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RESEARCH PAPER · Cell Reports Physical Science · 2023

Metal-catalyzed plastic depolymerization

Kishor V. Khopade, Samir H. Chikkali, Nagaraju Barsu

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Metal-catalyzed plastic depolymerizationOriginalHydrolytic depolymerisation of polyesters over heterogeneous ZnO catalyst26Recent advances in plastic recycling and upgrading under mild conditions147Ultrafast and Selective Chemical Recycling of Pla to Methyl Lactate by Using Mhmds as Facile Catalysts0Ionic Liquid‐Assisted Depolymerization of Condensation Polymers: A Review18Novel dragon fruit peel ash-derived solid catalyst for biodiesel production and PET waste recycling10Advances in catalytic chemical recycling of synthetic textiles43Chemical recycling of poly(butylene terephthalate) into value-added biodegradable poly(butylene adipate- co -terephthalate)21Closed-loop recyclable polymers: from monomer and polymer design to the polymerization–depolymerization cycle106Depolymerization of waste polyethylene to linear alkenes via sequential dehydrogenation and metathesis19Design of depolymerizable polymers toward a circular economy69Direct conversion of esters to imines/enamines and applications to polyester waste upcycling4Modern mechanistic approaches for the depolymerization of commodity plastics via organometallic catalysis0Ni-based catalysts supported on Hbeta zeolite for the hydrocracking of waste polyolefins17ZrH-Catalyzed Semi-Reduction of Esters Enabled by an Imine/Enamine Trap1Review on Catalytic Depolymerization of Polyolefin Waste by Hydrogenolysis: State-of-the-Art and Outlook57Ultrafast and selective chemical recycling of PLA to methyl lactate by using MHMDS as simple catalysts18A silica-supported organocatalyst for polycarbonate methanolysis under mild and economic conditions27Polymeric Carbon Nitride Nanosheets as a Metal‐Free Heterogeneous Catalyst for Highly Efficient Methanolysis of Polycarbonates14Recyclable and (Bio)degradable Polyesters in a Circular Plastics Economy400Hydrogenolysis of Urethanes and Ureas Catalyzed by Manganese Complex Supported by Bidentate PN Ligand11Co-pyrolysis of sewage sludge with hydrogen-rich polythene: Effects on synergistic promotion and bio-oil quality29Counterintuitive chemoselectivity in the reduction of carbonyl compounds27Iron in Organometallic Transformations: A Sustainable Substitute for Noble Metals15Efficient Photolytic Breakdown of Waste Polystyrene Foam Using an “All-in-One” Photo-HAT Reagent at Ambient Conditions21Shape Memory Temperature-Tunable Poly(butylene adipate- co -terephthalate)/Polylactic Acid Foams Prepared by Supercritical CO 2 Foaming15Industrial and Laboratory Technologies for the Chemical Recycling of Plastic Waste70Chemoselective Hydrogenolysis of Urethanes to Formamides and Alcohols in the Presence of More Electrophilic Carbonyl Compounds27Integration with biotechnological approaches for upcycling waste plastics0Study of the co-pyrolysis behavior and bio-oil characterization of walnut shell and polyethylene by thermogravimetric analyzer and bubbling fluidized bed9Hydroborative Depolymerization of Polyesters and Polycarbonates to Diols Catalyzed by Heterogeneous Lanthanum Materials La(CH2C6H4NMe2-o)3@SBA-155Selective Upcycling of Polyolefins into High-Value Nitrogenated Chemicals80Homogeneously catalyzed oxidations to produce chemical intermediates (pharmaceuticals, agrochemicals, and plastics)0Tetravalent metals modulated Zn-based layered double hydroxides and their mixed metal oxides for catalytic depolymerization of carbonyl-coordinating plastic waste13Challenges and opportunities in catalytic hydrogenolysis of oxygenated plastics waste: polyesters, polycarbonates, and epoxy resins44Investigation on co-gasification performances of sewage sludge and polyolefins by thermogravimetric analyze and two-stage fixed bed reactor3Waste to treasure: Upcycling waste express packing to sustainable packaging materials13Copper/Iron Cocatalyzed Depolymerization of Postconsumer Polycarbonate: A One-Pot Strategy to Synthesize Aryl Ethers5Stabilization of ZnO Catalysts for Polyesters Hydrolytic Depolymerization by Incorporation into ZrO2 Lattice: A Polylactic Acid Case Study5Upgrading polyethylene plastic waste into a biodegradable polymer: Harnessing a hybrid chemical oxidation–biological conversion approach18Harnessing borane-potassium cooperativity for sulfurated ring-opening copolymerisation8Harnessing synthetic biology to empower a circular plastics economy1Flash Joule heating for synthesis, upcycling and remediation138Catalyst‐Free Depolymerization of Aromatic and Aliphatic Polyesters Using Me3SiI1Electrochemical Deconstruction of Waste Polyvinylidene Chloride (PVDC) to Value‐Added Products in Batch and Flow16Ruthenium‐Catalyzed Deconstruction of Polyolefins: A Strategy to Up‐cycle Waste Polyethylene to Value‐Added Alkene1Ruthenium‐Catalyzed Deconstruction of Polyolefins: A Strategy to Up‐cycle Waste Polyethylene to Value‐Added Alkene20Recycling Methods of Plastic Materials for Circular and Sustainable Production Design: A Review1Air-Enabled Electricity-Driven Depolymerization of Polyesters1MOF Catalysts for Plastic Depolymerization4MOF Catalysts for Plastic Depolymerization52Synthesis and Characterization of Fully Bio-Based Butylene Succinate Oligomers with Varying Molecular Weights for Sustainable Food Packaging Applications2Promotion effect of nickel on the stability of NiMnAl catalysts for the PET glycolysis1Waste polyethylene to long-chain unsaturated esters and alcohols via alkene cross-metathesis0A Review on Sustainable Upcycling of Plastic Waste Through Depolymerization into High-Value Monomer38Emulsion polymerization of allyl sulfide copolymers for enhanced molar mass0Research and Developments of Heterogeneous Catalytic Technologies20High value olefins from polypropylene by in situ catalytic pyrolysis4AI-accelerated innovations in photodegradation and depolymerization of waste plastics: a critical review on mechanistic insights, environmental impact, and future perspectives6Low Temperature and Efficient Catalytic Depolymerization of Polyethylene Terephthalate Waste1Functional Materials for Environmental Energy Harvesting in Smart Agriculture via Triboelectric Nanogenerators24Metal–Organic Framework for Plastic Depolymerization and Upcycling5Synthesis and characterization of lanthanum supported halloysite nanotubes catalyst in obtaining low molecular weight of liquid epoxidized natural rubber0En route to realistic sustainable structural fiber-reinforced polymers in a circular economy9Oxidation of Biomass to Value-Added Chemicals Using Heterogeneous Solid Base Catalysts: A Recent Advancement0Mitigation strategies for micronanoplastics0Sustainable synthesis of value-added compounds from carbohydrates and carbohydrate-based platform molecules3A chemically recyclable thermosetting elastomer via ring-opening metathesis polymerization0Chemical recycling and repolymerization of poly(ethylene terephthalate), poly(ethylene furanoate), and their copolyesters0Cutting-Edge advances in chemical depolymerization-based recycling of waste polyethylene terephthalate plastics0Microwave-assisted recycling of plastic waste into value-added chemicals: challenges, recent advances, and perspectives0The Future of Waste Engineering and Technological Innovations0Upcycling waste polyoxymethylene to value-added chemicals using reusable polymeric acid catalysts at ppm levels2Chemical Upcycling of Waste Chlorinated Plastics into α,ω-Dienes via Consecutive Dehydrochlorination-Hydrogenation with HCl Trapping and Metathesis1Strong and recyclable bio-derived poly(ester amide) hot-melt adhesive6Transforming plastics at the interface: Electrochemical re- and upcycling strategies5Mechanocatalysis: background and challenges2Chemical Recycling of PET to Its Monomers via Heterogeneous ZnO-Catalysed Ethanolysis2Incorporation of Fully Bio-Based Butylene Succinate Oligomers into Poly(butylene succinate) by Melt Mixing1Noncovalent Interaction-Catalyzed High Conversion of Waste PET Plastics into Organic Esters under Mild Conditions0

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  1. Hydrolytic depolymerisation of polyesters over heterogeneous ZnO catalyst

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  2. Recent advances in plastic recycling and upgrading under mild conditions

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  3. Ultrafast and Selective Chemical Recycling of Pla to Methyl Lactate by Using Mhmds as Facile Catalysts

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  4. Ionic Liquid‐Assisted Depolymerization of Condensation Polymers: A Review

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  5. Novel dragon fruit peel ash-derived solid catalyst for biodiesel production and PET waste recycling

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  6. Advances in catalytic chemical recycling of synthetic textiles

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  7. Chemical recycling of poly(butylene terephthalate) into value-added biodegradable poly(butylene adipate- co -terephthalate)

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  8. Closed-loop recyclable polymers: from monomer and polymer design to the polymerization–depolymerization cycle

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  9. Depolymerization of waste polyethylene to linear alkenes via sequential dehydrogenation and metathesis

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  10. Design of depolymerizable polymers toward a circular economy

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  11. Direct conversion of esters to imines/enamines and applications to polyester waste upcycling

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  12. Modern mechanistic approaches for the depolymerization of commodity plastics via organometallic catalysis

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  13. Ni-based catalysts supported on Hbeta zeolite for the hydrocracking of waste polyolefins

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  14. ZrH-Catalyzed Semi-Reduction of Esters Enabled by an Imine/Enamine Trap

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  15. Review on Catalytic Depolymerization of Polyolefin Waste by Hydrogenolysis: State-of-the-Art and Outlook

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  16. Ultrafast and selective chemical recycling of PLA to methyl lactate by using MHMDS as simple catalysts

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  17. A silica-supported organocatalyst for polycarbonate methanolysis under mild and economic conditions

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  18. Polymeric Carbon Nitride Nanosheets as a Metal‐Free Heterogeneous Catalyst for Highly Efficient Methanolysis of Polycarbonates

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  19. Recyclable and (Bio)degradable Polyesters in a Circular Plastics Economy

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  20. Hydrogenolysis of Urethanes and Ureas Catalyzed by Manganese Complex Supported by Bidentate PN Ligand

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  21. Co-pyrolysis of sewage sludge with hydrogen-rich polythene: Effects on synergistic promotion and bio-oil quality

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  22. Counterintuitive chemoselectivity in the reduction of carbonyl compounds

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  23. Iron in Organometallic Transformations: A Sustainable Substitute for Noble Metals

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  24. Efficient Photolytic Breakdown of Waste Polystyrene Foam Using an “All-in-One” Photo-HAT Reagent at Ambient Conditions

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  25. Shape Memory Temperature-Tunable Poly(butylene adipate- co -terephthalate)/Polylactic Acid Foams Prepared by Supercritical CO 2 Foaming

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  28. Integration with biotechnological approaches for upcycling waste plastics

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  35. Investigation on co-gasification performances of sewage sludge and polyolefins by thermogravimetric analyze and two-stage fixed bed reactor

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  38. Stabilization of ZnO Catalysts for Polyesters Hydrolytic Depolymerization by Incorporation into ZrO2 Lattice: A Polylactic Acid Case Study

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  46. Ruthenium‐Catalyzed Deconstruction of Polyolefins: A Strategy to Up‐cycle Waste Polyethylene to Value‐Added Alkene

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