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RESEARCH PAPER · Advanced Functional Materials · 2018

Mg 3 B 7 O 13 Cl: A New Quasi‐Phase Matching Crystal in the Deep‐Ultraviolet Region

Zujian Wang, Huimin Qiao, Rongbing Su, Bing Hu, Xiaoming Yang, Chao He, Xifa Long

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Mg 3 B 7 O 13 Cl: A New Quasi‐Phase Matching Crystal in the Deep‐Ultraviolet RegionOriginalExploration of the deep-ultraviolet nonlinear optical materials in the derivatives of KBe2BO3F27β‐CsB9O14: A Triple‐Layered Borate with Edge‐Sharing BO4 Tetrahedra Exhibiting a Short Cutoff Edge and a Large Birefringence30Nontoxic KBBF Family Member Zn2BO3(OH): Balance between Beneficial Layered Structure and Layer Tendency81Emergent Deep‐Ultraviolet Nonlinear Optical Candidates324Neue Kandidaten für die nichtlineare Optik im Tief‐UV‐Bereich43Noncentrosymmetric Fluorooxoborates A10B13O15F19 (A = K and Rb) with Unexpected [B10O12F13]7– Units and Deep-Ultraviolet Cutoff Edges26Pushing periodic-disorder-induced phase matching into the deep-ultraviolet spectral region: theory and demonstration78A2SnS5: A Structural Incommensurate Modulation Exhibiting Strong Second‐Harmonic Generation and a High Laser‐Induced Damage Threshold (A=Ba, Sr)30A2SnS5: A Structural Incommensurate Modulation Exhibiting Strong Second‐Harmonic Generation and a High Laser‐Induced Damage Threshold (A=Ba, Sr)86Zn3B7O13Cl: A New Deep-Ultraviolet Transparency Nonlinear Optical Crystal with Boracite Structure24Ba 2 B 7 O 12 F with novel FBB [B 7 O 16 F] and deep-ultraviolet cut-off edge31Borates: A Rich Source for Optical Materials1089From centrosymmetric to noncentrosymmetric: effect of the cation on the crystal structures and birefringence values of (NH 4 ) n−2 AE(PO 2 F 2 ) n (AE = Mg, Sr and Ba; n = 2, 3 and 4)9Borosilicate Crystal LaBSiO5: A New Promising Ultraviolet Quasiphase Matching Material31π‑Conjugated Trigonal Planar [C(NH2)3]+ Cationic Group: A Superior Functional Unit for Ultraviolet Nonlinear Optical Materials52Fluorine‐Driven Enhancement of Birefringence in the Fluorooxosulfate: A Deep Evaluation from a Joint Experimental and Computational Study139Achieving Short‐Wavelength Phase‐Matching Second Harmonic Generation in Boron‐Rich Borosulfate with Planar [BO3] Units102Achieving Short‐Wavelength Phase‐Matching Second Harmonic Generation in Boron‐Rich Borosulfate with Planar [BO3] Units9Structure and Origin of the Second-Harmonic Generation Response of Nonlinear Optical Material Sr2Be2B2O713A Lanthanum Ammonium Sulfate Double Salt with a Strong SHG Response and Wide Deep‐UV Transparency15A Lanthanum Ammonium Sulfate Double Salt with a Strong SHG Response and Wide Deep‐UV Transparency96Li 6.58 Na 7.43 Sr 4 (B 9 O 18 )(B 12 O 24 )Cl: unprecedented combination of the largest two highly polymerized isolated B–O clusters with novel isolated B 9 O 18 FBB18Phase matching achieved by isomorphous substitution in IR nonlinear optical material Ba 2 SnSSi 2 O 7 with an undiscovered [SnO 4 S] functional motif47Crystal growth and functional properties of rare mineral Mn3B7O13Cl2Phosphogermanate Crystal: A New Ultraviolet–Infrared Nonlinear Optical Crystal with Excellent Optical Performances16Ultrawide Bandgap and Outstanding Second‐Harmonic Generation Response by a Fluorine‐Enrichment Strategy at a Transition‐Metal Oxyfluoride Nonlinear Optical Material51Ultrawide Bandgap and Outstanding Second‐Harmonic Generation Response by a Fluorine‐Enrichment Strategy at a Transition‐Metal Oxyfluoride Nonlinear Optical Material12Alkali metal sulfate: A new non-π-conjugated deep-ultraviolet quasi-phase matching crystal27An Optimized KBe2BO3F2‐Like Structure: The Unity of Deep‐Ultraviolet Transparency, Nonlinear Optical Property, and Ferroelectricity22Structural Characterization and ORR Activity of a Copper Complex Borate and an Unexpected [Ni(atta)(SO4)0.5]+ Borate-Sulfate7Ba5Ga2SiO4S6: a Phase-Matching Nonlinear Optical Oxychalcogenide Design via Structural Regulation Originated from Heteroanion Introduction25Discovery of SrZn 2 B 6 O 12 with an unprecedented quadruple-layered configuration0The origin of pyroelectricity in boracite at varying temperatures0Rational Design of the First Ammonium Magnesium Borate with Deep-Ultraviolet Cutoff Edge and Moderate Birefringence and Further Investigation into the Nature of Ammonium in the Borate System15Li3B8O13X (X = Cl and Br): Two New Noncentrosymmetric Crystals with Large Birefringence Induced by BO3 Units18Na2Mg2P2O7F2: A new diphosphate of the cuspidine family without disorder designed by targeted structural modulation1The Strategy to Improve the Phase Matching Ability in Tetrahedron‐Based Deep‐Ultraviolet Nonlinear Optical Crystals21Quadruple‐Bidentate Nitrate‐Ligated A 2 Hg(NO 3 ) 4 (A=K, Rb): Strong Second‐Harmonic Generation and Sufficient Birefringence59Quadruple‐Bidentate Nitrate‐Ligated A 2 Hg(NO 3 ) 4 (A=K, Rb): Strong Second‐Harmonic Generation and Sufficient Birefringence2Hydroxyl-Driven Enhanced Birefringence in Borophosphates3Crystal growth and spontaneous polarization mechanism of polar metal borate halides: Mn 3 B 7 O 13 Cl2Cadmium Hydroxyl Chloride with Balanced Band Gap and Second-Harmonic-Generation Response2Screening Strategy Identifies an Overlooked Deep‐Ultraviolet Transparent Nonlinear Optical Crystal3Screening Strategy Identifies an Overlooked Deep‐Ultraviolet Transparent Nonlinear Optical Crystal45LiNa2Ca8B12O24F6Cl and Li1.2Na2.8B6O11: A Case of Cation-Induced Birefringence Enhancement via Dimensional Changes of Highly Polymerized [B12O24] Motifs10Cationic substitution engineering induces a new quaternary chalcogenide in the A–M IIIA –M IVA –Q system for optical crystal applications1Nonlinear Metasurfaces: A New Paradigm for Short-Wavelength Generation and Modulation3Temperature dependence of optical parameters of a single crystal Mn3B7O13Cl in the THz frequency range1In Situ Synthesized Cobalt Nanocrystal via Bipyridine Ligand Cobaltic Borate Annealing Method for High‐performance Zinc‐air Battery5Finding a Novel Borate Ferroelectric with Random Domain Structures for Deep‐UV Quasi‐Phase‐Matching22CsGaGe₃Se₈: Enhanced optical anisotropy and bandgap via cation-substitution-driven dimensionality reduction0Inorganic Ge-based ferroelectric perovskites towards quasi-phase-matching in the infrared region0Pyrazole‐Protected Heteronuclear Rare‐Earth Boron‐Oxo Cluster Cage With Tunable Luminescence0NH 4 B 3 PO 6 (OH) 3 : A Hydroxyborophosphate with Short DUV Cutoff Edge and Large Birefringence2Tailoring a Solar‐Blind Ultraviolet Ferroelectric for Nonlinear Optics Through a Local Symmetry‐Breaking Cascaded Strategy1Emergent Deep‐Ultraviolet Ferroelectrics: Structure and Polarization Mechanism0

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  1. Exploration of the deep-ultraviolet nonlinear optical materials in the derivatives of KBe2BO3F2

    Acta Physica Sinica · 2019-01-01

    Minqiang Gai, Ying Wang, Shilie Pan

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  2. β‐CsB9O14: A Triple‐Layered Borate with Edge‐Sharing BO4 Tetrahedra Exhibiting a Short Cutoff Edge and a Large Birefringence

    Chemistry - A European Journal · 2019-06-18

    Shujuan Han, Chunmei Huang, Abudukadi Tudi, Shuaishuai Hu, Zhihua Yang, Shilie Pan

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  3. Nontoxic KBBF Family Member Zn2BO3(OH): Balance between Beneficial Layered Structure and Layer Tendency

    Advanced Science · 2019-09-16

    Xuefei Wang, Fangfang Zhang, Le Gao, Zhihua Yang, Shilie Pan

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  4. Emergent Deep‐Ultraviolet Nonlinear Optical Candidates

    Angewandte Chemie International Edition · 2019-12-10

    Miriding Mutailipu, Shilie Pan

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  5. Neue Kandidaten für die nichtlineare Optik im Tief‐UV‐Bereich

    Angewandte Chemie · 2019-12-10

    Miriding Mutailipu, Shilie Pan

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  6. Noncentrosymmetric Fluorooxoborates A10B13O15F19 (A = K and Rb) with Unexpected [B10O12F13]7– Units and Deep-Ultraviolet Cutoff Edges

    Inorganic Chemistry · 2020-02-10

    Wenyao Zhang, Zhonglei Wei, Zhihua Yang, Shilie Pan

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  7. Pushing periodic-disorder-induced phase matching into the deep-ultraviolet spectral region: theory and demonstration

    Light Science & Applications · 2020-03-18

    Mingchuan Shao, Fei Liang, Haohai Yu, Huaijin Zhang

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  8. A2SnS5: A Structural Incommensurate Modulation Exhibiting Strong Second‐Harmonic Generation and a High Laser‐Induced Damage Threshold (A=Ba, Sr)

    Angewandte Chemie · 2020-04-17

    Rui‐An Li, Zhengyang Zhou, Yu‐Kun Lian, Fei Jia, Xingxing Jiang, Mingcong Tang, Li‐Ming Wu, Junliang Sun, Ling Chen

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  9. A2SnS5: A Structural Incommensurate Modulation Exhibiting Strong Second‐Harmonic Generation and a High Laser‐Induced Damage Threshold (A=Ba, Sr)

    Angewandte Chemie International Edition · 2020-04-17

    Rui‐An Li, Zhengyang Zhou, Yu‐Kun Lian, Fei Jia, Xingxing Jiang, Mingcong Tang, Li‐Ming Wu, Junliang Sun, Ling Chen

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  10. Zn3B7O13Cl: A New Deep-Ultraviolet Transparency Nonlinear Optical Crystal with Boracite Structure

    ACS Applied Materials & Interfaces · 2020-08-24

    Zheyao Xiong, Jiangang He, Bing Hu, Pai Shan, Zujian Wang, Rongbing Su, Chao He, Xiaoming Yang, Xifa Long

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  11. Ba 2 B 7 O 12 F with novel FBB [B 7 O 16 F] and deep-ultraviolet cut-off edge

    Inorganic Chemistry Frontiers · 2020-10-30

    Zhaohong Miao, Yun Mo Yang, Zhonglei Wei, Zhihua Yang, Shilie Pan

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  12. Borates: A Rich Source for Optical Materials

    Chemical Reviews · 2020-12-14

    Miriding Mutailipu, Kenneth Reinhard Poeppelmeier, Shilie Pan

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  13. From centrosymmetric to noncentrosymmetric: effect of the cation on the crystal structures and birefringence values of (NH 4 ) n−2 AE(PO 2 F 2 ) n (AE = Mg, Sr and Ba; n = 2, 3 and 4)

    Dalton Transactions · 2021-01-01

    Wenyao Zhang, Wenqi Jin, Meng Cheng, Ruonan Zhang, Zhihua Yang, Shilie Pan

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  14. Borosilicate Crystal LaBSiO5: A New Promising Ultraviolet Quasiphase Matching Material

    Advanced Optical Materials · 2021-03-10

    Hongyuan Sha, Rongbing Su, Zheyao Xiong, Zujian Wang, Pai Shan, Chao He, Xiaoming Yang, Xifa Long

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  15. π‑Conjugated Trigonal Planar [C(NH2)3]+ Cationic Group: A Superior Functional Unit for Ultraviolet Nonlinear Optical Materials

    ACS Omega · 2021-03-23

    Yunxia Song, Min Luo, Donghong Lin, Chensheng Lin, Zujian Wang, Xifa Long, Ning Ye

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  16. Fluorine‐Driven Enhancement of Birefringence in the Fluorooxosulfate: A Deep Evaluation from a Joint Experimental and Computational Study

    Advanced Science · 2021-06-04

    Wenqi Jin, Wenyao Zhang, Abudukadi Tudi, Liying Wang, Xin Hua Zhou, Zhihua Yang, Shilie Pan

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  17. Achieving Short‐Wavelength Phase‐Matching Second Harmonic Generation in Boron‐Rich Borosulfate with Planar [BO3] Units

    Angewandte Chemie International Edition · 2021-10-09

    Zi‐Jian Li, Wenqi Jin, Fangfang Zhang, Zilong Chen, Zhihua Yang, Shilie Pan

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  18. Achieving Short‐Wavelength Phase‐Matching Second Harmonic Generation in Boron‐Rich Borosulfate with Planar [BO3] Units

    Angewandte Chemie · 2021-10-09

    Zi‐Jian Li, Wenqi Jin, Fangfang Zhang, Zilong Chen, Zhihua Yang, Shilie Pan

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  19. Structure and Origin of the Second-Harmonic Generation Response of Nonlinear Optical Material Sr2Be2B2O7

    The Journal of Physical Chemistry Letters · 2021-11-17

    Xiyue Cheng, Yueping Zhang, Lijuan Liu, Xiaoyang Wang, Myung‐Hwan Whangbo, Jing Chie Lin, Shuiquan Deng

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  20. A Lanthanum Ammonium Sulfate Double Salt with a Strong SHG Response and Wide Deep‐UV Transparency

    Angewandte Chemie · 2021-12-11

    Chao Wu, Xingxing Jiang, Yilei Hu, Chunbo Jiang, Tianhui Wu, Zheshuai Lin, Zhipeng Huang, Mark Graeme Humphrey, Chi Zhang

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  21. A Lanthanum Ammonium Sulfate Double Salt with a Strong SHG Response and Wide Deep‐UV Transparency

    Angewandte Chemie International Edition · 2021-12-11

    Chao Wu, Xingxing Jiang, Yilei Hu, Chunbo Jiang, Tianhui Wu, Zheshuai Lin, Zhipeng Huang, Mark Graeme Humphrey, Chi Zhang

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  22. Li 6.58 Na 7.43 Sr 4 (B 9 O 18 )(B 12 O 24 )Cl: unprecedented combination of the largest two highly polymerized isolated B–O clusters with novel isolated B 9 O 18 FBB

    Inorganic Chemistry Frontiers · 2022-01-01

    Feixiang Wang, Yun Mo Yang, Congcong Jin, Shilie Pan

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  23. Phase matching achieved by isomorphous substitution in IR nonlinear optical material Ba 2 SnSSi 2 O 7 with an undiscovered [SnO 4 S] functional motif

    Materials Chemistry Frontiers · 2022-01-01

    Yong‐Fang Shi, Zuju Ma, Bingxuan Li, Xin‐Tao Wu, Hua Lin, Qi‐Long Zhu

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  24. Crystal growth and functional properties of rare mineral Mn3B7O13Cl

    Journal of Crystal Growth · 2022-01-04

    Jiesen Guo, Ruijin Sun, Fei Chen, Munan Hao, Yuxin Ma, Qiangqiang Wang, Yuetong Wu, Dongxu Hou, Zeyu Zhang, Tianming Liu, Zhibin Li, Dezhong Meng, Changchun Zhao

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  25. Phosphogermanate Crystal: A New Ultraviolet–Infrared Nonlinear Optical Crystal with Excellent Optical Performances

    ACS Applied Materials & Interfaces · 2022-02-16

    Hongyuan Sha, Zheyao Xiong, Junxin Xu, Zujian Wang, Rongbing Su, Chao He, Xiaoming Yang, Xifa Long, Ying Liu

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  26. Ultrawide Bandgap and Outstanding Second‐Harmonic Generation Response by a Fluorine‐Enrichment Strategy at a Transition‐Metal Oxyfluoride Nonlinear Optical Material

    Angewandte Chemie International Edition · 2022-03-17

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  27. Ultrawide Bandgap and Outstanding Second‐Harmonic Generation Response by a Fluorine‐Enrichment Strategy at a Transition‐Metal Oxyfluoride Nonlinear Optical Material

    Angewandte Chemie · 2022-03-17

    Tianhui Wu, Xingxing Jiang, Chao Wu, Yilei Hu, Zheshuai Lin, Zhipeng Huang, Mark Graeme Humphrey, Chi Zhang

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  28. Alkali metal sulfate: A new non-π-conjugated deep-ultraviolet quasi-phase matching crystal

    Scripta Materialia · 2022-04-28

    Hongyuan Sha, Junxin Xu, Lingxiong Huang, Zheyao Xiong, Zujian Wang, Rongbing Su, Chao He, Xiaoming Yang, Xifa Long

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  29. An Optimized KBe2BO3F2‐Like Structure: The Unity of Deep‐Ultraviolet Transparency, Nonlinear Optical Property, and Ferroelectricity

    Advanced Optical Materials · 2022-05-02

    Hongyuan Sha, Junxin Xu, Zheyao Xiong, Zujian Wang, Rongbing Su, Chao He, Xiaoming Yang, Xifa Long, Ying Liu

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  30. Structural Characterization and ORR Activity of a Copper Complex Borate and an Unexpected [Ni(atta)(SO4)0.5]+ Borate-Sulfate

    Inorganic Chemistry · 2022-05-11

    Wei Li, Yan-Ling Deng, Chun‐Yang Pan

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  31. Ba5Ga2SiO4S6: a Phase-Matching Nonlinear Optical Oxychalcogenide Design via Structural Regulation Originated from Heteroanion Introduction

    Inorganic Chemistry · 2022-12-16

    Yong‐Fang Shi, Shenghua Zhou, Bingxuan Li, Yi Liu, Xintao Wu, Hua Lin, Qi‐Long Zhu

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  32. Discovery of SrZn 2 B 6 O 12 with an unprecedented quadruple-layered configuration

    New Journal of Chemistry · 2023-01-01

    Xiangyu Long, Yan An Lv, Xueyan Wu

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  33. The origin of pyroelectricity in boracite at varying temperatures

    Research Square · 2023-01-05

    Qiang-qiang wang, Ruijin Sun, Jiesen Guo, Yuetong Wu, Yuxin Ma, Fei Chen, Tianming Liu, Haodong Li, Fanshu Meng, Dezhong Meng, Changchun Zhao

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  34. Rational Design of the First Ammonium Magnesium Borate with Deep-Ultraviolet Cutoff Edge and Moderate Birefringence and Further Investigation into the Nature of Ammonium in the Borate System

    Inorganic Chemistry · 2023-01-18

    Feixiang Wang, Mengfan Wu, Zhihua Yang, Xifa Long, Yun Mo Yang, Shilie Pan

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  35. Li3B8O13X (X = Cl and Br): Two New Noncentrosymmetric Crystals with Large Birefringence Induced by BO3 Units

    Inorganic Chemistry · 2023-02-16

    Mei Hu, Nuerbiye Tuerhong, Zhaohui Chen, Qun Jing, Ming‐Hsien Lee

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  36. Na2Mg2P2O7F2: A new diphosphate of the cuspidine family without disorder designed by targeted structural modulation

    Inorganica Chimica Acta · 2023-06-07

    Yanhui Zhang, Yun Mo Yang, Xifa Long, Hualing Tian, Xiaofeng Gu, Zhi Guo Su

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  37. The Strategy to Improve the Phase Matching Ability in Tetrahedron‐Based Deep‐Ultraviolet Nonlinear Optical Crystals

    Advanced Optical Materials · 2023-07-09

    Hongyuan Sha, Yanran Shang, Zujian Wang, Rongbing Su, Chao He, Xiaoming Yang, Xifa Long

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  38. Quadruple‐Bidentate Nitrate‐Ligated A 2 Hg(NO 3 ) 4 (A=K, Rb): Strong Second‐Harmonic Generation and Sufficient Birefringence

    Angewandte Chemie International Edition · 2023-08-02

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  39. Quadruple‐Bidentate Nitrate‐Ligated A 2 Hg(NO 3 ) 4 (A=K, Rb): Strong Second‐Harmonic Generation and Sufficient Birefringence

    Angewandte Chemie · 2023-08-02

    Qi Lu, Xingxing Jiang, Kaining Duanmu, Chao Wu, Zheshuai Lin, Zhipeng Huang, Mark Graeme Humphrey, Chi Zhang

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  40. Hydroxyl-Driven Enhanced Birefringence in Borophosphates

    Inorganic Chemistry · 2023-11-22

    Yang Xia, Wen-Bin Zhang, Xueting Pan, Xueling Hou, Shujuan Han

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  41. Crystal growth and spontaneous polarization mechanism of polar metal borate halides: Mn 3 B 7 O 13 Cl

    CrystEngComm · 2024-01-01

    Haodong Li, Duo Zhang, Jiesen Guo, Qiangqiang Wang, Yuxin Ma, Munan Hao, Yuetong Wu, Fanshu Meng, Tianming Liu, Yibo Xu, Chen Xu, Changchun Zhao, Dezhong Meng, Zhiyuan Zheng, Ruijin Sun

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  42. Cadmium Hydroxyl Chloride with Balanced Band Gap and Second-Harmonic-Generation Response

    Inorganic Chemistry · 2024-03-28

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  43. Screening Strategy Identifies an Overlooked Deep‐Ultraviolet Transparent Nonlinear Optical Crystal

    Angewandte Chemie · 2024-08-12

    Jia-Xiang Zhang, Qing-Gang Yue, Shenghua Zhou, Xin‐Tao Wu, Hua Lin, Qi‐Long Zhu

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  44. Screening Strategy Identifies an Overlooked Deep‐Ultraviolet Transparent Nonlinear Optical Crystal

    Angewandte Chemie International Edition · 2024-08-12

    Jia-Xiang Zhang, Qing-Gang Yue, Shenghua Zhou, Xin‐Tao Wu, Hua Lin, Qi‐Long Zhu

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  45. LiNa2Ca8B12O24F6Cl and Li1.2Na2.8B6O11: A Case of Cation-Induced Birefringence Enhancement via Dimensional Changes of Highly Polymerized [B12O24] Motifs

    Inorganic Chemistry · 2024-08-21

    Ziting Yan, Jinbin Fan, Dongdong Chu, Zhihua Yang, Juanjuan Lu, Shilie Pan, Min Zhang

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  46. Cationic substitution engineering induces a new quaternary chalcogenide in the A–M IIIA –M IVA –Q system for optical crystal applications

    CrystEngComm · 2025-01-01

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  47. Nonlinear Metasurfaces: A New Paradigm for Short-Wavelength Generation and Modulation

    The Journal of Physical Chemistry C · 2025-03-28

    Zhihui Wang, Rong Lin, Chen Chen, Jiajun Wu, Jin Li Yao, Din Ping Tsai

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  48. Temperature dependence of optical parameters of a single crystal Mn3B7O13Cl in the THz frequency range

    Applied Optics · 2025-04-18

    Yibo Xu, Haodong Li, Zhiyuan Zheng, Chutong Gao, Mingrui Zhang, Tong Zhang, Haochong Huang, Changchun Zhao, Ruijin Sun

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  49. In Situ Synthesized Cobalt Nanocrystal via Bipyridine Ligand Cobaltic Borate Annealing Method for High‐performance Zinc‐air Battery

    Chemistry - A European Journal · 2025-05-03

    Lei Liu, Xiang‐Yu Huang, Hao Liu, An‐Na Chen, Chun‐Yang Pan

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  50. Finding a Novel Borate Ferroelectric with Random Domain Structures for Deep‐UV Quasi‐Phase‐Matching

    Advanced Materials · 2025-05-30

    Yabo Wu, Cui Chen, Zhongchang Wang, Junjie Li, Jian Wei Han, Miriding Mutailipu, Shilie Pan

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