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RESEARCH PAPER · Angewandte Chemie International Edition · 2024

Ultra‐Narrow Alkane Product Distribution in Polyethylene Waste Hydrocracking by Zeolite Micro‐Mesopore Diffusion Optimization

Shuai Wang, Weichen Wang, Mingyu Chu, Daowei Gao, Yong Wang, Yipin Lv, Rongyao Wang, Lianghao Song, Huaiqing Zhao, Jinxing Chen, Guozhu Chen

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Ultra‐Narrow Alkane Product Distribution in Polyethylene Waste Hydrocracking by Zeolite Micro‐Mesopore Diffusion OptimizationOriginalGradient-temperature control enhances oxi-upcycling of polyethylene plastics to dicarboxylic acids over TS-1 zeolite14Catalytic coproduction of renewable lubricant base oils and diesel fuels from bio-lipids and aromatics via alkylation and hydrodeoxygenation5Recent developments in recycling of post-consumer polyethylene waste33Insights into Chemical Recycling and Upgrading Strategies for Polyolefin-Based Plastics15Upgrading polyolefin plastics: experiences from petroleum refining and distinct characteristics19Hydrocracking of Polyethylene to Gasoline-Range Hydrocarbons over a Ruthenium-Zeolite Bifunctional Catalyst System with Optimal Synergy of Metal and Acid Sites9Enhancing Waste Plastic Hydrogenolysis on Ru/CeO 2 Through Concurrent Incorporation of Fe Single Atoms and FeO x Nanoclusters27Enhancing Waste Plastic Hydrogenolysis on Ru/CeO 2 Through Concurrent Incorporation of Fe Single Atoms and FeO x Nanoclusters4Co-recycling of plastics and other waste materials70Hydrogen Spillover‐Induced Brønsted Acidity Enables Controllable Hydrocracking of Polyolefin Waste to Liquid Fuels32Hydrogen Spillover‐Induced Brønsted Acidity Enables Controllable Hydrocracking of Polyolefin Waste to Liquid Fuels4Oxidation of n-alkanes using TS-1 and H2O2: Effects of chain length and solvents2A Minimalist Design for a Dual-Catalyst System for High-Efficiency Conversion of Waste Plastics into Liquid Fuel Products27ZSM-5/Y composite zeolite enabled via ZSM-5 refabrication and outstanding performance of the composite in VGO catalytic cracking6Transforming Textile Waste: Innovative Pathways to High-Value Material Upcycling8Dual-catalyst system without supported metals toward polyethylene waste upcycling3Impact of Acid Sites in ZSM-5 Zeolites on the Selective Catalytic Oxi-Upcycling of High-Density Polyethylene to Dicarboxylic Acid under Mild Conditions16Synthesis and Applications of Zeolite-Encapsulated Metal Catalysts13Toward Sustainable Plastic Waste Valorization: Green Synergistic Catalytic Strategies for Plastic Upcycling12Plasma Catalysis for Plastic Waste Conversion into Value‐Added Products: Advancements and Perspectives11Beyond Monosite Catalysis: Multi‐Tiered Site Engineering for Advanced CO 2 Valorization9A review of recent advances in thermal-catalytic cracking of plastic waste8Bayesian Optimization of Hierarchical ZSM-5 for High-Efficiency Polyolefin Waste Recycling to Light Olefins7Selective Hydrocracking of Polyethylene to Gasoline Over Bi‐Functional Ir/HBEA Catalysts Under Mild Condition2Surface and Interface Properties of Metal Species for Waste Plastic Hydroconversion6Research progress in metal-zeolite bifunctional systems for upcycling of waste polyolefins3Synergy between acidity and Pt in Pt/HY zeolite for boosting the hydrocracking of polyethylene to C5-C7 liquid fuels0Entropy Engineering for the Efficient Hydrogenolysis of Waste Polyolefins1Single-Atom Ni on Tungsten Oxides Drives Hydrogen Spillover for Efficient Plastic Waste Upcycling13Research progress of high value utilization of waste polyethylene plastics6Acidified montmorillonite (MMT)-supported ultrafine Ru nanoparticles for polyethylene plastic upcycling0Direct upcycling of mixed plastic waste into liquid alkanes3Highly selective hydrocracking of polypropylene to gasoline-range fuels over the Pt/MCM-22 catalyst0Plastic Waste Conversion into Monomers Using Microwaves0Synergistic pore-acidity engineering of hierarchical ZSM-5 for hydrogen-free upcycling of Polyethylene to C8–C12 Methylated Aromatics1Engineering atomic nickel on zeolite-encapsulated platinum nanoclusters for efficient hydrogenation of halonitrobenzenes1Honeycomb-like Mordenite Zeolite Monoliths with Hierarchical Porosity for Promoting Direct Air Capture of CO 22Long-Chain Branched α-Alkenes from Plastic Upcycling Using Mo 2 C–Zn Nanoclusters Embedded on Hierarchical Porous Carbon1Acid Site Engineering of Ni/BEA Zeolites Enables Efficient Upcycling of Polyolefin Plastics to Liquid Fuels1Advancing Waste Plastic Valorization: Catalytic Production of Aviation Fuel over Zeolite and Ru/CNT-Based Catalysts4Thermo-chemical upgrading of waste polyethylene and polypropylene plastics0Structure–performance relationships in heterogeneous catalysts for polyolefin plastic hydroconversion1Catalytic Upcycling of Polyolefins and Polystyrene: Integrating Active Site Design With Mass Transfer Considerations4Deciphering structure-activity relationships in La/Ce/Ga/In-modified Pt/Y zeolites for n-docosane hydrocracking to aviation fuel0Adaptive Brønsted Acidity From Heterolytic Dihydrogen Activation Enables Polyethylene Hydrogenolysis Over Pd‐Encapsulated Na‐Zeolites2NiW alloy catalyst for methane suppression in polyethylene hydrogenolysis to enhance liquid hydrocarbon yields1Interfacial Engineering of Zeolite-Based Multicomponent Catalysts Enables Synergistic Acid−Diffusion Coupling for Efficient Polyolefin Upcycling4iPDA-Assisted Design of Hierarchical Beta Zeolites for the Sustainable Upcycling of Polyethylene to Naphtha with Ultra-Low Pt Loading1Hydrocracking of LDPE to liquid fuel over HY zeolite supported Ni catalyst: synergistic effect among metal, porosity and acidity1Advances in Catalytic Hydrogenolysis of Waste Plastics to Value-Added Products0Catalyst‐Free Upcycling of Polyethylene Waste Into Oxidized Polyethylene Wax1Recent progress of zeolite-based catalysts for industrial applications2Bifunctional nanocatalyst design for polyolefin hydrocracking2Quantitative Polyethylene Upcycling to Liquid Olefins over Ru-Containing Layered Zeolites0Coupling Polyolefin Conversion and Methanol Reduction for C 9 –C 10 Alkylaromatic Production1Elucidating the Spatiotemporal Reaction Mechanism of Polyethylene Aromatization over ZSM-5 Zeolites1Sufficient Metal–Acid Site Matching in Co-Loaded WO x -ZrO2 Catalysts for Polyethylene Hydrocracking0Catalytic pyrolysis of waste plastics to liquid fuels: pathways, mechanisms, and challenges0Spatially orthogonal CeOx-Zn sites on diatomite-aerogel-derived hierarchical HZSM-5 enable gated dechlorination and BTX-selective upcycling of PVC/PET mixed plastics0A review on selective dealkylation of alkylaromatics: Feedstocks, catalysts, and reaction pathways0Self‐Pillared Pentasil Zeolite Microspheres as Self‐Supported Catalysts With Enhanced Molecular Diffusion for Waste Plastic Upcycling0Unraveling the effects of pore structure on the performance of Ru/SiO2 catalysts for the selective hydrogenation of dimethyl terephthalate to dimethyl 1,4-cyclohexanedicarboxylate0Mechanistic insights into the Cr-Zr/ZSM-5 catalyzed cracking of waste polyethylene: Steering product distribution toward BTX aromatics and sustainable aviation fuel0Hierarchical Accessibility and Framework‐Al Organization in Ultra‐High‐Silica ZSM‐5 Enable Efficient Cracking of Polyolefin Waste to Light Olefins0Reactive-Intermediate Channelling from Interfacial Hydrogen Peroxide Generation to Confined Catalysis for Water Decontamination0Defect-Engineered Pd/ZSM-5 for Hydroconversion of LDPE to Light Alkanes0

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  2. Catalytic coproduction of renewable lubricant base oils and diesel fuels from bio-lipids and aromatics via alkylation and hydrodeoxygenation

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  3. Recent developments in recycling of post-consumer polyethylene waste

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  5. Upgrading polyolefin plastics: experiences from petroleum refining and distinct characteristics

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  6. Hydrocracking of Polyethylene to Gasoline-Range Hydrocarbons over a Ruthenium-Zeolite Bifunctional Catalyst System with Optimal Synergy of Metal and Acid Sites

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  8. Enhancing Waste Plastic Hydrogenolysis on Ru/CeO 2 Through Concurrent Incorporation of Fe Single Atoms and FeO x Nanoclusters

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  9. Co-recycling of plastics and other waste materials

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  10. Hydrogen Spillover‐Induced Brønsted Acidity Enables Controllable Hydrocracking of Polyolefin Waste to Liquid Fuels

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  12. Oxidation of n-alkanes using TS-1 and H2O2: Effects of chain length and solvents

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