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RESEARCH PAPER · Advanced Materials · 2021

Synergistic Enzyme Mixtures to Realize Near‐Complete Depolymerization in Biodegradable Polymer/Additive Blends

Christopher DelRe, Boyce S. Chang, Ivan Jayapurna, Aaron Hall, Ariel Wang, Kyle Zolkin, Ting Xu

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Synergistic Enzyme Mixtures to Realize Near‐Complete Depolymerization in Biodegradable Polymer/Additive BlendsOriginalTrends in Polymer Degradation Across All Scales27Conductive Ink with Circular Life Cycle for Printed Electronics57Machine Learning on a Robotic Platform for the Design of Polymer–Protein Hybrids177Biofuel generation from food waste through immobilized enzymes on magnetic nanoparticles22Glass transition of random heteropolymers: A molecular dynamics simulation study in melt, in water, and in vacuum17Photocontrolled RAFT polymerization: past, present, and future290Recent advances in plastic recycling and upgrading under mild conditions147Sequence Design of Random Heteropolymers as Protein Mimics22Boosting Degradation of Biodegradable Polymers95Data-Driven Design of Polymer-Based Biomaterials: High-throughput Simulation, Experimentation, and Machine Learning109Nanomedicine-based treatment: An emerging therapeutical strategy for pulmonary hypertension7A Phase Engineering Strategy of Perovskite‐Type ZnSnO3:Nd for Boosting the Sonodynamic Therapy Performance43Solvent-Assisted Poly(lactic acid) Upcycling under Mild Conditions26Sequence Patterning, Morphology, and Dispersity in Single-Chain Nanoparticles: Insights from Simulation and Machine Learning33Probing the Effects of Antimicrobial‐Lysozyme Derivatization on Enzymatic Degradation of Poly(ε‐caprolactone) Film and Fiber9Protein modified cellulose nanocrystals on reinforcement and self-driven biodegradation of aliphatic polyester11High Thermal Stability of Enzyme-MOF Composites at 180 °C9Chemical Recycling of Polybutadiene Rubber with Tailored Depolymerization Enabled by Microencapsulated Metathesis Catalysts16Controlling the lifetime of biodegradable electronics: from dissolution kinetics to trigger acceleration21Designed to Degrade: Tailoring Polyesters for Circularity168Degradable living plastics programmed by engineered spores40Exploring biodegradable alternatives: microorganism-mediated plastic degradation and environmental policies for sustainable plastic management10Comparative studies on the effectiveness of proteases and enzymes from dietary supplements in the degradation of polylactide (PLA)8Practice and tactics in the construction of novel degradable plastics at polymer and molecular levels1Thermally and Base-Triggered “Debond-on-Demand” Chain-Extended Polyurethane Adhesives25Scalable nanoplastic degradation in water with enzyme-functionalized porous hydrogels21Enzymes offer a promising avenue for enhancing the competitiveness of biodegradable plastics in environmental restoration and the circular economy13Nanoplastics and microplastics released from an enzyme-embedded biodegradable polyester during hydrolysis20Targeted Upcycling of Poly(L‐lactide) Based on Stereocomplexation Technology0Simultaneous improvement of thermal stability, mechanical properties, and combustion safety in polycaprolactone via blending with a tiny amount of aramid nanofiber9Breaking Symmetry of Active Sites in Metal‐Organic Frameworks for Efficient Photocatalytic Valorization of Polyester Plastics5Breaking Symmetry of Active Sites in Metal‐Organic Frameworks for Efficient Photocatalytic Valorization of Polyester Plastics29Seeking Precise Protein-like Functions from Random Heteropolymer Ensemble and through Dimensionality Reduction9Random Heteropolymers Enable Nonspecific Protein Binding and Loop-Mediated Stabilization4Integrating chemical and biological conversion for waste plastics recycling and upcycling toward a circular bioeconomy0Poly(butylene adipate- co -terephthalate) with synergistically enhanced mechanical, moisture/oxygen barrier, and degradation performance via embedding immobilized enzyme0Recent advances in designing high-performance and enzymatically degradable plastics0Understanding Solvent-Induced Glass Transition in Polymer Thin Films Using Absorption–Desorption Isotherms1Computational design of functional random heteropolymers through atomistic simulations0Upcycling of polyethylene waste to biodegradable polyesters via oxidative conversion1Emerging Trends in Smart Nanozymes for Microplastic/Nanoplastic Remediation: Mechanistic Insights and Food System Applications0Degradable Living Plastics Programmed by Engineered Microbial Consortia0

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  1. Trends in Polymer Degradation Across All Scales

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    Juliet Veskova, Federica Sbordone, Hendrik Frisch

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  2. Conductive Ink with Circular Life Cycle for Printed Electronics

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    Junpyo Kwon, Christopher DelRe, Philjun Kang, Aaron Hall, Daniel P. Arnold, Ivan Jayapurna, Le Ma, Matthew Michalek, Robert O. Ritchie, Ting Xu

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  3. Machine Learning on a Robotic Platform for the Design of Polymer–Protein Hybrids

    Advanced Materials · 2022-05-20

    Matthew Tamasi, Roshan A. Patel, Carlos H. Borca, Shashank Kosuri, Heloise Mugnier, Rahul Upadhya, N. Sanjeeva Murthy, Michael E. Webb, Adam J. Gormley

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  4. Biofuel generation from food waste through immobilized enzymes on magnetic nanoparticles

    Materials Today Proceedings · 2022-06-06

    Pranay Amruth Maroju, Ramakrishnan Ganesan, Jayati Ray Dutta

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  5. Glass transition of random heteropolymers: A molecular dynamics simulation study in melt, in water, and in vacuum

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  6. Photocontrolled RAFT polymerization: past, present, and future

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  7. Recent advances in plastic recycling and upgrading under mild conditions

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    Shengbo Zhang, Mei Li, Zhenyang Zuo, Zhiqiang Niu

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  8. Sequence Design of Random Heteropolymers as Protein Mimics

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    Ivan Jayapurna, Zhiyuan Ruan, Marco Eres, Prajna Jalagam, Spencer Jenkins, Ting Xu

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  9. Boosting Degradation of Biodegradable Polymers

    Macromolecular Rapid Communications · 2023-01-17

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  10. Data-Driven Design of Polymer-Based Biomaterials: High-throughput Simulation, Experimentation, and Machine Learning

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  11. Nanomedicine-based treatment: An emerging therapeutical strategy for pulmonary hypertension

    Nano Research · 2023-02-15

    Shuya Wang, Qiaohui Chen, Tianjiao Zhao, Kelong Ai, Chang-Ping Hu

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  12. A Phase Engineering Strategy of Perovskite‐Type ZnSnO3:Nd for Boosting the Sonodynamic Therapy Performance

    Advanced Functional Materials · 2023-03-21

    Rui Zhang, Pengyu Zang, Dan Yang, Jiahao Li, Narisu Hu, Songnan Qu, Piaoping Yang

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  13. Solvent-Assisted Poly(lactic acid) Upcycling under Mild Conditions

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    Dion Hubble, Sarah L. Nordahl, Tianyu Zhu, Nawa Raj Baral, Corinne Donahue Scown, Gao Liu

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  14. Sequence Patterning, Morphology, and Dispersity in Single-Chain Nanoparticles: Insights from Simulation and Machine Learning

    ACS Polymers Au · 2023-06-05

    Roshan A. Patel, Sophia Colmenares, Michael A. Webb

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  15. Probing the Effects of Antimicrobial‐Lysozyme Derivatization on Enzymatic Degradation of Poly(ε‐caprolactone) Film and Fiber

    Macromolecular Bioscience · 2023-08-09

    Pranay Amruth Maroju, Ramakrishnan Ganesan, Jayati Ray Dutta

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  16. Protein modified cellulose nanocrystals on reinforcement and self-driven biodegradation of aliphatic polyester

    Carbohydrate Polymers · 2023-08-18

    Siwen Bi, Zhuang Zhang, Zhenzhen Yang, Zitong Shen, Jiahui Cai, Jintao Hu, Haoxiang Jin, Tianhao Qiu, Peng Yu, Bin Tan

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  17. High Thermal Stability of Enzyme-MOF Composites at 180 °C

    Chemistry · 2023-09-19

    Shitong Cui, Jun Yan Ge

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  18. Chemical Recycling of Polybutadiene Rubber with Tailored Depolymerization Enabled by Microencapsulated Metathesis Catalysts

    ACS Sustainable Chemistry & Engineering · 2023-09-25

    Matthew J. Warner, James P. Lassa, Hannah L. Narcross, Alex J. Commisso, Koushik Ghosh, Mikayla Romero, Jared M. Schwartz, Anthony Christian Engler, Paul A. Kohl, Samuel C. Leguizamon, Brad H. Jones

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  19. Controlling the lifetime of biodegradable electronics: from dissolution kinetics to trigger acceleration

    Soft Science · 2024-04-23

    Y. S. Park, Young‐In Ryu, Myung-Kyun Choi, Kyung‐Sub Kim, Seung‐Kyun Kang

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  20. Designed to Degrade: Tailoring Polyesters for Circularity

    Chemical Reviews · 2024-06-27

    Celine V. Aarsen, Anna Liguori, Rebecca Mattsson, Mika Henrikki Sipponen, Minna Hakkarainen

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  21. Degradable living plastics programmed by engineered spores

    Nature Chemical Biology · 2024-08-21

    Chenwang Tang, Lin Wang, Jing Sun, Guangda Chen, Junfeng Shen, Liang Wang, Ying Han, Jiren Luo, Zhiying Li, Pei Zhang, Simin Zeng, Dianpeng Qi, Jin Geng, Ji Liu, Zhuojun Dai

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  22. Exploring biodegradable alternatives: microorganism-mediated plastic degradation and environmental policies for sustainable plastic management

    Archives of Microbiology · 2024-11-05

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  23. Comparative studies on the effectiveness of proteases and enzymes from dietary supplements in the degradation of polylactide (PLA)

    International Biodeterioration & Biodegradation · 2024-11-10

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  24. Practice and tactics in the construction of novel degradable plastics at polymer and molecular levels

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    Yulong Niu, Fengying Pan, Yue Chen, Younes Ahmadi, Ki‐Hyun Kim, Xiaowei Li

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  25. Thermally and Base-Triggered “Debond-on-Demand” Chain-Extended Polyurethane Adhesives

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  26. Scalable nanoplastic degradation in water with enzyme-functionalized porous hydrogels

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  27. Enzymes offer a promising avenue for enhancing the competitiveness of biodegradable plastics in environmental restoration and the circular economy

    Waste Management · 2025-01-29

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  28. Nanoplastics and microplastics released from an enzyme-embedded biodegradable polyester during hydrolysis

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  29. Targeted Upcycling of Poly(L‐lactide) Based on Stereocomplexation Technology

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  30. Simultaneous improvement of thermal stability, mechanical properties, and combustion safety in polycaprolactone via blending with a tiny amount of aramid nanofiber

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  31. Breaking Symmetry of Active Sites in Metal‐Organic Frameworks for Efficient Photocatalytic Valorization of Polyester Plastics

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  35. Integrating chemical and biological conversion for waste plastics recycling and upcycling toward a circular bioeconomy

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