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RESEARCH PAPER · Journal of Materials Chemistry C · 2020

Na 3 Sc 2 (PO 4 ) 2 F 3 : rational design and synthesis of an alkali rare-earth phosphate fluoride as an ultraviolet nonlinear optical crystal with an enlarged birefringence

Feng Xu, Guang Peng, Chensheng Lin, Dan Zhao, Bingxuan Li, Ge Zhang, Shunda Yang, Ning Ye

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Na 3 Sc 2 (PO 4 ) 2 F 3 : rational design and synthesis of an alkali rare-earth phosphate fluoride as an ultraviolet nonlinear optical crystal with an enlarged birefringenceOriginalPolar polymorphism: α- and β-KCsWP 2 O 9 nonlinear optical materials with a strong second harmonic generation response25Nonlinear Optical Oxythiophosphate Approaching the Good Balance with Wide Ultraviolet Transparency, Strong Second Harmonic Effect, and Large Birefringence92Nonlinear Optical Oxythiophosphate Approaching the Good Balance with Wide Ultraviolet Transparency, Strong Second Harmonic Effect, and Large Birefringence13Na 1.5 Rb 0.5 PO 3 F·H 2 O: synthesis, properties, and stepwise reconstruction of the hydrogen bond network13Synthesis, characterization and theoretical investigation of a new chalcohalide, Ba 4 GaS 4 F 311Ba3Sb2(PO4)4 and Cd3Sb2(PO4)4(H2O)2: Two New Antimonous Phosphates with Distinct [Sb(PO4)2] Structure Types and Enhanced Birefringence37A2(TeO)P2O7 (A = K, Rb, Cs): Three new tellurite-pyrophosphates with large birefringence17[C(NH2)3]3PO4·2H2O: A new metal-free ultraviolet nonlinear optical phosphate with large birefringence and second-harmonic generation response70Toward the Enhancement of Critical Performance for Deep-Ultraviolet Frequency-Doubling Crystals Utilizing Covalent Tetrahedra137Struvite-type AMgPO4·6H2O (A = NH4, K): Two Natural Deep-Ultraviolet Transparent Nonlinear Optical Crystals13Tin(II)-Induced Large Birefringence Enhancement in Metal Phosphates22Syntheses, Structures and Properties of Alkali and Alkaline Earth Metal Diamond-Like Compounds Li2MgMSe4 (M = Ge, Sn)12Ba 2 Bi 2 [Zn(PO 4 ) 4 ]: ionic-isolation-activated first barium bismuth zincophosphate with unprecedented ∞ [Zn(PO 4 ) 4 ] 10− chains and balanced overall performance4Complex coordinated functional groups: A great genes for nonlinear optical materials64(N 2 H 6 )[HPO 3 F] 2 : maximizing the optical anisotropy of deep-ultraviolet fluorophosphates33A flexible functional module to regulate ultraviolet optical nonlinearity for achieving a balance between a second-harmonic generation response and birefringence43BaSc 2 (HPO 3 ) 4 (H 2 O) 2 : a new nonlinear optical phosphite exhibiting a 3D {[Sc 2 (HPO 3 ) 4 ] 2− } ∞ anionic framework and phase-matchable SHG effect32Halogen regulation triggers structural transformation from centrosymmetric to noncentrosymmetric switches in tin phosphate halides Sn 2 PO 4 X (X = F, Cl)47Nain(C2o4)(Hpo4)(H2o)5: An Ultraviolet Transparent Nonlinear Optical Oxalate-Phosphate with Large Birefringence0Lone Pair-Driven Enhancement of Birefringence in Polar Alkali Metal Antimony Phosphates46The Kurtz-Perry powder technique revisited: A case study on the importance of reference quality and broadband nonlinear optical measurements using LiInSe232Three polar indium phosphites exhibiting diverse structural networks and SHG-activity9Phosphites: A Nonlinear Optical Materials System with a Wide Band Gap and Moderate Second-Harmonic Generation Effect27A promising ultraviolet nonlinear optical crystal: Rb 3 Ba 3 Li 2 Al 4 B 6 O 20 F—crystal growth, physical properties, and 266 nm laser generation17Co-substitution design: a new glaserite-type rare-earth phosphate K 2 RbSc(PO 4 ) 2 with high structural tolerance6Evaluating refractive index and birefringence of nonlinear optical crystals: Classical methods and new developments45Single crystal growth and phase transition mechanism of KCsMoP 2 O 9 with efficient second harmonic generation via the emerging additional periodic phase technology4Structure and optical property evolution in PbM(PO 4 )X (M = Zn, Sn; X = halogen): SHG effect and birefringence21Isomeric Cd(NH4)2(PO3F)2·2H2O: Solution concentration-driven elimination of antiparallel dipole-dipole interaction generating an SHG β phase12Recent advances of inorganic phosphates with UV/DUV cutoff edge and large second harmonic response7(NH4)3(H3O)Zn4(PO4)4: A nonlinear optical zinc orthophosphate crystal9Li9Mg3[PO4]4F3 fluorophosphate as a new thermoluminescent material: Experimental and theoretical study6Novel antimony phosphates with enlarged birefringence induced by lone pair cations4The enhanced bandgap and birefringence of rare-earth phosphates XPO 4 (X = Sc, Y, La, and Lu): a first-principles investigation7The Birefringence Modulation in Short‐Wave Ultraviolet Sulfates with Functional π‐Conjugated Cations and Polymerized Heteroleptic Tetrahedral Anions18Optimization of Functional Building Blocks Generates a Substantial Improvement in Birefringence from Sn2OSO4 to Sn3O2(OH)(HSO4)6A2Cd(PO3)4 (A = K, Rb, Cs): Series of cadmium polyphosphates with infinite 1[(PO3)4]ꝏ chains and deep ultraviolet transparency windows2From Ba2Bi2Zn(PO4)4 to Ba2Bi2Cu(PO4)4: Rational design of an ultraviolet phosphate with enhanced birefringence2Functional assembly and modification of nonlinear optical fundamental motifs in phosphates27Deep ultraviolet transparent borophosphates LiAB 2 P 2 O 9 (A = NH 4 , K) and LiNaB 2 P 2 O 8 (OH) 2 ·H 2 O exhibiting a moderate second-harmonic generation response4A 3 Sc(PO 4 ) 2 (A = Li, Na): rare earth cations effectively regulate phosphate structures for enhanced birefringence4Tailoring UV waveplate materials via rational assembly of functional motifs in scandium fluoride phosphate2Na3Y2F3P2O8 and K4Y3F5P4O14: [YOF] Polyhedra Inducing Birefringence Enhancement in Non-π-Conjugated Phosphate Systems3Na2MP3O9 (M = K, Rb): Two Potential Zero-Order Waveplate Materials with DUV Cutoff Edges2The Layered Structure–Induced Enhanced Birefringence of LiMgPO 4 : A First‐Principles Investigation1Tuning the Anionic Configuration in ASc2(P2O7)2 (A = Ba, Pb) through A-Site Cationic Coordination Engineering0From the up-converting multimodal luminescent thermometer to ratiometric visual power density meter based on Er 3+ ,Yb 3+ emission3Ternary Anion‐Engineered Rare Earth Crystals for Broadband UV Transparency and Enhanced Second‐Harmonic Generation1Potential Deep Ultraviolet Phosphate With Y‐Based: 1 [(PO 3 ) 4 ] ∞ Chains AYP 4 O 12 (A = K, NH 4 ) and the First [P 3 O 10 ] Anionic Framework KLiYP 3 O 100

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  1. Polar polymorphism: α- and β-KCsWP 2 O 9 nonlinear optical materials with a strong second harmonic generation response

    Journal of Materials Chemistry C · 2020-01-01

    Tuohetijiang Baiheti, Shujuan Han, Abudukadi Tudi, Zhihua Yang, Shilie Pan

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  2. Nonlinear Optical Oxythiophosphate Approaching the Good Balance with Wide Ultraviolet Transparency, Strong Second Harmonic Effect, and Large Birefringence

    Angewandte Chemie International Edition · 2020-12-20

    Xinyuan Zhang, Lei Kang, Pifu Gong, Zheshuai Lin, Yicheng Wu

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  3. Nonlinear Optical Oxythiophosphate Approaching the Good Balance with Wide Ultraviolet Transparency, Strong Second Harmonic Effect, and Large Birefringence

    Angewandte Chemie · 2020-12-21

    Xinyuan Zhang, Lei Kang, Pifu Gong, Zheshuai Lin, Yicheng Wu

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  4. Na 1.5 Rb 0.5 PO 3 F·H 2 O: synthesis, properties, and stepwise reconstruction of the hydrogen bond network

    Inorganic Chemistry Frontiers · 2021-01-01

    Xinrui Yang, Xin Liu, Zujian Wang, Xue‐Bin Deng, Hejie Lu, Yujia Li, Xifa Long, Ling Chen, Li‐Ming Wu

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  5. Synthesis, characterization and theoretical investigation of a new chalcohalide, Ba 4 GaS 4 F 3

    Dalton Transactions · 2021-01-01

    Hongbo Gao, Ruijiao Chen, Kewang Zhang, Ailijiang Abudurusuli, Kangrong Lai, Junjie Li

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  6. Ba3Sb2(PO4)4 and Cd3Sb2(PO4)4(H2O)2: Two New Antimonous Phosphates with Distinct [Sb(PO4)2] Structure Types and Enhanced Birefringence

    Inorganic Chemistry · 2021-01-12

    Xiaobao Li, Chun‐Li Hu, Fang Kong, Jiang‐Gao Mao

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  7. A2(TeO)P2O7 (A = K, Rb, Cs): Three new tellurite-pyrophosphates with large birefringence

    Journal of Alloys and Compounds · 2021-02-02

    Min Zhao, Weimin Dong, Yuandong Wu, Dajiang Mei, Shaoguo Wen, Thomas Doert

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  8. [C(NH2)3]3PO4·2H2O: A new metal-free ultraviolet nonlinear optical phosphate with large birefringence and second-harmonic generation response

    Science China Materials · 2021-02-24

    Xin Wen, Chensheng Lin, Min Luo, Huixin Fan, Kaichuang Chen, Ning Ye

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  9. Toward the Enhancement of Critical Performance for Deep-Ultraviolet Frequency-Doubling Crystals Utilizing Covalent Tetrahedra

    Accounts of Materials Research · 2021-03-25

    Miriding Mutailipu, Zhihua Yang, Shilie Pan

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  10. Struvite-type AMgPO4·6H2O (A = NH4, K): Two Natural Deep-Ultraviolet Transparent Nonlinear Optical Crystals

    Inorganic Chemistry · 2021-05-24

    Feifei Yuan, Lei Hu, Zhiyong Bai, Lehui Liu, Yisheng Huang, Lizhen Zhang, Dongshan Wei, Zhoubin Lin

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  11. Tin(II)-Induced Large Birefringence Enhancement in Metal Phosphates

    Inorganic Chemistry · 2021-09-27

    Mengya Ji, Chun‐Li Hu, Zhi Gang Fang, Yan Chen, Jiang‐Gao Mao

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  12. Syntheses, Structures and Properties of Alkali and Alkaline Earth Metal Diamond-Like Compounds Li2MgMSe4 (M = Ge, Sn)

    Materials · 2021-10-18

    Hongbo Gao, Kewang Zhang, Ailijiang Abudurusuli, Chen Bai, Zhihua Yang, Kangrong Lai, Junjie Li, Shilie Pan

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  13. Ba 2 Bi 2 [Zn(PO 4 ) 4 ]: ionic-isolation-activated first barium bismuth zincophosphate with unprecedented ∞ [Zn(PO 4 ) 4 ] 10− chains and balanced overall performance

    Inorganic Chemistry Frontiers · 2021-11-23

    Yuxin Li, Meihong Duan, Peixin Ma, Xu-Kui Yang, Wenhua Ma, Baichuan Wang, Zhi Gang Fang

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  14. Complex coordinated functional groups: A great genes for nonlinear optical materials

    Chinese Chemical Letters · 2021-12-03

    Weikang Wang, Dajiang Mei, Shaoguo Wen, Jian Wang, Yuandong Wu

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  15. (N 2 H 6 )[HPO 3 F] 2 : maximizing the optical anisotropy of deep-ultraviolet fluorophosphates

    Chemical Communications · 2022-01-01

    Haotian Qiu, Fuming Li, Congcong Jin, Juanjuan Lu, Zhihua Yang, Shilie Pan, Miriding Mutailipu

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  16. A flexible functional module to regulate ultraviolet optical nonlinearity for achieving a balance between a second-harmonic generation response and birefringence

    Chemical Science · 2022-01-01

    Liling Cao, Haotian Tian, Donghong Lin, Chensheng Lin, Feng Xu, Yinglei Han, Tao Yan, Jindong Chen, Bingxuan Li, Ning Ye, Min Luo

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  17. BaSc 2 (HPO 3 ) 4 (H 2 O) 2 : a new nonlinear optical phosphite exhibiting a 3D {[Sc 2 (HPO 3 ) 4 ] 2− } ∞ anionic framework and phase-matchable SHG effect

    Inorganic Chemistry Frontiers · 2022-01-01

    Ru‐Ling Tang, Gang-Xiang Liu, Wen‐Dong Yao, Li-Nan Zhang, Wenlong Liu, Sheng‐Ping Guo

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  18. Halogen regulation triggers structural transformation from centrosymmetric to noncentrosymmetric switches in tin phosphate halides Sn 2 PO 4 X (X = F, Cl)

    Inorganic Chemistry Frontiers · 2022-01-01

    Ting Zheng, Qiang Wang, Jinxuan Ren, Liling Cao, Ling Huang, Daojiang Gao, Jian Bi, Guohong Zou

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  19. Nain(C2o4)(Hpo4)(H2o)5: An Ultraviolet Transparent Nonlinear Optical Oxalate-Phosphate with Large Birefringence

    SSRN Electronic Journal · 2022-01-01

    Xuqi Zhang, Yanyan Xue, Lei Yang, Chao Wu, Zhipeng Huang, Jun Xu, Mark Graeme Humphrey, Chi Zhang

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  20. Lone Pair-Driven Enhancement of Birefringence in Polar Alkali Metal Antimony Phosphates

    Chemistry of Materials · 2022-04-29

    Chenhui Hu, Xintong Cai, Mengfan Wu, Zhihua Yang, Jian Wei Han, Shilie Pan

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  21. The Kurtz-Perry powder technique revisited: A case study on the importance of reference quality and broadband nonlinear optical measurements using LiInSe2

    Journal of Alloys and Compounds · 2022-05-13

    Daniel J. Clark, Jian‐Han Zhang, Andrew J. Craig, Ashley Weiland, Jacilynn A. Brant, Jeong Bin Cho, Yong Soo Kim, Joon Ik Jang, Jennifer A. Aitken

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  22. Three polar indium phosphites exhibiting diverse structural networks and SHG-activity

    Journal of Solid State Chemistry · 2022-10-10

    Gang-Xiang Liu, Yu-Long Wei, Li-Nan Zhang, Wenlong Liu, Sheng‐Ping Guo, Ru‐Ling Tang

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  23. Phosphites: A Nonlinear Optical Materials System with a Wide Band Gap and Moderate Second-Harmonic Generation Effect

    Inorganic Chemistry · 2022-11-08

    Jingjing Zhang, Xiaomin Zhang, Ying Wang, Kui Wu, Bingbing Zhang

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  24. A promising ultraviolet nonlinear optical crystal: Rb 3 Ba 3 Li 2 Al 4 B 6 O 20 F—crystal growth, physical properties, and 266 nm laser generation

    Journal of Materials Chemistry C · 2022-12-15

    Jiankang Wang, Hongping Wu, Zhanggui Hu, Jiyang Wang, Yicheng Wu, Hongwei Yu

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  25. Co-substitution design: a new glaserite-type rare-earth phosphate K 2 RbSc(PO 4 ) 2 with high structural tolerance

    Dalton Transactions · 2023-01-01

    Jingfang Zhou, Pifu Gong, Mingjun Xia, Qian Wu

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  26. Evaluating refractive index and birefringence of nonlinear optical crystals: Classical methods and new developments

    Chinese Journal of Structural Chemistry · 2023-01-01

    Qi Shi, Lingyun Dong, Ying Wang

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  27. Single crystal growth and phase transition mechanism of KCsMoP 2 O 9 with efficient second harmonic generation via the emerging additional periodic phase technology

    Journal of Materials Chemistry C · 2023-01-01

    Mengdi Fan, Guangda Wu, Lili Li, Fapeng Yu, Chunhui Wang, Xiufeng Cheng, Xian Zhao

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  28. Structure and optical property evolution in PbM(PO 4 )X (M = Zn, Sn; X = halogen): SHG effect and birefringence

    Inorganic Chemistry Frontiers · 2023-01-01

    Xiaobao Li, Chun‐Li Hu, Fang Kong, Jiang‐Gao Mao

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  29. Isomeric Cd(NH4)2(PO3F)2·2H2O: Solution concentration-driven elimination of antiparallel dipole-dipole interaction generating an SHG β phase

    Materials Today Physics · 2023-01-31

    Xinrui Yang, Xin Liu, Xue‐Bin Deng, Ling Chen, Li‐Ming Wu

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  30. Recent advances of inorganic phosphates with UV/DUV cutoff edge and large second harmonic response

    Chinese Journal of Structural Chemistry · 2023-02-13

    Boxuan Zhang, Zhaohui Chen

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  31. (NH4)3(H3O)Zn4(PO4)4: A nonlinear optical zinc orthophosphate crystal

    Journal of Solid State Chemistry · 2023-06-22

    Yueling Sun, Gang-Xiang Liu, Yi‐Lei Lv, Liang Ma, Wen‐Dong Yao, Ru‐Ling Tang

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  32. Li9Mg3[PO4]4F3 fluorophosphate as a new thermoluminescent material: Experimental and theoretical study

    Optical Materials · 2023-10-03

    D.A. Akulov, N. I. Medvedeva, Michael O. Kalinkin, Vladimir G. Zubkov, R. M. Αbashev, Α. I. Surdo, Е. V. Zabolotskaya, Д. Г. Келлерман

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  33. Novel antimony phosphates with enlarged birefringence induced by lone pair cations

    Dalton Transactions · 2024-01-01

    Mei Hu, Jialong Wang, Nuerbiye Tuerhong, Zhiyuan Zhang, Qun Jing, Zhaohui Chen, Yonglei Yang, Ming‐Hsien Lee

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  34. The enhanced bandgap and birefringence of rare-earth phosphates XPO 4 (X = Sc, Y, La, and Lu): a first-principles investigation

    Physical Chemistry Chemical Physics · 2024-01-01

    Nuerbiye Tuerhong, Hongheng Chen, Mei Hu, X.Y. Cui, Haiming Duan, Qun Jing, Zhaohui Chen

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  35. The Birefringence Modulation in Short‐Wave Ultraviolet Sulfates with Functional π‐Conjugated Cations and Polymerized Heteroleptic Tetrahedral Anions

    Advanced Optical Materials · 2024-02-07

    Yanran Shang, Hongyuan Sha, Zujian Wang, Rongbing Su, Chao He, Xiaoming Yang, Xifa Long

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  36. Optimization of Functional Building Blocks Generates a Substantial Improvement in Birefringence from Sn2OSO4 to Sn3O2(OH)(HSO4)

    Inorganic Chemistry · 2024-07-31

    Yuqi Chen, Han Luo, Zeqiao Yin, Xuehua Dong, Daojiang Gao, Yuqiao Zhou, Ling Huang, Liling Cao, Guohong Zou

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  37. A2Cd(PO3)4 (A = K, Rb, Cs): Series of cadmium polyphosphates with infinite 1[(PO3)4]ꝏ chains and deep ultraviolet transparency windows

    Journal of Alloys and Compounds · 2024-09-26

    Huanhuan Zhao, Die Xu, Xuebin Yu, Qun Jing, Yi Huang, Zhaohui Chen

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  38. From Ba2Bi2Zn(PO4)4 to Ba2Bi2Cu(PO4)4: Rational design of an ultraviolet phosphate with enhanced birefringence

    Journal of Alloys and Compounds · 2024-11-26

    Yin-Jie Peng, Yanbo Li, Jun Li, Chao-Qian Li, Baichuan Wang, Zhi Gang Fang, Meihong Duan

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  39. Functional assembly and modification of nonlinear optical fundamental motifs in phosphates

    Coordination Chemistry Reviews · 2024-11-27

    Fan Liu, Pifu Gong, Zheshuai Lin, Lei Kang

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  40. Deep ultraviolet transparent borophosphates LiAB 2 P 2 O 9 (A = NH 4 , K) and LiNaB 2 P 2 O 8 (OH) 2 ·H 2 O exhibiting a moderate second-harmonic generation response

    Journal of Materials Chemistry C · 2024-12-23

    Huanhuan Zhao, Chenxu Li, Juanjuan Lu, Zhihua Yang, Jian Wei Han, Shilie Pan

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  41. A 3 Sc(PO 4 ) 2 (A = Li, Na): rare earth cations effectively regulate phosphate structures for enhanced birefringence

    Dalton Transactions · 2025-01-01

    Hongheng Chen, Xudong Leng, Mei Hu, Yibo Han, Haiming Duan, Qun Jing, Zhaohui Chen, Ming‐Hsien Lee

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  42. Tailoring UV waveplate materials via rational assembly of functional motifs in scandium fluoride phosphate

    Chemical Communications · 2025-01-01

    Huijian Zhao, Conggang Li, Ning Ye, Zhanggui Hu

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  43. Na3Y2F3P2O8 and K4Y3F5P4O14: [YOF] Polyhedra Inducing Birefringence Enhancement in Non-π-Conjugated Phosphate Systems

    Inorganic Chemistry · 2025-02-20

    Jiawei Zhao, Wei Wei, Meihui Chen, Donghai An, Yanna Chen, Hongsheng Shi

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  44. Na2MP3O9 (M = K, Rb): Two Potential Zero-Order Waveplate Materials with DUV Cutoff Edges

    Inorganic Chemistry · 2025-03-04

    Huanhuan Zhao, Chenxu Li, Yi Huang, Qun Jing, Xuebin Yu, Zhaohui Chen

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  45. The Layered Structure–Induced Enhanced Birefringence of LiMgPO 4 : A First‐Principles Investigation

    physica status solidi (b) · 2025-06-26

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  46. Tuning the Anionic Configuration in ASc2(P2O7)2 (A = Ba, Pb) through A-Site Cationic Coordination Engineering

    Inorganic Chemistry · 2025-09-05

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  47. From the up-converting multimodal luminescent thermometer to ratiometric visual power density meter based on Er 3+ ,Yb 3+ emission

    Materials Horizons · 2025-09-17

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  48. Ternary Anion‐Engineered Rare Earth Crystals for Broadband UV Transparency and Enhanced Second‐Harmonic Generation

    Chinese Journal of Chemistry · 2026-03-12

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  49. Potential Deep Ultraviolet Phosphate With Y‐Based: 1 [(PO 3 ) 4 ] ∞ Chains AYP 4 O 12 (A = K, NH 4 ) and the First [P 3 O 10 ] Anionic Framework KLiYP 3 O 10

    European Journal of Inorganic Chemistry · 2026-09-15

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