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RESEARCH PAPER · Angewandte Chemie International Edition · 2025

Giant Birefringence and Solar‐Blind Ultraviolet Transmission by Coordination‐Induced Assembly of π‐Conjugated Pyridine–Carboxylate

Peng‐Hui Guo, Xia Zhang, Xia Zhang, Yao Guo, Nan Zhang, Yi‐Gang Chen, Xingxing Jiang, Zheshuai Lin, Xian‐Ming Zhang, Xian‐Ming Zhang

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Giant Birefringence and Solar‐Blind Ultraviolet Transmission by Coordination‐Induced Assembly of π‐Conjugated Pyridine–CarboxylateOriginalA strongly birefringent sulfate crystal with a wide second-harmonic generation phase-matching range4K 2 GdB 3 O 6 F 2 : A Promising Short-Wave UV Birefringent Crystal via Optimized Assembly of π-Conjugated [B 3 O 6 ] Groups8Chiral-Unit-Driven Short-Wave Ultraviolet Nonlinear Optical Acetates with Balanced Overall Optical Properties3A mercury-based selenite with wide bandgap and moderate birefringence via cation substitution and partial fluorination1Achieving giant optical anisotropy in the mid-far infrared region via ideal alignment of dual functional motifs0Counterion engineering in open-framework crystals: dual enhancement of birefringence and UV transparency in Cd–oxalate framework via cation substitution0Covalent hybrid cadmium halides with heteroleptic tetrahedral units exhibiting a wideband nonlinear optical response0Strategically designed deep-ultraviolet optical crystals with balanced properties by small heteroatom substitution1Type I Framework Complex: Photocontrolled Superoxide Anion Generator4Realizing Phase‐Matching of Nonlinear Optical [ABa 3 Br 2 ][Ga 5 Se 10 ] (A = Cs, Rb, K, Na) Through Large Anisotropic Lattice Distortion11Halogen‐Bond Coupled Halogenated‐π‐Conjugation Enables Giant Birefringence in Hydrogen‐Bonded Organic Frameworks13Unit Symmetry‐Breaking and Layered Linear Ordering Enabling Superior Short‐Wave Ultraviolet Birefringent Crystal8Density-Compensated Polarizability Anisotropy for Record Birefringence in Short-Wavelength Ultraviolet Inorganic Crystals11Overcoming the Bandgap‐Birefringence Trade‐Off: Proton‐Transfer Engineering of High‐Performance Ultraviolet‐Transparent Organic Crystal5Ultrawide Bandgap and Record-High Birefringence in a Covalent Beryllium-Organic Framework7Electronegativity Adaption Approach for Solar‐Blind UV Birefringent Crystals With Ultrawide Bandgaps2Lock‐and‐Key Assembly Enables Record Birefringence in Monocyclic π‐Conjugated Crystals via Spatial Confinement of Linear Polyhalide5Bio-inspired proton-conformation-coupled hydrogen-bond network reconfiguration for adaptive optical anisotropy0From High Symmetry to High Symmetry: A Self‐Assembly Strategy for Synthesizing Large Birefringent Borates0Organic Metal Chalcogenide Films With Giant Birefringence0Organic Metal Chalcogenide Films With Giant Birefringence0Cation-Modulated Activation of Linear Units in an Ordered Arrangement Achieves the Largest Optical Anisotropy in Wide-Bandgap Metal Chalcogenides0Rational Construction of Fluoride Crystals With Record Birefringence via Water‐Regulated Hydrogen‐Bond Network Reconfiguration0Domino‐Effect Amplification via Covalent‐Chain Engineering for Giant Birefringence in NaAsQ 2 (Q = S, Se) Crystals0

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  1. A strongly birefringent sulfate crystal with a wide second-harmonic generation phase-matching range

    Journal of Materials Chemistry C · 2025-01-01

    Zhiyong Bai, Shanshan Chen, Xu Chen, Yong Wang, Xinwei Zhou, Yipeng Song, Yanqiang Li, Sangen Zhao, Junhua Luo

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  2. K 2 GdB 3 O 6 F 2 : A Promising Short-Wave UV Birefringent Crystal via Optimized Assembly of π-Conjugated [B 3 O 6 ] Groups

    Inorganic Chemistry · 2025-10-14

    Mengru Liu, Huijian Zhao, Xianghao Kong, Ning Ye, Zhanggui Hu, Conggang Li

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  3. Chiral-Unit-Driven Short-Wave Ultraviolet Nonlinear Optical Acetates with Balanced Overall Optical Properties

    The Journal of Physical Chemistry Letters · 2025-12-26

    Zi-Xuan Zhao, Wei Chen, Hui‐Yan Zhao, Mengjiao Xu, Chao He, Qi Wei, Guo-Ming Wang

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  4. A mercury-based selenite with wide bandgap and moderate birefringence via cation substitution and partial fluorination

    Dalton Transactions · 2026-01-01

    Chen Zhu, Xiao-Min Wu, Xiao-Xue Wang, Si-Qi Zhou, Jing-Jing Wu, Xin-Lei Liu, You-Qian Wu, Jiannian Yao, Peng-Fei Li, Yu-Wu Zhong

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  5. Achieving giant optical anisotropy in the mid-far infrared region via ideal alignment of dual functional motifs

    Inorganic Chemistry Frontiers · 2026-01-01

    Yi-Wen Shan, Ming‐Zhi Zhang, C Hu, Jiang‐Gao Mao

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  6. Counterion engineering in open-framework crystals: dual enhancement of birefringence and UV transparency in Cd–oxalate framework via cation substitution

    CrystEngComm · 2026-01-01

    Chenyuan Ma, Jingyi Xie, Zhi Fang, Meihong Duan

    Read original paper ↗ ·

  7. Covalent hybrid cadmium halides with heteroleptic tetrahedral units exhibiting a wideband nonlinear optical response

    Inorganic Chemistry Frontiers · 2026-01-01

    Yi-Fan Fu, Wen‐Dong Yao, Ruo‐Nan Li, Qiuwei Huang, Qiu-Xia Tang, Jiajing Wu, Sheng‐Ping Guo

    Read original paper ↗ ·

  8. Strategically designed deep-ultraviolet optical crystals with balanced properties by small heteroatom substitution

    Inorganic Chemistry Frontiers · 2026-01-01

    Mei Hu, Zhencheng Wu, Xin Su, Hongheng Chen, Qun Jing, Zhaohui Chen, Ming‐Hsien Lee

    Read original paper ↗ ·

  9. Type I Framework Complex: Photocontrolled Superoxide Anion Generator

    Research · 2026-01-01

    Zehao Jing, Yingying Zhang, Yelin Wu, Xiaoqiang Chen, Meizhen Yin, Mingwei Li, Xiaojun Peng

    Read original paper ↗ ·

  10. Realizing Phase‐Matching of Nonlinear Optical [ABa 3 Br 2 ][Ga 5 Se 10 ] (A = Cs, Rb, K, Na) Through Large Anisotropic Lattice Distortion

    Angewandte Chemie International Edition · 2026-01-05

    Meng‐Na Jing, Si‐Fan Lu, Xiao‐Ming Jiang, Bin‐Wen Liu, Guo‐Cong Guo

    Read original paper ↗ ·

  11. Halogen‐Bond Coupled Halogenated‐π‐Conjugation Enables Giant Birefringence in Hydrogen‐Bonded Organic Frameworks

    Advanced Science · 2026-01-14

    Miao‐Bin Xu, Yun‐Xia Hu, Ming‐Chang Wang, Jia‐jia Li, Jia‐Min Lian, Jin Chen, Ke‐Zhao Du

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  12. Unit Symmetry‐Breaking and Layered Linear Ordering Enabling Superior Short‐Wave Ultraviolet Birefringent Crystal

    Angewandte Chemie International Edition · 2026-01-14

    Xin Wen, Dequan Kong, Jingyao Lu, Jindong Chen, Haohai Yu, Huaijin Zhang, Zhanggui Hu, Jiyang Wang, Ning Ye, Guang Peng

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  13. Density-Compensated Polarizability Anisotropy for Record Birefringence in Short-Wavelength Ultraviolet Inorganic Crystals

    Journal of the American Chemical Society · 2026-03-05

    Chong‐An Chen, Yang Li, Congcong Jin, S. D. Lee, Zhihua Yang, Kang Min Ok

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  14. Overcoming the Bandgap‐Birefringence Trade‐Off: Proton‐Transfer Engineering of High‐Performance Ultraviolet‐Transparent Organic Crystal

    Angewandte Chemie · 2026-03-05

    Lin Qiu, Xing‐Yu Li, Bing-Wei Miao, Hongjian Yu, Wenlong Liu, Yifan Sun, Ru‐Ling Tang

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  15. Ultrawide Bandgap and Record-High Birefringence in a Covalent Beryllium-Organic Framework

    Journal of the American Chemical Society · 2026-04-21

    Peng-Hui Guo, Xia Zhang, Xia Zhang, Miriding Mutailipu, Sangen Zhao, Nan Zhang, Yao Guo, Lei Huai, Yi-Gang Chen, Xian-Ming Zhang, Xian-Ming Zhang

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  16. Electronegativity Adaption Approach for Solar‐Blind UV Birefringent Crystals With Ultrawide Bandgaps

    Angewandte Chemie International Edition · 2026-04-23

    Xinwei Zhou, Zhiyong Bai, Ji Qi, Yuexin Zhang, Weiqi Huang, Yipeng Song, Yong Wang, Chang Liu, Sangen Zhao, Junhua Luo

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  17. Lock‐and‐Key Assembly Enables Record Birefringence in Monocyclic π‐Conjugated Crystals via Spatial Confinement of Linear Polyhalide

    Angewandte Chemie International Edition · 2026-05-26

    Yun‐Xia Hu, Huai Yu Wu, Jia‐jia Li, Ming‐Chang Wang, Jia‐Min Lian, Jin Yu Luo, Yiru Fu, Zi‐Yan Chen, Yang‐Hang Guo, Jin Chen, Ke‐Zhao Du

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  18. Bio-inspired proton-conformation-coupled hydrogen-bond network reconfiguration for adaptive optical anisotropy

    Research Square · 2026-06-02

    Kang Min Ok, Yayong Sun, Jiachen Lu, Yanqiang Li, Wei Zeng, Chong‐An Chen, Congcong Jin, Hyungjin Lim, S. D. Lee, Hanjung Kim, Junhua Zhang, Tianhua Zhou

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  19. From High Symmetry to High Symmetry: A Self‐Assembly Strategy for Synthesizing Large Birefringent Borates

    Small · 2026-08-03

    Chunjie Shen, Junwei Feng, Zhihua Yang, Shilie Pan, Feng Zhang

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  20. Organic Metal Chalcogenide Films With Giant Birefringence

    Angewandte Chemie · 2026-09-01

    Zhi-Qing Lan, Li‐Hua Peng, Chao-Hong Xie, Liang‐Liang Peng, Shiyuan Liu, Xiaoqing Yu, Jiangfeng Lu, Honggang Gu, Guan‐E Wang, Gang Xu

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  21. Organic Metal Chalcogenide Films With Giant Birefringence

    Angewandte Chemie International Edition · 2026-09-01

    Zhi-Qing Lan, Li‐Hua Peng, Chao‐Hong Xie, Liang‐Liang Peng, Shiyuan Liu, Xiaoqing Yu, Jiangfeng Lu, Honggang Gu, Guan‐E Wang, Gang Xu

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  22. Cation-Modulated Activation of Linear Units in an Ordered Arrangement Achieves the Largest Optical Anisotropy in Wide-Bandgap Metal Chalcogenides

    Chemistry of Materials · 2026-09-09

    Wen‐Dong Yao, Xiao Huang, Qiu-Yang Du, Xu‐Bin Ni, Wenlong Liu, Sheng‐Ping Guo

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  23. Rational Construction of Fluoride Crystals With Record Birefringence via Water‐Regulated Hydrogen‐Bond Network Reconfiguration

    Angewandte Chemie International Edition · 2026-09-11

    Ru‐Ling Tang, Bing-Wei Miao, Ling Wang, Zheng-Yu Yang, Guo-Ren Zhu, Wenlong Liu, Sheng‐Ping Guo

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  24. Domino‐Effect Amplification via Covalent‐Chain Engineering for Giant Birefringence in NaAsQ 2 (Q = S, Se) Crystals

    Laser & Photonics Review · 2026-09-24

    Bo Zhang, Weiqi Huang, Yang Chi, Xin‐Tao Wu, Hua Lin, Qi‐Long Zhu

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