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RESEARCH PAPER · Aggregate · 2025

Engineered Integration of Diverse Functional Units Induces Multifunctionality in Malonate‐Borate Hybrids

Ziqi Chen, Chenxu Li, Xiaoyu Wu, Juanjuan Lu, Zhihua Yang, Xueling Hou, Miriding Mutailipu

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Engineered Integration of Diverse Functional Units Induces Multifunctionality in Malonate‐Borate HybridsOriginalA new ultraviolet-transparent molybdate featuring a layered structure and moderate birefringence0KNa 2 Y 2 B 2 O 6 F 3 : a beryllium free deep-UV nonlinear optical crystal with well-balanced properties2Exceptional Enhancement of Optical Anisotropy Achieved via the Strategy of Combining Rigid Groups with High Symmetry and π‐Conjugated Organic Groups in Hybrid Fluorides33The nonlinear optical properties and through-space charge-transfer effects of the twist donor-acceptor complexes4Quantum chemical investigation of Z-shaped Diradicaloid heptazethrene derivatives towards linear and nonlinear optical polarizability2Dual-anion synergy drives remarkable birefringence in sulfate–nitrate crystals1Integrating Fluorinated [BF 4 ] Anion With π‐Conjugated Six‐Membered Rings for Short‐Wavelength UV Frequency Conversion17Integrating Fluorinated [BF 4 ] Anion With π‐Conjugated Six‐Membered Rings for Short‐Wavelength UV Frequency Conversion2Broadband infrared-transparent crystals enabled by heterologous isomorphic substitution0Cation-dominated second-harmonic generation in chiral tetrahydro-1-naphthylammonium halides0Centimeter-scale chiral zero-dimensional manganese halide hybrids with green emission and second-harmonic generation0Chiral calcium thiocyanate hybrids: amino acid-enabled structural diversity and second-harmonic generation0Experimental measurements and density functional theory analysis of a novel Mannich base: structural and nonlinear optical perspectives1From centrosymmetric (C 4 H 8 N 5 )(SbF 4 ) to polar (C 4 H 7 N 4 O)(SbF 4 ): a new UV nonlinear optical material achieved by functional group modulation8K 7 MgY 2 (B 5 O 10 ) 3 : a novel ultraviolet nonlinear optical crystal based on the [B 5 O 10 ] functional unit2LiHgTeO 3 : a Hg( i )-containing tellurite crystal with typical Hg–Hg bonds0SnCl 2 [SC(NH 2 ) 2 ]: lone-pair and hydrogen-bonding triggered chromophore assembling for dual optical optimization0Solving the long-standing hygroscopicity and thermal stability issues of the nonlinear optical crystal α-LiIO 3 via homogeneous cation exchange0Te–Se replacement induced structural transition and enhanced band gaps in Cd 5 Se 4 O 12 Cl 2 and Cd 5 Se 4 O 12 Br 21UV and X-ray excited luminescence from m -terphenyl crystals grown by the vertical Bridgman technique0Zn 4 (BO 3 ) 2 (CO 2 CH 2 NH 2 ) 2 ·H 2 O: An Organic–Inorganic Hybridized KBe 2 BO 3 F 2 -like Ultraviolet Nonlinear Optical Crystal3Enhanced nonlinear optical characteristics of triarylmethane dye in various solvents using Z-scan and DFT method4Ba 5 Zn 4 (B 3 O 6 ) 2 (B 12 O 24 ): A Borate with Edge-Sharing [BO 4 ] Tetrahedral Connection by Introducing Zn into β-BaB 2 O 42Strategic Integration Between Trigonal Architecture Construction and Molecular Polarization Enhancement for Record SHG Effect in Selenates4Strategic Integration Between Trigonal Architecture Construction and Molecular Polarization Enhancement for Record SHG Effect in Selenates0Concentration-Dependent Enhancement of Linear and Nonlinear Optical Properties in Hybrid Systems of Perylenediimide and Silver Nanoparticles2Conformational Editing Drives Covalent Hybridization for Nonlinear Optical Crystals2Boosting Ultraviolet Phase‐Matching Performance of B 3 O 7 ‐Based Systems via Synergistic Fluorination and Organic Modification Strategy1Chirality-driven polar lattice engineering for high-performance organic nonlinear optical crystals3From Coplanarity to Coaxiality: A Linearity-Oriented Design Paradigm for Ultrahigh Ultraviolet Birefringent Inorganic Crystals4Research advances in rare-earth nonlinear optical crystalline materials in 20250Exploring third-order NLO response of Cu-doped Ag 2 S/PMMA thin films under CW laser excitation0First‐Principles Investigation of the Structural, Electronic, Optical, Elastic, and Thermal Properties of Defect Diamond‐Like Hg 3 P 2 S 80Halogen-Mediated Dimensionality Reduction in Bismuth Oxychlorides: Trade-off between Birefringence and Band Gap0Rational Design of a Strong Nonlinear Optical Crystal With Ultrawide Bandgap via Fine‐Tuning of Channel Structures0Reversible Symmetry Switching, Giant Birefringence, and UV Second‐Harmonic Generation in Hybrid Niobium Oxyfluorides0Reversible Symmetry Switching, Giant Birefringence, and UV Second‐Harmonic Generation in Hybrid Niobium Oxyfluorides0Proton-transfer-induced supramolecular assembly of 4-Aminopyridinium hydrogen maleate: Synthesis, structure-property correlation toward nonlinear optical (NLO) applications0The Multi‐Scale Paradigm: An Integrated Design Logic for Nonlinear Optical Crystals1The Multi‐Scale Paradigm: An Integrated Design Logic for Nonlinear Optical Crystals0Rational Construction of Fluoride Crystals With Record Birefringence via Water‐Regulated Hydrogen‐Bond Network Reconfiguration0Rational Construction of Fluoride Crystals With Record Birefringence via Water‐Regulated Hydrogen‐Bond Network Reconfiguration0Dual‐Role BF 3 Anchoring Enables Giant Birefringence in Short‐Wave UV‐Transparent Fluoroborates0Halogen‐Bond Dimensionality Controls π–π Packing to Unlock Ultrahigh Second‐Harmonic Generation and Giant Birefringence0

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  1. A new ultraviolet-transparent molybdate featuring a layered structure and moderate birefringence

    New Journal of Chemistry · 2025-01-01

    Shiyu Du, Paipai Zhang, Haozhen Liu, Donghai An, Yanna Chen

    Read original paper ↗ ·

  2. KNa 2 Y 2 B 2 O 6 F 3 : a beryllium free deep-UV nonlinear optical crystal with well-balanced properties

    Chemical Communications · 2025-01-01

    Huijian Zhao, Mengru Liu, Weina Nan, Ning Yang, Conggang Li, Ning Ye, Zhanggui Hu

    Read original paper ↗ ·

  3. Exceptional Enhancement of Optical Anisotropy Achieved via the Strategy of Combining Rigid Groups with High Symmetry and π‐Conjugated Organic Groups in Hybrid Fluorides

    Advanced Science · 2025-10-06

    Ru‐Ling Tang, Bing-Wei Miao, Guo-Ren Zhu, Wenlong Liu, Sheng‐Ping Guo

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  4. The nonlinear optical properties and through-space charge-transfer effects of the twist donor-acceptor complexes

    Dyes and Pigments · 2025-10-21

    Li Wang, Tongwei Liu, Yanli Liu, Mei‐Shan Wang

    Read original paper ↗ ·

  5. Quantum chemical investigation of Z-shaped Diradicaloid heptazethrene derivatives towards linear and nonlinear optical polarizability

    Journal of Molecular Graphics and Modelling · 2025-11-17

    Rao Aqil Shehzad, Javed Iqbal, Shaukat Ali, Hafeez Anwar

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  6. Dual-anion synergy drives remarkable birefringence in sulfate–nitrate crystals

    Inorganic Chemistry Frontiers · 2025-11-24

    LeHui Liu, FeiFei Yuan, YiSheng Huang, LiZhen Zhang, ZhouBin Lin

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  7. Integrating Fluorinated [BF 4 ] Anion With π‐Conjugated Six‐Membered Rings for Short‐Wavelength UV Frequency Conversion

    Angewandte Chemie International Edition · 2025-11-26

    Xiangyu Long, Fuming Li, Haotian Qiu, Xueling Hou, Juanjuan Lu, Junjie Li, Zhihua Yang, Jinhui Cao, Shilie Pan, Miriding Mutailipu

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  8. Integrating Fluorinated [BF 4 ] Anion With π‐Conjugated Six‐Membered Rings for Short‐Wavelength UV Frequency Conversion

    Angewandte Chemie · 2025-11-26

    Xiangyu Long, Fuming Li, Haotian Qiu, Xueling Hou, Juanjuan Lu, Junjie Li, Zhihua Yang, Jinhui Cao, Shilie Pan, Miriding Mutailipu

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  9. Broadband infrared-transparent crystals enabled by heterologous isomorphic substitution

    Dalton Transactions · 2026-01-01

    B Yang, Ziqi Chen, Zhenjiang Lu, Juanjuan Lu

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  10. Cation-dominated second-harmonic generation in chiral tetrahydro-1-naphthylammonium halides

    Dalton Transactions · 2026-01-01

    Youpei Zhang, Junjie Guan, Junhua Zhang, X Q Li, J Z Zhao, Yimin Yang, Yongshen Zheng, Jialiang Xu

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  11. Centimeter-scale chiral zero-dimensional manganese halide hybrids with green emission and second-harmonic generation

    Dalton Transactions · 2026-01-01

    Shanshan Wei, Yunfei Zhang, Guoming Lin, Yuqin Zhu, Lihua Yu, Cunqin Ji, Guoming Lin

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  12. Chiral calcium thiocyanate hybrids: amino acid-enabled structural diversity and second-harmonic generation

    Chemical Communications · 2026-01-01

    Xuemei Wen, Yingjie Wang, Guohong Zou, Zhien Lin, Kang Min Ok

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  13. Experimental measurements and density functional theory analysis of a novel Mannich base: structural and nonlinear optical perspectives

    CrystEngComm · 2026-01-01

    Dennis A. Raj, Mani Jeeva, R. Purusothaman, I. Vetha Potheher

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  14. From centrosymmetric (C 4 H 8 N 5 )(SbF 4 ) to polar (C 4 H 7 N 4 O)(SbF 4 ): a new UV nonlinear optical material achieved by functional group modulation

    Chemical Science · 2026-01-01

    Zhixiang Wang, Chun-Li Hu, Chuan‐Fu Sun, Jiang‐Gao Mao, Fang Kong

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  15. K 7 MgY 2 (B 5 O 10 ) 3 : a novel ultraviolet nonlinear optical crystal based on the [B 5 O 10 ] functional unit

    New Journal of Chemistry · 2026-01-01

    Haozhen Liu, Shiyu Du, Paipai Zhang, Jiawei Zhao, Yanna Chen, Donghai An

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  16. LiHgTeO 3 : a Hg( i )-containing tellurite crystal with typical Hg–Hg bonds

    Dalton Transactions · 2026-01-01

    Ruliu Zhou, Piao Tang, Xin Wen, Zhiyong Xue, J Chen, Guang Peng, Ning Ye, Zhanggui Hu

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  17. SnCl 2 [SC(NH 2 ) 2 ]: lone-pair and hydrogen-bonding triggered chromophore assembling for dual optical optimization

    Dalton Transactions · 2026-01-01

    Xing-Yu Bi, Yuting Gao, Chenyuan Ma, Zhi Gang Fang, Meihong Duan

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  18. Solving the long-standing hygroscopicity and thermal stability issues of the nonlinear optical crystal α-LiIO 3 via homogeneous cation exchange

    Inorganic Chemistry Frontiers · 2026-01-01

    Jiahao Wan, Zhengli Liang, Xiuying Zhang, Hongming Liu, Le Yang, Ping Wang, Lehui Liu, Xingxing Jiang, Zheshuai Lin, Qi Wu

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  19. Te–Se replacement induced structural transition and enhanced band gaps in Cd 5 Se 4 O 12 Cl 2 and Cd 5 Se 4 O 12 Br 2

    Dalton Transactions · 2026-01-01

    Maqsood Iqbal, Jiazheng Zhou, Aqsa Munawar, Juanjuan Lu, Junjie Li

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  20. UV and X-ray excited luminescence from m -terphenyl crystals grown by the vertical Bridgman technique

    Journal of Materials Chemistry C · 2026-01-01

    Praveen Joshwa Ramesh, Rajesh Paulraj, Mohit Tyagi

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  21. Zn 4 (BO 3 ) 2 (CO 2 CH 2 NH 2 ) 2 ·H 2 O: An Organic–Inorganic Hybridized KBe 2 BO 3 F 2 -like Ultraviolet Nonlinear Optical Crystal

    Inorganic Chemistry · 2026-01-27

    Yanming Han, Chensheng Lin, Xin Wen, Jindong Chen, Jiyang Wang, Zhanggui Hu, Ning Ye, Guang Peng

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  22. Enhanced nonlinear optical characteristics of triarylmethane dye in various solvents using Z-scan and DFT method

    Optics & Laser Technology · 2026-02-03

    Mohammad Ahmad Wadaan, Nawaf D. Almoutiri, Rohith Ramasamy, Rajadurai Vijay Solomon, A. G. Bharathi Dileepan, Madhappan Santhamoorthy, S. Jeyaram

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  23. Ba 5 Zn 4 (B 3 O 6 ) 2 (B 12 O 24 ): A Borate with Edge-Sharing [BO 4 ] Tetrahedral Connection by Introducing Zn into β-BaB 2 O 4

    Inorganic Chemistry · 2026-02-05

    Kaitong Liu, Yuan Rao, Zhaoxue Li, Shihang Zhou, Zhizhong Zhang, Yanhui Zhang

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  24. Strategic Integration Between Trigonal Architecture Construction and Molecular Polarization Enhancement for Record SHG Effect in Selenates

    Angewandte Chemie International Edition · 2026-02-17

    Jin Li, Deshuai Xiao, Xinyuan Zhang, Pifu Gong, Zheshuai Lin, Zhanggui Hu, Ning Ye

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  25. Strategic Integration Between Trigonal Architecture Construction and Molecular Polarization Enhancement for Record SHG Effect in Selenates

    Angewandte Chemie · 2026-02-17

    Jin Li, Deshuai Xiao, Xinyuan Zhang, Pifu Gong, Zheshuai Lin, Zhanggui Hu, Ning Ye

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  26. Concentration-Dependent Enhancement of Linear and Nonlinear Optical Properties in Hybrid Systems of Perylenediimide and Silver Nanoparticles

    Nanomaterials · 2026-03-05

    Tarek Mohamed, Majed H. El-Motlak, Fatma Abdel Samad, Mohamed E. El‐Khouly, Alaa Mahmoud

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  27. Conformational Editing Drives Covalent Hybridization for Nonlinear Optical Crystals

    Angewandte Chemie · 2026-03-09

    Ziqi Chen, Chenxu Li, Bowen Yang, Juanjuan Lu, Zhihua Yang, Junjie Li, Xueling Hou, Shilie Pan, Miriding Mutailipu

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  28. Boosting Ultraviolet Phase‐Matching Performance of B 3 O 7 ‐Based Systems via Synergistic Fluorination and Organic Modification Strategy

    Advanced Optical Materials · 2026-04-01

    Xueli Du, Haoran Liu, Wenhu Wang, Haoran Wang, Xueyan Wu, Min Zhang

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  29. Chirality-driven polar lattice engineering for high-performance organic nonlinear optical crystals

    Science China Materials · 2026-04-07

    Bo Liu, Jiali Chen, Yu-Peng Han, Qiaohong Li, Shangda Li, Fusong Wang, Jian Zhang

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  30. From Coplanarity to Coaxiality: A Linearity-Oriented Design Paradigm for Ultrahigh Ultraviolet Birefringent Inorganic Crystals

    Journal of the American Chemical Society · 2026-05-04

    Congcong Jin, Yang Li, Chong‐An Chen, Wei Zeng, S. D. Lee, Kang Min Ok

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  31. Research advances in rare-earth nonlinear optical crystalline materials in 2025

    Journal of Rare Earths · 2026-07-21

    Tiantian He, Dandan Zhou, Fang Kong, Jianggao Mao

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  32. Exploring third-order NLO response of Cu-doped Ag 2 S/PMMA thin films under CW laser excitation

    Materials Research Innovations · 2026-07-22

    Yuoraj S. Tamgadge, Prashant Gedam, Gajanan G. Muley, Rajesh Ganorkar, Kulbhushan Meghal, V. G. Pahurkar

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  33. First‐Principles Investigation of the Structural, Electronic, Optical, Elastic, and Thermal Properties of Defect Diamond‐Like Hg 3 P 2 S 8

    Advanced Physics Research · 2026-07-23

    Saravana Karthikeyan SKS, Sankar Ganesh Ramaraj, Ryo Watanabe, Choji Fukuhara, Chang Yi Kong

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  34. Halogen-Mediated Dimensionality Reduction in Bismuth Oxychlorides: Trade-off between Birefringence and Band Gap

    Journal of Molecular Structure · 2026-08-03

    Huaiqiang Xun, Shumei Cao, Qingyue Cui, Yi Feng, Rui Wu, Chunmei Huang, Leyan Nian

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  35. Rational Design of a Strong Nonlinear Optical Crystal With Ultrawide Bandgap via Fine‐Tuning of Channel Structures

    Laser & Photonics Review · 2026-08-15

    Zilong Geng, Zuju Ma, Ruibiao Fu, Xin-Tao Wu

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  36. Reversible Symmetry Switching, Giant Birefringence, and UV Second‐Harmonic Generation in Hybrid Niobium Oxyfluorides

    Angewandte Chemie International Edition · 2026-09-03

    S. D. Lee, Wei Zeng, Congcong Jin, Chong‐An Chen, Kang Min Ok

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  37. Reversible Symmetry Switching, Giant Birefringence, and UV Second‐Harmonic Generation in Hybrid Niobium Oxyfluorides

    Angewandte Chemie · 2026-09-03

    S. D. Lee, Wei Zeng, Congcong Jin, Chong‐An Chen, Kang Min Ok

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  38. Proton-transfer-induced supramolecular assembly of 4-Aminopyridinium hydrogen maleate: Synthesis, structure-property correlation toward nonlinear optical (NLO) applications

    Materials Science and Engineering B · 2026-09-08

    S. Balaji, B. Sahaya Infant Lasalle, Muthu Senthil Pandian, K. Anitha

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  39. The Multi‐Scale Paradigm: An Integrated Design Logic for Nonlinear Optical Crystals

    Angewandte Chemie International Edition · 2026-09-10

    Xiangqing Cao, Haotian Qiu, Juanjuan Lu, Yun Mo Yang, Xueling Hou, Junjie Li, Shilie Pan, Miriding Mutailipu

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  40. The Multi‐Scale Paradigm: An Integrated Design Logic for Nonlinear Optical Crystals

    Angewandte Chemie · 2026-09-10

    Xiangqing Cao, Haotian Qiu, Juanjuan Lu, Yun Mo Yang, Xueling Hou, Junjie Li, Shilie Pan, Miriding Mutailipu

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  41. Rational Construction of Fluoride Crystals With Record Birefringence via Water‐Regulated Hydrogen‐Bond Network Reconfiguration

    Angewandte Chemie · 2026-09-11

    Ru‐Ling Tang, Bing-Wei Miao, Ling Wang, Zheng-Yu Yang, Guo-Ren Zhu, Wenlong Liu, Sheng‐Ping Guo

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  42. Rational Construction of Fluoride Crystals With Record Birefringence via Water‐Regulated Hydrogen‐Bond Network Reconfiguration

    Angewandte Chemie International Edition · 2026-09-11

    Ru‐Ling Tang, Bing-Wei Miao, Ling Wang, Zheng-Yu Yang, Guo-Ren Zhu, Wenlong Liu, Sheng‐Ping Guo

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  43. Dual‐Role BF 3 Anchoring Enables Giant Birefringence in Short‐Wave UV‐Transparent Fluoroborates

    Advanced Functional Materials · 2026-09-30

    Jin Chen, Jia‐Min Lian, Huai‐Yu Wu, Yun‐Xia Hu, Jinyu Luo, Yiru Fu, Cai‐Yi Liu, Ke‐Zhao Du

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  44. Halogen‐Bond Dimensionality Controls π–π Packing to Unlock Ultrahigh Second‐Harmonic Generation and Giant Birefringence

    Small · 2026-10-04

    Jin Chen, Yun‐Xia Hu, Huai‐Yu Wu, Jia‐Min Lian, Jinyu Luo, Yiru Fu, Ke‐Zhao Du

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