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RESEARCH PAPER · Journal of the American Chemical Society · 2022

Catalytic Chemical Recycling of Post-Consumer Polyethylene

Alejandra Arroyave, Shilin Cui, Jaqueline C. Lopez, Andrew L. Kocen, Anne M. LaPointe, Massimiliano Delferro, Geoffrey W. Coates

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Catalytic Chemical Recycling of Post-Consumer PolyethyleneOriginalStimuli-cleavable moiety enabled vinyl polymer degradation and emerging applications12Tandem oxidative and thermal cracking of polypropylene at low temperatures21Cationic Tantalum Hydrides Catalyze Hydrogenolysis and Alkane Metathesis Reactions of Paraffins and Polyethylene38Notizen aus der Chemie0Recent Advances in Catalytic Chemical Recycling of Polyolefins104Ring‐opening Polymerization of Enantiopure Bicyclic Ether‐ester Monomers toward Closed‐loop Recyclable and Crystalline Stereoregular Polyesters via Chemical Upcycling of Bioplastic69Ring‐opening Polymerization of Enantiopure Bicyclic Ether‐ester Monomers toward Closed‐loop Recyclable and Crystalline Stereoregular Polyesters via Chemical Upcycling of Bioplastic2Hybrid Monomer Design Synergizing Property Trade‐offs in Developing Polymers for Circularity and Performance63Hybrid Monomer Design Synergizing Property Trade‐offs in Developing Polymers for Circularity and Performance4Degradation of Polyacrylates by One-Pot Sequential Dehydrodecarboxylation and Ozonolysis82Polyethylene Incorporating Diels–Alder Comonomers: A “Trojan Horse” Strategy for Chemically Recyclable Polyolefins3Polyethylene Incorporating Diels–Alder Comonomers: A “Trojan Horse” Strategy for Chemically Recyclable Polyolefins87Sustainable developments in polyolefin chemistry: Progress, challenges, and outlook204α,ω-Diene Generation from Ethylene and Butadiene by Copolymer Upcycling6Hydrogen-free catalytic depolymerization of waste polyolefins at mild temperatures43Upcycling of polyethylenes by catalysis0Regulating crystalline morphology jointly by dynamic shearing and solid phase stretching endows polyethylene high modulus, strength and heat-resistance6Modular Alcohol Click Chemistry Enables Facile Synthesis of Recyclable Polymers with Tunable Structure23Modular Alcohol Click Chemistry Enables Facile Synthesis of Recyclable Polymers with Tunable Structure1Treasuring trash: Pt/SrTiO3 catalysts process plastic waste into high-value materials25Activity of Silica-Alumina for the Conversion of Polyethylene into Tunable Aromatics Below Pyrolytic Temperatures20High‐Density Polyethylene with In‐Chain Photolyzable and Hydrolyzable Groups Enabling Recycling and Degradation59High‐Density Polyethylene with In‐Chain Photolyzable and Hydrolyzable Groups Enabling Recycling and Degradation6Homogeneous Catalysis in Plastic Waste Upcycling: A DFT Study on the Role of Imperfections in Polymer Chains15Current Advances and Challenges in Chemical Recycling of Polymeric Materials5Circularizing PET-G Multimaterials: Life Cycle Assessment and Techno-Economic Analysis24Recent Advances in the Functionalized Poly(α-Hydroxy Acids) Synthesized fromO-Carboxyanhydrides4Thermally Robust yet Deconstructable and Chemically Recyclable High‐Density Polyethylene (HDPE)‐Like Materials Based on Si−O Bonds55Thermally Robust yet Deconstructable and Chemically Recyclable High‐Density Polyethylene (HDPE)‐Like Materials Based on Si−O Bonds17Acrylate-Induced β-H Elimination in Coordination Insertion Copolymerizaton Catalyzed by Nickel24High-performance chlorinated polyvinyl chloride/polyurea nanocomposite foam with excellent solvent resistance, flame-triggered shape memory effect and its upcycling14Cyclic Polyesters with Closed‐Loop Recyclability from A New Chemically Reversible Alternating Copolymerization13Selective Electrocatalytic Degradation of Ether‐Containing Polymers31Selective Electrocatalytic Degradation of Ether‐Containing Polymers1A butadiene-derived semicrystalline polyolefin with two-tiered chemical recyclability23A facile methodology for side- and upcycling of HDPE waste via partial creation of unsaturated double bonds12Controlled degradation of chemically stable poly(aryl ethers) via directing group-assisted catalysis6Depolymerization of waste polyethylene to linear alkenes via sequential dehydrogenation and metathesis19Modern mechanistic approaches for the depolymerization of commodity plastics via organometallic catalysis0Sustainable carbonaceous raw materials: A contribution to reduce the negative environmental impacts of chemical industry7Sustainable high-density polyethylene via chemical recycling: From modification to polymerization methods45A Closed‐Loop Recyclable Low‐Density Polyethylene23Dynamic Chemistry Toolbox for Advanced Sustainable Materials24Chemically Recyclable Linear and Branched Polyethylenes Synthesized from Stoichiometrically Self-Balanced Telechelic Polyethylenes82Upcycling Waste Plastics with a C–C Backbone by Heterogeneous Catalysis45Circular olefin copolymers made de novo from ethylene and α-olefins83Supported Platinum Nanoparticles Catalyzed Carbon–Carbon Bond Cleavage of Polyolefins: Role of the Oxide Support Acidity27Synthesis and Deconstruction of Polyethylene-type Materials194Chloride and Hydride Transfer as Keys to Catalytic Upcycling of Polyethylene into Liquid Alkanes3Chloride and Hydride Transfer as Keys to Catalytic Upcycling of Polyethylene into Liquid Alkanes29Industrialized fine physical regeneration process and economic benefit assessment for recycling waste HDPE containers13Enabling Closed‐Loop Circularity of “Non‐Polymerizable” α, β‐Conjugated Lactone Towards High‐Performance Polyester with the Assistance of Cyclopentadiene23Enabling Closed‐Loop Circularity of “Non‐Polymerizable” α, β‐Conjugated Lactone Towards High‐Performance Polyester with the Assistance of Cyclopentadiene2The Overlooked Potential of Sulfated Zirconia: Reexamining Solid Superacidity Toward the Controlled Depolymerization of Polyolefins11Recyclable and (Bio)degradable Polyesters in a Circular Plastics Economy400Mechanism-Guided Discovery of Cleavable Comonomers for Backbone Deconstructable Poly(methyl methacrylate)44Solvent-Regulated Tandem Oxidative Degradation of Polyethylene to Multifunctional Chemicals17Conversion of Polyethylene to Low-Molecular-Weight Oil Products at Moderate Temperatures Using Nickel/Zeolite Nanocatalysts6i PP/HDPE blends compatibilized by a polyester: An unconventional concept to valuable products25Deconstruction of Polymers through Olefin Metathesis101Closed‐Loop Recycling of Mixed Plastics of Polyester and CO2‐Based Polycarbonate to a Single Monomer33Closed‐Loop Recycling of Mixed Plastics of Polyester and CO2‐Based Polycarbonate to a Single Monomer3Hydrocarboxylation of C═C Bonds in Polycyclooctene: Progress Toward Valorization of Waste Polyolefins8Catalytic chemical recycling and upcycling of polyolefin plastics27Designed to Degrade: Tailoring Polyesters for Circularity168Mild Catalytic Degradation of Crystalline Polyethylene Units in a Solid State Assisted by Carboxylic Acid Groups23Pyrolysis of high-density polyethylene: Degradation behaviors, kinetics, and product characteristics73Deconstruction of unsaturated polymers through photo-mediated oxidation under O27Copolymerization of Olefins and Conjugated Dienes: A Promising Approach to Produce Recyclable Polyolefins14Dehydrogenated Polyethylene from Discarded Plastics as a Synthon for Functional Polyolefins9Synthesis, Characterization, and Application of High-Molecular-Weight Polyethylene-like Polycarbonates: Toward Sustainable and Recyclable Fibers20Circular Melt-Spun Textile Fibers from Polyethylene-like Long-Chain Polyesters7Oxidative Polymer Degradation via Cope Elimination10New sustainable polymers with on-demand depolymerization property88Catalytic Upcycling of Polyolefins316Modulating the Contact Angle between Nonpolar Polymers and SiO2 Nanoparticles4Depolymerization of Polycarbonates by Transesterification without Using Base, Ionic Liquid, and Additives8Oxidative degradation and upcycling of polyethylene wastes40N2O deconstruction of polycyclooctene to generate carbonyl-functionalized macromonomers3Selective Upcycling of Polyolefins into High-Value Nitrogenated Chemicals80Electrochemical Postpolymerization Modification and Deconstruction of Macromolecules23Installing a Trigger to Upcycle High-Density Polyethylene42Chemically recyclable polyvinyl chloride-like plastics24Upcycling of polyethylene waste to biodegradable adhesive and coating via Baeyer-Villiger reaction: A new view on oxidation-fracture mechanism and structure-function relationship10Upcycling polyethylene into closed-loop recyclable polymers through titanosilicate catalyzed C-H oxidation and in-chain heteroatom insertion50Photooxidation of Polyolefins to Produce Materials with In‐Chain Ketones and Improved Materials Properties2Photooxidation of Polyolefins to Produce Materials with In‐Chain Ketones and Improved Materials Properties32Hydroesterification of Polycyclooctene to Access Linear Ethylene Ethyl Acrylate Copolymers as a Step Toward Polyolefin Functionalization6Room-temperature co-upcycling of polyvinyl chloride and polypropylene50Kinetic Models for Polymer Upcycling by Tag-and-Cut Strategies6Highly Selective, Catalyst‐Free, and Low Temperature Depolymerizable Styrene Copolymer With Incorporated α‐Methylstyrene Structural Units3Depolymerization by transition metal complexes: strategic approaches to convert polymeric waste into feedstocks3Co-upcycling of mixed polypropylene and polyesters5Ethylene and alkyl acrylate copolymers made-to-order using dynamic cation switching polymerization and evidence for improved polymer degradability with low polar group density0Low temperature polyolefin deconstruction via tandem cracking-hydrogenation2Oxidation upcycling of polyethylene into degradable, recyclable and high-performance materials4Recent developments in recycling of post-consumer polyethylene waste33Sustainability in Thermoplastics and Polymer Composites0Upcycling Polynorbornene Derivatives into Chemically Recyclable Multiblock Linear and Thermoset Plastics8Upcycling Polynorbornene Derivatives into Chemically Recyclable Multiblock Linear and Thermoset Plastics6Strategies and technologies for sustainable plastic waste treatment and recycling17Ruthenium‐Catalyzed Deconstruction of Polyolefins: A Strategy to Up‐cycle Waste Polyethylene to Value‐Added Alkene1Ruthenium‐Catalyzed Deconstruction of Polyolefins: A Strategy to Up‐cycle Waste Polyethylene to Value‐Added Alkene20Synthesis of Telechelic Isotactic Polypropylenes for Circular Polypropylene-like Materials via Chain Transfer Polymerization32Synthesis of Polyamides Bearing Directing Groups and Their Catalytic Depolymerization3Modulating Polyethylene Mimics with Degradability via Synthesis and Modeling22Catalytic closed-loop recycling of polyethylene-like materials produced by acceptorless dehydrogenative polymerization of bio-derived diols45Repurposing Post‐Consumer Polyethylene to Access Cross‐Linked Polyethylene with Reprocessability, Recyclability, and Tunable Properties18Repurposing Post‐Consumer Polyethylene to Access Cross‐Linked Polyethylene with Reprocessability, Recyclability, and Tunable Properties2Tailored synthesis of circular polyolefins27Advances and Challenges in Low‐Temperature Upcycling of Waste Polyolefins via Tandem Catalysis25Advances and Challenges in Low‐Temperature Upcycling of Waste Polyolefins via Tandem Catalysis2High Molecular Weight Biobased Long-Chain Aliphatic Polyesters with Degradability: Insights into Mimicking Polyethylene24Synthesis and Tunable Properties of Chemically Recyclable Multiblock Copolymers via Tandem Olefin Metathesis Polymerizations6Upcycling of Polyethylene through Sustainable Introduction of In-Chain Amides Using Zeolite Catalysis5Probing the Catalytic Degradation of Unsaturated Polyolefin Materials via Fe‐Based Lewis Acids‐Initiated Carbonyl–Olefin Metathesis18Probing the Catalytic Degradation of Unsaturated Polyolefin Materials via Fe‐Based Lewis Acids‐Initiated Carbonyl–Olefin Metathesis1On-demand, readily degradable Poly-2,3-dihydrofuran enabled by anion-binding catalytic copolymerization3Fluoropolymer Composites from Partially Perfluoroalkylated Waste Polyethylene4Short chain branched polyethylene polyester segmented copolymers2From Polyethylene to Conjugated Polyenes: a Mechanochemical One‐Pot Upcycling Strategy for Selective Functionalization1Catalytic and selective chemical recycling of post-consumer rubbers into cycloalkenes17Nitroarene Photoactivation Promotes Oxidative Deconstruction of Olefinic Polymers8Recyclable Cross-Linked Polyethylene from Self-Condensing Telechelic Polyethylene by Combining Olefin Metathesis, Hydrogenation, and Transesterification4Photocatalytic Transformation of Isotactic Polypropylene Using Phthalimide N‐Oxyl Radicals Under Mild Conditions2Sustainable and Orthogonally Closed-Loop Recyclable Acetal-Based Long-Chain Polyesters19Brewing By-Products: Source, Nature, and Handling in the Dawn of a Circular Economy Age8Polyethylene-like Polyesters: Strategies for Tailoring Mechanical Properties and Adhesion Performance6Post‐Synthetic Amide Insertion Into Polyethylenes Augments Diverse Physical Properties and Enables Branching‐Dependent Recyclability5High‐Density Polyethylenes with Dual Degradability Enabled by In‐Chain Photolyzable and Mechanoresponsive Units6Waste Rubber-Polyethylene Composite Materials for Enhancement of Mechanical, Thermal, and Electrical Properties–A Critical Review0Incorporation of Oxime Functionality into Polyolefins via Iron-Catalyzed C–H Imidoylation4Chemoenzymatic cascade depolymerization of plastics7Recyclable Biomass-Derived Polyethylene-like Plastics6A comprehensive review on the sustainable approach of fossil-based polymers toward bio-based polymers9Upcycling Waste Polyvinyl Chloride into Single‐Atom Catalysts for Versatile Electrocatalytic and Hydrogenation Reactions1Waste plastic upcycling via homogeneous catalytic hydrogenation/dehydrogenation/transfer hydrogenation4Catalytic Alternating Copolymerization to Access Mechanoresponsive Cyclic Olefin Copolymers with On-Demand Recyclability12Interfacial chain-growth polymerization enables polypropylene-like and circular polythioglycolide14Functionalizations of C─H and C═C Bonds in Polyolefins Catalyzed by Transition‐Metal Complexes14Main-Chain Ketone Installation in Polyethylene Chains: A Metal-Free Strategy toward Photodegradable Plastics18Precision Oligomeric Building Blocks toward Chemically Recyclable Polyolefin-like Materials4A Multiply and Long‐Chain Branched Polyolefin with Low Density Polyethylene (LDPE)‐Like Properties Containing Two Types of Functional Groups3A Multiply and Long‐Chain Branched Polyolefin with Low Density Polyethylene (LDPE)‐Like Properties Containing Two Types of Functional Groups0Advances in sustainable polyolefins: synthesis, chemical transformation and recycling23Research on the manufacture and environmental assessment of vibration and structure-borne sound insulation foams from packaging film waste0Transforming Waste Cooking Oil into Linear and Branched Polyethylene Mimics9Tuning High-Density Polyethylene Microstructure and Properties from Known Distributions of Dynamic Bonds7From inert carbon chains to closed-loop recycling: emerging polyolefin chemistry enabled by telechelic (macro)monomers0Vinylsilanes as Chain-Transfer Agents in Ethylene Polymerization: Direct Synthesis of Heterotelechelic Polyolefins3

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