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RESEARCH PAPER · Angewandte Chemie International Edition · 2024

Production of Branched Alkanes by Upcycling of Waste Polyethylene over Controlled Acid Sites of SO 4 /ZrO 2 ‐Al 2 O 3 Catalyst

Wanying Han, Longfei Lin, Longfei Lin, Ziyu Cen, Yubin Ke, Qian Xu, Junfa Zhu, Xuelei Mei, Zhanghui Xia, Xinrui Zheng, Yaqin Wang, Yani Liu, Mingyuan He, Haihong Wu, Haihong Wu, Buxing Han

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Production of Branched Alkanes by Upcycling of Waste Polyethylene over Controlled Acid Sites of SO 4 /ZrO 2 ‐Al 2 O 3 CatalystOriginalSynthesis of mesoporous Al 2 O 3 microspheres via hydrogen bond-enhanced monomicelle assembly strategy6Insights into Chemical Recycling and Upgrading Strategies for Polyolefin-Based Plastics15Advances and Challenges in Low‐Temperature Upcycling of Waste Polyolefins via Tandem Catalysis25Advances and Challenges in Low‐Temperature Upcycling of Waste Polyolefins via Tandem Catalysis2Polyethylene Upcycling to Liquid Alkanes in Molten Salts under Neat and External Hydrogen Source-Free Conditions17Individual Functionality and Synergistic Effects of Redox Site–Acid Site in Propane Oxidation35Rational design of zeolite-based composite catalysts in catalytic cracking of polyethylene6A Universal Micelle Assembly Strategy for Coating Mesoporous Al2O3 Shells on Diverse Interfaces0The silent partner in catalysis: How support architectures dictate efficiency in polyolefin hydrogenolysis1Plasma catalytic hydrogenolysis of polyethylene to gasoline-range fuels over Sm/USY catalysts10DFT Study of Oxygen Ion Migration in Mg-Doped Cubic Zirconia7Solar-Driven Upcycling of Polylactic Acid to Alanine over Pt/CdS–TiO 2 Heterojunction Single-Atom Photocatalyst35Dialectical Effects of MoO 3 Modification on the Pt/Al 2 O 3 Catalyst for VOC Combustion due to the Molecular Structure Sensitivity8Catalytic transfer reductive conversion of plastic wastes into fuel and chemicals0Acid sites in hydrogen-involved polyolefin upcycling: mechanistic insights and design principles0Carrier confinement of BiOI (001)/BiOI (010) facet junction mediated by crystal facet engineering: From experimental to theoretical perspectives on photocatalytic performance2Selective Upcycling of Waste Polyethylene into Propane Facilitated by the Undulation Confinement Effect in Zeolite Channels5Low-Temperature Pyrolysis of Aliphatic Polymers Using a Fluorinated Amorphous Silica–Alumina: Cooperative Reactivity between a Redox-Active Radical and an Aluminum Lewis Site0A Panoramic View on Plastic Waste Recycling and Upcycling: Heterogeneous Catalytic Strategies for Diverse Plastics and Multiple Pathways6Polyethylene as a Hydrogen Source for C─O Bond Cleavage Via Transfer Hydrogenation2Stepwise Hydrodeoxygenation of Mixed Oxygenated Plastics Enables Sequential Production of Jet- and Gasoline-Range Fuels0Solvent-free chemical recycling of polyolefins and polystyrene under mild conditions via GaCl3-based molten catalysts0Quantitative Polyethylene Upcycling to Liquid Olefins over Ru-Containing Layered Zeolites0Implementable and Sustainable Upcycling of Medical Plastic Waste to Liquid Highly Branched Alkanes via Tandem Catalytic Cracking-Hydrogenation Strategy0Influence of Water Molecule Adsorption and H2 Reduction Treatment on Acid Sites of WO3 with the (002) Crystal Facet Studied by Solid-State NMR Spectroscopy0Hydroxyl Surface Enrichment Strategy to Achieve Dual‐Mechanism Pathway for Overcoming the Activity–Stability Trade‐Off of Oxygen Evolution Reaction0Metal-Acid Balance Enables Earth-Abundant Metal Upcycling of Polyolefins to Jet Fuel0

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  1. Synthesis of mesoporous Al 2 O 3 microspheres via hydrogen bond-enhanced monomicelle assembly strategy

    Nano Research · 2024-06-01

    Kerun Zhu, Shuai Li, Tong Wang, Luo Lu, Bing Ma, Liang Qiao, Ao Guo, Jiwei Wang, Wei Zhang, Wei Li

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  2. Insights into Chemical Recycling and Upgrading Strategies for Polyolefin-Based Plastics

    Industrial & Engineering Chemistry Research · 2025-03-05

    Mei Lu, Shengdi Wang, Min Su, Zhenghui Weng, Jiawen Zheng, Navneet Kumar Gupta, Kejian Cai, Zhoupeng Shou, Quanli Ke

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  3. Advances and Challenges in Low‐Temperature Upcycling of Waste Polyolefins via Tandem Catalysis

    Angewandte Chemie International Edition · 2025-03-13

    Wei Zhang, Sung Min Kim, Michele L. Sarazen, Mingyuan He, Jingguang G. Chen, Johannes A. Lercher

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  4. Advances and Challenges in Low‐Temperature Upcycling of Waste Polyolefins via Tandem Catalysis

    Angewandte Chemie · 2025-03-13

    Wei Zhang, Sung Min Kim, Michele L. Sarazen, Mingyuan He, Jingguang G. Chen, Johannes A. Lercher

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  5. Polyethylene Upcycling to Liquid Alkanes in Molten Salts under Neat and External Hydrogen Source-Free Conditions

    Journal of the American Chemical Society · 2025-04-07

    Liqi Qiu, Felipe Polo‐Garzon, Luke L. Daemen, Min-Jae Kim, Jinghua Guo, Bobby G. Sumpter, Michael Köehler, Carlos Alberto Steren, Tao Wang, Logan T. Kearney, Tomonori Saito, Zhenzhen Yang, Sheng Dai

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  6. Individual Functionality and Synergistic Effects of Redox Site–Acid Site in Propane Oxidation

    ACS Catalysis · 2025-06-06

    Cai-Hao Wen, Lin‐Ya Xu, You‐Zeng Hao, Qian Zhou, Yi-Wei Xian, Mao-Di Wang, Wei Tan, Lin Dong, Jian Chen, Meng‐Fei Luo, Qihua Yang

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  7. Rational design of zeolite-based composite catalysts in catalytic cracking of polyethylene

    Fuel · 2025-07-01

    Yanjun Li, Zhe Ma, Jingyuan Shang, Ting Wang, Xingong Zhang, Peng Xu, Chenzhao Wang, Xiang Feng, De Chen, Chaohe Yang, Xiaobo Chen

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  8. A Universal Micelle Assembly Strategy for Coating Mesoporous Al2O3 Shells on Diverse Interfaces

    Advanced Materials Technologies · 2025-07-05

    Haijun Yu, Kuoyan Ma, Luo Lu, Tong Wang, Kerun Zhu, Jie Zhao, Jie Tang, Xiangmin Lv, Hongli Li, Peng Wang, Yuncan Chen, Keyi Xiao, Yupu Liu, Wei Zhang

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  9. The silent partner in catalysis: How support architectures dictate efficiency in polyolefin hydrogenolysis

    Nano Research · 2025-08-22

    Xueping Zhang, Wenli Wang, Mei Hong, Yamei Lin, Guoping Lu

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  10. Plasma catalytic hydrogenolysis of polyethylene to gasoline-range fuels over Sm/USY catalysts

    Applied Catalysis B: Environmental · 2025-09-08

    Chengxin Hou, Yanan Diao, Tianqi Yun, Jianhui Han, Tianhao Shi, Bingbing Chen, Chuan Shi

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  11. DFT Study of Oxygen Ion Migration in Mg-Doped Cubic Zirconia

    Solids · 2025-09-25

    Zh.M. Salikhodzha, Guldari B. Bairbayeva, Anatoli I. Popov, Raigul N. Kassymkhanova, Keleshek B. Zhangylyssov, Elena Popova, Marina Koņuhova

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  12. Solar-Driven Upcycling of Polylactic Acid to Alanine over Pt/CdS–TiO 2 Heterojunction Single-Atom Photocatalyst

    Journal of the American Chemical Society · 2025-11-21

    Zhanghui Xia, Longfei Lin, Xiao Chen, Jianxin Zhai, Cheng Xue, Shuaiqiang Jia, Jiapeng Jiao, Mengke Dong, Wanying Han, Xinrui Zheng, Ting Deng, Xinyu Zou, Chensheng Xian, Haihong Wu, Buxing Han

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  13. Dialectical Effects of MoO 3 Modification on the Pt/Al 2 O 3 Catalyst for VOC Combustion due to the Molecular Structure Sensitivity

    Environmental Science & Technology · 2025-12-27

    Jiawei Yang, Zhan Yu, Qing Tong, Bifeng Zhang, Xin Wang, Zixi Li, Xiuwen Wang, A. Liu, Wei Tan, Lin Dong

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  14. Catalytic transfer reductive conversion of plastic wastes into fuel and chemicals

    Green Chemistry · 2026-01-01

    Yinghui Chen, Huayang Lin, Ruixing Wang, Jiaqi Qiao, Sibao Liu, Guozhu Liu

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  15. Acid sites in hydrogen-involved polyolefin upcycling: mechanistic insights and design principles

    Science China Chemistry · 2026-01-27

    Qi Zhang, Xiang Wang

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  16. Carrier confinement of BiOI (001)/BiOI (010) facet junction mediated by crystal facet engineering: From experimental to theoretical perspectives on photocatalytic performance

    Surfaces and Interfaces · 2026-02-07

    Guangri Chen, Fanbing Yan, Jingjing Bi, Xuejiao Li, Lianwei Shan, Haitao Wu

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  17. Selective Upcycling of Waste Polyethylene into Propane Facilitated by the Undulation Confinement Effect in Zeolite Channels

    Journal of the American Chemical Society · 2026-03-25

    Yangyang Liu, Bing Ma, Jingqing Tian, Chen Zhao

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  18. Low-Temperature Pyrolysis of Aliphatic Polymers Using a Fluorinated Amorphous Silica–Alumina: Cooperative Reactivity between a Redox-Active Radical and an Aluminum Lewis Site

    Journal of the American Chemical Society · 2026-04-27

    Jiaxin Gao, Avijit Mondal, Riley Pritchett, Paul H. Oyala, Matthew P. Conley

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  19. A Panoramic View on Plastic Waste Recycling and Upcycling: Heterogeneous Catalytic Strategies for Diverse Plastics and Multiple Pathways

    Advanced Materials · 2026-05-12

    Chang‐Jie Yang, Xin-Yu Wang, Mei‐Qi Zhu, Tianyou Zhao, Yong-Zhou Pan, Yuhai Dou, Jie Yang, Zechao C. Zhuang, Zhenglong Li, Zhijun Wu, Wen‐Gang Cui, Hongge Pan, Weiwei Li, Dingsheng S. Wang

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  20. Polyethylene as a Hydrogen Source for C─O Bond Cleavage Via Transfer Hydrogenation

    Angewandte Chemie International Edition · 2026-05-13

    Weilong Wen, Ziyu Cen, Tianrui Bi, Zhiye Ma, Xiaqian Lin, Cong Luo, Zhenpeng Wang, Qinglei Meng, Longfei Lin, Bo Han

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  21. Stepwise Hydrodeoxygenation of Mixed Oxygenated Plastics Enables Sequential Production of Jet- and Gasoline-Range Fuels

    Environmental Science & Technology · 2026-06-16

    Yue Zhu, Zhouying Mao, Pengfei An, Buxing Han, Qingqing Mei

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  22. Solvent-free chemical recycling of polyolefins and polystyrene under mild conditions via GaCl3-based molten catalysts

    CHINESE JOURNAL OF CATALYSIS (CHINESE VERSION) · 2026-07-01

    Lei Yuan, Zhiwen Gao, Libin Shi, Cuishi Guan, Dongyue Peng, Shuhui Fang, Wei Zhang, Y Liu

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  23. Quantitative Polyethylene Upcycling to Liquid Olefins over Ru-Containing Layered Zeolites

    Journal of the American Chemical Society · 2026-07-03

    Malin Eqi, Yi Yang, Jiashuo Zheng, Guangjun Wu, Yuchao Chai, Landong Li

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  24. Implementable and Sustainable Upcycling of Medical Plastic Waste to Liquid Highly Branched Alkanes via Tandem Catalytic Cracking-Hydrogenation Strategy

    ACS Sustainable Chemistry & Engineering · 2026-08-04

    Guanyu Zhang, Yuan Jiang, Qing Cheng, Xin Zhang, Ge Kong, Tianqi Cao, Chun Shan, Jin Wang, Fangqi Liu, Roger R. Ruan, Hanwu Lei, Xuesong Zhang, Lujia Han

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  25. Influence of Water Molecule Adsorption and H2 Reduction Treatment on Acid Sites of WO3 with the (002) Crystal Facet Studied by Solid-State NMR Spectroscopy

    The Journal of Physical Chemistry C · 2026-08-12

    Hengshun Zhao, Li Zhang, Qingying Yao, Yuting Miao, Yuanhang Ren, Xueying Chen, Bin Yue, Heyong He

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  26. Hydroxyl Surface Enrichment Strategy to Achieve Dual‐Mechanism Pathway for Overcoming the Activity–Stability Trade‐Off of Oxygen Evolution Reaction

    Angewandte Chemie International Edition · 2026-08-14

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  27. Metal-Acid Balance Enables Earth-Abundant Metal Upcycling of Polyolefins to Jet Fuel

    Journal of the American Chemical Society · 2026-08-27

    Jicong Yan, Shuheng Tian, Qi Zhang, Yujia Ding, Hongbo Xie, Fuping Tian, Tao Hu, Junzhong Xie, Xiang Wang, Ding Ma

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