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RESEARCH PAPER · Chem · 2022

Catalytic strategies for upvaluing plastic wastes

Meiqi Zhang, Meng Wang, Bo Sun, Chaoquan Hu, Dequan Xiao, Ding Ma

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Catalytic strategies for upvaluing plastic wastesOriginalRecent progress in photoelectrocatalysis beyond water oxidation46Catalytic hydroconversion processes for upcycling plastic waste to fuels and chemicals94Advancements in catalysis for plastic resource utilization21Selective oxidative upgrade of waste polystyrene plastics by nitric acid to produce benzoic acid43Ultrafast and Selective Chemical Recycling of Pla to Methyl Lactate by Using Mhmds as Facile Catalysts0Converting Plastic Wastes to Naphtha for Closing the Plastic Loop187Valorization of waste biodegradable polyester for methyl methacrylate production111Ultrafast activation of Ni foam by electro-corrosion and its use for upcycling PBT plastic waste57Solvent‐Free Heterogeneous Catalytic Hydrogenation of Polyesters to Diols48Solvent‐Free Heterogeneous Catalytic Hydrogenation of Polyesters to Diols6Photothermal Catalysis: An Emerging Green Approach to Upcycling Plastic Waste39Upcycling contaminated plastics21Novel catalysts in catalytic upcycling of common polymer wastes26Sustainable developments in polyolefin chemistry: Progress, challenges, and outlook204Direct catalytic plastics waste upcycling7Heterogeneous Photocatalytic Oxidative Cleavage of Polystyrene to Aromatics at Room Temperature76Processing Plastic Wastes into Value-Added Carbon Adsorbents by Sulfur-Based Solvothermal Synthesis14Molecular oxygen-assisted in defect-rich ZnO for catalytic depolymerization of polyethylene terephthalate25Integrated Photochromic‐Photothermal Processes for Catalytic Plastic Upcycling17Integrated Photochromic‐Photothermal Processes for Catalytic Plastic Upcycling84Recent advances on solar-driven valorization of polyethylene terephthalate plastics into value-added chemicals14In Situ Construction of an Intramolecular Donor–Acceptor Conjugated Copolymer via Terephthalic Acid Derived from Plastic Waste for Photocatalysis of Plastic to Hydrogen Peroxide43Aromatization of HDPE and PP over Ga-promoted zeolite: Effects of pretreatment and zeolite type11Chemical recycling of plastic wastes with alkaline earth metal oxides: A review39Highly Efficient Depolymerization of Waste Polyesters Enabled by Transesterification/Hydrogenation Relay Under Mild Conditions4Highly Efficient Depolymerization of Waste Polyesters Enabled by Transesterification/Hydrogenation Relay Under Mild Conditions87From Plastic Waste to Treasure: Selective Upcycling through Catalytic Technologies100Quantifying synergy for mixed end-scission and random-scission catalysts in polymer upcycling12Solar-driven photocatalysis for recycling and upcycling plastics122Stapler Strategies for Upcycling Mixed Plastics0Mixed Plastics Wastes Upcycling with High-Stability Single-Atom Ru Catalyst188Recent Advances in the Functionalized Poly(α-Hydroxy Acids) Synthesized fromO-Carboxyanhydrides4Electrocatalytic Waste-Treating-Waste Strategy for Concurrently Upgrading of Polyethylene Terephthalate Plastic and CO 2 into Value-Added Formic Acid134Dual Photo‐Responsive Diphenylacetylene Enables PET In‐Situ Upcycling with Reverse Enhanced UV‐Resistance and Strength3Dual Photo‐Responsive Diphenylacetylene Enables PET In‐Situ Upcycling with Reverse Enhanced UV‐Resistance and Strength51Catalytic depolymerization of polyester plastics toward closed-loop recycling and upcycling127Excavating the Potential of Photo‐ and Electroupcycling Platforms Toward a Sustainable Future for Waste Plastics11Chemical recycling of plastic wastes via homogeneous catalysis: A review78The thermodynamics and kinetics of depolymerization: what makes vinyl monomer regeneration feasible?98Precise activation of C–C bonds for recycling and upcycling of plastics81Synthesis of bio-based polyesters from carvone-derived epoxides3Recent advancement on photocatalytic plastic upcycling90Monomer recycling of polyethylene terephthalate, polycarbonate and polyethers: Scalable processes to achieve high carbon circularity62Advances in solar-driven, electro/photoelectrochemical, and microwave-assisted upcycling of waste polyesters15Beyond biodegradation: upcycling of polylactic acid plastic waste into amino acids via cascade catalysis under mild conditions60Self-supported Ni/Ni 3 N 1− x heterostructures with abundant nitrogen vacancies as efficient electrocatalysts for ethylene glycol oxidation23Selective Upcycling of Polyethylene Terephthalate towards High‐valued Oxygenated Chemical Methyl p‐Methyl Benzoate using a Cu/ZrO2 Catalyst94Selective Upcycling of Polyethylene Terephthalate towards High‐valued Oxygenated Chemical Methyl p‐Methyl Benzoate using a Cu/ZrO2 Catalyst5Solvent-Promoted Catalyst-Free Recycling of Waste Polyester and Polycarbonate Materials39One-Pot Conversion of Polyester and Carbonate into Formate without External H240A Unified View of Carbon Neutrality: Solar-Driven Selective Upcycling of Waste Plastics30Catalytic conversion of mixed polyolefins under mild atmospheric pressure48Population Balance Equations for Reactive Separation in Polymer Upcycling20Upcycling Waste Plastics with a C–C Backbone by Heterogeneous Catalysis45Ultrafast and selective chemical recycling of PLA to methyl lactate by using MHMDS as simple catalysts18Chemical recycling of waste plastics: Current challenges and perspectives37Tandem catalysis enables chlorine-containing waste as chlorination reagents48Polymeric Carbon Nitride Nanosheets as a Metal‐Free Heterogeneous Catalyst for Highly Efficient Methanolysis of Polycarbonates14Closed‐Loop Polymer‐to‐Polymer Upcycling of Waste Poly (Ethylene Terephthalate) into Biodegradable and Programmable Materials27Perspectives on sustainable plastic treatment: A shift from linear to circular economy39High-efficiency Ce-modified ZSM-5 nanosheets for waste plastic upgrading43Electro-Reforming of PET Plastic to C 2 Chemicals with Concurrent Generation of Hydrogen and Electric Energy188Grave-to-cradle photothermal upcycling of waste polyesters over spent LiCoO2111Rethinking Chlorinated Plastic: Can Direct Upcycling of Mixed Plastic Wastes Surpass Preseparation?2Nanomaterials for the Catalytic Degradation and Detection of Microplastics: A Review31Micelles Cascade Assembly to Tandem Porous Catalyst for Waste Plastics Upcycling3Micelles Cascade Assembly to Tandem Porous Catalyst for Waste Plastics Upcycling50Brønsted-acid sites induced photocatalytic cracking of low-polarity polyethylene plastics17Iron‐Catalyzed Oxidative Deconstruction of Polyethylene Terephthalate to Terephthalic Acid under O223Advancements and future directions in waste plastics recycling: From mechanical methods to innovative chemical processes136Navigating the hydrogen prospect: A comprehensive review of sustainable source-based production technologies, transport solutions, advanced storage mechanisms, and CCUS integration92Chemical Upcycling of Polyolefin Plastics Using Structurally Well-defined Catalysts35Closed‐Loop Recycling of Mixed Plastics of Polyester and CO2‐Based Polycarbonate to a Single Monomer33Closed‐Loop Recycling of Mixed Plastics of Polyester and CO2‐Based Polycarbonate to a Single Monomer3Progress and Perspective for “Green” Strategies of Catalytic Plastics Conversion into Fuels by Regulating Half-Reactions102Ir(triNHC)‐Catalyzed Upcycling of Waste PET for Lactic Acid Production with Sustainable Isolation via Bipolar Membrane Electrodialysis5Ir(triNHC)‐Catalyzed Upcycling of Waste PET for Lactic Acid Production with Sustainable Isolation via Bipolar Membrane Electrodialysis9Sustainable upcycling of waste polyethylene terephthalate into hierarchically porous carbon nanosheet for interfacial solar steam and hydroelectricity generation17Stapler Strategies for Upcycling Mixed Plastics49Amide wax-assisted interfacial compatibilization of maleic anhydride-grafted polyethylene for high-performance wood-plastic composites2Advancing Recyclable Thermosets through C═C/C═N Dynamic Covalent Metathesis Chemistry36Co-upcycling of Plastic Waste and Biowaste via Tandem Transesterification Reactions10Electrocatalytic upcycling of plastic waste: Progress, challenges, and future53One-Step Upcycling the Engineering Plastic of Polyoxymethylene toward a Flowing Telechelic Polyester: From Poly(A) to Poly(A-alt-B)4Catalytic Upcycling of Polyolefins316Energy‐Saving Ambient Electrosynthesis of Nylon‐6 Precursor Coupled with Electrocatalytic Upcycling of Polyethylene Terephthalate15Oxidative degradation and upcycling of polyethylene wastes40Catalytic recycling of plastics into value-added products28The interaction between sludge and microplastics during thermal hydrolysis of sludge13Grave-to-cradle dry reforming of plastics via Joule heating64Potential cycling boosts the electrochemical conversion of polyethylene terephthalate-derived alcohol into valuable chemicals79Simultaneous electrochemical upgrading of polyethylene terephthalate plastic and carbon dioxide into valuable chemicals31Noble metal-free tandem catalysis enables efficient upcycling plastic waste into liquid fuel components22Exploring enzymatic degradation, reinforcement, recycling, and upcycling of poly(ester)-poly(urethane) with movable crosslinks20Upcycling of polyolefins into detergents2Highly active cobalt oxide-palladium nanohybrid catalyst enables selective electrocatalytic synthesis of glycolic acid21Photocatalytic Perception for Degradation of Macro- and Micro-plastics2Challenges and opportunities in catalytic hydrogenolysis of oxygenated plastics waste: polyesters, polycarbonates, and epoxy resins44Chemical transformation of polyurethane into valuable polymers26Accurately tuning the pore size and acidity of mesoporous zeolites for enhancing the catalytic hydrocracking of polypropylene24Aerobic oxidation of alkylarenes and polystyrene waste to benzoic acids via a copper-based catalyst28Recent Progress for Designing of Catalysts for Photothermal Conversion of Plastic Wastes48Photoreforming of Plastic Waste to Sustainable Fuels and Chemicals: Waste to Energy59Research progress and challenges in the upcycling of polyolefin plastics through chemical oxidation4A pair of strongly reductive and oxidative photocatalysts for the general upcycling of biomass derivatives and plastic wastes12Boosting the hydrodeoxygenation of PET waste to cycloalkanes by electron transfer and hydrogen spillover in H x WO 3− y incorporated dendritic fibrous nanosilica supported Ni catalysts15Chemical degradation and recycling of polyethylene terephthalate (PET): a review107g-C 3 N 5 -based photocatalysts for energy and environmental applications: insights into properties, structural modifications, challenges, and future directions24Hydrogenation-induced selective degradation of PET wastes8Innovative recycling strategies for non-recycled plastics: advancing the circular economy for a sustainable future22Synergistic effect of acidic sites and mesoporous confinement in Ce-doped Ru/SBA-15 catalysts for efficient hydrogenolysis of low-density polyethylene to liquid fuels7Thermodynamically leveraged solventless aerobic deconstruction of polyethylene-terephthalate plastics over a single-site molybdenum-dioxo catalyst12Tunable Syngas Production from Photocatalytic PET Reforming over TiO2/CdZnS S-Scheme Heterojunction0Catalytic conversion of polyolefins to aromatics by ultra-thin b-axis oriented ZSM-5 zeolite1Nitrogenative Degradation of Polystyrene Waste44Recyclable Zinc Cyanamide Dual-Site Catalyst Enables Efficient PET Glycolysis11Ionic Liquid–Catalyzed Recycling of Spent Polymers0Recycling homocarbon backbone polymers toward a circular materials economy12Preparation of Al2O3 Nanoparticles via Fluidized Roasting and Their Application in the Pyrolysis of Spent Mulching Film for Hydrocarbon Production4Morphology Optimization of Spinel Catalysts for High‐Efficiency Photothermal Catalytic Upcycling of Polyethylene Terephthalate47Electronic Configuration‐Modulated Dual‐Active Nanocomposite NiAlOx for Promoting Plastic‐To‐Green Hydrogen9Selective Asymmetric Hydrogenation of Waste Polyethylene Terephthalate via Controlled Sorption through Precisely Tuned Moderate Acid Sites50Cold plasma-assisted co-conversion of polyolefin wastes and CO2 into aromatics over hierarchical Ga/ZSM-5 catalyst24Multicomponent Polymerizations Provide Sustainable Sulfur (Selenium)-Containing Polyesters10One-Pot Conversion of Polyethylene Terephthalate into 1,4-Cyclohexanedicarboxylic Acid without External H219Advances in Solar-Driven, Electro/Photoelectrochemical, and Photothermal-Assisted Upcycling of Waste Plastics10Advances in catalytic transformations of waste plastic resources with zeolites0Synthesis of Graft‐Modified Polyolefin Compatibilizers for Compatibilizing Mixed Plastics8Recent advances in pyrolysis upcycling of waste plastics into hydrocarbon fuels on biochar-based catalysts28Co-recycling of plastics and other waste materials70Microwave-Assisted Catalytic Upcycling of Plastic Wastes over Heterojunction-Structured Layered Triple Oxides8Synergistic Catalysis for Recycling and Upcycling of Plastics35Lattice and electronic structural engineering toward PET waste upcycling over PVP-incorporated Ni(OH)219Photocatalytic Hydrogen Evolution Driven by Advanced Metal Sulfides from Sustainable Multilevel Biomass and Waste Plastics51Recent Advances in the Thermo-Catalytic Upcycling of Polyethylene Waste13Ambient solar thermal catalysis for polyolefin upcycling using copper encapsulated in silicon nanosheets and chloroaluminate ionic liquid32Mechanistic Insight into the Role of Bi in Bi-rich PdBi Alloy Structure for Promoting Electrocatalytic Upcycling of Polyethylene Terephthalate Plastics into Formate4Recent advances in hydrogen production by solar photoreforming of plastic feedstocks using nanocatalytic materials: A review9Conversion of polyethylene terephthalate and ammonium polyphosphate into P/N-doped porous carbon nanobulks for efficient sulfadiazine degradation2Syngas from waste plastics and water using Joule heating19Addressing the plastic waste crisis: Advanced catalytic strategies for upcycling and fuel production6A catalytic approach to the valorization of polyesters and biogenic waste for the production of amines9Effects of Conduction Band Edge Regulation on the Photoreforming Efficiency of Plastic Waste: Taking BPNS/TiO 2 as a Photocatalyst21Recyclable Inorganic Subnanowire Plastics8Zinc oxide-mediated C H activation of polypropylene waste for thermochemical valorization1Ir(triNHC)-catalyzed upcycling of waste poly(butylene terephthalate) into biodegradable plastic2Catalytic Depolymerization of Plastics to Valuable Products7Upcycling Waste Polypropylene into Multifunctional Homogeneous Additives for Simultaneously Enhanced Mechanical Performance and Processability6A solid gelator from plastic waste for selectively and fast congealing liquid/gaseous chloroform2Catalytic Upcycling of PET: From Waste to Chemicals and Degradable Polymers48

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  5. Ultrafast and Selective Chemical Recycling of Pla to Methyl Lactate by Using Mhmds as Facile Catalysts

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  47. Selective Upcycling of Polyethylene Terephthalate towards High‐valued Oxygenated Chemical Methyl p‐Methyl Benzoate using a Cu/ZrO2 Catalyst

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  48. Selective Upcycling of Polyethylene Terephthalate towards High‐valued Oxygenated Chemical Methyl p‐Methyl Benzoate using a Cu/ZrO2 Catalyst

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  49. Solvent-Promoted Catalyst-Free Recycling of Waste Polyester and Polycarbonate Materials

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  50. One-Pot Conversion of Polyester and Carbonate into Formate without External H2

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