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RESEARCH PAPER · Advanced Optical Materials · 2022

An Optimized KBe2BO3F2‐Like Structure: The Unity of Deep‐Ultraviolet Transparency, Nonlinear Optical Property, and Ferroelectricity

Hongyuan Sha, Junxin Xu, Zheyao Xiong, Zujian Wang, Rongbing Su, Chao He, Xiaoming Yang, Xifa Long, Ying Liu

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An Optimized KBe2BO3F2‐Like Structure: The Unity of Deep‐Ultraviolet Transparency, Nonlinear Optical Property, and FerroelectricityOriginalLiNaB6O9F2: A Promising UV NLO Crystal Having Fluorine‐Directed Optimal Performances and Double Interpenetrating 3[B6O9F2]∞ Networks33M(NH2SO3)2·xH2O (M = Ca, Pb, x = 0, 1, 4): Effect of Hydrogen Bonding on Structural Transformations and Second Harmonic Generation of Metal Sulfamates26A series of novel phosphites/phosphates with deep-ultraviolet cut-off edges from 0D polar to 3D non-polar architectures13Achieving broadband ultraviolet to mid-infrared transparency in germanate-based nonlinear optical crystals Cs 3 REGe 3 O 9 (RE = Y, Gd)16Anisotropic structure building unit involving diverse chemical bonds: a new opportunity for high-performance second-order NLO materials181Tetrahedron-based deep-ultraviolet nonlinear optical crystal with optimized KBe 2 BO 3 F 2 -like structure and disordered cations2Recent advances in non-π-conjugated nonlinear optical sulfates with deep-UV absorption edge53Spatial Frequency Manipulation of a Quartz Crystal for Phase‐Matched Second‐Harmonic Vacuum Ultraviolet Generation16The Strategy to Improve the Phase Matching Ability in Tetrahedron‐Based Deep‐Ultraviolet Nonlinear Optical Crystals21Nonlinear optical inorganic sulfates: The improvement of the phase matching ability driven by the structural modulation41Li2RbSO4Cl with a Short Ultraviolet Absorption Edge and an Acentric Structure through Assembling Heteroleptic [LiO3Cl] Tetrahedra2A chiral sodium lanthanum sulfate for second-order nonlinear optics and proton conduction6KBa 3 M 2 F 14 Cl (M = Zr, Hf): novel short-wavelength mixed metal halides with the largest second-harmonic generation responses contributed by mixed functional moieties37Trithionic guanidine: A novel semi-organic short-wave ultraviolet nonlinear optical sulfate with dimeric heteroleptic tetrahedra14A3Sc(SO4)3 (A = K, Rb, Cs): Three Deep‐Ultraviolet Transparent Alkali‐Scandium Sulfates with Strong Second‐Harmonic Generation Response and High Thermal Stability14Promising Functional Structural Building Unit Trisulfimide (SO2N)33– and Its Contributions to Second Harmonic Generation and Birefringence1A new-type electro-optic crystal: K3Nb3B2O125Hg 2 (HTe 2 O 5 )(PO 4 ): a novel phosphate crystal with enhanced birefringence enabled by the synergistic modification of multiple functional groups12Designing a 3‐Hydroxypropane‐1‐Sulfonate Deep‐Ultraviolet Nonlinear Optical Crystal9Tailoring ordered structures with distorted [TeO 3 ] and aligned [ScO 6 ] motifs for balanced nonlinear optical properties in rare-earth tellurate crystals5Confinement π‐Conjugated Moiety Tailoring to Achieve Record Deep‐UV Nonlinearity in Sulfates0Emergent Deep‐Ultraviolet Ferroelectrics: Structure and Polarization Mechanism0

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  1. LiNaB6O9F2: A Promising UV NLO Crystal Having Fluorine‐Directed Optimal Performances and Double Interpenetrating 3[B6O9F2]∞ Networks

    Advanced Optical Materials · 2022-12-03

    Xiaojing Li, Zilong Chen, Fuming Li, Fangfang Zhang, Zhihua Yang, Shilie Pan

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  2. M(NH2SO3)2·xH2O (M = Ca, Pb, x = 0, 1, 4): Effect of Hydrogen Bonding on Structural Transformations and Second Harmonic Generation of Metal Sulfamates

    Inorganic Chemistry · 2022-12-12

    Danyang Dou, Bingjie Cai, Bingbing Zhang, Ying Wang

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  3. A series of novel phosphites/phosphates with deep-ultraviolet cut-off edges from 0D polar to 3D non-polar architectures

    CrystEngComm · 2023-01-01

    Yucheng Hao, Yang Zhang, Yuying Zhang, Zixiang Fu, Chunyang Heng, Junjie Li, Jiatian You, Kunhong Hu, Yuan Hua Lin, Haijian Li

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  4. Achieving broadband ultraviolet to mid-infrared transparency in germanate-based nonlinear optical crystals Cs 3 REGe 3 O 9 (RE = Y, Gd)

    Inorganic Chemistry Frontiers · 2023-01-01

    Jinmiao Jiao, Conggang Li, Yuheng She, Ning Ye, Zhanggui Hu, Yicheng Wu

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  5. Anisotropic structure building unit involving diverse chemical bonds: a new opportunity for high-performance second-order NLO materials

    Chemical Society Reviews · 2023-01-01

    Xin Liu, Yi‐Chang Yang, Mengyue Li, Ling Chen, Li‐Ming Wu

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  6. Tetrahedron-based deep-ultraviolet nonlinear optical crystal with optimized KBe 2 BO 3 F 2 -like structure and disordered cations

    New Journal of Chemistry · 2023-01-01

    Junxin Xu, Hongyuan Sha, Yanran Shang, Zujian Wang, Rongbing Su, Chao He, Xiaoming Yang, Xifa Long

    Read original paper ↗ ·

  7. Recent advances in non-π-conjugated nonlinear optical sulfates with deep-UV absorption edge

    Chinese Journal of Structural Chemistry · 2023-02-24

    Chen Xu, Yanqiang Li, Junhua Luo, Sangen Zhao

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  8. Spatial Frequency Manipulation of a Quartz Crystal for Phase‐Matched Second‐Harmonic Vacuum Ultraviolet Generation

    Laser & Photonics Review · 2023-06-27

    Mingchuan Shao, Fei Liang, Zhongmian Zhang, Haohai Yu, Huaijin Zhang

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  9. The Strategy to Improve the Phase Matching Ability in Tetrahedron‐Based Deep‐Ultraviolet Nonlinear Optical Crystals

    Advanced Optical Materials · 2023-07-09

    Hongyuan Sha, Yanran Shang, Zujian Wang, Rongbing Su, Chao He, Xiaoming Yang, Xifa Long

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  10. Nonlinear optical inorganic sulfates: The improvement of the phase matching ability driven by the structural modulation

    Coordination Chemistry Reviews · 2023-08-02

    Yanran Shang, Junxin Xu, Hongyuan Sha, Zujian Wang, Chao He, Rongbing Su, Xiaoming Yang, Xifa Long

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  11. Li2RbSO4Cl with a Short Ultraviolet Absorption Edge and an Acentric Structure through Assembling Heteroleptic [LiO3Cl] Tetrahedra

    Inorganic Chemistry · 2023-08-08

    Huanhuan Cheng, Fuming Li, Juanjuan Lu, Xueling Hou

    Read original paper ↗ ·

  12. A chiral sodium lanthanum sulfate for second-order nonlinear optics and proton conduction

    Inorganic Chemistry Frontiers · 2024-01-01

    Hao Fu, Xiaohui Zhang, Peiyu Liu, Bo Li, Baolin Wu, Ye Tao, Qianshuang Lu, Yingjie Li, Jiaxi Huang, Fangfang Zhang, Tingchao He, Zhi Chen, Heng Wang, Chenliang Su, Hong‐Ying Zang, Xiujun Yu, Xiaopeng Li

    Read original paper ↗ ·

  13. KBa 3 M 2 F 14 Cl (M = Zr, Hf): novel short-wavelength mixed metal halides with the largest second-harmonic generation responses contributed by mixed functional moieties

    Chemical Science · 2024-01-01

    Mei Yan, Chun‐Li Hu, Ru‐Ling Tang, Wen‐Dong Yao, Wenlong Liu, Sheng‐Ping Guo

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  14. Trithionic guanidine: A novel semi-organic short-wave ultraviolet nonlinear optical sulfate with dimeric heteroleptic tetrahedra

    Chinese Chemical Letters · 2024-03-08

    Hongyuan Sha, Dongling Yang, Yanran Shang, Zujian Wang, Rongbing Su, Chao He, Xiaoming Yang, Xifa Long

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  15. A3Sc(SO4)3 (A = K, Rb, Cs): Three Deep‐Ultraviolet Transparent Alkali‐Scandium Sulfates with Strong Second‐Harmonic Generation Response and High Thermal Stability

    Advanced Optical Materials · 2024-07-16

    Zilong Geng, Ruibiao Fu, Zuju Ma, Xintao Wu

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  16. Promising Functional Structural Building Unit Trisulfimide (SO2N)33– and Its Contributions to Second Harmonic Generation and Birefringence

    Crystal Growth & Design · 2024-08-14

    Chu‐Feng Zhu, Xin Liu, Rui‐Xi Wang, Li‐Ming Wu, Ling Chen

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  17. A new-type electro-optic crystal: K3Nb3B2O12

    Journal of Materiomics · 2024-12-14

    Lingfei Lv, Xiaoming Yang, Hongjiang Wu, Rongbing Su, Zujian Wang, Bin Su, Pai Shan, Bingxuan Li, Xifa Long, Ge Zhang, Feng Xu, Chao He

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  18. Hg 2 (HTe 2 O 5 )(PO 4 ): a novel phosphate crystal with enhanced birefringence enabled by the synergistic modification of multiple functional groups

    Inorganic Chemistry Frontiers · 2025-01-01

    Pengfei Li, Chun‐Li Hu, Bo Zhang, Jiang‐Gao Mao, Fang Kong

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  19. Designing a 3‐Hydroxypropane‐1‐Sulfonate Deep‐Ultraviolet Nonlinear Optical Crystal

    Small · 2025-05-02

    Yuexin Zhang, Zhengnan Yuan, Yanqiang Li, Yipeng Song, Weiqi Huang, Yao Yao, Ji Qi, Zhiyong Bai, Sangen Zhao, Junhua Luo

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  20. Tailoring ordered structures with distorted [TeO 3 ] and aligned [ScO 6 ] motifs for balanced nonlinear optical properties in rare-earth tellurate crystals

    Chemical Science · 2025-11-18

    Xiaoxu Wang, Tinghui Zhang, Huijian Zhao, Ning Jia, Hongjun Liu, Ning Ye, Zhanggui Hu, Conggang Li

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  21. Confinement π‐Conjugated Moiety Tailoring to Achieve Record Deep‐UV Nonlinearity in Sulfates

    Angewandte Chemie · 2026-03-05

    Yujie Fan, Cheng Hu, Li Wu, Chensheng Lin, Chao Wang, Huixin Fan, Tao Yan, Min Luo

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  22. Emergent Deep‐Ultraviolet Ferroelectrics: Structure and Polarization Mechanism

    Advanced Functional Materials · 2026-08-31

    Zujian Wang, Hongyuan Sha, Xiaoming Yang, Chao He, Fangfang Zhang, Xifa Long, Shilie Pan

    Read original paper ↗ ·
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