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RESEARCH PAPER · Science · 2023

Chemical upcycling of polyethylene, polypropylene, and mixtures to high-value surfactants

Zhen Xu, Nuwayo Eric Munyaneza, Qikun Zhang, Mengqi Sun, Carlos Posada, Paul Venturo, Nicholas A. Rorrer, Joel Miscall, Bobby G. Sumpter, Guoliang Liu

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Chemical upcycling of polyethylene, polypropylene, and mixtures to high-value surfactantsOriginalProduction of Low Molecular Oil from Typical Polyolefin Plastics Through Molten Salts Thermal Treatment9Plastic waste recycling is gaining momentum115Stapler Strategies for Upcycling Mixed Plastics0Design of Copolymer‐Based Blend Compatibilizers for Mixed Plastic Recycling38Adulteration of endogenous substances as a next challenge in dairy safety: High-throughput analysis of flavours in goat milk based on the molecular mechanism of flavouring components dynamic changes6Selective Electrocatalytic Degradation of Ether‐Containing Polymers31Selective Electrocatalytic Degradation of Ether‐Containing Polymers1Precise activation of C–C bonds for recycling and upcycling of plastics81Transformation of medical plastic waste to valuable carbon dots: A sustainable recycling of medical waste to efficient fluorescent marker24A facile methodology for side- and upcycling of HDPE waste via partial creation of unsaturated double bonds12A great many Rs0Depolymerization of waste polyethylene to linear alkenes via sequential dehydrogenation and metathesis19Design of depolymerizable polymers toward a circular economy69Heterogeneous oxidative upcycling of polystyrene plastics to benzoic acid under air conditions15Hydroxyl carboxylate anion catalyzed depolymerization of biopolyesters and transformation to chemicals8Mild aqueous metal catalyzed oxidative conversion of low-density polyethylene to low molecular weight aliphatic carboxylic acids15Non-equilibrium plasma co-upcycling of waste plastics and CO 2 for carbon-negative oleochemicals35Solvent-Induced Mobility of Polymer Chains and Solvent-Induced Mobility of Polymer Chains and Metallocene Migration into Ldpe: A Hrmas Nmr Study0Thermal oxo-degradation of plastic wastes to valuable compounds0Upcycling Polyolefin Blends into High-Performance Materials by Exploiting Azidotriazine Chemistry Using Reactive Extrusion69High-performance plastic-derived metal-free catalysts for organic pollutants degradation via Fenton-like reaction10Review on Catalytic Depolymerization of Polyolefin Waste by Hydrogenolysis: State-of-the-Art and Outlook57A novel approach for accurate determination of polyethylene and polypropylene content in polyolefin blends and recyclates by cross-fractionation chromatography17Recycled polymer: Green roads for polyester plastics65Catalytic conversion of mixed polyolefins under mild atmospheric pressure48Upcycling Waste Plastics with a C–C Backbone by Heterogeneous Catalysis45Catalytic Strategies for the Upcycling of Polyolefin Plastic Waste30Chemical recycling of waste plastics: Current challenges and perspectives37Implementing a Doping Approach for Poly(methyl methacrylate) Recycling in a Circular Economy55Ring-Opening Polymerization of Lactones to Prepare Closed-Loop Recyclable Polyesters116Recent Progresses and Challenges in Upcycling of Plastics through Selective Catalytic Oxidation15Synthesis and Deconstruction of Polyethylene-type Materials194Light-driven polymer recycling to monomers and small molecules112Main-Chain Carborane-Embedded Polyethylene14Hydrogen production synergy in non-thermal plasma copyrolysis of low-density polyethylene and cellulose14Complete Degradation of Polyolefin Plastic Wastes to High‐Value Products7Biomimetic versatile wood hybrids with gradient structure towards lightweight, high strength, fire-retardant, and deterioration-resistant materials30Hydrothermal route upcycling surgical masks into dual-emitting carbon dots as ratiometric fluorescent probe for Cr (VI) and corrosion inhibitor in saline solution29Hydrodeoxygenation of Oxygen‐Containing Aromatic Plastic Wastes into Cycloalkanes and Aromatics11Radicals mediated polypropylene waste plastics oxidation into ketone fuel12Thermodynamic and economic analysis of a deployable and scalable process to recover Monomer-Grade styrene from waste polystyrene22The environmental effects of microplastics and microplastic derived dissolved organic matter in aquatic environments: A review70Efficient degradation of vulcanized natural rubber into liquid rubber by catalytic oxidation6Progress and Challenges in Polystyrene Recycling and Upcycling87Oxidative Upcycling of Polyethylene to Long Chain Diacid over Co‐MCM‐41 Catalyst12Oxidative Upcycling of Polyethylene to Long Chain Diacid over Co‐MCM‐41 Catalyst58Positioning dynamic polymeric materials within the modern polymer economy: From application to recycling and circularity10Ternary Single-Use Packaging Plastic Alloy5i PP/HDPE blends compatibilized by a polyester: An unconventional concept to valuable products25Recent progress of waste plastic upcycling based on multifunctional zeolite catalysts13Advancements and future directions in waste plastics recycling: From mechanical methods to innovative chemical processes136A Mechanistic Understanding of the Activity-Stability Trade-off in PETase2Influence of Autoclave Liner on Polyethylene Hydrogenolysis Selectivity7Lifecycle Management for Sustainable Plastics: Recent Progress from Synthesis, Processing to Upcycling87Catalytic chemical recycling and upcycling of polyolefin plastics27A Highly Sustainable Supramolecular Bioplastic Film with Superior Hydroplasticity and Biodegradability4Chemical upcycling of high-density polyethylene into upcycled waxes as rheology modifiers and paper coating materials12Driving selective upcycling of mixed polyethylene waste with table salt11Stapler Strategies for Upcycling Mixed Plastics49Selective and Controllable Cracking of Polyethylene Waste by Beta Zeolites with Different Mesoporosity and Crystallinity33Bimetal-carbon engineering for polypropylene conversion into hydrocarbons and ketones in a Fenton-like system10High Molecular Weight Product Formation in Polyolefin Chemical Recycling: A Comprehensive Review on Primary and Secondary Products18Polyoxymethylene Upcycling into Methanol and Methyl Groups Catalyzed by a Manganese Pincer Complex18Membrane‐Free Electrocatalytic Co‐Conversions of PBS Waste Plastics and Maleic Acid into High‐Purity Succinic Acid Solid6Membrane‐Free Electrocatalytic Co‐Conversions of PBS Waste Plastics and Maleic Acid into High‐Purity Succinic Acid Solid47Pyrolytic Depolymerization of Polyolefins Catalysed by Zirconium‐based UiO‐66 Metal–Organic Frameworks38Pyrolytic Depolymerization of Polyolefins Catalysed by Zirconium‐based UiO‐66 Metal–Organic Frameworks10Catalyst‐ and Solvent‐Free Upcycling of Poly(Ethylene Terephthalate) Waste to Biodegradable Plastics52Industrial and Laboratory Technologies for the Chemical Recycling of Plastic Waste70Catalytic Upcycling of Polyolefins316Upcycling of polyethylene/polypropylene mixtures promoted by well-controlled multiblock olefin copolymers20Oxidative degradation and upcycling of polyethylene wastes40Selective Upcycling of Polyolefins into High-Value Nitrogenated Chemicals80Key Terms in Plastic Waste Transformation Reactions3Task‐Specific Deep Eutectic Solvent for Efficient Dissolution and Further Accelerating Alkaline Hydrolysis of Polyesters Into Their Monomers18Converting Waste Polyethylene Terephthalate to High Value Monomers by Synergistic Catalysts14Catalytic Installation of Primary Amines Onto Polyolefins for Oligomer Valorization2In-suit cemented strategy enables intumescent flame retardant transition from hyper-hydrophilic to hydrophobic and aggregation flame retardant effect simultaneously in polypropylene47Diethyl phthalate removal in waste gas from plastic formulations by membrane biofilm reactor1Upcycling of polyethylene waste to biodegradable adhesive and coating via Baeyer-Villiger reaction: A new view on oxidation-fracture mechanism and structure-function relationship10Catalytic Hydrodeoxygenation of Mixed Plastic Wastes into Sustainable Naphthenes47Hyperbranched anionic surfactant with superwettability and high alkaline resistance from isobutene upgrading12Polyethylene Recycling via Water Activation by Ball Milling5Polyethylene Recycling via Water Activation by Ball Milling23Reinforcing the Efficiency of Plastic Upgrading through Full‐Spectrum Photothermal Effect Integration of Heat Isolator15Hydroaminoalkylation for Amine Functionalization of Vinyl‐Terminated Polyethylene Enables Direct Access to Responsive Functional Materials14Hydroaminoalkylation for Amine Functionalization of Vinyl‐Terminated Polyethylene Enables Direct Access to Responsive Functional Materials3Electrothermal synthesis of commodity chemicals64HRMAS NMR for Studying Solvent‐Induced Mobility of Polymer Chains and Metallocene Migration Into Low‐Density Polyethylene (LDPE)1Aqu‐Thermoplastics: Recycling Plastics with Water9Chain-length-controllable upcycling of polyolefins to sulfate detergents41Upcycling of polyolefins into detergents2Efficient Hydrogenolysis of Consumer-Grade High-Density Polyethylene Wastes over MgAl-Layered Double Oxide-Supported Ru Catalysts11Microplastics’ impact on soil health and quality: Effect of incubation time and soil properties in soil fertility and pollution extent under the circular economy concept8Room-temperature co-upcycling of polyvinyl chloride and polypropylene50Photothermal Upcycling of Waste Polyvinyl Chloride Plastics27Study on enrichment of value-added oxygenated compounds from lignite by a low carbon cascading utilization4The carbonate exchange reaction strategy for chemical recycling of poly(bisphenol A carbonate) into an epoxy-curing agent8Heterogeneous catalysis strategies for polyolefin plastic upcycling: co-reactant-assisted and direct transformation under mild conditions15Microwave‐Powered Liquid Metal Degradation of Polyolefins30Research progress and challenges in the upcycling of polyolefin plastics through chemical oxidation4Upgrading polyethylene plastic waste into a biodegradable polymer: Harnessing a hybrid chemical oxidation–biological conversion approach18Advances and Challenges for Catalytic Recycling and Upgrading of Real-World Mixed Plastic Waste100Recent Progress in Polyolefin Plastic: Polyethylene and Polypropylene Transformation and Depolymerization Techniques22Upcycling of waste plastics: strategies, status-quo, and prospects3Base-Metal Heterogeneous Catalysts for Upgrading Plastics to Light Olefins3Can mixed plastics be recycled and upcycled without separation?11Circular plastic economy for sustainable development: current advances and future perspectives49Circular polyethylene with low-density in-chain functionalities2Co-upcycling of mixed polypropylene and polyesters5Efficient upgrading of polystyrene plastics to nitriles through a catalytic oxidative amination process9Enhancing the Potential of Hydrothermal Waxes from Polyethylene: Product Characterization and Insights from Solvent Effects0Enhancing the Potential of Hydrothermal Waxes from Polyethylene: Product Characterization and Insights from Solvent Effects0Heterogeneous Fenton-type oxidative degradation of low-density polyethylene to valuable acid products using a nanostructured Fe–CeO 2 solid solution catalyst5Highly energy-efficient hydrogenolysis of high-density polyethylene via hydrogen nonthermal plasma reaction engineering4Influence of functional additives, fillers, and pigments on thermal and catalytic pyrolysis of polyethylene for waste plastic upcycling61Low temperature polyolefin deconstruction via tandem cracking-hydrogenation2Oxidation upcycling of polyethylene into degradable, recyclable and high-performance materials4Recycling of polystyrene waste to mono-aromatic hydrocarbons via intermittent thermal scission5State-of-the-art and perspectives of hydrogen generation from waste plastics80Upcycling of mixed polyolefin wastes to 3D structured carbon Joule heaters for decarbonized hydrogen production12Upcycling of poly(ethylene terephthalate) waste plastics to terephthalonitrile6Upcycling polyethersulfones to luminescent materials by aminolysis4Upgrading of waste polyolefins with non-noble metal catalysts21UV-driven anchor carbon dots towards flame-retardant polypropylene with durable anti-UV aging and recyclable performance0Physicochemical profiles of mixed ruminal microbes in response to surface tension and specific surface area1Conversion of Polypropylene to Light Olefins by HMFI Catalysts below Pyrolytic Temperature: Catalytic, Spectroscopic, and Theoretical Studies3Molecular Design for Dual Circularity: Polyester with Complementary Mechanical and Chemical Recyclability under Mild Conditions3Molecular Design for Dual Circularity: Polyester with Complementary Mechanical and Chemical Recyclability under Mild Conditions1Co-upcycling of polyethylene terephthalate and polyoxymethylene into valuable chemicals13Toward Sustainable Polydienes26Upcycling Polynorbornene Derivatives into Chemically Recyclable Multiblock Linear and Thermoset Plastics8Upcycling Polynorbornene Derivatives into Chemically Recyclable Multiblock Linear and Thermoset Plastics6Progress and prospects in polymer science addressing plastic pollution in marine environments, including the deep-sea floor8Ruthenium‐Catalyzed Deconstruction of Polyolefins: A Strategy to Up‐cycle Waste Polyethylene to Value‐Added Alkene1Ruthenium‐Catalyzed Deconstruction of Polyolefins: A Strategy to Up‐cycle Waste Polyethylene to Value‐Added Alkene20Integrating Community Service into Student Learning: A Model Event of a Plastic Waste Cleanup2Anionic Surfactants from Reactive Separation of Hydrocarbons Derived from Polyethylene Upcycling8Recycling homocarbon backbone polymers toward a circular materials economy12Solar refinery: a disruptive strategy for upcycling plastic wastes3Highly selective upcycling of plastic mixture waste by microwave-assisted catalysis over Zn/b-ZnO68Synthesis and Properties of Isononyl-Extended Multibranched Alcohol Polyether Nonionic Surfactants7Development of Mechanically Tunable Polythiourethane Elastomers for Recyclable Energetic Material3Photocatalytic Conversion of Polyester‐Derived Alcohol into Value‐Added Chemicals by Engineering Atomically Dispersed Pd Catalyst1Photocatalytic Conversion of Polyester‐Derived Alcohol into Value‐Added Chemicals by Engineering Atomically Dispersed Pd Catalyst47Catalytic deconstruction of organic additive-containing plastics44Valorization of Waste Polyester for 1,4-Cyclohexanedimethanol Production22Insights into Chemical Recycling and Upgrading Strategies for Polyolefin-Based Plastics15Advances and Challenges in Low‐Temperature Upcycling of Waste Polyolefins via Tandem Catalysis25Advances and Challenges in Low‐Temperature Upcycling of Waste Polyolefins via Tandem Catalysis2

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