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RESEARCH PAPER · Chemical Science · 2022

A flexible functional module to regulate ultraviolet optical nonlinearity for achieving a balance between a second-harmonic generation response and birefringence

Liling Cao, Haotian Tian, Donghong Lin, Chensheng Lin, Feng Xu, Yinglei Han, Tao Yan, Jindong Chen, Bingxuan Li, Ning Ye, Min Luo

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A flexible functional module to regulate ultraviolet optical nonlinearity for achieving a balance between a second-harmonic generation response and birefringenceOriginalLarge optical anisotropy-oriented construction of a carbonate-nitrate chloride compound as a potential ultraviolet birefringent material44Rbcl·(H2seo3)2: A New Salt-Inclusion Selenite as a Promising Uv Birefringent Material0Pb5(GeO4)(Ge2O7) and Pb3.32Ca1.68(GeO4)(Ge2O7): Two Nonlinear Optical Germanates Induced by Diverse PbOx Polyhedra17RbCl·(H2SeO3)2: A Salt-Inclusion Selenite Featuring Short UV Cut-Off Edge and Large Birefringence15A 0.5 H 2 C 6 N 7 O 3 ·4H 2 O (A = Ca 2+ , Sr 2+ ) iso-cyamelurates with ultra-large π-conjugated group and excellent nonlinear optical properties10From H 12 C 4 N 2 CdI 4 to H 11 C 4 N 2 CdI 3 : a highly polarizable CdNI 3 tetrahedron induced a sharp enhancement of second harmonic generation response and birefringence50The transformation of a zero-dimensional cluster into a one-dimensional chain structure achieving a dramatically enhanced birefringence in tin( ii )-based oxalates33Recent Development of Sn II , Sb III ‐based Birefringent Material: Crystal Chemistry and Investigation of Birefringence130Recent Development of SnII, SbIII‐based Birefringent Material: Crystal Chemistry and Investigation of Birefringence6Recent progress of newly developed functional building units and corresponding nonlinear optical materials14Design of the Ionic Organic Nonlinear Optical Material NH 4 [LiC 3 H(CH 3 )O 4 ] with Ultrawide Band Gap and Moderate Birefringence79Design of the Ionic Organic Nonlinear Optical Material NH 4 [LiC 3 H(CH 3 )O 4 ] with Ultrawide Band Gap and Moderate Birefringence9New Functional Groups Design toward High Performance Ultraviolet Nonlinear Optical Materials95Salt-inclusion chalcogenides with d-orbital components: unveiling remarkable nonlinear optical properties and dual-band photoluminescence10Synergistic combination of different types of functional motif in Rb(NO 3 )(SO 3 NH 3 ) for realizing excellent ultraviolet optical nonlinearity18Synthesis, structures and properties of two new nitrate optical materials: Rb3ZnNO3Cl4 and Rb5Na(NO3)4Cl24Designing Strong Polarity and High Configurational Entropy Flexible Units toward Excellent Ultraviolet Nonlinear Optical Materials42Intramolecular Hydrogen Bonds Enhance Structure Coplanarity, Resulting in Significant Birefringence in Bridged-Bipyridine Halides7Optimization of Functional Building Blocks Generates a Substantial Improvement in Birefringence from Sn2OSO4 to Sn3O2(OH)(HSO4)6A remarkable solar-blind ultraviolet nonlinear optical crystal with comprehensive performance and enhanced thermal stability4Co-ligand tuning of MOF structural anisotropy for giant optical birefringence7Design of a high-performance infrared birefringent crystal Ba 4 HgP 2 Se 10 via a low-dimensional motif intercalation strategy2Histidine-directed synthesis and optical properties of two indium phosphite–oxalates with three-dimensional structures4K3[HCO3]2F: a new deep-UV birefringent crystal exhibiting strong optical anisotropy17Inch‐sized K[NH2(CH2COO)2]: a High‐Performance UV Nonlinear Optical Crystal Enabled by Novel Flexible π‐Conjugated Building Units, [NH2(CH2COO)2]−13Multifunctional Cd‐based Hybrid with Large Birefringence Achieving Excellent Second Harmonic Generation and Reversible Temperature‐Activated Fluorescence for Anti‐counterfeiting16Decoupling the SHG‐Birefringence Trade‐off in UV NLO Materials via Triple‐Control Coordination Engineering: Achieving Synergistic Performance Optimization88Decoupling the SHG‐Birefringence Trade‐off in UV NLO Materials via Triple‐Control Coordination Engineering: Achieving Synergistic Performance Optimization13Designing an all-organic wide bandgap ultraviolet nonlinear optical crystal3Deprotonation-Regulated Conformational Switching in Malonates Enables High-Performance Ultraviolet Polar Crystals3Isoniazid nitrate: synergistic dual π-conjugation triggering prominent second-harmonic generation0Stable lead succinate-iodides with strong second-harmonic generation response and large birefringence0Truss bridge-like anhydrous stacking in hybrid crystals triggers ultra-high stability and robust birefringence0氢键组装的新型紫外非线性光学晶体（R/S‑DACH）Mal·H2O的设计及性能研究（特邀）0Confinement π‐Conjugated Moiety Tailoring to Achieve Record Deep‐UV Nonlinearity in Sulfates0Anion Size‐Dependent Conformational Folding of Guanidinopropionate: Enabling Tunable Birefringence and Balanced Second‐Harmonic Generation Performance3Anion Size‐Dependent Conformational Folding of Guanidinopropionate: Enabling Tunable Birefringence and Balanced Second‐Harmonic Generation Performance0Local Conformational Confinement and Dipole Engineering for Phase-Matchable Solar-Blind Ultraviolet Nonlinear Optical Crystals11Cation-sulfur-driven dimensional reduction engineering for tailoring sulfonate birefringent crystals with enhanced anisotropy2Second-order nonlinear optical organic crystals exhibit reversible photoisomerization0The Parallel Coplanar Alignment of Planar Non‐π‐Conjugated [Pb 3 Br 3 ] Rings for a Stable Ultraviolet Nonlinear Optical Crystal0The Multi‐Scale Paradigm: An Integrated Design Logic for Nonlinear Optical Crystals1The Multi‐Scale Paradigm: An Integrated Design Logic for Nonlinear Optical Crystals0

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  1. Large optical anisotropy-oriented construction of a carbonate-nitrate chloride compound as a potential ultraviolet birefringent material

    Chemical Science · 2022-01-01

    Meng Cheng, Wenqi Jin, Zhihua Yang, Shilie Pan

    Read original paper ↗ ·

  2. Rbcl·(H2seo3)2: A New Salt-Inclusion Selenite as a Promising Uv Birefringent Material

    SSRN Electronic Journal · 2022-01-01

    Huan Wang, Lili Liu, Zhaowei Hu, Junbo Wang, Mengmeng Zhu, Jiayue Xu

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  3. Pb5(GeO4)(Ge2O7) and Pb3.32Ca1.68(GeO4)(Ge2O7): Two Nonlinear Optical Germanates Induced by Diverse PbOx Polyhedra

    Inorganic Chemistry · 2022-08-17

    Mei Yan, Ru‐Ling Tang, Gang-Xiang Liu, Lei Huai, Wenlong Liu, Sheng‐Ping Guo

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  4. RbCl·(H2SeO3)2: A Salt-Inclusion Selenite Featuring Short UV Cut-Off Edge and Large Birefringence

    Inorganic Chemistry · 2022-12-23

    Huan Wang, Lili Liu, Zhaowei Hu, Junbo Wang, Mengmeng Zhu, Yu Meng, Jiayue Xu

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  5. A 0.5 H 2 C 6 N 7 O 3 ·4H 2 O (A = Ca 2+ , Sr 2+ ) iso-cyamelurates with ultra-large π-conjugated group and excellent nonlinear optical properties

    Inorganic Chemistry Frontiers · 2023-01-01

    Xiaoguang Du, Fangyan Wang, Fei Liang, Zhanggui Hu, Yicheng Wu, Xinyuan Zhang

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  6. From H 12 C 4 N 2 CdI 4 to H 11 C 4 N 2 CdI 3 : a highly polarizable CdNI 3 tetrahedron induced a sharp enhancement of second harmonic generation response and birefringence

    Chemical Science · 2023-01-01

    Huai‐Yu Wu, Chun‐Li Hu, Miao‐Bin Xu, Qianqian Chen, Nan Ma, Xiao‐Ying Huang, Ke‐Zhao Du, Jin Chen

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  7. The transformation of a zero-dimensional cluster into a one-dimensional chain structure achieving a dramatically enhanced birefringence in tin( ii )-based oxalates

    Inorganic Chemistry Frontiers · 2023-01-01

    Liying Ren, Linhong Cheng, Xiaoyan Zhou, Jinxuan Ren, Liling Cao, Ling Huang, Xuehua Dong, Yuqiao Zhou, Daojiang Gao, Guohong Zou

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  8. Recent Development of Sn II , Sb III ‐based Birefringent Material: Crystal Chemistry and Investigation of Birefringence

    Angewandte Chemie International Edition · 2023-03-13

    Shujuan Han, Abudukadi Tudi, Wenbin Zhang, Xueling Hou, Zhihua Yang, Shilie Pan

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  9. Recent Development of SnII, SbIII‐based Birefringent Material: Crystal Chemistry and Investigation of Birefringence

    Angewandte Chemie · 2023-03-13

    Shujuan Han, Abudukadi Tudi, Wenbin Zhang, Xueling Hou, Zhihua Yang, Shilie Pan

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  10. Recent progress of newly developed functional building units and corresponding nonlinear optical materials

    Chinese Journal of Structural Chemistry · 2023-05-11

    Wenjing Tan, Chenyang Zhang, Chenyang Zhang, Tingting Huang, Bingbing Zhang

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  11. Design of the Ionic Organic Nonlinear Optical Material NH 4 [LiC 3 H(CH 3 )O 4 ] with Ultrawide Band Gap and Moderate Birefringence

    Angewandte Chemie International Edition · 2023-05-22

    Haotian Tian, Chensheng Lin, Yuqiao Zhou, Xin Lei Zhao, Huixin Fan, Tao Yan, Ning Ye, Min Luo

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  12. Design of the Ionic Organic Nonlinear Optical Material NH 4 [LiC 3 H(CH 3 )O 4 ] with Ultrawide Band Gap and Moderate Birefringence

    Angewandte Chemie · 2023-05-22

    Haotian Tian, Chensheng Lin, Yuqiao Zhou, Xin Lei Zhao, Huixin Fan, Tao Yan, Ning Ye, Min Luo

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  13. New Functional Groups Design toward High Performance Ultraviolet Nonlinear Optical Materials

    Accounts of Chemical Research · 2023-10-27

    Huixin Fan, Ning Ye, Min Luo

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  14. Salt-inclusion chalcogenides with d-orbital components: unveiling remarkable nonlinear optical properties and dual-band photoluminescence

    Chemical Science · 2024-01-01

    Shao‐Min Pei, Ming‐Shu Zhang, Fan Wu, Yan Guo, Xiao‐Ming Jiang, Bin‐Wen Liu, Guo‐Cong Guo

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  15. Synergistic combination of different types of functional motif in Rb(NO 3 )(SO 3 NH 3 ) for realizing excellent ultraviolet optical nonlinearity

    Inorganic Chemistry Frontiers · 2024-01-01

    Yunxia Song, Chensheng Lin, Xin Yi Zhao, Tao Yan, Ning Ye, Haotian Tian, Min Luo

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  16. Synthesis, structures and properties of two new nitrate optical materials: Rb3ZnNO3Cl4 and Rb5Na(NO3)4Cl2

    Results in Physics · 2024-01-21

    Changyou Liu, Ketian Hou, Bei Zhang

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  17. Designing Strong Polarity and High Configurational Entropy Flexible Units toward Excellent Ultraviolet Nonlinear Optical Materials

    Advanced Functional Materials · 2024-04-15

    Haotian Tian, Chensheng Lin, Bingxuan Li, Xin Lei Zhao, Tao Yan, Ning Ye, Min Luo

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  18. Intramolecular Hydrogen Bonds Enhance Structure Coplanarity, Resulting in Significant Birefringence in Bridged-Bipyridine Halides

    Crystal Growth & Design · 2024-05-30

    Wenjie He, Xin Liu, Ling Chen, Li‐Ming Wu

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  19. Optimization of Functional Building Blocks Generates a Substantial Improvement in Birefringence from Sn2OSO4 to Sn3O2(OH)(HSO4)

    Inorganic Chemistry · 2024-07-31

    Yuqi Chen, Han Luo, Zeqiao Yin, Xuehua Dong, Daojiang Gao, Yuqiao Zhou, Ling Huang, Liling Cao, Guohong Zou

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  20. A remarkable solar-blind ultraviolet nonlinear optical crystal with comprehensive performance and enhanced thermal stability

    Materials Chemistry Frontiers · 2025-01-01

    Jialin Zeng, Shuangcheng Li, Ruibiao Fu, Zilong Geng, Yiting Luo, Senfu Lei, Zuju Ma

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  21. Co-ligand tuning of MOF structural anisotropy for giant optical birefringence

    Chemical Communications · 2025-01-01

    Svyatoslav A. Povarov, Ekaterina D Iukhnevich, Pavel V. Alekseevskiy, Dmitry I. Pavlov, Аndrei S. Potapov, Irina D. Yushina, Valentin A. Milichko, Alena N. Kulakova

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  22. Design of a high-performance infrared birefringent crystal Ba 4 HgP 2 Se 10 via a low-dimensional motif intercalation strategy

    Dalton Transactions · 2025-01-01

    Zhihui Xiong, Haotian Tian, Zhixi Li, Guowei Deng, Fang Ding, Qian Wu, Mingjun Xia

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  23. Histidine-directed synthesis and optical properties of two indium phosphite–oxalates with three-dimensional structures

    CrystEngComm · 2025-01-01

    Xuemei Wen, Ying Li, Yan Zhao, Jing Li, Hongmei Zeng, Guohong Zou, Zhien Lin

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  24. K3[HCO3]2F: a new deep-UV birefringent crystal exhibiting strong optical anisotropy

    Science China Materials · 2025-03-03

    Wenbin Zhang, Yabo Wu, Zhihua Yang, Shujuan Han, Shilie Pan

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  25. Inch‐sized K[NH2(CH2COO)2]: a High‐Performance UV Nonlinear Optical Crystal Enabled by Novel Flexible π‐Conjugated Building Units, [NH2(CH2COO)2]−

    Laser & Photonics Review · 2025-03-05

    Yujie Fan, Lingli Wu, Chensheng Lin, Haotian Tian, Chao Wang, Tao Yan, Min Luo

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  26. Multifunctional Cd‐based Hybrid with Large Birefringence Achieving Excellent Second Harmonic Generation and Reversible Temperature‐Activated Fluorescence for Anti‐counterfeiting

    Advanced Optical Materials · 2025-05-21

    Duanliang Wang, Qiwei Xing, Defu Sun, Chuanrui Zhu, Kui Wu, Bingbing Zhang, Guangxia Liu, Jiyang Wang, Chuanying Shen

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  27. Decoupling the SHG‐Birefringence Trade‐off in UV NLO Materials via Triple‐Control Coordination Engineering: Achieving Synergistic Performance Optimization

    Angewandte Chemie International Edition · 2025-05-22

    Yaolong Zhu, Jie Gou, Can Yang, Qingwen Zhu, Yi Xiong, Qi Wu

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  28. Decoupling the SHG‐Birefringence Trade‐off in UV NLO Materials via Triple‐Control Coordination Engineering: Achieving Synergistic Performance Optimization

    Angewandte Chemie · 2025-05-22

    Yaolong Zhu, Jie Gou, Can Yang, Qingwen Zhu, Yi Xiong, Qi Wu

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  29. Designing an all-organic wide bandgap ultraviolet nonlinear optical crystal

    Science China Chemistry · 2025-06-30

    Shanshan Chen, Zhiyong Bai, Liangmeng Zhu, Tao Ouyang, Chen Xu, Shoufeng Wang, Yanqiang Li, Weiqi Huang, Sangen Zhao, Junhua Luo

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  30. Deprotonation-Regulated Conformational Switching in Malonates Enables High-Performance Ultraviolet Polar Crystals

    Inorganic Chemistry · 2025-10-03

    Zhengyan Lin, Huili Liu, Liling Cao, Ling Huang, Xuehua Dong, Yuqiao Zhou, Daojiang Gao, Ning Ye

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  31. Isoniazid nitrate: synergistic dual π-conjugation triggering prominent second-harmonic generation

    Chemical Communications · 2026-01-01

    Yang Chi, Ya-Ping Zhao, Sheng‐Ping Guo

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  32. Stable lead succinate-iodides with strong second-harmonic generation response and large birefringence

    Inorganic Chemistry Frontiers · 2026-01-01

    Yulu Wu, Jialin Zeng, Rui Biao Fu, Wen Jing Yang, Zilong Geng, Senfu Lei, Yiting Luo, Xiaofan Tong, Zuju Ma

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  33. Truss bridge-like anhydrous stacking in hybrid crystals triggers ultra-high stability and robust birefringence

    Inorganic Chemistry Frontiers · 2026-01-01

    Ping Wang, Qiya Huang, Xiaoli Meng, Lehui Liu, Qi Wu, Hongming Liu

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  34. 氢键组装的新型紫外非线性光学晶体（R/S‑DACH）Mal·H2O的设计及性能研究（特邀）

    Chinese Journal of Lasers · 2026-01-01

    阚子钧 Kan Zijun, 李雷鸣 Li Leiming, 吴红萍 Wu Hongping, 张玉杰 ZHANG Yujie, 俞洪伟 Yu Hongwei, 吴以成 Wu Yicheng

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  35. Confinement π‐Conjugated Moiety Tailoring to Achieve Record Deep‐UV Nonlinearity in Sulfates

    Angewandte Chemie · 2026-03-05

    Yujie Fan, Cheng Hu, Li Wu, Chensheng Lin, Chao Wang, Huixin Fan, Tao Yan, Min Luo

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  36. Anion Size‐Dependent Conformational Folding of Guanidinopropionate: Enabling Tunable Birefringence and Balanced Second‐Harmonic Generation Performance

    Angewandte Chemie International Edition · 2026-04-13

    Si‐Qian Jiang, Shuang Zhao, Yi‐Chang Yang, Jingyu Guo, Wenkai Zhao, Xuefei Wang, Li‐Ming Wu, Ling Chen

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  37. Anion Size‐Dependent Conformational Folding of Guanidinopropionate: Enabling Tunable Birefringence and Balanced Second‐Harmonic Generation Performance

    Angewandte Chemie · 2026-04-13

    Si‐Qian Jiang, Shuang Zhao, Yi‐Chang Yang, Jingyu Guo, Wenkai Zhao, Xuefei Wang, Li‐Ming Wu, Ling Chen

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  38. Local Conformational Confinement and Dipole Engineering for Phase-Matchable Solar-Blind Ultraviolet Nonlinear Optical Crystals

    Journal of the American Chemical Society · 2026-04-13

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  39. Cation-sulfur-driven dimensional reduction engineering for tailoring sulfonate birefringent crystals with enhanced anisotropy

    Chinese Journal of Structural Chemistry · 2026-05-02

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  40. Second-order nonlinear optical organic crystals exhibit reversible photoisomerization

    Chinese Journal of Structural Chemistry · 2026-07-01

    Zhu Xiangzhao, Songhua Chen, Zi Wang, Yan Jianfeng, Xin DanDan, Jialiang Xu, Yaofeng Yuan

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  41. The Parallel Coplanar Alignment of Planar Non‐π‐Conjugated [Pb 3 Br 3 ] Rings for a Stable Ultraviolet Nonlinear Optical Crystal

    Advanced Optical Materials · 2026-08-27

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  42. The Multi‐Scale Paradigm: An Integrated Design Logic for Nonlinear Optical Crystals

    Angewandte Chemie International Edition · 2026-09-10

    Xiangqing Cao, Haotian Qiu, Juanjuan Lu, Yun Mo Yang, Xueling Hou, Junjie Li, Shilie Pan, Miriding Mutailipu

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  43. The Multi‐Scale Paradigm: An Integrated Design Logic for Nonlinear Optical Crystals

    Angewandte Chemie · 2026-09-10

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