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RESEARCH PAPER · ACS Catalysis · 2025

Synergistic Catalysis for Recycling and Upcycling of Plastics

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Synergistic Catalysis for Recycling and Upcycling of PlasticsOriginalIn-situ capture and upgrading of carbonate and aromatic units during PC depolymerization: from environmental crisis to circular opportunity5Solar‐Driven Plastic Upcycling Coupled with Valuable Reduction Reactions3NbOx-Based Catalysts for Biomass Conversion: Progress in the Past 20 Years18Plasma catalytic hydrogenolysis of polyethylene to gasoline-range fuels over Sm/USY catalysts10Toward Sustainable Plastic Waste Valorization: Green Synergistic Catalytic Strategies for Plastic Upcycling12Degradation and utilization of polyvinyl chloride (PVC): Challenges and opportunities toward a circular economy24Mechanistic insights into plastic degradation via catalytic bond breaking: a comprehensive review1Chemoselective depolymerization of polyurethane via solvent-engineered glycolysis0Key components for realistic application of plastic photoreforming coupled with H2 evolution9Tuning ruthenium states for enhanced polyethylene hydroconversion over HZSM-5 catalysts0Dendritic mesoporous silica nanospheres supported NiCo bimetallic catalysts for efficient cleavage of CC with formic acid for lignin depolymerization2Acid sites in hydrogen-involved polyolefin upcycling: mechanistic insights and design principles0Stepwise hydrogen spillover–engineered synergistic sites enable near-quantitative conversion of waste PET to p-xylene10Long-Chain Branched α-Alkenes from Plastic Upcycling Using Mo 2 C–Zn Nanoclusters Embedded on Hierarchical Porous Carbon1Prospective future of zeolites – From molecular to systems level2Inverse Al-ZrO 2 /Cu Catalysts Enable the On-Purpose Production of Separable Para -Xylene and Ethylene Glycol from PET Wastes7Catalytic Upcycling of Polyolefins and Polystyrene: Integrating Active Site Design With Mass Transfer Considerations4Precision bond cleavage in waste plastics: Directed catalytic upcycling1Dynamic coordination transformation from single-to dual-metal sites in MOFs for cascaded photoreforming of plastics into CO1Single-Atom Nickel Dispersed on Mo 2 TiC 2 T x MXene for Upcycling of Polyolefins via Catalytic Hydropyrolysis for Fuels and Lubricants0Photo‐ and Electrocatalytic Waste PET Plastic to Valuable Chemicals: Catalyst Engineering and Reaction Mechanism6Synergy Between Ru 3 Nanoclusters and Pt Nanoparticles for High‐Efficiency Alkaline Hydrogen Evolution Reaction0Synergy Between Ru 3 Nanoclusters and Pt Nanoparticles for High‐Efficiency Alkaline Hydrogen Evolution Reaction2Well‐Defined Heterocatalysts for Plastic Upcycling: From Design to Applications3Stepwise Hydrodeoxygenation of Mixed Oxygenated Plastics Enables Sequential Production of Jet- and Gasoline-Range Fuels0Stabilizing single-atom Ni on an Al2O3/N-C composite for efficient H2 production from polypropylene via pyrolysis-catalytic reforming0Spatially orthogonal CeOx-Zn sites on diatomite-aerogel-derived hierarchical HZSM-5 enable gated dechlorination and BTX-selective upcycling of PVC/PET mixed plastics0Mechanochemical AlCl3-Catalyzed Cracking of Waste Polyolefins and Synthetic Rubbers into Liquid Fuel0Atomically dispersed cerium enabling mild polyolefin hydrocracking to simple gas streams0Unlocking the Catalytic Potential of PFAS: Upcycling Forever Chemicals Into Effective Catalysts0Unlocking the Catalytic Potential of PFAS: Upcycling Forever Chemicals Into Effective Catalysts0Defect-Engineered Pd/ZSM-5 for Hydroconversion of LDPE to Light Alkanes0Fe–Ca‐Catalyzed Conversion of Cellulose Into Highly Ordered Graphitic Carbon Revealed by Solid‐State 1 3 C NMR and Mössbauer Spectroscopy0In Situ Hydrogen Utilization in Plastic Waste Recycling and Upcycling0Artificial Photoreforming Technology for Plastic Waste Valorization0

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  1. In-situ capture and upgrading of carbonate and aromatic units during PC depolymerization: from environmental crisis to circular opportunity

    中国科学通报:英文版 · 2025-08-18

    Minghao Zhang, Zhizheng Wu, Jun Guan, Qingqing Mei

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  2. Solar‐Driven Plastic Upcycling Coupled with Valuable Reduction Reactions

    Advanced Sustainable Systems · 2025-08-20

    Xiang Gao, Longfei Hong, Huiyan Zhang, Sheng Chu

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  3. NbOx-Based Catalysts for Biomass Conversion: Progress in the Past 20 Years

    ACS Catalysis · 2025-08-26

    Yaxuan Jing, Xiaohui Liu, Qineng Xia, Lin Dong, Yong Quan Guo, Yanqin Wang

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  4. Plasma catalytic hydrogenolysis of polyethylene to gasoline-range fuels over Sm/USY catalysts

    Applied Catalysis B: Environmental · 2025-09-08

    Chengxin Hou, Yanan Diao, Tianqi Yun, Jianhui Han, Tianhao Shi, Bingbing Chen, Chuan Shi

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  5. Toward Sustainable Plastic Waste Valorization: Green Synergistic Catalytic Strategies for Plastic Upcycling

    Advanced Sustainable Systems · 2025-10-10

    Luyao Zhang, Junliang Chen, Jinzhou Li, Jing Wu, Pin Gao, Jianping Yang

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  6. Degradation and utilization of polyvinyl chloride (PVC): Challenges and opportunities toward a circular economy

    Green Energy & Environment · 2025-10-28

    Rui Huang, Jiaolong Meng, Xuefeng Jiang

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  7. Mechanistic insights into plastic degradation via catalytic bond breaking: a comprehensive review

    European Polymer Journal · 2025-12-19

    Mengxia Ren, Hao Liu, Hao Liu, Zhen Yu, Zhaobin Tang, Yanlin Liu

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  8. Chemoselective depolymerization of polyurethane via solvent-engineered glycolysis

    RSC Advances · 2026-01-01

    Sajid Hussain

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  9. Key components for realistic application of plastic photoreforming coupled with H2 evolution

    CHINESE JOURNAL OF CATALYSIS (CHINESE VERSION) · 2026-01-01

    Jinpeng Zhang, Teng Liang, Jaenudin Ridwan, Chen Tian, Elhussein M. Hashem, Meijun Guo, Amin Talebian‐Kiakalaieh, Le Yu, Ping She, Jingrun Ran

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  10. Tuning ruthenium states for enhanced polyethylene hydroconversion over HZSM-5 catalysts

    Chemical Communications · 2026-01-01

    Zeyuan Zhu, Junhong Liu, Hongyu Wang, Qiao Hu, Dong Liang, Ling Zhang, Zhichao Tao, Jiajing Pei, Xi Liu, Liwei Chen

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  11. Dendritic mesoporous silica nanospheres supported NiCo bimetallic catalysts for efficient cleavage of CC with formic acid for lignin depolymerization

    Chemical Engineering Journal · 2026-01-16

    Chang Li, Hongzhi Luo, Chunhui Zhou, Haiping Chen, Yishuang Wang, Shihai Yang, Chenhuan Nie, Defang Liang, Mingqiang Chen

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  12. Acid sites in hydrogen-involved polyolefin upcycling: mechanistic insights and design principles

    Science China Chemistry · 2026-01-27

    Qi Zhang, Xiang Wang

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  13. Stepwise hydrogen spillover–engineered synergistic sites enable near-quantitative conversion of waste PET to p-xylene

    Nature Communications · 2026-01-28

    Wenyi Ni, Hongshun Ran, Rui Wang, Yifan Liu, Zhou Pa, Tao Guo, Junjie Shan, Zhuangzhuang Lai, Beibei Liu, S. Liang, Feng Miao, Xinyi Cui, Yaxuan Jing

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  14. Long-Chain Branched α-Alkenes from Plastic Upcycling Using Mo 2 C–Zn Nanoclusters Embedded on Hierarchical Porous Carbon

    Nano Letters · 2026-02-10

    Yuan Jiang, Guanyu Zhang, Qing Cheng, Ge Kong, Xin Zhang, Xin Zhang, Chun Shan, Fangqi Liu, Jin Wang, Tianqi Cao, Xuesong Zhang, Xuesong Zhang, Lujia Han

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  15. Prospective future of zeolites – From molecular to systems level

    Catalysis Today · 2026-02-12

    David Bajec, Gleb Veryasov

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  16. Inverse Al-ZrO 2 /Cu Catalysts Enable the On-Purpose Production of Separable Para -Xylene and Ethylene Glycol from PET Wastes

    Journal of the American Chemical Society · 2026-03-13

    Zehui Sun, Kaizhi Wang, Chen Chen, Mugeng Chen, Xin Chen, Fan Yang, Y P Liu, Heyong He, Yong Cao

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  17. Catalytic Upcycling of Polyolefins and Polystyrene: Integrating Active Site Design With Mass Transfer Considerations

    ChemSusChem · 2026-03-29

    Xinlei Han, Jie Sun, Jiuxuan Zhang, Zhengyan Qu, Hong Jiang, Zhenchen Tang, Rui Chen

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  18. Precision bond cleavage in waste plastics: Directed catalytic upcycling

    Renewable and Sustainable Energy Reviews · 2026-04-25

    Yusong Zhang, Yinxiang Wang, Aimin Li

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  19. Dynamic coordination transformation from single-to dual-metal sites in MOFs for cascaded photoreforming of plastics into CO

    CHINESE JOURNAL OF CATALYSIS (CHINESE VERSION) · 2026-05-01

    Jian Li, Zhenfa Wu, Xinru Zhang, Tongan Yan, Jin Luo, Wenjuan Xue, Zhaolin Lv, Hongliang Huang, Chongli Zhong

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  20. Single-Atom Nickel Dispersed on Mo 2 TiC 2 T x MXene for Upcycling of Polyolefins via Catalytic Hydropyrolysis for Fuels and Lubricants

    Precision Chemistry · 2026-05-01

    Jonathan Tjioe, Wei-Ling Huang, Harish Radhakrishnan, Ruoyu Cui, Yuting Li, Alex Gatiba, Tao Ma, Dapeng Jing, Long Hao Qi, Jeffrey T. Miller, Xianglan Bai, Yue Wu

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  21. Photo‐ and Electrocatalytic Waste PET Plastic to Valuable Chemicals: Catalyst Engineering and Reaction Mechanism

    Advanced Functional Materials · 2026-05-13

    Yu Zheng, Xiaohui Tang, Yanxi Qi, Shengbo Zhang, Na Ji

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  22. Synergy Between Ru 3 Nanoclusters and Pt Nanoparticles for High‐Efficiency Alkaline Hydrogen Evolution Reaction

    Angewandte Chemie · 2026-05-15

    Xiuting Fu, Xuxin Kang, Ruhao Wang, Zhenfei Zhang, Ruicong Chen, Youqi Zhu, Xiangmei Duan, Haifeng Jiang, Dingsheng S. Wang, Shubo Tian

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  23. Synergy Between Ru 3 Nanoclusters and Pt Nanoparticles for High‐Efficiency Alkaline Hydrogen Evolution Reaction

    Angewandte Chemie International Edition · 2026-05-15

    Xiuting Fu, Xuxin Kang, Ruhao Wang, Zhenfei Zhang, Ruicong Chen, Youqi Zhu, Xiangmei Duan, Haifeng Jiang, Dingsheng S. Wang, Shubo Tian

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  24. Well‐Defined Heterocatalysts for Plastic Upcycling: From Design to Applications

    Advanced Materials · 2026-05-22

    Minhao Tang, Ji Shen, Zhimin Liu

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  25. Stepwise Hydrodeoxygenation of Mixed Oxygenated Plastics Enables Sequential Production of Jet- and Gasoline-Range Fuels

    Environmental Science & Technology · 2026-06-16

    Yue Zhu, Zhouying Mao, Pengfei An, Buxing Han, Qingqing Mei

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  26. Stabilizing single-atom Ni on an Al2O3/N-C composite for efficient H2 production from polypropylene via pyrolysis-catalytic reforming

    Journal of Analytical and Applied Pyrolysis · 2026-07-20

    Dexin Kong, Rui Shan, Shuxiao Wang, Hui Li, Haoran Yuan, Yong Chen

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  27. Spatially orthogonal CeOx-Zn sites on diatomite-aerogel-derived hierarchical HZSM-5 enable gated dechlorination and BTX-selective upcycling of PVC/PET mixed plastics

    Applied Catalysis B: Environmental · 2026-09-04

    Jie Li, Yuxiang Yang, Guangtong Xu, Xiangxu Du, Anbang Dai, Yangchuan Ke

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  28. Mechanochemical AlCl3-Catalyzed Cracking of Waste Polyolefins and Synthetic Rubbers into Liquid Fuel

    ACS Sustainable Chemistry & Engineering · 2026-09-07

    Xiaojuan Zhao, Lizheng Chen, Wenjuan Zhang, Gang Liu, Dayang Wang

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  29. Atomically dispersed cerium enabling mild polyolefin hydrocracking to simple gas streams

    Journal of Energy Chemistry · 2026-09-11

    Yüe Zhao, Yue Wu, Biao Meng, WeiHao Guan, Qizhi Hu, Jiameng Gao, Qihong Yue, Xiaoling Liu, Jun Wang, Yu Ting Zhou

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  30. Unlocking the Catalytic Potential of PFAS: Upcycling Forever Chemicals Into Effective Catalysts

    Angewandte Chemie · 2026-09-22

    Mengying Zheng, Pengfei Zhou, Kangjun Zhou, Hongshun Ran, Wenyi Ni, Yifan Liu, Xinyi Cui, Yaxuan Jing

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  31. Unlocking the Catalytic Potential of PFAS: Upcycling Forever Chemicals Into Effective Catalysts

    Angewandte Chemie International Edition · 2026-09-22

    Mengying Zheng, Pengfei Zhou, Kangjun Zhou, Hongshun Ran, Wenyi Ni, Yifan Liu, Xinyi Cui, Yaxuan Jing

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  32. Defect-Engineered Pd/ZSM-5 for Hydroconversion of LDPE to Light Alkanes

    ACS Sustainable Chemistry & Engineering · 2026-09-26

    Yi Lu, Tiancheng Fang, Jiankun Yang, Yanshuang Zhang, Jun Wan, Hui Lan, Yongtao Wang, Zidi Yan, Yunbo Yu, Yunbo Yu, Hong He

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  33. Fe–Ca‐Catalyzed Conversion of Cellulose Into Highly Ordered Graphitic Carbon Revealed by Solid‐State 1 3 C NMR and Mössbauer Spectroscopy

    Chemistry - A European Journal · 2026-10-06

    Shamala Gowri Krishnan, Yannick Coppel, Jean‐François Meunier, Ange Nzihou

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  34. In Situ Hydrogen Utilization in Plastic Waste Recycling and Upcycling

    ACS Catalysis · 2026-10-06

    Xinyang Sun, Hongshun Ran, Tao Guo, Yaxuan Jing

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  35. Artificial Photoreforming Technology for Plastic Waste Valorization

    Advanced Materials · 2026-10-07

    Haiyin Zhan, Guanqi Yu, Xiangkun Jia, Wei Liu, Sihui Zhan

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