catalytic pyrolysis of mixed plastics over zeolites31Polyethylene hydrogenolysis over bimetallic catalyst with suppression of methane formation15Recent advances in polyolefin plastic waste upcycling via mild heterogeneous catalysis route from catalyst development to process design25Constructing the Al deficiency in Si-O(H)-Al units based on Pt/ZSM-5 for enhanced hydrocracking of polyethylene into high-quality liquid fuel20Insight into the Competitive Adsorption Behavior of Polymer Chains in Silica Nanopores by Small-Angle Neutron Scattering3Catalytic Upcycling of Polyolefins316The role of size and structure of catalytic active sites in polyolefin hydrogenolysis12Interfacial Reactions in Chemical Recycling and Upcycling of Plastics18Ultra‐Narrow Alkane Product Distribution in Polyethylene Waste Hydrocracking by Zeolite Micro‐Mesopore Diffusion Optimization12Ultra‐Narrow Alkane Product Distribution in Polyethylene Waste Hydrocracking by Zeolite Micro‐Mesopore Diffusion Optimization66Ultrathin Porous Carbon Nitride Anchored with Pt Nanoclusters for Synergistic Enhancement of Hydrogen Production in Alkaline Photocatalytic Polyester Reforming15Upconversion Phosphor-Driven Photodegradation of Plastics11Efficient Hydrogenolysis of Consumer-Grade High-Density Polyethylene Wastes over MgAl-Layered Double Oxide-Supported Ru Catalysts11Challenges and opportunities in catalytic hydrogenolysis of oxygenated plastics waste: polyesters, polycarbonates, and epoxy resins44Heterogeneous catalysis strategies for polyolefin plastic upcycling: co-reactant-assisted and direct transformation under mild conditions15Co-upcycling of mixed polypropylene and polyesters5Selectivity control by zeolites during methanol-mediated CO 2 hydrogenation processes51Sustainable thermochemical plastic valorization towards a circular economy: a critical review27Synergistic effect of acidic sites and mesoporous confinement in Ce-doped Ru/SBA-15 catalysts for efficient hydrogenolysis of low-density polyethylene to liquid fuels7Conversion of Polypropylene to Light Olefins by HMFI Catalysts below Pyrolytic Temperature: Catalytic, Spectroscopic, and Theoretical Studies3Tandem Catalysis for Plastic Depolymerization: In Situ Hydrogen Generation via Methanol Aqueous Phase Reforming for Sustainable Polyethylene Hydrogenolysis2Tandem Catalysis for Plastic Depolymerization: In Situ Hydrogen Generation via Methanol Aqueous Phase Reforming for Sustainable Polyethylene Hydrogenolysis27Effective Methane Suppression in Upcycling of Polyethylene into Fuels via Alloying Platinum with Ruthenium Supported on ZSM-5 Zeolite17Hydrocarbon Deposition during Polyolefin Upcycling: Irreversible Adsorption and Surface Reactions of Polyethylene and Ethylene Oligomers on Silica Supports2Upgrading polyolefin plastics: experiences from petroleum refining and distinct characteristics19Engineering porous Beta zeolite-encapsulated nickel catalyst for waste polyolefins upcycling26Synergistic Co‐Recycling: Selective Oxidation of Polyethylene to Dicarboxylic Acids over Spent LiCoO 2 Cathodes22Synergistic Co‐Recycling: Selective Oxidation of Polyethylene to Dicarboxylic Acids over Spent LiCoO 2 Cathodes3Enhancing Waste Plastic Hydrogenolysis on Ru/CeO 2 Through Concurrent Incorporation of Fe Single Atoms and FeO x Nanoclusters27Enhancing Waste Plastic Hydrogenolysis on Ru/CeO 2 Through Concurrent Incorporation of Fe Single Atoms and FeO x Nanoclusters4Population Balance Models for Catalytic Depolymerization: From Elementary Steps to Multiphase Reactors8Hydrocracking of Polypropylene to Light Alkanes over HMFI Zeolite Catalysts under H 27Methods for Carbon Mass Closure in Polyolefin Hydrocracking6Chemical recycling of polyethylenes with low gas products by catalytic hydrogenolysis with heterogeneous CeO2-supported Cu-doped Ru catalyst5Polymer Upcycling by Catalytic Hydrogenolysis: The Role of Polyolefin Short-Chain Branching3In-situ encapsulation synthesis of Ni-Ce/SBA-15 by EISA for promoting CO2 methanation5Orchestrating catalytic hotspots and macromolecular architectures: molecular engineering toward zero-waste polymer circularity4Molar-Mass-Dependent Partitioning of Polyethylene in Nanopores of Model Catalyst Supports from Small-Angle Neutron Scattering2Advancing chemical recycling for waste plastic conversion1Synergy Effects in a Bimetallic Ru ─ Pt Alloy Catalyst for Low‐H 2 ‐Pressure Hydrogenolysis of Low‐Density Polyethylene3Plasma Catalysis for Plastic Waste Conversion into Value‐Added Products: Advancements and Perspectives11Chemical recycling of polycarbonate waste into advanced aviation fuel candidates via nickel–oxygen vacancy dual sites4Research progress in the detection of tumor markers by field-effect transistor biosensors based on different biorecognition elements4Entropy Engineering for the Efficient Hydrogenolysis of Waste Polyolefins1A self-regenerative Sn–W/γ-Al 2 O 3 catalyst for low-carbon and scalable polyolefin upcycling via tandem dehydrogenation–metathesis2Carbon–carbon bond cleavage for lignin and plastics deconstruction0Electronegativity-driven d-band center shifts in Ru–Ni alloys for low methane hydrogenolysis of polyolefin plastics2Highly selective production of gasoline-range hydrocarbons via hydroconversion of polyolefins over Ru/CeO 2 and BEA hybrid catalysts0Programming Atomic Aggregates and Single Atoms Synergy in Advanced Oxidation Systems0Synergistic bifunctional catalysis and plasma activation for valorizing polypropylene and CO2 to gasoline-range olefins1Structure–performance relationships in heterogeneous catalysts for polyolefin plastic hydroconversion1Techno-economic analysis and life cycle assessment for the catalytic hydrogenolysis and hydrocracking of polyethylene6Proton‐Exchanged Montmorillonite With Interlayer Accessibility as a Solid Acid Catalyst for the Upcycling of Polyoxymethylene0Hydrocracking of LDPE to liquid fuel over HY zeolite supported Ni catalyst: synergistic effect among metal, porosity and acidity1Polyethylene as a Hydrogen Source for C─O Bond Cleavage Via Transfer Hydrogenation2Advances in Catalytic Hydrogenolysis of Waste Plastics to Value-Added Products0A Mesopore-Confined and Graphene Oxide-Localized Ruthenium Catalyst Increases Rates of Mid-Chain Polyolefin Hydrogenolysis0Elucidating the Spatiotemporal Reaction Mechanism of Polyethylene Aromatization over ZSM-5 Zeolites1Biodegradable microplastics as a solution, not just a problem: Plastic waste for PPCP removal from hospital wastewater0Ambient‐Pressure Polyolefin Upcycling With Earth‐Abundant Catalyst0Ambient‐Pressure Polyolefin Upcycling With Earth‐Abundant Catalyst0A confinement-driven redox platform: CoNi-MOF/PDA@LDH for rapid and complete Cr(VI) sequestration from acidic wastewater0

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  1. Consumer Grade Polyethylene Recycling via Hydrogenolysis on Ultrafine Supported Ruthenium Nanoparticles

    Angewandte Chemie · 2023-12-17

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  2. Consumer Grade Polyethylene Recycling via Hydrogenolysis on Ultrafine Supported Ruthenium Nanoparticles

    Angewandte Chemie International Edition · 2023-12-18

    Shibashish D. Jaydev, Antonio José Martín, Marc‐Eduard Usteri, Katia Chikri, Henrik Eliasson, Rolf Erni, Javier Pérez‐Ramírez

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  3. Increase in the effective viscosity of polyethylene under extreme nanoconfinement

    The Journal of Chemical Physics · 2024-01-12

    Tian Ren, Zachary R. Hinton, Renjing Huang, Thomas H. III Epps, LaShanda T. J. Korley, Raymond J. Gorte, Daeyeon Lee

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  4. Review on Catalytic Depolymerization of Polyolefin Waste by Hydrogenolysis: State-of-the-Art and Outlook

    Energy & Fuels · 2024-01-22

    Abdulrahman Musa, E. A. Jaseer, Samir Barman, Néstor Garcı́a

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  5. Upcycling Waste Plastics with a C–C Backbone by Heterogeneous Catalysis

    Langmuir · 2024-02-15

    Huidong Lv, Fei Huang, Fan Zhang

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  6. Hydrogen Bubbles: Harmonizing Local Hydrogen Transfer for Efficient Plastic Hydro-Depolymerization

    ACS Nano · 2024-04-16

    Qingyun Kang, Xiaofang Zhang, Qianyue Feng, Lin Zhang, Mingyu Chu, Chaoran Li, Panpan Xu, Muhan Cao, Le He, Qiao Zhang, Jinxing Chen

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  7. Recent progress of waste plastic upcycling based on multifunctional zeolite catalysts

    Chemical Synthesis · 2024-05-28

    Xiaomei Wang, Jing Xu, Meng Ke Zhao, Wenjie Cui, Xiaowei Mu, Xiao Wang, Shuyan Song, Hongjie Zhang

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  8. Chemical Upcycling of Polyolefin Plastics Using Structurally Well-defined Catalysts

    JACS Au · 2024-06-04

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  9. Poisoning effect of polyvinyl chloride on the catalytic pyrolysis of mixed plastics over zeolites

    Science China Chemistry · 2024-06-04

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  10. Polyethylene hydrogenolysis over bimetallic catalyst with suppression of methane formation

    Frontiers of Chemical Science and Engineering · 2024-06-24

    Xiangkun Zhang, Bingyan Sun, Zhigang Zhao, Tan Li, Marc Mate, Kaige Wang

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  11. Recent advances in polyolefin plastic waste upcycling via mild heterogeneous catalysis route from catalyst development to process design

    Cell Reports Physical Science · 2024-07-01

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  12. Constructing the Al deficiency in Si-O(H)-Al units based on Pt/ZSM-5 for enhanced hydrocracking of polyethylene into high-quality liquid fuel

    Nano Research · 2024-08-09

    Xia Zhong, Jie Liu, Li Gao, Junnan Chen, Xiyang Wang, Ying Zhang, Yimin A. Wu, Mozaffar Shakeri, Xia Zhang, Bingsen Zhang

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  13. Insight into the Competitive Adsorption Behavior of Polymer Chains in Silica Nanopores by Small-Angle Neutron Scattering

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  14. Catalytic Upcycling of Polyolefins

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  15. The role of size and structure of catalytic active sites in polyolefin hydrogenolysis

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    Jueun Kim, Simin Sun, Donghyeon Kim, Byung Gwan Park, Hojeong Lee, Wenyu Huang, Kwangjin An

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  16. Interfacial Reactions in Chemical Recycling and Upcycling of Plastics

    ACS Applied Materials & Interfaces · 2024-08-30

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  17. Ultra‐Narrow Alkane Product Distribution in Polyethylene Waste Hydrocracking by Zeolite Micro‐Mesopore Diffusion Optimization

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  18. Ultra‐Narrow Alkane Product Distribution in Polyethylene Waste Hydrocracking by Zeolite Micro‐Mesopore Diffusion Optimization

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  19. Ultrathin Porous Carbon Nitride Anchored with Pt Nanoclusters for Synergistic Enhancement of Hydrogen Production in Alkaline Photocatalytic Polyester Reforming

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  20. Upconversion Phosphor-Driven Photodegradation of Plastics

    Nano Letters · 2024-10-22

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  21. Efficient Hydrogenolysis of Consumer-Grade High-Density Polyethylene Wastes over MgAl-Layered Double Oxide-Supported Ru Catalysts

    ACS Sustainable Chemistry & Engineering · 2024-11-20

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  22. Challenges and opportunities in catalytic hydrogenolysis of oxygenated plastics waste: polyesters, polycarbonates, and epoxy resins

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  23. Heterogeneous catalysis strategies for polyolefin plastic upcycling: co-reactant-assisted and direct transformation under mild conditions

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  24. Co-upcycling of mixed polypropylene and polyesters

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  25. Selectivity control by zeolites during methanol-mediated CO 2 hydrogenation processes

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  27. Synergistic effect of acidic sites and mesoporous confinement in Ce-doped Ru/SBA-15 catalysts for efficient hydrogenolysis of low-density polyethylene to liquid fuels

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  28. Conversion of Polypropylene to Light Olefins by HMFI Catalysts below Pyrolytic Temperature: Catalytic, Spectroscopic, and Theoretical Studies

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  29. Tandem Catalysis for Plastic Depolymerization: In Situ Hydrogen Generation via Methanol Aqueous Phase Reforming for Sustainable Polyethylene Hydrogenolysis

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  30. Tandem Catalysis for Plastic Depolymerization: In Situ Hydrogen Generation via Methanol Aqueous Phase Reforming for Sustainable Polyethylene Hydrogenolysis

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  31. Effective Methane Suppression in Upcycling of Polyethylene into Fuels via Alloying Platinum with Ruthenium Supported on ZSM-5 Zeolite

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  32. Hydrocarbon Deposition during Polyolefin Upcycling: Irreversible Adsorption and Surface Reactions of Polyethylene and Ethylene Oligomers on Silica Supports

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  33. Upgrading polyolefin plastics: experiences from petroleum refining and distinct characteristics

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  34. Engineering porous Beta zeolite-encapsulated nickel catalyst for waste polyolefins upcycling

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  35. Synergistic Co‐Recycling: Selective Oxidation of Polyethylene to Dicarboxylic Acids over Spent LiCoO 2 Cathodes

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  36. Synergistic Co‐Recycling: Selective Oxidation of Polyethylene to Dicarboxylic Acids over Spent LiCoO 2 Cathodes

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  37. Enhancing Waste Plastic Hydrogenolysis on Ru/CeO 2 Through Concurrent Incorporation of Fe Single Atoms and FeO x Nanoclusters

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  39. Population Balance Models for Catalytic Depolymerization: From Elementary Steps to Multiphase Reactors

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  40. Hydrocracking of Polypropylene to Light Alkanes over HMFI Zeolite Catalysts under H 2

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  41. Methods for Carbon Mass Closure in Polyolefin Hydrocracking

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  42. Chemical recycling of polyethylenes with low gas products by catalytic hydrogenolysis with heterogeneous CeO2-supported Cu-doped Ru catalyst

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  43. Polymer Upcycling by Catalytic Hydrogenolysis: The Role of Polyolefin Short-Chain Branching

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  44. In-situ encapsulation synthesis of Ni-Ce/SBA-15 by EISA for promoting CO2 methanation

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  45. Orchestrating catalytic hotspots and macromolecular architectures: molecular engineering toward zero-waste polymer circularity

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  46. Molar-Mass-Dependent Partitioning of Polyethylene in Nanopores of Model Catalyst Supports from Small-Angle Neutron Scattering

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  47. Advancing chemical recycling for waste plastic conversion

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  49. Plasma Catalysis for Plastic Waste Conversion into Value‐Added Products: Advancements and Perspectives

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  50. Chemical recycling of polycarbonate waste into advanced aviation fuel candidates via nickel–oxygen vacancy dual sites

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