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RESEARCH PAPER · Scripta Materialia · 2022

Alkali metal sulfate: A new non-π-conjugated deep-ultraviolet quasi-phase matching crystal

Hongyuan Sha, Junxin Xu, Lingxiong Huang, Zheyao Xiong, Zujian Wang, Rongbing Su, Chao He, Xiaoming Yang, Xifa Long

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Alkali metal sulfate: A new non-π-conjugated deep-ultraviolet quasi-phase matching crystalOriginalRecent advances in non-π-conjugated nonlinear optical sulfates with deep-UV absorption edge53Sn9O4Br9X (X = Cl, Br): Two new Sn(II) oxyhalides exhibiting large birefringence derived from highly distortive polyhedra of lone pair cations9The Strategy to Improve the Phase Matching Ability in Tetrahedron‐Based Deep‐Ultraviolet Nonlinear Optical Crystals21(NH 4 ) 2 (I 5 O 12 )(IO 3 ) and K 1.03 (NH 4 ) 0.97 (I 5 O 12 )(IO 3 ): Mixed‐Valent Polyiodates with Unprecedented I 5 O 12 − Unit Exhibiting Strong Second‐Harmonic Generation Responses and Giant Birefringence22Nonlinear optical inorganic sulfates: The improvement of the phase matching ability driven by the structural modulation41A Sharp Improvement of Sulfate's Birefringence Induced by the Synergistic Effect of Heteroleptic and Dimeric Strategies14Exploration of antimony( iii ) oxyhalides via single-site substitution in quest of large birefringence10AYSO4F2 (A = K, Rb): [YO4F4] Polyhedra Enhancement of Birefringence in Non-π-Conjugated Sulfate Systems9Hg4(Te2O5)(SO4): A Giant Birefringent Sulfate Crystal Triggered by a Highly Selective Cation153Trithionic guanidine: A novel semi-organic short-wave ultraviolet nonlinear optical sulfate with dimeric heteroleptic tetrahedra14Old tree blossoms anew: Research progress on the structures and optical properties of ultraviolet selenites56Screening Strategy Identifies an Overlooked Deep‐Ultraviolet Transparent Nonlinear Optical Crystal3Screening Strategy Identifies an Overlooked Deep‐Ultraviolet Transparent Nonlinear Optical Crystal45Promising Functional Structural Building Unit Trisulfimide (SO2N)33– and Its Contributions to Second Harmonic Generation and Birefringence1Electronic, optical, elastic, piezoelectric and vibrational properties of P63 KLiSO42The New Paradigm of Ligand Substitution-Driven Enhancement of Anisotropy from SO4 Units in Short-Wavelength Region14Dual Lone Pair Strategy for High Birefringence in Antimony(III)-Based Tellurite Sulfates with Short-Wave UV Transparency10From AgHgI(SO4) to AgHg3I3.2Cl1.8(SO4): Symmetry Breaking of the Belousovite‐Type Topology by Mixed Halides to Achieve Strong Nonlinear Optical Effect14Direct Deep‐UV Second‐Harmonic Generation in Disordered Χ 2 ‐Modulated Ferroelectric Crystals18π-Conjugated unit bridge for giant second-harmonic generation and birefringence in hybrid materials with dual heteroleptic polyhedra5Rational design of novel mixed metal sulfates with diverse dimensional structures and short UV cutoff edges1Confinement π‐Conjugated Moiety Tailoring to Achieve Record Deep‐UV Nonlinearity in Sulfates0Crystal Growth, Structure and Optical Properties of (NH 4 ) 2 Mg(SO 4 ) 2 ·6H 2 O: A Crystal With a Wide Deep Ultraviolet Window0The Enhancement of Phase‐Matching Capability by Recombining π‐Conjugated Group in Nonlinear Optical Sulfates1Toward the vacuum-ultraviolet frontier in nonlinear optical frequency conversion: phase-matching mechanisms across dimensions and architectures2Emergent Deep‐Ultraviolet Ferroelectrics: Structure and Polarization Mechanism0Two Rare Earth-Based Sulfates with Enhanced Birefringence and Broad Optical Transparency Window0

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  1. Recent advances in non-π-conjugated nonlinear optical sulfates with deep-UV absorption edge

    Chinese Journal of Structural Chemistry · 2023-02-24

    Chen Xu, Yanqiang Li, Junhua Luo, Sangen Zhao

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  2. Sn9O4Br9X (X = Cl, Br): Two new Sn(II) oxyhalides exhibiting large birefringence derived from highly distortive polyhedra of lone pair cations

    Scripta Materialia · 2023-03-27

    Mei Hu, Chenchen Tu, Zhihua Yang, Shujuan Han, Shilie Pan

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  3. The Strategy to Improve the Phase Matching Ability in Tetrahedron‐Based Deep‐Ultraviolet Nonlinear Optical Crystals

    Advanced Optical Materials · 2023-07-09

    Hongyuan Sha, Yanran Shang, Zujian Wang, Rongbing Su, Chao He, Xiaoming Yang, Xifa Long

    Read original paper ↗ ·

  4. (NH 4 ) 2 (I 5 O 12 )(IO 3 ) and K 1.03 (NH 4 ) 0.97 (I 5 O 12 )(IO 3 ): Mixed‐Valent Polyiodates with Unprecedented I 5 O 12 − Unit Exhibiting Strong Second‐Harmonic Generation Responses and Giant Birefringence

    Small · 2023-07-25

    Nan Ma, Jin Chen, Bingxuan Li, Chun‐Li Hu, Jiang‐Gao Mao

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  5. Nonlinear optical inorganic sulfates: The improvement of the phase matching ability driven by the structural modulation

    Coordination Chemistry Reviews · 2023-08-02

    Yanran Shang, Junxin Xu, Hongyuan Sha, Zujian Wang, Chao He, Rongbing Su, Xiaoming Yang, Xifa Long

    Read original paper ↗ ·

  6. A Sharp Improvement of Sulfate's Birefringence Induced by the Synergistic Effect of Heteroleptic and Dimeric Strategies

    Small · 2023-12-10

    Hongyuan Sha, Yanran Shang, Zujian Wang, Rongbing Su, Chao He, Xiaoming Yang, Xifa Long

    Read original paper ↗ ·

  7. Exploration of antimony( iii ) oxyhalides via single-site substitution in quest of large birefringence

    Inorganic Chemistry Frontiers · 2024-01-01

    Chenhui Hu, Dongdong Chu, Xueling Hou, Feng Zhang, Jian Wei Han

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  8. AYSO4F2 (A = K, Rb): [YO4F4] Polyhedra Enhancement of Birefringence in Non-π-Conjugated Sulfate Systems

    Inorganic Chemistry · 2024-02-27

    Zhencheng Wu, Huimin Li, Xueling Hou, Zhihua Yang, Hongsheng Shi

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  9. Hg4(Te2O5)(SO4): A Giant Birefringent Sulfate Crystal Triggered by a Highly Selective Cation

    Journal of the American Chemical Society · 2024-03-08

    Pengfei Li, Chun‐Li Hu, Yafeng Li, Jiang‐Gao Mao, Fang Kong

    Read original paper ↗ ·

  10. Trithionic guanidine: A novel semi-organic short-wave ultraviolet nonlinear optical sulfate with dimeric heteroleptic tetrahedra

    Chinese Chemical Letters · 2024-03-08

    Hongyuan Sha, Dongling Yang, Yanran Shang, Zujian Wang, Rongbing Su, Chao He, Xiaoming Yang, Xifa Long

    Read original paper ↗ ·

  11. Old tree blossoms anew: Research progress on the structures and optical properties of ultraviolet selenites

    Coordination Chemistry Reviews · 2024-06-15

    Pengfei Li, Chun‐Li Hu, Jiang‐Gao Mao, Fang Kong

    Read original paper ↗ ·

  12. Screening Strategy Identifies an Overlooked Deep‐Ultraviolet Transparent Nonlinear Optical Crystal

    Angewandte Chemie · 2024-08-12

    Jia-Xiang Zhang, Qing-Gang Yue, Shenghua Zhou, Xin‐Tao Wu, Hua Lin, Qi‐Long Zhu

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  13. Screening Strategy Identifies an Overlooked Deep‐Ultraviolet Transparent Nonlinear Optical Crystal

    Angewandte Chemie International Edition · 2024-08-12

    Jia-Xiang Zhang, Qing-Gang Yue, Shenghua Zhou, Xin‐Tao Wu, Hua Lin, Qi‐Long Zhu

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  14. Promising Functional Structural Building Unit Trisulfimide (SO2N)33– and Its Contributions to Second Harmonic Generation and Birefringence

    Crystal Growth & Design · 2024-08-14

    Chu‐Feng Zhu, Xin Liu, Rui‐Xi Wang, Li‐Ming Wu, Ling Chen

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  15. Electronic, optical, elastic, piezoelectric and vibrational properties of P63 KLiSO4

    Physica Scripta · 2024-11-06

    Zhen‐Long Lv, Shijie Lv, Hong‐Ling Cui

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  16. The New Paradigm of Ligand Substitution-Driven Enhancement of Anisotropy from SO4 Units in Short-Wavelength Region

    ACS Central Science · 2024-11-27

    Chenhui Hu, Huimin Li, Guangsheng Xu, Zhihua Yang, Jian Wei Han, Shilie Pan

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  17. Dual Lone Pair Strategy for High Birefringence in Antimony(III)-Based Tellurite Sulfates with Short-Wave UV Transparency

    Inorganic Chemistry · 2025-01-24

    Jiale Xue, Shuyao Wang, Xiande Peng, Zhengyan Lin, Xuehua Dong, Liling Cao, Ling Huang, Guohong Zou

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  18. From AgHgI(SO4) to AgHg3I3.2Cl1.8(SO4): Symmetry Breaking of the Belousovite‐Type Topology by Mixed Halides to Achieve Strong Nonlinear Optical Effect

    Laser & Photonics Review · 2025-04-30

    Qian‐Qian Chen, Ming‐Zhi Zhang, Jin Chen, Bingxuan Li, Chun‐Li Hu, Jiang‐Gao Mao

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  19. Direct Deep‐UV Second‐Harmonic Generation in Disordered Χ 2 ‐Modulated Ferroelectric Crystals

    Advanced Materials · 2025-09-07

    Yabo Wu, Cui Chen, Guopeng Han, Ying Wang, Fuming Li, Fangfang Zhang, Zhihua Yang, Shilie Pan

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  20. π-Conjugated unit bridge for giant second-harmonic generation and birefringence in hybrid materials with dual heteroleptic polyhedra

    Chinese Chemical Letters · 2025-11-01

    Yumei Zhang, Wen‐Dong Yao, Yifan Fu, Zhen-Cheng Wu, Zhen-Cheng Wu, Wenlong Liu, Wenlong Liu, Jiajing Wu, Sheng‐Ping Guo

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  21. Rational design of novel mixed metal sulfates with diverse dimensional structures and short UV cutoff edges

    Journal of Molecular Structure · 2025-11-22

    Bingchen Xiao, Yanyan Ding, Jindan Tian, Lei Hou, Ming Xi, Ruoyan Qv, Yaoqing Chu, Lili Liu

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  22. Confinement π‐Conjugated Moiety Tailoring to Achieve Record Deep‐UV Nonlinearity in Sulfates

    Angewandte Chemie · 2026-03-05

    Yujie Fan, Cheng Hu, Li Wu, Chensheng Lin, Chao Wang, Huixin Fan, Tao Yan, Min Luo

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  23. Crystal Growth, Structure and Optical Properties of (NH 4 ) 2 Mg(SO 4 ) 2 ·6H 2 O: A Crystal With a Wide Deep Ultraviolet Window

    ChemistrySelect · 2026-04-01

    Ling Chen, Qianzhen Zhang, Xifa Long, Yun Mo Yang

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  24. The Enhancement of Phase‐Matching Capability by Recombining π‐Conjugated Group in Nonlinear Optical Sulfates

    Advanced Optical Materials · 2026-04-25

    Lilin Yang, Qinghe Li, Dongling Yang, Hongyuan Sha, Zujian Wang, Xiaoming Yang, Rongbing Su, Bin Su, Chao He, Xifa Long

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  25. Toward the vacuum-ultraviolet frontier in nonlinear optical frequency conversion: phase-matching mechanisms across dimensions and architectures

    Progress in Materials Science · 2026-07-09

    Zhihua Yang, Shilie Pan

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  26. Emergent Deep‐Ultraviolet Ferroelectrics: Structure and Polarization Mechanism

    Advanced Functional Materials · 2026-08-31

    Zujian Wang, Hongyuan Sha, Xiaoming Yang, Chao He, Fangfang Zhang, Xifa Long, Shilie Pan

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  27. Two Rare Earth-Based Sulfates with Enhanced Birefringence and Broad Optical Transparency Window

    Crystal Growth & Design · 2026-09-08

    Chang Liu, Ji Qi, Zhenchao Bai, Yong Wang, Weiqi Huang, Lina Li, Junhua Luo

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