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RESEARCH PAPER · ACS Applied Materials & Interfaces · 2024

Interfacial Reactions in Chemical Recycling and Upcycling of Plastics

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Interfacial Reactions in Chemical Recycling and Upcycling of PlasticsOriginalLow‐Temperature Catalytic Approaches for Upcycling Plastics into Oxygenated Aromatic Compounds14Can mixed plastics be recycled and upcycled without separation?11Toward a Circular Economy of Heteroatom Containing Plastics: A Focus on Heterogeneous Catalysis in Recycling21Interfacial catalysis in enzymatic PET plastic depolymerization28Eco-friendly additives for biodegradable polyesters: Recent progress in performance optimization and environmental impact reduction23MOF Catalysts for Plastic Depolymerization4MOF Catalysts for Plastic Depolymerization52Understanding the Surface Acidity Mediated Reaction Pathway in CO 2 Assisted Aromatization of Polyolefin Waste8Polymer Upcycling by Catalytic Hydrogenolysis: The Role of Polyolefin Short-Chain Branching3Plasma Catalysis for Plastic Waste Conversion into Value‐Added Products: Advancements and Perspectives11Enzymatic degradation of biopolymers in amorphous and molten states: mechanisms and applications10Upcycling Waste Polyethylene and Polypropylene into Carbon Oxides and Hydrocarbons via a Mechanochemistry-Photocatalysis Combined Technology under Mild Conditions1Methods for the establishment of enzymatic mechanisms – from QM to ML0Thermodynamic exclusion of alkaline ionic crystals from polymers and interfacial-controlled subcritical water degradation0Precision bond cleavage in waste plastics: Directed catalytic upcycling1Aqueous-Based Biomimetic Porphyrin-Catalyzed Surface Oxidation of Polyethylenes for Enhanced 3D-Printability0Accelerating Biocatalysis in Interface-Regulated Nano–Bio Hybrid System via Increasing Substrate Accessibility0Photothermal Catalytic Depolymerization and Glycolytic Regeneration of Polyethylene Terephthalate0

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  1. Low‐Temperature Catalytic Approaches for Upcycling Plastics into Oxygenated Aromatic Compounds

    ChemCatChem · 2024-11-19

    Jason Y. C. Lim

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  2. Can mixed plastics be recycled and upcycled without separation?

    Green Chemistry · 2025-01-01

    Jaime J. M. Pang, Yan Hui Lee, Haonan Zhao, Albert Ong, Jason Y. C. Lim

    Read original paper ↗ ·
  3. Toward a Circular Economy of Heteroatom Containing Plastics: A Focus on Heterogeneous Catalysis in Recycling

    Langmuir · 2025-03-03

    Gabriel Perli, Ion Olazabal, Louise Breloy, Ina Vollmer, Fernando López‐Gallego, Haritz Sardón

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  4. Interfacial catalysis in enzymatic PET plastic depolymerization

    Trends in Chemistry · 2025-03-27

    Jie Zhou, Zhongli Cui, Ren Wei, Weiliang Dong, Min Jiang

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  5. Eco-friendly additives for biodegradable polyesters: Recent progress in performance optimization and environmental impact reduction

    Sustainable materials and technologies · 2025-04-11

    Ahmad Fayyazbakhsh, Nima Hajinajaf, Hamed Bakhtiari, Michael Feuchter, Ilaria Improta, Ehsan Salehi, Sara Kamal Shahsavar, Markéta Julinová, Amirehsan Ghasemi, Bita Ghasemi, Reza Afsharnia, Marek Koutný, Young‐Cheol Chang

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  6. MOF Catalysts for Plastic Depolymerization

    Angewandte Chemie · 2025-04-30

    Bao‐Nguyen T. Nguyen, Tristan Tsai Yuan Tan, Ken‐ichi Otake, Susumu Kitagawa, Jason Y. C. Lim

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  7. MOF Catalysts for Plastic Depolymerization

    Angewandte Chemie International Edition · 2025-04-30

    Bao‐Nguyen T. Nguyen, Tristan Tsai Yuan Tan, Ken‐ichi Otake, Susumu Kitagawa, Jason Y. C. Lim

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  8. Understanding the Surface Acidity Mediated Reaction Pathway in CO 2 Assisted Aromatization of Polyolefin Waste

    ACS Sustainable Chemistry & Engineering · 2025-08-16

    Xiaoyue Xiao, Jiuxuan Zhang, Zhengyan Qu, Y. Li, Feng Zeng, Hong Li Jiang, Zhenchen Tang, Rizhi Chen

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  9. Polymer Upcycling by Catalytic Hydrogenolysis: The Role of Polyolefin Short-Chain Branching

    ACS Catalysis · 2025-09-23

    Zachary M. Gdowski, Rishi Raj, Aditya Bhan, K. Andre Mkhoyan, Mahesh K. Mahanthappa, Frank S. Bates

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  10. Plasma Catalysis for Plastic Waste Conversion into Value‐Added Products: Advancements and Perspectives

    Advanced Functional Materials · 2025-11-10

    Yanan Diao, Xuetao Qin, Chengxin Hou, Bingbing Chen, Tianqi Yun, Xinwen Guo, Ding Ma, Chuan Shi

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  11. Enzymatic degradation of biopolymers in amorphous and molten states: mechanisms and applications

    FEBS Open Bio · 2025-12-10

    Anđela Pustak, Aleksandra Maršavelski

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  12. Upcycling Waste Polyethylene and Polypropylene into Carbon Oxides and Hydrocarbons via a Mechanochemistry-Photocatalysis Combined Technology under Mild Conditions

    ACS Applied Materials & Interfaces · 2025-12-28

    Fei Liu, Yuan He, Pengfei Li, Guixue Liang, Yi Dan, Yun Huang, Long Jiang

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  13. Methods for the establishment of enzymatic mechanisms – from QM to ML

    Chemical Science · 2026-01-01

    Rui P. P. Neves, João T. S. Coimbra, Pedro Paiva, Umberto Raucci, Sudip Das, Ana Rita Calixto, António J. M. Ribeiro, João P. M. Sousa, Pedro Ferreira, Enrico Trizio, Pedro Alexandrino Fernandes, Michele Parrinello, Maria João Ramos

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  14. Thermodynamic exclusion of alkaline ionic crystals from polymers and interfacial-controlled subcritical water degradation

    Chemical Engineering Science · 2026-03-25

    Li Yan, Lin-Han Wang, Xiao-Sa Liu, Qi Zeng, Zibin Huang, Jingyi Yang, Pei‐Qing Yuan

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  15. Precision bond cleavage in waste plastics: Directed catalytic upcycling

    Renewable and Sustainable Energy Reviews · 2026-04-25

    Yusong Zhang, Yinxiang Wang, Aimin Li

    Read original paper ↗ ·
  16. Aqueous-Based Biomimetic Porphyrin-Catalyzed Surface Oxidation of Polyethylenes for Enhanced 3D-Printability

    Journal of the American Chemical Society · 2026-05-27

    Haonan Zhao, Danwei Zhang, Wei Wei Loh, Shih Jia Yam, Jaime J. M. Pang, Debbie Hwee Leng Seng, Zhuang Mao Png, Xue Qi Koh, Yan Hui Lee, Lewis Queh, Jason Y. C. Lim

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  17. Accelerating Biocatalysis in Interface-Regulated Nano–Bio Hybrid System via Increasing Substrate Accessibility

    ACS Applied Bio Materials · 2026-07-16

    Ziyang Xing, Kailiang Hua, R Li, 容习习, Li Mi

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  18. Photothermal Catalytic Depolymerization and Glycolytic Regeneration of Polyethylene Terephthalate

    ChemSusChem · 2026-08-21

    Haishui Xu, Chao Chen, Zhang Cao, Jiabao Chen, Jiacheng Zhao, Guiyin Xu, Xijiang Chang

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