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RESEARCH PAPER · ACS Sustainable Chemistry & Engineering · 2021

Chemical Upcycling of Polyethylene to Value-Added α,ω-Divinyl-Functionalized Oligomers

Manhao Zeng, Yu‐Hsuan Lee, Garrett Strong, Anne M. LaPointe, Andrew L. Kocen, Zhiqiang Qu, Geoffrey W. Coates, Susannah L. Scott, Mahdi M. Abu‐Omar

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Chemical Upcycling of Polyethylene to Value-Added α,ω-Divinyl-Functionalized OligomersOriginalChemical Upcycling of Poly(3-hydroxybutyrate) into Bicyclic Ether–Ester Monomers toward Value-Added, Degradable, and Recyclable Poly(ether ester)45Chemically Recyclable Ester-Linked Polypropylene124Metathesis, molecular redistribution of alkanes, and the chemical upgrading of low-density polyethylene44Catalytic deconstruction of waste polyethylene with ethylene to form propylene419RETRACTED: Hydrogenolysis of Polyethylene and Polypropylene into Propane over Cobalt-Based Catalysts72Upcycling plastic waste into high value-added chemicals under mild conditions1Polyolefins Vitrimers: Design Principles and Applications108Catalytic Chemical Recycling of Post-Consumer Polyethylene188“Functional upcycling” of polymer waste towards the design of new materials226Functionalization of polyethylene with hydrolytically-stable ester groups6Heterogeneous Pt-catalyzed transfer dehydrogenation of long-chain alkanes with ethylene7Solvent-induced competing processes in polycarbonate degradation: depolymerization, chain scission, and branching/crosslinking12Tandem oxidative and thermal cracking of polypropylene at low temperatures21A comprehensive review of sustainable approaches for synthetic lubricant components67Upcycling of Polybutadiene Facilitated by Selenium‐Mediated Allylic Amination23Upcycling of Polybutadiene Facilitated by Selenium‐Mediated Allylic Amination4Waste PVC upcycling: Transferring unmanageable Cl species into value-added Cl-containing chemicals61Machine Learning and Informatics Based Elucidation of Reaction Pathways for Upcycling Model Polyolefin to Aromatics11Metal-catalyzed plastic depolymerization79Recent Advances in Catalytic Chemical Recycling of Polyolefins104Degradation of Polyvinyl Chloride by Sequential Dehydrochlorination and Olefin Metathesis26Polyethylene Incorporating Diels–Alder Comonomers: A “Trojan Horse” Strategy for Chemically Recyclable Polyolefins3Polyethylene Incorporating Diels–Alder Comonomers: A “Trojan Horse” Strategy for Chemically Recyclable Polyolefins87Sustainable developments in polyolefin chemistry: Progress, challenges, and outlook204α,ω-Diene Generation from Ethylene and Butadiene by Copolymer Upcycling6Hydrogen-free catalytic depolymerization of waste polyolefins at mild temperatures43Upcycling of polyethylenes by catalysis0Circular Polyolefins: Advances toward a Sustainable Future76Mechanistic Insights Enable Divergent Product Selectivity in Catalyst-Controlled Photooxidative Degradation of Polystyrene90Biodegradable polymers from lignocellulosic biomass and synthetic plastic waste: An emerging alternative for biomedical applications63Controlled degradation of chemically stable poly(aryl ethers) via directing group-assisted catalysis6Modern mechanistic approaches for the depolymerization of commodity plastics via organometallic catalysis0Significantly Tunable Foaming Behavior of Blowing Agent for the Polyethylene Foam Resin with a Unique Designed Blowing Agent System6Upcycling Waste Plastics with a C–C Backbone by Heterogeneous Catalysis45Synthesis and Deconstruction of Polyethylene-type Materials194Multi-color polymer carbon dots synthesized from waste polyolefins through phenylenediamine-assisted hydrothermal processing13Mechanism-Guided Discovery of Cleavable Comonomers for Backbone Deconstructable Poly(methyl methacrylate)44Progress and Challenges in Polystyrene Recycling and Upcycling87Deconstruction of Polymers through Olefin Metathesis101Hydrocarboxylation of C═C Bonds in Polycyclooctene: Progress Toward Valorization of Waste Polyolefins8Catalytic chemical recycling and upcycling of polyolefin plastics27Driving selective upcycling of mixed polyethylene waste with table salt11Designed to Degrade: Tailoring Polyesters for Circularity168Copolymerization of Olefins and Conjugated Dienes: A Promising Approach to Produce Recyclable Polyolefins14Catalytic Upcycling of Polyolefins316N2O deconstruction of polycyclooctene to generate carbonyl-functionalized macromonomers3Polyolefin melt-phase effects on alkane hydrogenolysis over Pt catalysts5Installing a Trigger to Upcycle High-Density Polyethylene42Incorporation of Thioacetate Pendants on a Polyalkenamer Enables High Extensibility3Two-step conversion of waste plastic into light olefins and aromatics on metal-free carbon felt catalyst under radiofrequency heating11Kinetic Models for Polymer Upcycling by Tag-and-Cut Strategies6From Waste to Worth: Upcycling Plastic into High-Value Carbon-Based Nanomaterials42Chemical upcycling of polybutadiene into size controlled α,ω-dienes and diesters via sequential hydrogenation and cross-metathesis14Recent developments in recycling of post-consumer polyethylene waste33Recyclable Polypentenamers with Precise Crystallization and Versatile Functionalization15Ruthenium‐Catalyzed Deconstruction of Polyolefins: A Strategy to Up‐cycle Waste Polyethylene to Value‐Added Alkene1Ruthenium‐Catalyzed Deconstruction of Polyolefins: A Strategy to Up‐cycle Waste Polyethylene to Value‐Added Alkene20Synthesis of Polyamides Bearing Directing Groups and Their Catalytic Depolymerization3Modulating Polyethylene Mimics with Degradability via Synthesis and Modeling22Emerging Biochemical Conversion for Plastic Waste Management: A Review8High Molecular Weight Biobased Long-Chain Aliphatic Polyesters with Degradability: Insights into Mimicking Polyethylene24Probing the Catalytic Degradation of Unsaturated Polyolefin Materials via Fe‐Based Lewis Acids‐Initiated Carbonyl–Olefin Metathesis18Probing the Catalytic Degradation of Unsaturated Polyolefin Materials via Fe‐Based Lewis Acids‐Initiated Carbonyl–Olefin Metathesis1Synthesis and Blending of Two Poly(ethylene-co-vinyl alcohol) Polymers with Mixed 1,2-Diol Stereochemistry3From Polyethylene to Conjugated Polyenes: a Mechanochemical One‐Pot Upcycling Strategy for Selective Functionalization1TsOH-assisted photocatalytic aerobic upcycling of polystyrene waste6A Review on Sustainable Upcycling of Plastic Waste Through Depolymerization into High-Value Monomer38Recyclable Biomass-Derived Polyethylene-like Plastics6Molar-Mass-Dependent Partitioning of Polyethylene in Nanopores of Model Catalyst Supports from Small-Angle Neutron Scattering2Sustainable polymers for battery applications7Advances in sustainable polyolefins: synthesis, chemical transformation and recycling23Tuning High-Density Polyethylene Microstructure and Properties from Known Distributions of Dynamic Bonds7Supported Organoiridium-Pincer Catalysts for the Nonoxidative Dehydrogenation of High-Density Polyethylene1Chemical Upcycling of Polybutadiene Into Polyolefin‐Based Dynamic Covalent Polymer Networks4Recent developments in recycling technologies for polymeric plastics8Carbon–carbon bond cleavage for lignin and plastics deconstruction0Electrophilic substitution in poly(ethylene terephthalate) waste for upcycling to functional metal–organic frameworks0Upcycling waste polyoxymethylene to value-added chemicals using reusable polymeric acid catalysts at ppm levels2Chemical Upcycling of Waste Chlorinated Plastics into α,ω-Dienes via Consecutive Dehydrochlorination-Hydrogenation with HCl Trapping and Metathesis1Olefin metathesis-driven deconstruction and upcycling of chloroprene rubber2Varying the Oxidative Functionalization of Polypropylene Films under Quiescent Conditions2Heterogeneous Transfer Dehydrogenation for Catalytic Upcycling of Polyethylene0Beyond Recycling: Vitrimer and Chemical Valorization Strategies for Thermoplastic Polyolefin Upcycling0Accessing Degradable Polyethylenes via Catalytic Ethylene Copolymerization1Recent advances in the directed degradation of polyolefins into oligomers0Pyrolysis of waste plastics in the rotary-kiln reactor2Ring-Opening Metathesis Polymerization of Caged FLP Monomers and Uncaged Alkene Macromonomers0Catalytic Hydrosilylation Deoxygenation: Synthesizing Polysiloxanes While Upcycling Polymers to Alkanes0Catalytic Hydrosilylation Deoxygenation: Synthesizing Polysiloxanes While Upcycling Polymers to Alkanes0A General Strategy for the Degradation of Nitrile-Containing Plastics and Rubbers via Nickel-Catalyzed Decyanation and Sequential Ethenolysis0From Dicyclopentadiene to Chemically Recyclable Polymeric Materials0Challenges in polyolefin re/upcycling catalysis specific to polymer feedstock0

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  5. RETRACTED: Hydrogenolysis of Polyethylene and Polypropylene into Propane over Cobalt-Based Catalysts

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  18. Machine Learning and Informatics Based Elucidation of Reaction Pathways for Upcycling Model Polyolefin to Aromatics

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