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RESEARCH PAPER · Advanced Optical Materials · 2021

Borosilicate Crystal LaBSiO5: A New Promising Ultraviolet Quasiphase Matching Material

Hongyuan Sha, Rongbing Su, Zheyao Xiong, Zujian Wang, Pai Shan, Chao He, Xiaoming Yang, Xifa Long

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Borosilicate Crystal LaBSiO5: A New Promising Ultraviolet Quasiphase Matching MaterialOriginalFrom β‐Na2B6O10 to Na3AlB8O15 and Na3Al2B7O15: Structural Tuning of Anionic‐Group Architectures by Substitution of [BO4] by [AlO4] Covalent Tetrahedra10AZn 2 (BO 3 )Si 2 O 5 (A = Rb, Cs): first examples of KBe 2 BO 3 F 2 structure type in the borosilicate family exhibiting a deep-ultraviolet cutoff edge25Hexameric poly-fluoroberyllophosphate Na 4 Be 2 PO 4 F 5 with moderate birefringence and deep-ultraviolet transmission as a potential zero-order-waveplate crystal17Phosphogermanate Crystal: A New Ultraviolet–Infrared Nonlinear Optical Crystal with Excellent Optical Performances16Alkali metal sulfate: A new non-π-conjugated deep-ultraviolet quasi-phase matching crystal27An Optimized KBe2BO3F2‐Like Structure: The Unity of Deep‐Ultraviolet Transparency, Nonlinear Optical Property, and Ferroelectricity22Triple-Wavelength Lasing with a Stabilized β-LaBSiO5:Nd3+ Crystal27Oxychalcogenides as Promising Ultraviolet Nonlinear Optical Candidates: Experimental and Theoretical Studies of AEGeOS2(AE = Sr and Ba)24Borate-Based Compounds as Mixed Polyanion Cathode Materials for Advanced Batteries22Rb 3 B 11 P 2 O 23 : Materials Design of a New Chemically Benign Deep-Ultraviolet Nonlinear Optical Material58Deep-ultraviolet nonlinear-optical crystal BaNa2[PO3(OH)]2 with large birefringence and strong second-harmonic-generation response8Recent progress in borate-based short-wavelength nonlinear optical crystals with boron–oxygen skeleton modification28The Strategy to Improve the Phase Matching Ability in Tetrahedron‐Based Deep‐Ultraviolet Nonlinear Optical Crystals21Enlargement of Bandgap and Birefringence in Nonlinear Optical Alkali‐Metal Sulfate Crystals by the Substitution of Asymmetrical Non‐π‐Conjugated Cation8The structural origin and boundaries of thermal transitions in stillwellite-type LnBSiO54Hierarchical chiral MOFs with the induced chirality of AIE ligands exhibiting non-reciprocal CPL17Trithionic guanidine: A novel semi-organic short-wave ultraviolet nonlinear optical sulfate with dimeric heteroleptic tetrahedra14PbBeB2O5: A High-Performance Ultraviolet Nonlinear-Optical Crystal with Functional [BeB2O8]8– Group3High second-order nonlinearity in single-domain tetragonal PMN-PT single crystal10Ba2ScBSi2O9: A Mixed-Coordination Borosilicate with a Low B/Si Ratio Exhibiting Enhanced Second Harmonic Generation Response7K0.9Rb2.1B8PO16: Design and Synthesis of a Deep-Ultraviolet Nonlinear Optical Crystal with Balanced Performance Derived from π-Conjugated and Non-π-Conjugated Groups11Two α‐SiO 2 ‐Related Deep‐Ultraviolet Phase‐Matchable Optical Nonlinear Beryllium Silicate Crystals Na 2 BeSiO 4 and Li 2 BeSiO 4 with Enhanced SHG Effect10Deep ultraviolet transparent borophosphates LiAB 2 P 2 O 9 (A = NH 4 , K) and LiNaB 2 P 2 O 8 (OH) 2 ·H 2 O exhibiting a moderate second-harmonic generation response4BaAlPO 4 F 2 : structure and properties of the first barium fluoroaluminophosphate with the mixed anion group [Al 2 PO 8 F 5 ]1Non-equivalent terminating roles of hydroxyl and fluorine in hydroxy/fluorooxo-borate optical functional materials2Design and Synthesis of a Deep-Ultraviolet Nonlinear Optical Crystal KRb3B6Ge3O17 Composed of [B3O8] Units and [GeO4] Tetrahedra6Borosilicates as deep-ultraviolet transparent nonlinear optical crystals: Structural motifs, performance limits and future directions9Record‐Short Phase Matchability of Silicate: Charge‐Driven Lattice Distortion Enables Deep‐UV Phase Matching and Strong Optical Nonlinearity0Breakthrough in High Quality LaBGeO 5 Crystal for Deep Ultraviolet Quasi-Phase Matching Application0Fluorine‐Driven Chemical Scissor Effect in Scandium Borates: Structural Evolution with Retained Optically Active Motifs0Emergent Deep‐Ultraviolet Ferroelectrics: Structure and Polarization Mechanism0

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  1. From β‐Na2B6O10 to Na3AlB8O15 and Na3Al2B7O15: Structural Tuning of Anionic‐Group Architectures by Substitution of [BO4] by [AlO4] Covalent Tetrahedra

    Chemistry - A European Journal · 2021-11-24

    Jiahao Jiao, Wenqi Jin, Min Zhang, Zhiyong Guo, Zhihua Yang, Shilie Pan

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  2. AZn 2 (BO 3 )Si 2 O 5 (A = Rb, Cs): first examples of KBe 2 BO 3 F 2 structure type in the borosilicate family exhibiting a deep-ultraviolet cutoff edge

    Journal of Materials Chemistry C · 2021-12-24

    Tuohetijiang Baiheti, Abudukadi Tudi, Jian Wei Han, Zhihua Yang, Shilie Pan

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  3. Hexameric poly-fluoroberyllophosphate Na 4 Be 2 PO 4 F 5 with moderate birefringence and deep-ultraviolet transmission as a potential zero-order-waveplate crystal

    Inorganic Chemistry Frontiers · 2022-01-01

    Yuanyu Yang, Yao Guo, Yi-Gang Chen, Xiwei Hu, Xia Zhang, Xian‐Ming Zhang, Xian-Ming Zhang, Xian-Ming Zhang

    Read original paper ↗ ·

  4. Phosphogermanate Crystal: A New Ultraviolet–Infrared Nonlinear Optical Crystal with Excellent Optical Performances

    ACS Applied Materials & Interfaces · 2022-02-16

    Hongyuan Sha, Zheyao Xiong, Junxin Xu, Zujian Wang, Rongbing Su, Chao He, Xiaoming Yang, Xifa Long, Ying Liu

    Read original paper ↗ ·

  5. Alkali metal sulfate: A new non-π-conjugated deep-ultraviolet quasi-phase matching crystal

    Scripta Materialia · 2022-04-28

    Hongyuan Sha, Junxin Xu, Lingxiong Huang, Zheyao Xiong, Zujian Wang, Rongbing Su, Chao He, Xiaoming Yang, Xifa Long

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  6. An Optimized KBe2BO3F2‐Like Structure: The Unity of Deep‐Ultraviolet Transparency, Nonlinear Optical Property, and Ferroelectricity

    Advanced Optical Materials · 2022-05-02

    Hongyuan Sha, Junxin Xu, Zheyao Xiong, Zujian Wang, Rongbing Su, Chao He, Xiaoming Yang, Xifa Long, Ying Liu

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  7. Triple-Wavelength Lasing with a Stabilized β-LaBSiO5:Nd3+ Crystal

    Journal of the American Chemical Society · 2022-06-09

    Lingyun Li, Fazheng Huang, Yi Shi, Zhong‐Zhen Luo, Guoqiang Wang, Xin‐Xiong Li, Bingxuan Li, Lizhen Zhang, Yi Yu, Yi Yu, Ya‐Nan Feng, Chengkai Yang, Yan Yu, Yan Yu, Kenneth Reinhard Poeppelmeier

    Read original paper ↗ ·

  8. Oxychalcogenides as Promising Ultraviolet Nonlinear Optical Candidates: Experimental and Theoretical Studies of AEGeOS2(AE = Sr and Ba)

    Inorganic Chemistry · 2022-09-21

    Hedi Yang, Shenghua Zhou, Mao‐Yin Ran, Xintao Wu, Hua Lin, Qi‐Long Zhu

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  9. Borate-Based Compounds as Mixed Polyanion Cathode Materials for Advanced Batteries

    Molecules · 2022-11-19

    Giancarlo Dominador D. Sanglay, Jayson S. Garcia, Mecaelah S. Palaganas, Maurice Sorolla, Sean Benson A. See, Lawrence A. Limjuco, Joey Duran Ocon

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  10. Rb 3 B 11 P 2 O 23 : Materials Design of a New Chemically Benign Deep-Ultraviolet Nonlinear Optical Material

    ACS Materials Letters · 2022-12-12

    Haonan Liu, Hongping Wu, Zhanggui Hu, Jiyang Wang, Yicheng Wu, P. Shiv Halasyamani, Hongwei Yu

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  11. Deep-ultraviolet nonlinear-optical crystal BaNa2[PO3(OH)]2 with large birefringence and strong second-harmonic-generation response

    Chinese Journal of Structural Chemistry · 2023-01-01

    Yuanyu Yang, Yao Guo, Yi-Gang Chen, Chengbo Li, Xian‐Ming Zhang

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  12. Recent progress in borate-based short-wavelength nonlinear optical crystals with boron–oxygen skeleton modification

    Materials Chemistry Frontiers · 2023-01-01

    Meng Cheng, Xueling Hou, Zhihua Yang, Shilie Pan

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  13. The Strategy to Improve the Phase Matching Ability in Tetrahedron‐Based Deep‐Ultraviolet Nonlinear Optical Crystals

    Advanced Optical Materials · 2023-07-09

    Hongyuan Sha, Yanran Shang, Zujian Wang, Rongbing Su, Chao He, Xiaoming Yang, Xifa Long

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  14. Enlargement of Bandgap and Birefringence in Nonlinear Optical Alkali‐Metal Sulfate Crystals by the Substitution of Asymmetrical Non‐π‐Conjugated Cation

    Advanced Optical Materials · 2023-10-02

    Pengfei Zhu, Pifu Gong, Zhenyan Wang, Huatong Jiang, Jianfu Zhao, Chao Li, Zheshuai Lin, Xiulan Duan, Fapeng Yu

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  15. The structural origin and boundaries of thermal transitions in stillwellite-type LnBSiO5

    Optical Materials · 2023-12-08

    Maria Georgievna Krzhizhanovskaya, Олег Сергеевич Верещагин, Yu.O. Kopylova, Liudmila A. Gorelova, Dmitrii Vasil'evich Pankin, Valentina A. Yukhno, Natalia S. Vlasenko, Vladimir M. Bocharov, Sergey N. Britvin

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  16. Hierarchical chiral MOFs with the induced chirality of AIE ligands exhibiting non-reciprocal CPL

    Chemical Communications · 2024-01-01

    Hong‐Ru Fu, Dan‐Dan Ren, Kun Zhang, Shuang Wang, Xu-Jing Yang, Qing-Rong Ding, Ya‐Pan Wu

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  17. Trithionic guanidine: A novel semi-organic short-wave ultraviolet nonlinear optical sulfate with dimeric heteroleptic tetrahedra

    Chinese Chemical Letters · 2024-03-08

    Hongyuan Sha, Dongling Yang, Yanran Shang, Zujian Wang, Rongbing Su, Chao He, Xiaoming Yang, Xifa Long

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  18. PbBeB2O5: A High-Performance Ultraviolet Nonlinear-Optical Crystal with Functional [BeB2O8]8– Group

    Inorganic Chemistry · 2024-05-17

    Fang Wang, Mengke Zi, Qin Chen, Zixu Wang, Jianguang Wang, Xingxing Jiang, Yi-Gang Chen, Yao Guo, Zheshuai Lin, Xian‐Ming Zhang

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  19. High second-order nonlinearity in single-domain tetragonal PMN-PT single crystal

    Applied Physics Letters · 2024-07-22

    Peng Luan, Xin Liu, Hongliang Du, Wanghua Wu, Hailong Hu, Fei Li, Xiaoyong Wei, Zhuo Xu

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  20. Ba2ScBSi2O9: A Mixed-Coordination Borosilicate with a Low B/Si Ratio Exhibiting Enhanced Second Harmonic Generation Response

    Inorganic Chemistry · 2024-08-21

    Ming Yang, Hongwei Yu, Zhanggui Hu, Jiyang Wang, Yicheng Wu, Hongping Wu

    Read original paper ↗ ·

  21. K0.9Rb2.1B8PO16: Design and Synthesis of a Deep-Ultraviolet Nonlinear Optical Crystal with Balanced Performance Derived from π-Conjugated and Non-π-Conjugated Groups

    Inorganic Chemistry · 2024-09-22

    Wenyu He, Xianchao Zhu, Zhanggui Hu, Jiyang Wang, Yicheng Wu

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  22. Two α‐SiO 2 ‐Related Deep‐Ultraviolet Phase‐Matchable Optical Nonlinear Beryllium Silicate Crystals Na 2 BeSiO 4 and Li 2 BeSiO 4 with Enhanced SHG Effect

    Small · 2024-10-29

    Yi-Gang Chen, Xingxing Jiang, Hongxiao Lv, Dajiang Mei, Xia Zhang, Xia Zhang, Yao Guo, Zheshuai Lin, Xian‐Ming Zhang, Xian‐Ming Zhang

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  23. Deep ultraviolet transparent borophosphates LiAB 2 P 2 O 9 (A = NH 4 , K) and LiNaB 2 P 2 O 8 (OH) 2 ·H 2 O exhibiting a moderate second-harmonic generation response

    Journal of Materials Chemistry C · 2024-12-23

    Huanhuan Zhao, Chenxu Li, Juanjuan Lu, Zhihua Yang, Jian Wei Han, Shilie Pan

    Read original paper ↗ ·

  24. BaAlPO 4 F 2 : structure and properties of the first barium fluoroaluminophosphate with the mixed anion group [Al 2 PO 8 F 5 ]

    Dalton Transactions · 2025-01-01

    Yanhui Zhang, Jiajia Li, Yaqing Ding, Kaitong Liu, Xiaofeng Gu

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  25. Non-equivalent terminating roles of hydroxyl and fluorine in hydroxy/fluorooxo-borate optical functional materials

    Science China Chemistry · 2025-06-03

    Huanhuan Cheng, Shilie Pan, Zhihua Yang

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  26. Design and Synthesis of a Deep-Ultraviolet Nonlinear Optical Crystal KRb3B6Ge3O17 Composed of [B3O8] Units and [GeO4] Tetrahedra

    Inorganic Chemistry · 2025-06-27

    Ziqi Guo, Xianchao Zhu, Zhanggui Hu, Jiyang Wang, Yicheng Wu

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  27. Borosilicates as deep-ultraviolet transparent nonlinear optical crystals: Structural motifs, performance limits and future directions

    Chinese Journal of Structural Chemistry · 2025-09-01

    Yangfeifei Ou, Xiaoliang Zhou, You‐Zhao Lan, Jian‐Wen Cheng

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  28. Record‐Short Phase Matchability of Silicate: Charge‐Driven Lattice Distortion Enables Deep‐UV Phase Matching and Strong Optical Nonlinearity

    Advanced Functional Materials · 2026-02-28

    Yi‐Gang Chen, Qin Chen, Mengke Zi, Xia Zhang, Xia Zhang, Yao Guo, Miriding Mutailipu, Xingxing Jiang, Zheshuai Lin, Xian‐Ming Zhang, Xian‐Ming Zhang

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  29. Breakthrough in High Quality LaBGeO 5 Crystal for Deep Ultraviolet Quasi-Phase Matching Application

    ACS Applied Materials & Interfaces · 2026-06-29

    Jiahao Wang, Lingfei Lv, Rongbing Su, Z G Zhu, Hongjiang Wu, Hongyuan Sha, Zujian Wang, Bin Su, Chao He

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  30. Fluorine‐Driven Chemical Scissor Effect in Scandium Borates: Structural Evolution with Retained Optically Active Motifs

    Chinese Journal of Chemistry · 2026-08-03

    Linsen Wang, Qianzhen Zhang, Ran An, Zhihua Yang, Yun Yang, Xueyan Wu

    Read original paper ↗ ·

  31. Emergent Deep‐Ultraviolet Ferroelectrics: Structure and Polarization Mechanism

    Advanced Functional Materials · 2026-08-31

    Zujian Wang, Hongyuan Sha, Xiaoming Yang, Chao He, Fangfang Zhang, Xifa Long, Shilie Pan

    Read original paper ↗ ·
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