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RESEARCH PAPER · Langmuir · 2024

Upcycling Waste Plastics with a C–C Backbone by Heterogeneous Catalysis

Huidong Lv, Fei Huang, Fan Zhang

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Upcycling Waste Plastics with a C–C Backbone by Heterogeneous CatalysisOriginalRecent advances in oxidative degradation of plastics227Ruthenium-catalyzed “open-loop” recycling of polyethylene via tandem isomerization-metathesis (ISOMET)12Oxidative degradation and upcycling of polyethylene wastes40Catalytic recycling of plastics into value-added products28Chirality and Local Electron Density of States in a Two-Dimensional Molecular Crystal Self-Assembled by Prochiral Radical Molecules1Silicate Derived from Phaeodactylum tricornutum for Removal of Polystyrene: Interfacial Effects of Living Organism and Its Derivatives with Nanoplastics2Photooxidation of Polystyrene into High‐Value Chemicals16Chain-length-controllable upcycling of polyolefins to sulfate detergents41Electricity Generation and Plastic Waste Reduction Using the Fungus Paecilomyces as a Biodegrader in Microbial Fuel Cells3Research progress and challenges in the upcycling of polyolefin plastics through chemical oxidation4Upgrading polyethylene plastic waste into a biodegradable polymer: Harnessing a hybrid chemical oxidation–biological conversion approach18A review of commercial plastic waste recycling into graphene materials14Enhancing liquified petroleum gas selectivity through hierarchical porosity in MWW-type MCM-49 zeolite for polyethylene hydrocracking0Morphology engineering of 2D Zn-catalysts to wrinkled particles using NaCl microcrystals: enhanced recyclability for the synthesis of poly(caprolactone)s1Conversion of Polypropylene to Light Olefins by HMFI Catalysts below Pyrolytic Temperature: Catalytic, Spectroscopic, and Theoretical Studies3Anionic Surfactants from Reactive Separation of Hydrocarbons Derived from Polyethylene Upcycling8Advances and Challenges in Low‐Temperature Upcycling of Waste Polyolefins via Tandem Catalysis25Advances and Challenges in Low‐Temperature Upcycling of Waste Polyolefins via Tandem Catalysis2Upgrading polyolefin plastics: experiences from petroleum refining and distinct characteristics19Predicting a generalized mechanism of branched alkane hydrogenolysis on Ru, Ir, and Pt surfaces relevant to polymer upcycling applications3Synthesis, properties, and chemical recyclability of aromatic polyesters using alkylamide diphenolic acid0Recent Advances in the Thermo-Catalytic Upcycling of Polyethylene Waste13Mechanistic alteration of polyethylene oxidation via heterogenous catalysis for enhanced fatty di-carboxylic acid yields6Enzymatic mechanism of polystyrene biodegradation: key depolymerization enzymes in the Stenotrophomonas maltophilia sp. ZSL24937Long-lived metal-zeolite catalysts for polyolefin aromatization via synergistic tandem dehydroaromatization and hydrogenolysis12Recent advances in thermal oxidative upcycling strategy of waste plastics under mild conditions2Phyllosilicate Clay Blended with Semiconductor Nanocomposite for Enhanced Dye Removal and CO 2 Adsorption1Acidified montmorillonite (MMT)-supported ultrafine Ru nanoparticles for polyethylene plastic upcycling0Carbon-modified TiO 2 catalysts for oxidative upcycling of waste polyethylene to dicarboxylic acids1Catalytic valorization of polyolefins: from catalysts and processes to reactors0Highly efficient photoreforming of plastic waste for hydrogen production: recent advances and prospects1Integrating chemical and biological conversion for waste plastics recycling and upcycling toward a circular bioeconomy0Acid sites in hydrogen-involved polyolefin upcycling: mechanistic insights and design principles0Thermal and kinetic modeling of waste plastic pyrolysis process to enhance the process scalability: A state-of-the-art review3Recent advancements in catalytic processes for plastic upcycling into fuels: a major step in sustainable waste management and energy production3Tailoring the polyolefin hydrogenolysis performance of Ru/TiO2 through TiO2 support facet engineering1Oxidative Upcycling of Polybutylene Terephthalate to Dicarboxylic Acids over a Cubic Au/Ca(OH) 2 Catalyst0Revealing the Native Multi-Enzyme Synergy of Acinetobacter calcoaceticus SDH15 for Ultra-Long-Chain Alkane Biodegradation0Enhancing catalytic cracking of polyolefin plastics to heavy waxes over modified calcium aluminate catalysts1Synergistic optimization of catalyst screening and reaction temperature for the catalytic cracking of polyolefins to light olefins0Elucidating the Spatiotemporal Reaction Mechanism of Polyethylene Aromatization over ZSM-5 Zeolites1A Molten Salt-Like Strategy for the Synthesis of Hierarchical NiCoMn-LDH Electrocatalysts for Electrocatalytic Upcycling of Polyethylene Terephthalate Waste0Solar-driven programmable polystyrene upcycling to aromatic hydrocarbons via plasmonic iron nanoparticles0Engineering microbial consortia for polyethylene biodegradation and valorization using a function-driven strategy0

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  1. Recent advances in oxidative degradation of plastics

    Chemical Society Reviews · 2024-01-01

    Sewon Oh, Erin E. Stache

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  2. Ruthenium-catalyzed “open-loop” recycling of polyethylene via tandem isomerization-metathesis (ISOMET)

    Green Chemistry · 2024-01-01

    Vajk Farkas, Pascal Albrecht, Ádám Erdélyi, Márton Nagyházi, Beatrix Csutorás, Gábor Turczel, Norbert Miskolczi, Janka Bobek‐Nagy, Ole Osterthun, Jürgen Klankermayer, Róbert Tuba

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  3. Oxidative degradation and upcycling of polyethylene wastes

    Science China Chemistry · 2024-08-23

    Yizhen Che, Yanfen Wu, Zhiqiang Niu

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  4. Catalytic recycling of plastics into value-added products

    Nano Research · 2024-09-09

    Tianyu Wei, Pengcheng Zhou, Wenxian Liu, Xijun Liu, Tairong Kuang

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  5. Chirality and Local Electron Density of States in a Two-Dimensional Molecular Crystal Self-Assembled by Prochiral Radical Molecules

    Langmuir · 2024-10-03

    Xiangqian Tang, Wenyu Wang, Haitao Tang, Ye Xia, Xinyan Shan, Xinghua Lu

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  6. Silicate Derived from Phaeodactylum tricornutum for Removal of Polystyrene: Interfacial Effects of Living Organism and Its Derivatives with Nanoplastics

    Langmuir · 2024-10-15

    Tingting Yu, Xiong Huang, Hong Li, Jishu Zheng, Lihong Gao, Song Wang, Yuxin Zhang

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  7. Photooxidation of Polystyrene into High‐Value Chemicals

    European Journal of Organic Chemistry · 2024-11-05

    Shaokai Jiang, Yunhan Chen, Yahao Huang, Yahao Huang, Peng Hu

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  8. Chain-length-controllable upcycling of polyolefins to sulfate detergents

    Nature Sustainability · 2024-11-18

    Nuwayo Eric Munyaneza, Ruiyang Ji, Adrian DiMarco, Joel Miscall, Lisa Stanley, Nicholas A. Rorrer, Rui Qiao, Guoliang Liu

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  9. Electricity Generation and Plastic Waste Reduction Using the Fungus Paecilomyces as a Biodegrader in Microbial Fuel Cells

    Sustainability · 2024-12-19

    Segundo Rojas-Flores, Magaly De La Cruz-Noriega, Nélida Milly Otiniano, Luis Cabanillas-Chirinos, Luis Manuel Angelats Silva

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  10. Research progress and challenges in the upcycling of polyolefin plastics through chemical oxidation

    Chinese Science Bulletin (Chinese Version) · 2024-12-19

    Guoli Chen, Lei Huang

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  11. Upgrading polyethylene plastic waste into a biodegradable polymer: Harnessing a hybrid chemical oxidation–biological conversion approach

    Chemical Engineering Journal · 2024-12-21

    Siti Nurjanah Firmansyah, Huashan Sun, Chun‐Jae Yoo, Ja Kyong Ko

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  12. A review of commercial plastic waste recycling into graphene materials

    RSC Advances · 2025-01-01

    Phuoc-Anh Le

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  13. Enhancing liquified petroleum gas selectivity through hierarchical porosity in MWW-type MCM-49 zeolite for polyethylene hydrocracking

    Catalysis Science & Technology · 2025-01-01

    Ruoyan Bai, Juhong Nie, Roudan Lian, Jian Zhang, Maolin Zhang

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  14. Morphology engineering of 2D Zn-catalysts to wrinkled particles using NaCl microcrystals: enhanced recyclability for the synthesis of poly(caprolactone)s

    Journal of Materials Chemistry A · 2025-01-01

    Seram Kim, Jong Doo Lee, Seung Uk Son

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  15. Conversion of Polypropylene to Light Olefins by HMFI Catalysts below Pyrolytic Temperature: Catalytic, Spectroscopic, and Theoretical Studies

    The Journal of Physical Chemistry C · 2025-01-10

    Yuriko Ando, Takumi Miyakage, Akihiko Anzai, Mengwen Huang, Abdellah Ait El Fakir, Takashi Toyao, Yuta Nakasaka, Alisa Phuekphong, Makoto Ogawa, Alexander A. Kolganov, Evgeny A. Pidko, Ken‐ichi Shimizu

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  16. Anionic Surfactants from Reactive Separation of Hydrocarbons Derived from Polyethylene Upcycling

    Langmuir · 2025-02-04

    Yu-Hsuan Lee, Alexandra Heuston, Enze Jin, Jia‐Kai Sun, Xichen Liang, Yangying Zhu, Matthew E. Helgeson, Eric R. Masanet, Susannah L. Scott, Mahdi M. Abu‐Omar

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  17. Advances and Challenges in Low‐Temperature Upcycling of Waste Polyolefins via Tandem Catalysis

    Angewandte Chemie International Edition · 2025-03-13

    Wei Zhang, Sung Min Kim, Michele L. Sarazen, Mingyuan He, Jingguang G. Chen, Johannes A. Lercher

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  18. Advances and Challenges in Low‐Temperature Upcycling of Waste Polyolefins via Tandem Catalysis

    Angewandte Chemie · 2025-03-13

    Wei Zhang, Sung Min Kim, Michele L. Sarazen, Mingyuan He, Jingguang G. Chen, Johannes A. Lercher

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  19. Upgrading polyolefin plastics: experiences from petroleum refining and distinct characteristics

    Science China Chemistry · 2025-03-19

    Rongxin Zhang, Guangchao Deng, Zhuoyang Jiang, Yiyi Fan, Yanqi Guo, Zhongwen Dong, Wenjun Chen, Bo Peng, Fan Zhang

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  20. Predicting a generalized mechanism of branched alkane hydrogenolysis on Ru, Ir, and Pt surfaces relevant to polymer upcycling applications

    Journal of Catalysis · 2025-05-08

    Andy Simonson, Lydia Thies, David D. Hibbitts

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  21. Synthesis, properties, and chemical recyclability of aromatic polyesters using alkylamide diphenolic acid

    European Polymer Journal · 2025-05-31

    Sorato Omura, Sho Fukushima, Tsubasa Sakiyama, Tatsuki Morita, Mai Takase, Yoshiaki Yoshida, Tomoyuki Suzuki, Yasuteru Mawatari

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  22. Recent Advances in the Thermo-Catalytic Upcycling of Polyethylene Waste

    ACS Applied Polymer Materials · 2025-06-03

    Yi Hao, Xin Che, Xueyang Hou, Liyi Shi, Lei Huang

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  23. Mechanistic alteration of polyethylene oxidation via heterogenous catalysis for enhanced fatty di-carboxylic acid yields

    Science China Chemistry · 2025-07-10

    Huidong Lv, Yi Ji, Wenjun Chen, Yuan Xiang, Yue Liu, Jianrong Zeng, Fei Huang, Fan Zhang

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  24. Enzymatic mechanism of polystyrene biodegradation: key depolymerization enzymes in the Stenotrophomonas maltophilia sp. ZSL2493

    Environmental Research · 2025-08-23

    Yue Yu, Kejian Tian, Pengfei Hao, Yibing Wang, Menghan Chang, Dandan Zhou, Jinming Gu, Fenglin Zhang, Hongliang Huo

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  25. Long-lived metal-zeolite catalysts for polyolefin aromatization via synergistic tandem dehydroaromatization and hydrogenolysis

    Journal of Energy Chemistry · 2025-09-11

    Wenjun Chen, Yiyi Fan, Yue Liu, Xiaobin Xie, Fan Zhang

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  26. Recent advances in thermal oxidative upcycling strategy of waste plastics under mild conditions

    Chemical Engineering Journal · 2025-09-15

    Bo Wang, Lan‐Lan Lou, Cheng Peng, Zhengyi Wu, Yuanling Zhang, Changzheng Liu, Shuangxi Liu, Kai Yu

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  27. Phyllosilicate Clay Blended with Semiconductor Nanocomposite for Enhanced Dye Removal and CO 2 Adsorption

    ACS Applied Nano Materials · 2025-09-25

    Shivam Kumar, Prarthana Puzari, Sarathi Kundu

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  28. Acidified montmorillonite (MMT)-supported ultrafine Ru nanoparticles for polyethylene plastic upcycling

    Green Chemistry · 2026-01-01

    Ruoyan Bai, Roudan Lian, Jian Zhang, Maolin Zhang

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  29. Carbon-modified TiO 2 catalysts for oxidative upcycling of waste polyethylene to dicarboxylic acids

    Green Chemistry · 2026-01-01

    Yi Hao, Kaili Wang, Rongrong Jia, Ping Cheng, Liyi Shi, Xiang Wang, Lei Huang

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  30. Catalytic valorization of polyolefins: from catalysts and processes to reactors

    Chemical Society Reviews · 2026-01-01

    Cuncun Wu, Chaojie Guo, Xinquan Xu, Kun Liu, Lu Bai, Nan Yang, Donglong Fu, Jinlong Gong

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  31. Highly efficient photoreforming of plastic waste for hydrogen production: recent advances and prospects

    Journal of Materials Chemistry A · 2026-01-01

    Ting Sun, Ayesha Obaid, Li Gao, Vipul Bansal, Rajesh Ramanathan, Zhen Wei, Yichao Wang, Derek Hao

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  32. Integrating chemical and biological conversion for waste plastics recycling and upcycling toward a circular bioeconomy

    Green Chemistry · 2026-01-01

    Schadrack Niyonkuru, Xiaoman He, Chen Deng, Eid S. Gaballah, Saeid Baroutian, Alec Foster, Bing Song, Francesco Barracco, David Chiaramonti, Richen Lin

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  33. Acid sites in hydrogen-involved polyolefin upcycling: mechanistic insights and design principles

    Science China Chemistry · 2026-01-27

    Qi Zhang, Xiang Wang

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  34. Thermal and kinetic modeling of waste plastic pyrolysis process to enhance the process scalability: A state-of-the-art review

    Journal of Analytical and Applied Pyrolysis · 2026-02-09

    Arshad Ali, Iyman Abrar, Pratik N. Sheth, Ibrahim Gbolahan Hakeem, Kalpit V. Shah

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  35. Recent advancements in catalytic processes for plastic upcycling into fuels: a major step in sustainable waste management and energy production

    Fuel · 2026-02-26

    Sudipta Nayak, Rajat Singhal, S. M. A. Hakim Siddiki, Ken Motokura, Navya Subray Bhat, Navneet Kumar Gupta

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  36. Tailoring the polyolefin hydrogenolysis performance of Ru/TiO2 through TiO2 support facet engineering

    Journal of Catalysis · 2026-03-02

    Qinge Fan, Ziyi zhang, Penglong Wang, Penglong Wang, Jicong Yan, Yongna Zhang, Caixia Feng, Li Wang, Li Wang, 常志显, Xiang Wang, Ruifeng Chong

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  37. Oxidative Upcycling of Polybutylene Terephthalate to Dicarboxylic Acids over a Cubic Au/Ca(OH) 2 Catalyst

    ACS Catalysis · 2026-03-14

    Ke Zhao, Xin Zhou, Chenao Zhou, Changtong Yue, Ying Liao, Mengnan Ma, Mengzhen Zhu, Liliang Jiang, Hao Yan, Xiaobo Chen, Yibin Liu, X Xiuzhen Feng, De Chen, Chaohe Yang, Ning Yan

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  38. Revealing the Native Multi-Enzyme Synergy of Acinetobacter calcoaceticus SDH15 for Ultra-Long-Chain Alkane Biodegradation

    Engineering · 2026-04-01

    Xianrui Liu, Donghuan Su, Shaojie Wang, Zhenxia Du, Haijia Su

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  39. Enhancing catalytic cracking of polyolefin plastics to heavy waxes over modified calcium aluminate catalysts

    Journal of the Energy Institute · 2026-04-30

    Jie Li, Xingxin Zhang, Fansheng Meng, Hongbo Chen, Qiang Zhao, Qi Li, Dan Luo, Wenshuo Ma, Chengbiao Wang, Jingxian Wang, Yingyun Qiao, Yuanyu Tian

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  40. Synergistic optimization of catalyst screening and reaction temperature for the catalytic cracking of polyolefins to light olefins

    Journal of the Energy Institute · 2026-05-07

    Jie Li, Wenshuo Ma, Houfu Bao, Qi Li, Shuya Li, Zhihao Yang, Bowen Xu, Chengyang Du, J Wang, Yingyun Qiao, Yuanyu Tian

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  41. Elucidating the Spatiotemporal Reaction Mechanism of Polyethylene Aromatization over ZSM-5 Zeolites

    ACS Catalysis · 2026-07-14

    Wenjun Chen, Yue Liu, Xiaoliang Liu, Fan Zhang

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  42. A Molten Salt-Like Strategy for the Synthesis of Hierarchical NiCoMn-LDH Electrocatalysts for Electrocatalytic Upcycling of Polyethylene Terephthalate Waste

    Langmuir · 2026-08-22

    Huanxu Du, Ranran Zhai, Xinru Xing, Wei Kong, Wenying Shi, Hua Zhou, Xianggui Kong, Mingfei Shao

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  43. Solar-driven programmable polystyrene upcycling to aromatic hydrocarbons via plasmonic iron nanoparticles

    Applied Catalysis B: Environmental · 2026-08-23

    Yifei Sun, Xupeng Liu, Yuqing Hu, Di Yang, Zhihui Ai

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  44. Engineering microbial consortia for polyethylene biodegradation and valorization using a function-driven strategy

    Chinese Journal of Chemical Engineering · 2026-09-01

    Xianrui Liu, Donghuan Su, Shaojie Wang, Haijia Su

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