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RESEARCH PAPER · Chemical Reviews · 2024

Synthesis and Deconstruction of Polyethylene-type Materials

Simon Timm Schwab, Maximilian Baur, Taylor F. Nelson, Stefan Mecking

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Synthesis and Deconstruction of Polyethylene-type MaterialsOriginalAdvances in catalytic chemical recycling of synthetic textiles43Controlled degradation of chemically stable poly(aryl ethers) via directing group-assisted catalysis6Electrochemical recycling of polymeric materials56Ruthenium-catalyzed “open-loop” recycling of polyethylene via tandem isomerization-metathesis (ISOMET)12Balancing Degradability and Mechanical Strength in Keto Modified Polyethylene through Hydrogen Bonds6Encoding Circularity in Polydiketoenamine Thermoplastics via Oxy-Functionalization1Terpenoid-based high-performance polyester with tacticity-independent crystallinity and chemical circularity21Synthesis of long-chain aliphatic poly(β-thioester)s via thiol-Michael polyaddition and their applications in noble metal recovery and information encryption4Circular Melt-Spun Textile Fibers from Polyethylene-like Long-Chain Polyesters7Aldehyde End‐Capped Degradable Polyethylenes From Hydrogen‐Controlled Ethylene/CO Copolymerization29Aldehyde End‐Capped Degradable Polyethylenes From Hydrogen‐Controlled Ethylene/CO Copolymerization2Spontaneous Amino-Acetoacetate Click Polymerization: A Powerful Tool toward Closed-Loop Recyclable Poly(vinylogous urethane)s8Oxidative degradation and upcycling of polyethylene wastes40Correlation of Enzymatic Depolymerization Rates with the Structure of Polyethylene-Like Long-Chain Aliphatic Polyesters15Cross-Linked Polyolefins: Opportunities for Fostering Circularity Throughout the Materials Lifecycle28Tailoring the Properties of Chemically Recyclable Polyethylene‐Like Multiblock Polymers by Modulating the Branch Structure32Tailoring the Properties of Chemically Recyclable Polyethylene‐Like Multiblock Polymers by Modulating the Branch Structure9Enhanced Gas/Oil Production from Catalytic Fast Pyrolysis of Polyethylene over Cu/Ce Co-Modified ZSM-55Oxidative Upcycling of Polyolefin Wastes into the Dynamically Cross-Linked Elastomer25Photooxidation of Polyolefins to Produce Materials with In‐Chain Ketones and Improved Materials Properties2Photooxidation of Polyolefins to Produce Materials with In‐Chain Ketones and Improved Materials Properties32The chemistry of oleates and related compounds in the 2020s16Circular Cross-Linked Polyethylene Enabled by In-Chain Ketones11Research progress and challenges in the upcycling of polyolefin plastics through chemical oxidation4Sustainable Terephthalic Polyesters with Medium/Long Methylene Sequence: Structure–Property Relationships and Closed-Loop Chemical Recycling10Backbone editing and deconstruction of polyethylene by Beckmann rearrangement and hydrogenolysis21Biocatalytic recycling of plastics: facts and fiction25Circular polyethylene with low-density in-chain functionalities2Closed-loop recycling of bio-based disulfide vitrimer via a solvent-and waste-free strategy15Photothermally-driven cobalt catalysed atom transfer radical polymerisation enables isocyanide copolymer synthesis3Recent developments in recycling of post-consumer polyethylene waste33Exploiting unique NP1 interface: Oriented immobilization via electrostatic and affinity interactions in a tailored PDA/PEI microenvironment enhanced by concanavalin A3Molecular Design for Dual Circularity: Polyester with Complementary Mechanical and Chemical Recyclability under Mild Conditions3Molecular Design for Dual Circularity: Polyester with Complementary Mechanical and Chemical Recyclability under Mild Conditions1Functional Polyolefins and Composites76Functional Polyolefins and Composites3Circularity in polydiketoenamine thermoplastics via control over reactive chain conformation4Synthesis of Telechelic Isotactic Polypropylenes for Circular Polypropylene-like Materials via Chain Transfer Polymerization32Synthesis of Polyamides Bearing Directing Groups and Their Catalytic Depolymerization3Modulating Polyethylene Mimics with Degradability via Synthesis and Modeling22Catalytic closed-loop recycling of polyethylene-like materials produced by acceptorless dehydrogenative polymerization of bio-derived diols45Repurposing Post‐Consumer Polyethylene to Access Cross‐Linked Polyethylene with Reprocessability, Recyclability, and Tunable Properties18Repurposing Post‐Consumer Polyethylene to Access Cross‐Linked Polyethylene with Reprocessability, Recyclability, and Tunable Properties2Effect of Cooling Rate and Molecular Weight on the Nonisothermal Crystallization of Polyethylene3Boosting Degradation of Polyethylene at Room Temperature4Innovative upcycling of polyesters and polycarbonates via manganese-catalyzed hydrogenolysis13Tailored synthesis of circular polyolefins27Upcycling waste commodity polymers into high-performance polyarylate materials with direct utilization of capping agent impurities34Catalytic pyrolysis of polyethylene over bimetallic-modified ZSM-5: Role of alkaline sites on structure regulation, thermal behavior and aromatics production9Recyclable plastics from a manganese catalyst3Skeletal Editing of Polymer Backbones and Its Impact Across the Polymer Lifecycle18Graphene quantum dot for thermoplastic nanocomposites—Scope and opportunities1Chain Dynamics of Halogenated Precision Polyethylenes in Different Crystal Polymorphs1Degradation of polyethylene by three bacteria isolated from coastal beach8Upcycling of Polyethylene through Sustainable Introduction of In-Chain Amides Using Zeolite Catalysis5End-Functionalized Biobased Aliphatic Polyesters Exhibiting Unique Emission/Thermal Properties0Efficient catalytic upcycling of polyester and polycarbonate plastics using NNN-based iron catalyst0Direct Synthesis of Poly(adipate)Esters via Catalytic Isomerizing Dual Hydroesterificative Polymerization of 1,3‐Butadiene4Direct Synthesis of Poly(adipate)Esters via Catalytic Isomerizing Dual Hydroesterificative Polymerization of 1,3‐Butadiene7From metabolism to lifespan trade-offs: polyethylene microplastics induce circadian disruption and sex-specific aging in Drosophila melanogaster0Mechanochromic Branched Polyethylenes Synthesized through Ring-opening Metathesis Terpolymerization1Thiol- and Disulfide-Functionalized Polycyclooctene: Metathesis Polymerization, Degradation, and Reformation6Overcoming limitations in polyolefins upcycling by codesigning endothermic-exothermic magnetocatalytic system8Series-parallel structure-directed photogenerated carriers migration accelerates photocatalytic polyolefins-plastics to acetic acid valorization over Co3O4/ZnO@g-C3N4 hollow nanoreactors9Influence of Ester Functionalization on Crystallization and Melting of Polyethylene: Insights from Coarse-Grained Modeling8Re-directing mixed-feed deconstruction products to hybrid polyesters: Tolerance windows for commodity plastics reconstruction3Effect of Nano-Refractory Bricks on the Morphological and Thermal Properties of PVC/LDPE Polymer Blend0Rational design of zeolite-based composite catalysts in catalytic cracking of polyethylene6Polar Functionalization of Polyalphaolefin Lubricants and Polyisobutylenes by Cationic Copolymerization from Ionic Cluster-Type Polar Monomers1Performance-Guided Design of Chemically Recyclable Polymeric Materials: A Case Study on Thermoplastic Elastomers9On-Demand Nonalternating Copolymerization Enables Upcycling of Mixed Polyethylene and Nylon Plastics14Facile Synthesis of Polyhydroperoxides from Ethylene and Carbon Monoxide10Efficient catalytic upcycling of polyester and polycarbonate plastics using an NNN-based iron catalyst7Dual-catalyst system without supported metals toward polyethylene waste upcycling3High‐Density Polyethylenes with Dual Degradability Enabled by In‐Chain Photolyzable and Mechanoresponsive Units6Crystallization of Biobased Long-Chain Aliphatic Polyesters as Sustainable Polymers: Effects of the Diol Structure in the Monomer Unit6Chemically Recyclable and Tunable Polyolefin‐Like Multiblock Copolymer Adhesives2Chemically Recyclable and Tunable Polyolefin‐Like Multiblock Copolymer Adhesives13Waste plastic upcycling via homogeneous catalytic hydrogenation/dehydrogenation/transfer hydrogenation4Synthesis of Hydroxy‐Functionalized Polyethylene via Radical Copolymerization of Ethylene with Alkenyl Boronate and Post‐Polymerization Oxidation1Synthesis of Hydroxy‐Functionalized Polyethylene via Radical Copolymerization of Ethylene with Alkenyl Boronate and Post‐Polymerization Oxidation0Concept of Recycling‐on‐Demand Investigated on Linear Poly(Ester‐Co‐Acetal)s1Sustainable Long-Spaced Polycondensates toward Polyethylene-Like Materials15Advancements in catalyst design and reactor engineering for efficient olefin synthesis from alcohol (C2+) dehydration3Main-Chain Ketone Installation in Polyethylene Chains: A Metal-Free Strategy toward Photodegradable Plastics18Stereospecific Hydroxyl–Yne Click Polymerization to Selectively Construct High-Performance Plastics and Elastomers4Precision Oligomeric Building Blocks toward Chemically Recyclable Polyolefin-like Materials4A comprehensive review on microbial degradation of polyethylene plastics: ecotoxicity, deterioration process, recurrent intermediates and key enzymes involved7Dual-control strategy for selective upgrading of polyethylene waste into jet fuel-range alkanes2Microplastics from Food Packaging: Polymer Degradation Pathways, Environmental Distribution, and Effects on the Human Gastrointestinal Tract34Designing truly sustainable polymers through an integrated three-pillar framework3Advances in sustainable polyolefins: synthesis, chemical transformation and recycling23Biorecycling of polyethylene (PE): an integrated effort in pretreatment, degradation, and upcycling8Plasma Catalysis for Plastic Waste Conversion into Value‐Added Products: Advancements and Perspectives11Synthesis of recyclable polyesters via a cis -fused ring strategy6A scientometric review of polymer foam for core sandwich composites: Trends, networks, and prospects0Selective, Oxygen‐Tunable, and Metal‐Free Functionalization of Polyethylene Through Dual‐Mode Nitrosation and Carbonylation1Selective, Oxygen‐Tunable, and Metal‐Free Functionalization of Polyethylene Through Dual‐Mode Nitrosation and Carbonylation7Rethinking plastics through microbial biodegradation and circular economy innovation – A review21Recent advances in chemical upcycling of plastic waste: microwave-assisted heating and heterogeneous catalysis11Chemically recyclable, fully biobased polyolefins with performance parity to low-density polyethylene11Synthesis and Upcycling of All‐Carbon‐Backbone Degradable Polyethylene with Dispersed On‐Chain Ketones5Synthesis and Upcycling of All‐Carbon‐Backbone Degradable Polyethylene with Dispersed On‐Chain Ketones0Impact of Degradable Linkages on the Crystallization Behaviors of Polyethylene Mimics4Recent advancement on heterogeneous metal catalysts for the upgradation of polyethylene terephthalate plastic waste into bis(2-hydroxyethyl) terephthalate2Living Carbonylative Polymerization of Vinylarenes Using P ‐Chirogentic Pd Catalyst: A Route to Functionalized Polyketone with Chirality Recognition1Living Carbonylative Polymerization of Vinylarenes Using P ‐Chirogentic Pd Catalyst: A Route to Functionalized Polyketone with Chirality Recognition2A study on Sn-doped SrFeO3-δ oxygen carriers for chemical looping oxidative dehydrogenation of ethane3The effect of plastic type on the product distribution and Cr (VI) removal in the co-pyrolysis of plastics and chromium-containing slag1Vinylsilanes as Chain-Transfer Agents in Ethylene Polymerization: Direct Synthesis of Heterotelechelic Polyolefins3Environmental performance of single-use plastic packaging: A life cycle assessment of end-of-life scenarios in the agri-food sector2Incorporating Carbamate Groups into Polyolefin Elastomers for High Performance and Closed-Loop Recyclability5Research progress of high value utilization of waste polyethylene plastics6Benchmarking electro-Fenton-driven decomposition of synthetic polymers0Catalytic valorization of polyolefins: from catalysts and processes to reactors0Controlled ring-opening polymerization of xylose-derived lactones towards sustainable polyesters0Controlling crystallinity in degradable poly(ethylene carbonate) polymers by precision carbonate placement0Flash Joule Heating Conversion of Waste Cross-linked Polyethylene (XLPE) into Graphene: Effects of XLPE Particle Size and Cross-linking0Fully bio-based monopyrrolidone-containing monomers towards the synthesis of renewable polyesters with high T g and hydrolyzable closed-loop recycling0Microstructure of amide-functionalized polyethylenes determined by NMR relaxometry2Palladium-catalyzed copolymerization to synthesize sulfur-containing polyethylene materials0Recent advances in designing high-performance and enzymatically degradable plastics0Selective solvent-free upcycling of polyethylene to lube-oil-range hydrocarbons via tuned acid–metal interactions on TiO 2 –ZrO 2 /Ni0Selectively controlled ring-opening copolymerization to chemically recyclable thermoplastic elastomers1The Coordination Microenvironment Tailoring in 2D MOFs for Enhancing Photocatalytic Acetylene Semi‐Hydrogenation0The Coordination Microenvironment Tailoring in 2D MOFs for Enhancing Photocatalytic Acetylene Semi‐Hydrogenation5Synthesis of discrete oligoethylenes towards chemically recyclable polyolefins3Valorization of Velvet Bean Pod Agricultural Residues in Recycled HDPE Composites: The Role of Recycling Cycles and Maleic Anhydride0On-Demand CO Delivery and Incorporation from Solid Surrogate Enable Compatible Slurry-Phase Ethylene Polymerization4Adaptive laboratory evolution unlocks membrane permeability as a key limitation in long-chain alcohol metabolism by Pseudomonas putida KT24400Mechanically Triggered Chemical Recyclable Polyethylene‐Like Materials1Mechanically Triggered Chemical Recyclable Polyethylene‐Like Materials5Mechanistic pathways and influencing factors in the liquefaction of single and mixed plastics toward waste-to-energy conversion: A structured and critical review1Effect of Middle Diol Repeat Units in Biobased Aliphatic Polyesters on Thermal and Tensile Properties2Fast-Dissociative and Slow-Associative Dual Dynamic Bonds Enable Self-Healing and Recyclable Polyethylene Networks for Sustainable High-Voltage Cable Insulation1Microbe-Mediated Degradation of Polyethylene and Release of Associated Pollutants under Simulated Dark Environments2Dual-Pathway Strategy for Click-Type Functionalization and Programmable Polymer Deconstruction10All-Hydrocarbon Polymers with Chemical Recyclability via a Catalyst-Free and Solvent-Free Method1Sustainable Hybrid Films Based on Ecovio, Sodium Nitrite, and Babassu Mesocarp Starch for Potential Packaging Applications1Light-Programmable Polyester Networks with Movable Cross-Links for On-Demand Enzymatic Degradation1Cooperatively Halide‐ and Benzhydryl‐Modified Bis(imino)pyridylcobalt Complexes for Linear α‐Olefin‐Type Polyethylenes1A plant-receptor-inspired cuprous complex for wearable trace-level ethylene gas sensing1Comparative evaluation of enzymatic, acidic, and alkaline digestion protocols for organic matrix removal from lyophilized and frozen mussel samples (Mytilus galloprovincialis)2Unsaturated biobased polyesters from bicyclic α ‐pinene‐based diols0Accessing Degradable Polyethylenes via Catalytic Ethylene Copolymerization1Safety and Innovation in Conventional Plastics: A Review of Polymer Synthesis and Emerging Technologies2Aqueous Slurry Polymerization of Ethylene by Phosphinephenolato Nickel(II) Complexes: Catalyst Tailoring and Synthesis of Bimodal Polyethylene1Advances in photocatalytic plastics reforming for concurrent hydrogen evolution and selective upgrading0A Comparison of Polyethylene and Polyurethane Blocks on the Stability of Dental Implants: An In Vitro Study0Living and Controlled Ring-Opening (co)Polymerization of PDL Catalyzed by N -Heterocyclic Olefin/Al(C 6 F 5 ) 3 Lewis Pair1

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