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RESEARCH PAPER · Advanced Functional Materials · 2024

Looking Back the Nonlinear Optical Crystals in a Functionalized Unit's Perspective

Miriding Mutailipu, Junjie Li, Shilie Pan

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Looking Back the Nonlinear Optical Crystals in a Functionalized Unit's PerspectiveOriginalA wide band gap selenohalide Cs 9 Si 8 Se 20 Cl with unprecedented [CsSe 7 Cl] mixed anionic units2Carbon-Rich Copper(I) Tetranuclear Complexes with Tunable Electrochemical, Luminescence, and Nonlinear Optical Properties0Cd 5 Te 4 O 12 X 2 (X = Cl, Br, I): a new oxyhalide family with [CdO 4 X] mixed anionic units and adjustable optical properties4Enhanced second-harmonic generation response in a chiral lead iodide induced by amino acid coordination8Expanding silver fluorooxoborate crystal chemistry: Ag 2 B 5 O 8 F with 3D double interpenetrating frameworks and Ag 3 B 5 O 8 F 2 with 2D layers5Hg 2 (HTe 2 O 5 )(PO 4 ): a novel phosphate crystal with enhanced birefringence enabled by the synergistic modification of multiple functional groups12Hg 2 (SeO 3 )(TeO 3 ): a novel tellurite–selenite birefringent crystal achieved by assembling multiple functional groups11Hydrogen bonding regulation-oriented design of pyridine sulfonate as a promising UV birefringent crystal characterized by enhanced structural anisotropy11Numerical simulation and modified Bridgman growth of high-quality and large-sized LiGaS 2 mid-infrared optical crystals1Prismatic crystal field stabilized divalent rare-earth chalcogenide REIIBII6CIII6QVI16 with bifunctionality30Synthesis, Photophysical Properties, and Two-Photon Absorption Behavior of Pyrimidinyl Urea Derivatives0The Nonlinear Optical Properties and Through-Space Charge-Transfer Effects of the Twist Donor-acceptor complexes0Reinforced Nonlinear Optical Performances Induced by P‐P Homoatomic Bond in Phosphide SrIn 3 Si 4 P 1131Reinforced Nonlinear Optical Performances Induced by P‐P Homoatomic Bond in Phosphide SrIn 3 Si 4 P 116ISOLATION, CHARACTERIZATION AND EVALUATION OF ANTIOXIDANT ACTIVITY OF SILICA CELLULOSE NANOCOMPOSITE (SiO2-CNC) EXTRACTED FROM BIO-WASTE (RICE HUSK) INTEGRATED WITH CALLISTEMON CITRINUS EXTRACT2Rb 7 PbY 2 (B 5 O 10 ) 3 : A Noncentrosymmetric Rare-Earth Borate Nonlinear Optical Crystal with [B 5 O 10 ] Unit16Synergically Assembling Advantageous Groups toward High‐Performance Infrared Nonlinear Optical Materials A II CdSiSe 4 (A II = Sr, Ba)40Red Emissive 1D Copper(I) Thiolates and Green Emissive 2D Copper(I) Halide Thiolates Displaying Second Harmonic Generation and Two‐Photon Absorption Processes2SrZnGeSe 4 : a promising infrared nonlinear optical material with strong second harmonic generation and high laser-induced damage threshold4Na[B3IO7(OH)] and Na2[B4IO9](IO3): Explorations of Boroiodates with Strong Second Harmonic Generation Response and Large Birefringence54Unearthing Hydrogen Bonded Metal‐Free Crystal with Remarkable Optical Anisotropy9Giant Birefringence Enabled by the Highly Anisotropic Linear IX 2 − (X = Cl, Br) Building Blocks6Giant Birefringence Enabled by the Highly Anisotropic Linear IX 2 − (X = Cl, Br) Building Blocks32Breaking the Natural Tendency of Deep‐UV Polyborate Anion Clusters to Inducing Strong Optical Anisotropy13Bridging the Interlayer Binding to Ordered π‐Conjugated Units for Constructing High‐Performing Light Polarization Crystals8Bridging the Interlayer Binding to Ordered π‐Conjugated Units for Constructing High‐Performing Light Polarization Crystals48Hydrogen‐Bonded Assembly of Functional Units for Constructing Linear and Nonlinear Optical Crystals10The Dugganite Structure as a Host for New Colored Compounds and for Oxygen Evolution Studies1Ca 7 (TeO 3 ) 6 (MoO 4 ): A Promising Mid-Infrared Nonlinear Optical Crystal Activated via a Module-Oriented Dimensionality Reduction Strategy34Multifunctional Cd‐based Hybrid with Large Birefringence Achieving Excellent Second Harmonic Generation and Reversible Temperature‐Activated Fluorescence for Anti‐counterfeiting16Giant Birefringence and Solar‐Blind Ultraviolet Transmission by Coordination‐Induced Assembly of π‐Conjugated Pyridine–Carboxylate8Giant Birefringence and Solar‐Blind Ultraviolet Transmission by Coordination‐Induced Assembly of π‐Conjugated Pyridine–Carboxylate24La3Ga5HfO14: Rare-Earth Polyhedron Coupled with Structural Protected Octahedron for Designing Nonlinear Optical Material with Wide Bandgap and Well-Balanced Properties5Atomic-Scale Dynamics of Five-Fold Twin Mediated Coalescence: Pathway-Dependent and Defect-Governed Nonclassical Growth Mechanisms30Polar Lithium l -Aspartate Monohydrate: A Semiorganic Ultraviolet Transparent Nonlinear Optical Crystal1Designing an all-organic wide bandgap ultraviolet nonlinear optical crystal3A novel metal-free crystal demonstrating superior birefringence attributed to the synergistic interaction of dual π-conjugated units8DFT investigation of functional group effects on the structure of tetraphenyl porphyrin for enhanced nonlinear optical properties2Optimizing the Hydrogen-Bond Network Drives Cadmium Ce(IV) Fluoride Hydrate with Significantly Enhanced Optical Anisotropy8Achieving the birefringence-bandgap trade-off: Hydrogen-bond engineered biuret-cyanurate14Design and engineering of Diaqua(nitrato-kO,O’)bis(L-phenylalaninato- kO,O’)lead(II) nitrate using machine learning for optical limiting applications8Hydrogen‐Bond‐Directed Modular Assembly of Polar Chains for Rational Construction of UV Nonlinear Optical Crystals14Engineered Integration of Diverse Functional Units Induces Multifunctionality in Malonate‐Borate Hybrids44Synergistic Design of UV Nonlinear Optical Crystals: Harnessing Flexible π-Conjugated Anions and Guanidinium Cations for Enhanced Performance4BaZn2(HPO3)3: A New Barium Zincophosphite with Short Ultraviolet Cutoff Edge2[HgX 2 ] Linear Group Enabled Ultraviolet Birefringent Crystal RbHg 5 Br 11 with Strong Optical Anisotropy and Wide Bandgap12Na6(SO4)2SiF6: A Stable Sulfate Fluosilicate with Wide Deep-Ultraviolet Transparency Window and Strong Second-Harmonic Generation Response4NaAg3Ga8S14: A new diamond-like framework infrared nonlinear optical material derived from AgGaS26Unlocking Advanced UV NLO Crystals in Rare‐Earth Metal Borate Fluorides via [B 3 O 6 ]‐Mediated Structural Modulation18Hydrogen-bond-driven noncentrosymmetric structure formation in π-conjugated (C3H7N6)(IO3): achieving both strong SHG response and wide bandgap5The nonlinear optical properties and through-space charge-transfer effects of the twist donor-acceptor complexes4Theoretical Insights into Alanine Maleate and Alanine Fumarate: NLO‐Active Single Crystals Stabilized by N─H Intramolecular Hydrogen Bonding0Integrating Fluorinated [BF 4 ] Anion With π‐Conjugated Six‐Membered Rings for Short‐Wavelength UV Frequency Conversion17Integrating Fluorinated [BF 4 ] Anion With π‐Conjugated Six‐Membered Rings for Short‐Wavelength UV Frequency Conversion2Halogen-substitution-driven crystal engineering of chalcones: mechanisms and optimization for spatial ordering and nonlinear optical performance1Nd-doped LYSB: A new multifunctional crystal for efficient multi-wavelength laser emission and frequency conversion0Chiral Lead-Oxyiodide Nonlinear Optical Crystals Constructed on l -Malate Groups5Achieving Ultra‐High Optical Anisotropy via Structural Regulation and Coplanar Engineering of Extended π‐Conjugated [H 2–x C 3 N 3 S 3 ] (x = 1, 2) Groups3Navigating the Landscape of Next-Generation Nonlinear Optical Materials Discovery: Opportunities and Challenges Driven by Artificial Intelligence4Achieving an optimal performance balance in UV nonlinear optical crystals via hydrogen-bond regulation1Broadband infrared-transparent crystals enabled by heterologous isomorphic substitution0Design of borate-squarate hybrid crystals with large birefringence by synergistic assembly of planar π-conjugated groups0Effects of pressure on structural, electronic and optical properties of noncentrosymmetric monoclinic Na3Sr(PO4)(CO3) with discrete [PO4] and [CO3] units0K 7 MgY 2 (B 5 O 10 ) 3 : a novel ultraviolet nonlinear optical crystal based on the [B 5 O 10 ] functional unit2Multifunctional Tetranuclear Copper(I) Complexes with Alkynyl-Imine Bridges: Electrochemical, Luminescent, and Nonlinear Optical Properties0Polyhedral replacement-guided design of Ce3MnGaSe7 featuring strong second-harmonic genera-tion and high laser-induced damage threshold0Stable lead succinate-iodides with strong second-harmonic generation response and large birefringence0Te–Se replacement induced structural transition and enhanced band gaps in Cd 5 Se 4 O 12 Cl 2 and Cd 5 Se 4 O 12 Br 21Two hydrated ionic cocrystals of phenylphosphonate exhibiting second-harmonic generation and proton conductivity0UV and X-ray excited luminescence from m -terphenyl crystals grown by the vertical Bridgman technique0氢键组装的新型紫外非线性光学晶体（R/S‑DACH）Mal·H2O的设计及性能研究（特邀）0Confinement-assembled ultraviolet nonlinear optical crystal from pyridine-expanded π-systems with exhibiting strong SHG and birefringence18Synthesis, photophysical properties, and two-photon absorption behavior of pyrimidinyl urea derivatives1Harnessing tetrahedral diversity: The path to superior diamond-like IR NLO crystals13Enhanced nonlinear optical characteristics of triarylmethane dye in various solvents using Z-scan and DFT method4KHg 4 Ga 5 S 12 : A Diamond-like Tetrahedral Chalcogenide Exhibiting Giant Phase-Matching Second Harmonic Generation6Coordination Geometry-Directed Optical Anisotropy and Phase-Matched Nonlinear Optics in Chiral Metal–Organic Frameworks2[C 3 N 2 H 5 ]B 7 O 10 F 2 : Demonstrating a New Hydrogen‐Bond‐Induced Intralayer Charge‐Balanced Structure Model with Large Birefringence3Nonlinear optical properties of pyrene-based chalcones: Insights from experimental and computational studies4Boosting Linear and Nonlinear Optical Properties of Pt 1 Ag 18 Nanoclusters by Manipulating Ligand‐Shell Rigidity2Origin of Large Second-Harmonic Generation in Nonpolar Molybdenum Tellurite Compounds0Concentration-Dependent Enhancement of Linear and Nonlinear Optical Properties in Hybrid Systems of Perylenediimide and Silver Nanoparticles2Ternary Anion‐Engineered Rare Earth Crystals for Broadband UV Transparency and Enhanced Second‐Harmonic Generation1Rational design of a quasi-0D tungsten tellurite nonlinear optical crystal with exceptionally balanced properties1Exploring the Effect of Electronic Symmetry on the Hyperpolarizabilities of Co(II) and Ni(II) Coordination Complexes with Cytidine Nucleotide6NH 4 B 3 PO 6 (OH) 3 : A Hydroxyborophosphate with Short DUV Cutoff Edge and Large Birefringence2K 3 Mg 2 [K 6 MgCl 3 ][Ga 20 S 36 ]: A Diamond-like Framework Based on Mixed-Type Supertetrahedra for Excellent Nonlinear Optical Property1NaNO 3 [(NH 2 ) 2 SO 2 ] 2 : A Halogen‐Free KBBF‐Type Nitrate Crystal with Record Birefringence for Ultraviolet Applications0Circumventing the Eg–SHG trade-off in selenides: Salt-inclusion [X4Br2][MGa4Se10] with concurrent large band gap and strong nonlinear optical response1Cation-sulfur-driven dimensional reduction engineering for tailoring sulfonate birefringent crystals with enhanced anisotropy2Linear [ICl 2 ] Units Induced Giant Optical Anisotropy in AICl 2 (A = NH 4 , Rb): A Pathway to Advanced Birefringent Materials4A Strategy for Enhancing the Optical Anisotropy of Phosphates via Tetrahedral Unit Modification0π ‐Conjugated Aligned Polar [CO 3 ] Triangulars Synergizing Hydroxylation Enables Stress‐Enhanced Geometric–Electronic Asymmetries for Hydrogen Piezoevolution0Mid‐ to Far‐Infrared Nonlinear Optical Crystals: Design Strategies, Structure–Property Relationships and Engineering Prospects0Growth, Structural Characterization, and Nonlinear Optical Properties of L-Lysinium Hydrogen Adipate Single Crystals: An Integrated Experimental and DFT Study0Fluorine‐Driven Chemical Scissor Effect in Scandium Borates: Structural Evolution with Retained Optically Active Motifs0MZnCO3OH: A family of hydroxycarbonate nonlinear optical crystals in the UV and DUV regions0Chiral Supramolecular Templating Enables Tunable Second‐Harmonic Generation in Hybrid Zinc Thiocyanates0Chiral Supramolecular Templating Enables Tunable Second‐Harmonic Generation in Hybrid Zinc Thiocyanates0Molecular Design and Optical Property Study of D–A– π –A Type Benzothiadiazole Derivatives0The Multi‐Scale Paradigm: An Integrated Design Logic for Nonlinear Optical Crystals1The Multi‐Scale Paradigm: An Integrated Design Logic for Nonlinear Optical Crystals0An Excellent Deep‐Ultraviolet Nonlinear Optical Crystal Realized via a Functional Group Based on a Two‐in‐One Strategy0Assembly of dual π-conjugated units toward enhanced birefringence in a 2D organic sulfonate crystal0Theoretical Study on the Effects of External Electric Field on Nonlinear Optical Properties of Azobenzene0Surface-initiated atom transfer radical polymerization of PHEMA-grafted PVA films: optical parameters, and thermal degradation kinetics0Luminescent materials based on aluminoborate compositions: a review0

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  41. Design and engineering of Diaqua(nitrato-kO,O’)bis(L-phenylalaninato- kO,O’)lead(II) nitrate using machine learning for optical limiting applications

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  42. Hydrogen‐Bond‐Directed Modular Assembly of Polar Chains for Rational Construction of UV Nonlinear Optical Crystals

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  43. Engineered Integration of Diverse Functional Units Induces Multifunctionality in Malonate‐Borate Hybrids

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  44. Synergistic Design of UV Nonlinear Optical Crystals: Harnessing Flexible π-Conjugated Anions and Guanidinium Cations for Enhanced Performance

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  45. BaZn2(HPO3)3: A New Barium Zincophosphite with Short Ultraviolet Cutoff Edge

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  46. [HgX 2 ] Linear Group Enabled Ultraviolet Birefringent Crystal RbHg 5 Br 11 with Strong Optical Anisotropy and Wide Bandgap

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